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23 records · Page 2

Long-Term Dynamics of Atmospheric Sulfur Dioxide in Urban and Rural Regions of China: Urbanization and Policy Impacts

High levels of sulfur dioxide (SO 2 ) due to human activities pose a serious air pollution issue in China, especially in urban agglomerations. However, limited research has investigated the impact of anthropogenic emissions on higher SO 2 concentrations in urban regions compared to rural areas in China. Here, we analyzed the trends in SO 2 concentrations from 1980 to 2021 in China using the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) dataset. SO 2 column concentrations from the Copernicus Atmosphere Monitoring Service (CAMS) and the Ozone Monitoring Instrument (OMI) during the years 2007–2021 were also examined for validation and comparison purposes. Eight representative areas, including four urban regions (Pearl River Delta [PRD], Beijing-Tianjin-Hebei [BTH], Yangtze River Delta [YRD], and Sichuan Basin [SCB]) and four rural regions (Northeast Region [NER], Mongolian Region [MR], West Region [WR], and Tibetan Plateau Region [TR]) were selected for the analysis. Overall, a significant but fluctuating increase in SO 2 concentrations over China was observed during 1980–2021. During 1980–1997 and 2000–2010, there was an increase in SO 2 concentration, while during 1997–2000 and 2010–2021, a decreasing trend was observed. The average increase in SO 2 concentration was approximately 16 times higher in urban regions than in the rural background. We also found that SO 2 dynamics were highly associated with expansion of urban areas, population density, and gross domestic product. Nonetheless, since 2007, SO 2 concentrations have exhibited a downward trend, which is mainly attributed to the air pollution policies implemented by the Chinese government. Our findings highlight the need for further studies on the impact of SO 2 on regional climate change in China.

54 ENVIRONMENTAL SCIENCES↗

Uncertainty Quantification of Global Net Methane Emissions From Terrestrial Ecosystems Using a Mechanistically Based Biogeochemistry Model

Quantification of methane (CH4) emissions from wetlands and its sinks from uplands is still fraught with large uncertainties. Here, a methane biogeochemistry model was revised, parameterized, and verified for various wetland ecosystems across the globe. The model was then extrapolated to the global scale to quantify the uncertainty induced from four different types of uncertainty sources including parameterization, wetland type distribution, wetland area distribution, and meteorological input. We found that global wetland emissions are 212 ± 62 and 212 ± 32 Tg CH4 year -1 (1Tg = 10 12 g) due to uncertain parameters and wetland type distribution, respectively, during 2000–2012. Using two wetland distribution data sets and three sets of climate data, the model simulations indicated that the global wetland emissions range from 186 to 212 CH 4 year -1 for the same period. The parameters were the most significant uncertainty source. After combining the global methane consumption in the range of -34 to -46 Tg CH 4 year -1 , we estimated that the global net land methane emissions are 149–176 Tg CH 4 year -1 due to uncertain wetland distribution and meteorological input. Spatially, the northeast United States and Amazon were two hotspots of methane emission, while consumption hotspots were in the Eastern United States and eastern China. During 1950–2016, both wetland emissions and upland consumption increased during El Niño events and decreased during La Niña events. This study highlights the need for more in situ methane flux data, more accurate wetland type, and area distribution information to better constrain the model uncertainty.

58 GEOSCIENCES↗

Influence of the Kuroshio Intrusion on Deep Flow Intraseasonal Variability in the Northern South China Sea

Abstract Interactions between the open ocean and marginal seas have been suggested to be critical to the redistribution and dissipation of global energy. Here, we propose a mechanism for the upper open ocean influencing the deep flow in marginal seas that hinges on the formation and propagation of topographic Rossby waves (TRWs). Observations and high‐resolution simulations suggest substantial intraseasonal variability with periods of 5–60 days associated with the deep flow over continental slopes of the northern South China Sea (NSCS). These fluctuations generally account for over 40% of the total deep kinetic energy variability and the number can reach 70% over the slopes to the west of the Luzon Strait, southwest of the Dongsha Islands, and northeast of the Xisha Islands. By examining the spatiotemporal features of the fluctuations, we demonstrate that the intraseasonal variability of the deep flow in the NSCS is closely associated with TRWs. Using a recently developed multiscale energetics analysis in combination with a ray tracing model, we show that the energy sources of TRWs can be traced back to the east of the Dongsha Islands, where the Kuroshio intrusion and related eddies energize the TRWs primarily through pressure work. These waves propagate westward across the NSCS and drive the intraseasonal variability of the deep flow over continental slopes. Our findings highlight an energy pathway from the open ocean western boundary current to the abyssal marginal sea that could modulate regional circulation as well as exchanges between major ocean basins.

Quan, Qi↗

Impact of the mid-latitude zonal circulation on dynamic mechanism of anomalous precipitation over China in summer 2021

China was hit by extreme precipitation in July and August of 2021 along with significant monthly variation. The positive precipitation anomalies observed in July were mainly located in eastern China, but these anomalies shifted to the middle and lower reaches of the Yangtze River (MLYR) in August. In this study, we investigated the July and August precipitation anomaly dynamics based on the three-pattern decomposition of global atmospheric circulation (3P-DGAC) method. The results showed that the mid-latitude zonal circulation played a dominant role in July 2021, causing anomalous positive relative vorticity advection over the center of the positive precipitation anomalies, thus providing strong convective activity for the anomalous precipitation. Nevertheless, the August anomalies could be better explained from a climate perspective. The anomalous relative vorticity distribution patterns recorded in August were often accompanied by extreme precipitation in the MLYR, and the negative relative vorticity anomalies identified in Northeast Asia also played a crucial role. In conclusion, the mechanisms of precipitation anomalies in July and August 2021 were almost completely disparate. In this study, we emphasized the role of the mid-latitude zonal circulation in extreme precipitation events, and suggested that the impact of mid-latitude zonal circulation will be further accentuated under global warming.

54 ENVIRONMENTAL SCIENCES↗

Evaluation of regional transport of PM2.5 during severe atmospheric pollution episodes in the western Yangtze River Delta, China

During winter 2018, the 16 prefecture-level cities in Anhui Province, Western Yangtze River Delta region, China had very high PM2.5 concentrations and prolonged pollution days. The impact of regional transport in the formation, accumulation, as well as dispersion of fine particulate matter (PM2.5) in Anhui Province was very significant. This study quantified and analyzed the vertical transport of PM2.5 in three major cities (Hefei, Fuyang, and Suzhou) of Anhui Province in January and July 2018 using the Weather Research and Forecasting (WRF) model coupled with the Community Multiscale Air Quality (CMAQ) model. The results of the inter-regional transport of PM2.5 revealed the dominant transport pathways for the three cities. The flux mainly flowed into Fuyang from Henan (2.23 and 1.42 kt/day in January and July, respectively) and Bozhou (1.96 and 1.21 kt/day in January and July, respectively), while the main flux from Fuyang flowed into Henan (-2.15 kt/day) and Lu'an (-1.91 kt/day) in January and Henan (-0.34 kt/day) and Bozhou (-0.29 kt/day) in July. In addition, the dominant transport pathways and the heights at which they occurred were identified: the northwest-southeast and northeast-south pathways in both winter and summer at both lower (?300 m) and higher (=300 m) levels for Fuyang; the northwest-south and northeast-southwest pathways in winter (at both lower and upper levels) and northwest-east and northeast-southwest pathways in summer at lower and upper levels for Hefei; and the northwest-southeast and northeast-south pathways in both winter (from 50 m up to the top level) and summer (between 100 and 300 m) for Suzhou. Furthermore, the intensities of daily PM2.5 transport fluxes in Fuyang during the atmospheric pollution episode (APE1) were stronger than the monthly average. These results show that joint emission controls across multiple cities along the identified pathways are urgently needed to reduce winter episodes.

Sulaymon, Ishaq D.↗