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At least 37 records · Page 2

Improving Nb 3 Sn cavity performance using centrifugal barrel polishing

Abstract In this study we will show a new method of polishing for Nb 3 Sn cavities known as centrifugal barrel polishing (CBP). Using this method, Nb 3 Sn coated samples are polished to a surface roughness comparable to a traditional Nb cavity after electropolishing. We also investigate different methods of cleaning the Nb 3 Sn surface after CBP to remove residual abrasive particles. The polished Nb 3 Sn surface is analyzed using confocal laser microscopy, and scanning electron microscopy is used to image the surface and measure the surface roughness after polishing. Transmission electron microscopy is also used for high resolution analysis of the surface after polishing. Finally, we show that CBP can improve the performance of a Nb 3 Sn superconducting radiofrequency cavity.

43 PARTICLE ACCELERATORS↗

Nb 3 Sn Superconducting RF Cavities: R&D Progress at Fermilab and Opportunities [Poster]

Nb 3 Sn becomes superconducting at twice as high temperature as our standard SRF material niobium. This allows us to efficiently operate Nb 3 Sn cavities at 4.4 K instead of the usual 2 K. This reduces cryogenic costs and even makes it possible to use a cryocooler instead of a large, complex cryogenic plant. The superheating field Hsh of Nb 3 Sn is twice that of niobium. Hsh is thought to be the ultimate limit for a defect-free superconductor. Nb 3 Sn cavities being made today are still about a factor of 4 away from this ultimate limit, but R&D has been leading to substantial progress towards this goal

43 PARTICLE ACCELERATORS↗

Optimization of Nb 3 Sn sputtering on SRF structures

Superconducting radiofrequency (SRF) cavities are the key technology to compact, high-efficiency, and cost-effective CW SRF accelerators. Further improvements in the efficiency can be realized by using novel materials such as Nb 3 Sn coated on the inner surface of SRF cavities. The Nb 3 Sn coatings enable cavity operation at 4 K, where the Nb 3 Sn coated cavities are already very efficient and have high intrinsic quality factors. Advances in Nb3Sn coatings on the inner surface of SRF cavities showed the potential for this material to significantly cut the capital and operating costs of SRF accelerators. Several approaches have been and are being investigated for coating SRF cavities with Nb 3 Sn. Magnetron sputtering is a versatile technique in that it has been shown to produce Nb 3 Sn films on flat Nb target in a single phase and a precisely controlled thickness, low defect levels, and a favorable morphology. Deposition of Nb 3 Sn films on SRF cavities have also shown promising RF superconducting properties. However, sputter coating of Nb 3 Sn on SRF cavities requires further development to be used in accelerators.

43 PARTICLE ACCELERATORS↗

Multi-scale nonlinear stress analysis of Nb 3 Sn superconducting accelerator magnets

A multi-scale nonlinear procedure to analyze the stress in Nb 3 Sn superconducting accelerator magnets is presented to address one of the most challenging obstacles currently facing the successful development of high-field superconducting magnets—the issue of stress management. The study demonstrates that gaskets (special nonlinear materials) are capable of modeling the complex nonlinear deformation behavior of insulation layers within the Nb 3 Sn coil block and that Hill materials (orthotropic materials utilizing the Hill yield criterion) are suitable to enable homogenization of the filamentary regions and the resin-impregnated Nb 3 Sn Rutherford cables. With the whole magnet under preload, cool-down, and Lorentz forces, the nonlinear behavior of the Nb 3 Sn coil was simulated, in three orthongonal axes, by the combined properties of the gaskets (insulation layers) and Hill materials (resin-impreganted cable). The procedure entailes minimal material assumptions because it incorporated measured stress-strain curves in the analysis. The coil was simulated to a high level of detail consisting of the insulation layers and resin-impregnated cables. The computed compressive azimuthal stresses of the cables were used to assess the stress-induced performance degradation. Through submodeling, the area-weighted average axial strains of the strands were computed and employed to evaluate the strain-induced performance degradation. The overall performance degradation of the Nb 3 Sn coil was thus obtained, and this information was subsequently used to guide the design of the overall magnet. Besides Nb 3 Sn magnets, this procedure can also be employed in the design of LTS, HTS, and room temperature magnets or in any composite structures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A Metallurgical Inspection Method to Assess the Damage in Performance-Limiting Nb 3 Sn Accelerator Magnet Coils

The design and production of Nb 3 Sn-based dipole and quadrupole magnets is critical for the realization of the High-Luminosity Large Hadron Collider (HL-LHC) at the European Organization for Nuclear Research (CERN). Nb 3 Sn superconducting coils are aimed at enhancing the bending and focusing strengths of accelerator magnets for HL-LHC and beyond. Due to the brittle nature of Nb 3 Sn, the coil fabrication steps are very challenging and require very careful QA/QC. Flaws in the Nb 3 Sn filaments may lead to quenches, and eventually, performance limitation below nominal during magnet testing. A novel inspection method, including advanced non-destructive and destructive techniques, was developed to explore the root-causes of quenches occurring in performance-limiting coils. The most relevant results obtained for MQXF coils through this innovative inspection method are presented. This approach allows for precise assessment of the physical events associated to the quenches experienced b y magnet coils, mainly occurring under the form of damaged strands with transversely broken sub-elements. Coil-slice preparation, micro-optical observations of transverse and longitudinal cross-sections, and a deep etching technique of copper will be illustrated in the present work, with a focus on the results achieved for a CERN coil from a non-conforming quadrupole magnet prototype, and two coils fabricated in the US, in the framework of the Accelerator Upgrade Project (AUP) collaboration, from two different non-conforming quadrupole magnets, respectively. The results obtained through the proposed inspection method will be illustrated.

43 PARTICLE ACCELERATORS↗

Investigations Towards Ultra-Low Cost Nb 3 Sn SRF Fabrication via Melt Casted Bronze Route Processing

Here, a novel approach to fabricating Nb 3 Sn SRF cavities and other RF components using an ultra-low-cost melt casting fabrication process has been investigated. This simple, low cost melt casting technique has the potential to be used to fabricate nearly any superconducting Nb3Sn structure using either the Bronze Route (BR), Internal Tin (IT), External Tin (ET) processes as well as normal conducting pure copper (Cu) cavities. Most of the heat treated samples that were examined using SEM/EDX seemed to show a reasonable correlation of T c onset and transition width (ΔT c ) of the ingots initial/starting Sn content to the desired stoichiometric Nb 3 Sn phase, where the lower starting Sn content coupons resulted in lower T c 's with broader transition widths and the higher starting Sn coupons resulted in higher T c 's with narrower ΔT c ’s. The best samples had T c onsets ~17-18 K and ΔT c 's < 2 K. Two samples were further tested for RF surface resistance (R s ) and Quality Factor (Q) at JLAB. Here, these RF measurements were performed at 7.4 GHz using a calorimetric technique and showed two transitions, one at ~ 8 K and another at ~ 14 K; values of R s were at least two orders of magnitude higher than similar high quality Nb 3 Sn films directly deposited substrates by JLAB and with another superconducting transition close to the superconducting transition temperature of niobium. Substantial improvements in the processing variables ranging from higher quality of the initial ingots with higher Sn content, to better electropolishing and reaction heat treatment regimens will be necessary to realize improved RF performance metrics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Smooth, homogeneous, high-purity Nb 3 Sn superconducting RF resonant cavity by seed-free electrochemical synthesis

Abstract Workbench-size particle accelerators, enabled by Nb 3 Sn-based superconducting radio-frequency (SRF) cavities, hold the potential of driving scientific discovery by offering a widely accessible and affordable source of high-energy electrons and x-rays. Thin-film Nb 3 Sn RF superconductors with high quality factors, high operation temperatures, and high-field potentials are critical for these devices. However, surface roughness, non-stoichiometry, and impurities in Nb 3 Sn deposited by conventional Sn-vapor diffusion prevent them from reaching their theoretical capabilities. Here we demonstrate a seed-free electrochemical synthesis that pushes the limit of chemical and physical properties in Nb 3 Sn. Utilization of electrochemical Sn pre-deposits reduces the roughness of converted Nb 3 Sn by five times compared to typical vapor-diffused Nb 3 Sn. Quantitative mappings using chemical and atomic probes confirm improved stoichiometry and minimized impurity concentrations in electrochemically synthesized Nb 3 Sn. We have successfully applied this Nb 3 Sn to the large-scale 1.3 GHz SRF cavity and demonstrated ultra-low BCS surface resistances at multiple operation temperatures, notably lower than vapor-diffused cavities. Our smooth, homogeneous, high-purity Nb 3 Sn provides the route toward high efficiency and high fields for SRF applications under helium-free cryogenic operations.

Physics↗

Field Measurement Results of the 15 T Nb 3 Sn Dipole Demonstrator MDPCT1b

A 15 T Nb 3 Sn dipole with cos-theta-type coils was developed to demonstrate a possible magnet design for a post-LHC proton-proton Collider. The magnet has 4-layer coils with 60-mm aperture, and has graded current density between the inner and outer layers to maximize performance. The coils are constrained by vertically-split, thick iron laminations, connected by aluminum Iclamps, and a thick stainless-steel skin. The magnet was previously tested at the Vertical Magnet Test Facility (VMTF) at Fermilab with reduced pre-load, and achieved record 14.1 T fields at maximum current. Now the magnet has been reassembled with full pre-load and has been cryogenically retested at VMTF. We report here on the magnetic measurements results of these tests, including field strength, geometrical harmonics, coil magnetization, and iron saturation characteristics of the demonstrator.

43 PARTICLE ACCELERATORS↗

Critical current and stability tests of Nb 3 Sn for LBNL CCT magnet project

The Nb 3 Sn wires received from LBNL include the original round wires as well as the extracted wires from Rutherford cables. Total of 12 samples were prepared and heat treated. Five of them were tested for electric field versus current (E-I), among them 4 samples were further tested for electric field versus magnetic field (E-H). E-I traces were measured in magnetic field between 5 T and 8 T at 4.2 K. The critical currents of these sample are between 924 A and 993 A at 5 T. E-H measurements were performed at currents between 900 and 1500 A at 4.2 K. The stability currents, which is defined as the maximum current without quench during the E-H test, are determined to be between 1100 A and 1400 A. A separate Excel file presenting all the critical current and E-H curves is attached.

36 MATERIALS SCIENCE↗

Three-Dimensional Reconstruction of Nb 3 Sn Films by Focused Ion Beam Cross Sectional Microscopy

Niobium has been the material of choice for SRF cavities for several decades due to its formability and superconducting properties. The accelerating gradient of niobium cavities is, however, rapidly approaching a theoretical limit. To achieve higher accelerating gradients a new material is needed that can sustain high fields. Nb 3 Sn is a promising competitor with a higher superconducting transition temperature and a higher critical field than pure niobium. However, Nb 3 Sn is very brittle and cannot be formed readily into a cavity. The main method for creating Nb 3 Sn cavities is to form a Nb 3 Sn film into a niobium surface using a tin vapor-diffusion method. This technique creates a microcrystalline Nb 3 Sn thin film on the inner surface of the cavity. Tin depleted regions are known to form in the film during this process. Previous studies have analyzed these regions using transmission electron microscopy on cross-sectional lamellae prepared by focused ion beam/scanning electron microscope (FIB/SEM). This method does not provide any three-dimensional (3-D) information about the distribution of tin-deficient regions. In this study we employ a focused ion beam tomographic technique to analyze the 3-D structure of the film. Electron dispersive X-ray spectroscopy is used to image the tin concentration of the film in 3-D. Tin-deficient regions are discovered close to the surface of the Nb 3 Sn film.

Viklund, E.↗

Development and Understanding of Nb 3 Sn films for radiofrequency applications through a sample-host 9-cell cavity

Nb 3 Sn is a promising advanced material under development for superconducting radiofrequency cavities. Past efforts have been focused primarily on small development-scale cavities, but large, often multi-celled cavities, are needed for particle accelerator applications. In this work, we report on successful Nb 3 Sn coatings on Nb in a 1 m-long 9-cell Nb sample-host cavity at Fermilab. The geometry of the first coating with only one Sn source made it possible to study the influence of Sn flux on the microstructure. Based on these results, we postulate a connection between recently observed anomalously large thin grains and uncovered niobium spots observed in the past by other authors (Trenikhina et al 2018 Supercond. Sci. Technol. 32 015004). A phenomenological model to explain how these anomalously large grains could form is proposed. Overall, this model is invoked to provide possible explanations for literature results from several groups and to guide key process parameters to achieve uniform vapor-diffusion coatings, when applied to complex structures as the multi-cell cavity under study.

43 PARTICLE ACCELERATORS↗

Pathway to tune sputter coated Nb$_3$Sn with Zr

Superconducting radio frequency (SRF) cavities are essential elements of many modern-day particle accelerators such as, European XFEL (DESY), LCLS II-HE (SLAC) and PIP II (Fermilab). Nb$_3$Sn superconducting material promises significant potential to exceed the performance of conventional niobium based SRF cavities. We aim to advance the ongoing R$&$D efforts to achieve Nb$_3$Sn coated cavities with high material quality. In this work, we have developed to achieve a route for effectively reducing the intrinsic defects in magnetron sputter coated Nb$_3$Sn SRF cavities and eventually improve the overall RF performance. We have observed that Zr is mainly being incorporated as ZrO$_2$ precipitates of average dimensions ranging from 20-100nm. By increasing the concentration of Zr, we have three major effects in the physical properties. Firstly, we noted that the density of the surface and bulk voids as well as their average dimensions are dramatically reduced on increasing the Zr content in Nb$_3$Sn. These surface voids are believed to be detrimental to cavity applications due to increase the local dissipation of electric and magnetic fields. These results indicate that inclusion of Zr in Nb$_3$Sn sputtered coating will improve the material quality and might help to reduce the overall RF power dissipation. Secondly, we observed that increasing Zr concentration from 0 to 2.4% substantially improves both superconducting transition temperature (Tc) and upper critical magnetic field (Hc2). However, on further increasing the Zr concentration to 24%, we noticed a small decrement in the Hc2 value. These results infer that the increase in Zr concentration up to an optimal concentration will be beneficial to enhance the superconducting properties. Increase in Tc promises lesser RF losses and improvement in accelerating gradient, whereas the increase in Hc2 suggests more efficient flux pinning which could give rise to high quality factors in presence of multi-Tesla magnetic field. Additionally, we also observed that increasing Zr concentration possibly prevents the oxygen diffusion and leads to thinner formation of primary surface oxide (Nb$_2$O$_5$ and SnO). This study gives a route to tune Zr fraction in Nb3Sn to modify the physical properties that control the high field performance of Nb3Sn RF cavities.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Comparison of Multi-Scale Nonlinear and Conventional Linear Methods for Stress Analysis of Nb 3 Sn Superconducting Magnets

Here this is an extension of the work on a multi-scale nonlinear procedure that demonstrated how to conduct nonlinear stress analysis of Nb 3 Sn superconducting accelerator magnets. The nonlinear procedure uses measured stress-strain curves of annealed copper, Nb 3 Sn strands and coil samples as inputs, which reduces the number of assumptions made for material properties—key uncertainties of any engineering analysis. The results from nonlinear analysis, semi-nonlinear analysis, and linear analysis of the same QFFB2 Nb 3 Sn quadrupole magnet under the same temperature and loads, were compared and discussed. The comparison illustrates that nonlinear stress analysis is significantly more accurate than other methods. As the superconducting coil block is a complex, composite material, it would be inadequate to assume the whole coil block to be linear, either isotropic or orthotropic. It is imperative to conduct nonlinear analysis by simulating the superconducting coil to the level of detail of the individual cables and individual strands. The nonlinear stress analysis procedure can be used to simulate not only Nb 3 Sn magnets, but also NbTi and HTS magnets.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Superconducting low-beta Nb 3 Sn cavity for ATLAS and future ion accelerators

We report on a Nb 3 Sn-coated low-beta superconducting radio frequency (RF) cavity intended for accelerating ions. We aim to apply the cavity in ATLAS, our Argonne National Laboratory user facility for nuclear physics studies with ion beams in the energy range of 5–20 MeV u −1 . The Nb 3 Sn-coated cavity, a 145 MHz quarter-wave optimized for ions moving with velocity β = $v/c$ = 0.08 exhibits an order-of-magnitude reduction in RF losses into helium at 4.4 K compared to a superconducting niobium (Nb) cavity at the same frequency and temperature. Experimentally measured fields are among the highest to date for any Nb 3 Sn-coated cavity, reaching a peak surface magnetic field of 105 mT. We also present a practical solution to the problem of cavity frequency tuning. Tuning by mechanical deformation has been a challenge with Nb 3 Sn due to its brittle nature, however, using a set of techniques tailored to the properties of thin-film Nb 3 Sn on Nb, we can repeatably tune the cavity to the ATLAS master clock frequency after it is cooled, while maintaining the excellent performance characteristics. The same Nb 3 Sn cavity technology offers broad benefits for future ion accelerators.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Assessment of Training Performance, Degradation and Robustness of Paraffin-Wax Impregnated Nb 3 Sn Demonstrator Under High Magnetic Field

In the context of high-energy physics, the use of Nb 3 Sn superconducting magnets as a cost-effective and reliable technology depends on improvements in the following areas: long development and manufacturing cycles, conductor degradation after thermal cycling, long training, as well as a demonstration in accelerator magnets with a beam aperture of the full potential of modern Nb 3 Sn conductors. In short, performance, robustness, and cost are the three issues to be addressed. The Magnet Development project (MagDev) of the Swiss Accelerator Research and Technology initiative (CHART) at the Paul Scherrer Institute (PSI) aims to contribute to the solutions to each of these issues, re-thinking the manufacturing and design process. Here in our program, every innovation is to be validated by means of a panoply of fast-turnaround tools: from non-powered and powered samples and coils, tested under background field, to low-field subscale magnets and high field short prototypes. This work presents one element in this panoply of R&D vehicles: a stress-managed Nb 3 Sn coil called BigBOX, impregnated with paraffin wax, and tested, through a collaboration with the Magnet Development Program of the United States (US-MDP), in the background field of Brookhaven National Laboratory (BNL)’s common coils dipole DCC17.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Evidence of Kramer extrapolation inaccuracy for predicting high field Nb 3 Sn properties

Future applications requiring high magnetic fields, such as the proposed Future Circular Collider, demand a substantially higher critical current density, J c , at fields ≥16 T than is presently available in any commercial strand, so there is a strong effort to develop new routes to higher J c Nb 3 Sn. As a consequence, evaluating the irreversibility field (H irr ) of any new conductor to ensure reliable performance at these higher magnetic fields becomes essential. To predict the irreversibility field for Nb 3 Sn wires, critical current measurements, I c , are commonly performed in the 12-15 T range and the Kramer extrapolation is used to predict higher field properties. Here, the Kramer extrapolation typically models the contribution only for sparse grain boundary pinning, yet Nb 3 Sn wires rely on a high density of grain boundaries to provide the flux pinning that enables their high critical current density. However, whole-field range VSM measurements up to 30 T recently showed for Nb 3 Sn RRP® wires that the field dependence of the pinning force curve significantly deviates from the typical grain boundary shape, leading to a 1-2 T overestimation of Hirr when extrapolated from the typical mid-field data taken only up to about 15 T. In this work we characterized a variety of both RRP® and PIT Nb 3 Sn wires by transport measurements up to 29 T at the Laboratoire National des Champs Magnétiques Intenses (LNCMI), part of the European Magnetic Field Laboratory in Grenoble, to verify whether or not such overestimation is related to the measurement technique and whether or not it is a common feature across different designs. Indeed we also found that when measured in transport the 12-15 T Kramer extrapolation overestimates the actual H irr in both types of conductor with an inaccuracy of up to 1.6 T, confirming that high field characterization is a necessary tool to evaluate the actual high field performance of each Nb 3 Sn wire.

36 MATERIALS SCIENCE↗

First Field Measurements of the 15 T Nb 3 Sn Dipole Demonstrator MDPCT1

Within the US Magnet Development Program (MDP) a 15 T Nb 3 Sn dipole was developed, to demonstrate a magnet design for a post-LHC pp Collider. Specifically, the magnet design is based on 60 mm aperture 4-layer shell-type coils, graded between the inner and outer layers to maximize the magnet performance. The cable in the two innermost layers has 28 strands 1.0 mm in diameter and the cable in the two outermost layers has 40 strands 0.7 mm in diameter. Both cables use RRP Nb3Sn wires produced by Bruker-OST. Magnet coils are surrounded by vertically-split thick iron laminations, con-nected by aluminum I-clamps, and a thick stainless-steel skin. The magnet was tested at the Vertical Magnet Test Facility (VMTF) at Fermilab. This paper reports the first results of magnetic measure-ments of the 15 T Nb 3 Sn dipole demonstrator including geometrical harmonics, coil magnetization and iron saturation effects. The ex-perimental data are compared with the magnetic calculations.

43 PARTICLE ACCELERATORS↗

Analysis of vapor diffusion Nb$^{3}$Sn coating at Fermilab: Minimizing impurities using TOF-SIMS

Nb₃Sn demonstrates steady advancements nowadays offering reduced power cost in superconducting radio-frequency cavities due to its high critical temperature, quality factor, and achieved accelerating gradient. However, theoretical estimates of its radio-frequency parameters have not been achieved due to several potentially limiting mechanisms: tin spots, patchy regions, defects, thermal impedance, and impurities. While some of these limitations have been intensively studied, impurity analysis in Nb$_3$Sn coatings have received less attention. We report an investigation of impurities in several vapor-diffused Nb₃Sn coated samples using time-of-flight secondary ion mass spectroscopy (TOF-SIMS) and show allowable impurity levels in view of superconducting cavity performance. Challenges and lessons learned in maintaining clean Nb$_3$Sn coatings are also discussed.

Tagdulang, Nikki [Fermilab]↗