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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2

Signal Processing of Multiplexed Optical PWM Signals for Sensor Arrays in Nuclear Environments

Safe and effective generation of terrestrial nuclear power greatly benefits from the actionable data provided by the array of sensors located throughout a plant to provide a holistic online indication of reactor operation. This array includes sensors for monitoring coolant flow and pressure, temperature and heat transfer, radiation levels, structure health monitoring, and other critical parameters for reactor operation. While sensors capable of measuring these parameters have been developed, the electronics used in the pre-amplification and analog-to-digital conversion of the small signals they produce are extremely sensitive and susceptible to damage by high-temperatures and radiation environments nuclear reactors encounter while generating power. The small signals from sensors in nuclear power plants (NPPs) are transmitted over long cable runs which introduce dispersion artifacts into the signals of interest as well as electromagnetic interference (EMI) from lighting fixtures, pumps, mains electricity, and other equipment. To overcome these challenges, a front-end digitization (FREND) platform has been developed to use radiation-tolerant electronics to multiplex, amplify, and optically encode signals from an array of sensors for transmission over an optical fiber to mitigate dispersion and EMI artifacts from long runs of electrical cabling. To recover the optically transmitted data, a signal processing scheme based on 1-dimensional template matching to an indexing channel is described herein and demonstrated to have an effective bit-depth of 9.2 bits (1%). This scheme has been validated in proof-of-concept, non-nuclear testing and preliminary experimental results show good agreement between the measured optical output and and sensor input signals. The FREND system represents a low-loss data link between sensors in nuclear environments and data acquisition hardware which is aimed at improving the signal-to-noise ratio of the data acquired from these sensors to provide better information to operators and researchers.

Sweeney, Dan↗

Thermodynamic Modeling of Complex Solid Solutions in the Lu-H-N System via Graph Neural Network Accelerated Monte Carlo Simulations

Metal hydrides are important across diverse applications, such as hydrogen storage, batteries, gas sensors, nuclear reactions, and high-temperature superconductivity. Previous computational studies of metal hydrides under extreme pressures, e.g., 𝑂⁡(10 2 ) ⁢GPa, usually treat them as stoichiometric compounds without considering interstitial lattice disorder. As pressures become more moderate in the 𝑂⁡(10 0 ) ⁢GPa and below range, hydrogen disorder at interstitial lattice sites becomes prominent, e.g., in the N-doped Lu hydride that was recently claimed superconducting near 1 GPa. Further adding compositional complexity from alloying and/or multielement interstitial occupation makes elucidating pressure- and temperature-dependent observables intractable by first-principles calculations alone. We therefore propose a lattice graph neural-network surrogate modeling approach to predict configuration- and pressure-dependent equation-of-state properties. Their efficiency permits Monte Carlo simulations to calculate Gibbs energies and pressure-dependent phase diagrams, thereby revealing insights into the synthesis conditions required for achieving desired phase equilibria. We demonstrate this concept for the compositionally complex cubic Lu(H,N,Va) 3 system where three constituents (hydrogen, nitrogen and vacancy) have disordered multielement interstitial occupancies and insights into pressure-dependent phase equilibria are critically needed, e.g., N-doping levels can significantly lower dehydrogenation temperatures and provide a new strategy to optimize hydrogen-storage alloys. This work can improve the thermodynamic understanding of the Lu-H-N system and help rational synthesis of N-doped Lu hydrides, but more generally demonstrates an efficient approach to model pressure-dependent thermodynamics of multicomponent solid solutions.

Monte Carlo methods↗

Testing piezoelectric sensors in a nuclear reactor environment

Several Department of Energy Office of Nuclear Energy (DOE-NE) programs, such as the Fuel Cycle Research and Development (FCRD), Advanced Reactor Concepts (ARC), Light Water Reactor Sustainability, and Next Generation Nuclear Power Plants (NGNP), are investigating new fuels, materials, and inspection paradigms for advanced and existing reactors. A key objective of such programs is to understand the performance of these fuels and materials during irradiation. In DOE-NE’s FCRD program, ultrasonic based technology was identified as a key approach that should be pursued to obtain the high-fidelity, high-accuracy data required to characterize the behavior and performance of new candidate fuels and structural materials during irradiation testing. The radiation, high temperatures, and pressure can limit the available tools and characterization methods. In this work piezoelectric transducers capable of making these measurements are developed. Specifically, three piezoelectric sensors (Bismuth Titanate, Aluminum Nitride, and Zinc Oxide) are tested in the Massachusetts Institute of Technology Research reactor to a fast neutron fluence of 8.65x1020 nf/cm2. It is demonstrated that Bismuth Titanate is capable of transduction up to 5 x1020 nf/cm2, Zinc Oxide is capable of transduction up to at least 6.27 x1020 nf/cm2 , and Aluminum Nitride is capable of transduction up to at least 8.65x x1020 nf/cm2.

T. Reinhardt, Brian↗

Presentation: Sensor Anomaly Detection for Nuclear Reactor Systems Utilizing Linear Regression and K-Means Unsupervised Machine Learning: An overview of methods and results

This presentation is a culmination of work which has occurred over the course of a 10-week internship. Anomaly detection methods must be both robust enough to detect subtle anomalies yet not so sensitive to report false positives, which would result significant loss of revenue. Methods currently being developed for autonomous systems are often pursuing a Digital Twin method, which will look at the entire system and model it as a whole. This presentation, however, focuses less on direct application to an NPP, rather acting as a proof of concept for the methods developed. For the project, we look to develop methods to analyze steady-state data and report anomalies.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Statistical and Neural Network for Real Sensor-Data-Driven Anomaly Detection in Nuclear Applications

Anomaly detection (AD) in sensor data is critical to ensure uninterrupted functionality of nuclear power plants (NPPs). Consequently, AD model validation through real-world sensor data is important for applications in nuclear facilities. In this paper, we propose an Autoencoder (AE)—a multi-layered neural network, for AD in sensor data from an operational NPP testbed. Since the dataset lacks labels for irregularities, we introduce random noise and label them to effectively train our model. The proposed AE model assigns a higher reconstruction error to the abnormal samples that deviate from those encountered during the training phase and uses the reconstruction loss to detect anomalies in a representative imbalanced dataset. We also introduce an analytical solution—seasonal trend decomposition (STD)—as another AD scheme for identifying irregularities withinthe same time-series dataset. In contrast to the AE model which relies on reconstruction loss, the STD scheme decomposes the entire dataset into its trend, seasonality, and residual components to pinpoint irregularities. Our findings indicate that the proposed AE and STD models individually achieve recall scores of 97% and 92%, respectively. We validate the performance of the two models on both balanced and imbalanced data. We further solidify the results by picking the combined selected anomalies of the two solutions with an "AND" operator for more reliable predictions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Statistical and Neural Network for Real Sensor-Data-Driven Anomaly Detection in Nuclear Applications

Anomaly detection (AD) in sensor data is critical to ensure uninterrupted functionality of nuclear power plants (NPPs). Consequently, validation of AD models through real-world sensor data is important for their application in nuclear facilities. In this paper, we propose an Autoencoder (AE)— a multi-layered neural network, for AD in sensor data from an operational NPP testbed. Since the dataset lacks labels for irregularities, we introduce random noise and label them to effectively train our model. The proposed AE model assigns a higher reconstruction error to the abnormal samples that deviate from those encountered during the training phase and uses the reconstruction loss to detect anomalies in a representative imbalanced dataset. We also introduce an analytical solution—seasonal trend decomposition (STD) — as another AD scheme for identifying irregularities within the same time-series dataset. In contrast to the AE model which relies on reconstruction loss, the STD scheme decomposes the entire dataset into its trend, seasonality, and residual components to pinpoint irregularities. Our findings indicate that the proposed AE and STD models individually achieve recall scores of 97% and 92%, respectively. We also validate the performance of the two models on both balanced and imbalanced data. We further solidify the results by picking the combined selected anomalies of the two solutions with an "AND" operator for more reliable predictions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Toward local core outlet temperature monitoring in gas-cooled nuclear reactors using distributed fiber-optic temperature sensors

Gas-cooled nuclear reactors operate at temperatures up to 950 °C with significant spatial variations in power generation and coolant flow through hundreds of parallel flow channels, resulting in complex mixing at the core outlet. The high temperatures and complex mixing can damage downstream components, challenge reactor calorimetry for power determination, and result in significant conservatism in calculated peak fuel temperatures, which ultimately limits the total power output. Directly measuring each gas stream individually is unrealistic using single point thermocouples, requiring more robust sensing techniques. Fiber-optic sensors are resilient to high temperatures (up to 1,000 °C) and radiation damage. Moreover, distributed measurements can be made along the length of one fiber, making them potential candidates for monitoring local core outlet temperatures to improve core calorimetry and identify hot channels. Here, to the authors’ knowledge, this manuscript is the first to report spatially distributed fiber optic temperature measurements to quantify mixing at the outlet of a relevant orifice plate under prototypic temperature and flow regimes to assess the feasibility of using fiber-optic sensors for distributed measurements of coolant temperature in gas-cooled reactors. A single optical fiber captured dynamic changes in local temperatures, whereas the mixed outlet temperature exhibited a muted response and could not identify which channels were responsible for the change in the mixed outlet temperature. The discussion focuses on potential challenges for deploying distributed optical fibers in gas-cooled reactors, including the effects of vibrations, radiation-induced signal attenuation and drift, and routing of the fiber while minimizing flow obstructions.

42 ENGINEERING↗

Sensor Anomaly Detection for Nuclear Reactor Systems Utilizing Linear Regression and K-Means Unsupervised Machine Learning

Nuclear reactors and related systems are becoming increasingly complex due to advancing technologies in next-generation power reactors. This increased complexity necessitates enhanced automation and data management capabilities. To successfully realize autonomous systems, methods must be developed to handle vast volumes of data and effectively distinguish anomalous data from noise and expected data. While impressive models utilizing digital twins and similar approaches are under development, here we propose a simplified model for analyzing fundamental methods and techniques. Initially, we created a general dataset by using initial data from PCTRAN in order to represent ideal steady-state conditions. We then inserted anomalies based on prevalent sensor anomaly types (e.g., point anomalies, linear drift, and downward deviations), along with unusual anomalies such as exponential drift and upward deviations. To detect anomalies, we developed a program that employs data partitioning and linear regression to preprocess and filter the anomalous data. A K-Means machine learning (ML) method was then applied to separate and count the data within the anomalous partition. The results from all datasets—apart from exponential growth—demonstrated positive outcomes, with each returning multiple instances of greaterthan-95% accuracy. We conducted further investigations using Idaho National Laboratory’s RAVEN software to perform a sensitivity analysis on the input variables (R 2 Tolerance, Slope Tolerance, and Window Size) and found that the output variables (Accuracy and Time) were most sensitive to the Window Size. Despite the promising results published, further development is required to effectively apply these methods to nuclear systems. Nevertheless, the strengths of this approach are evident and hold promise for future applications in the field.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Wireless Sensor Modalities at a Nuclear Plant Site to Collect Vibration Data

One of the major contributors to the total operating costs of domestic nuclear fleet of reactors today is the operation and maintenance (O&M) costs. These include labor-intense preventive maintenance programs involving manually-performed inspection, calibration, testing, and maintenance of plant assets at periodic frequency and time-based replacement of assets at periodic frequency, irrespective of their conditions. This has resulted in a labor-centric business model to achieve high capacity factors. To build an optimal maintenance program, it’s time to transition from this labor-centric business model to a technology-centric business model. Fortunately, there are technologies (advanced sensor, data analytics, and risk assessment methodologies) that will support this transition. The technology-centric business model will result in significant plant life extension and reduction of time-based maintenance activities. This will drive down O&M costs as labor is a rising cost and technology is a declining cost. This approach will lay the foundation for real-time condition assessment of plant assets, allowing condition-based maintenance to enhance plant safety, reliability, and economics of operation. The goal of this project is to address challenges in the area of digital monitoring, i.e., the application of advanced sensor technologies (particularly wireless sensor technologies) and science-based data analytic capabilities to advance online monitoring and predictive maintenance in nuclear plants to improve plant performance (efficiency gain and economic competitiveness). To achieve the project goal, in partnership with Exelon Generating Company (Exelon), researchers from Idaho National Laboratory (INL) and Oak Ridge National Laboratory (ORNL) are performing research and development (R&D) to demonstrate application of wireless sensors using the distributed antenna system and advanced data analytics to achieve predictive maintenance. In the report, wireless vibration sensors, vibration data and its indicator are described. The wireless vibration sensors presented in this report support three types of wireless communication, namely, Wi-Fi, cellular, and 900 MHz. These wireless vibration sensors are considered by partner plant site for installation on plant asset to enable online vibration monitoring to replace periodic measurements. These vibration data along with other plant process data will be utilized to develop diagnostic and prognostic models.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Precision spectroscopy of nuclear decays using quantum optomechanical sensors

This project developed and demonstrated a fundamentally new way to detect individual nuclear decays: rather than capturing the energy that decay products deposit in a detector, we measure the tiny mechanical recoil of the entire micron- or nanometer-sized particle in which the decaying nucleus is embedded. Because momentum is conserved, this approach is sensitive even to neutral, weakly interacting particles, including neutrinos, that escape conventional detectors. During the award, the Yale group reported the first-ever mechanical detection of single nuclear decays, a result featured widely in the scientific press, and pushed the sensitivity of smaller levitated nanoparticles into the quantum measurement regime, reaching an impulse resolution within a factor of five of the fundamental Standard Quantum Limit (SQL), good enough in principle to detect the momentum kicked to the particle by a single emitted neutrino. In parallel, the LBNL group developed the theory of quantum-enhanced (sub-SQL) readout tailored to this experiment, showing how squeezed light can push the sensitivity below the SQL. Together these results establish levitated optomechanical sensors as a new tool for precision nuclear decay spectroscopy, with further applications in neutrino physics, quantum metrology, and nuclear forensics and safeguards.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Comparing Sensor Fusion and Multimodal Chemometric Models for Monitoring U(VI) in Complex Environments Representative of Irradiated Nuclear Fuel

Optical sensors and chemometric models were leveraged for the quantification of uranium(VI) (0–100 μg mL –1 ), europium (0–150 μg mL –1 ), samarium (0–250 μg mL –1 ), praseodymium (0–350 μg mL –1 ), neodymium (0–1000 μg mL –1 ), and HNO 3 (2–4 M) with varying corrosion product (iron, nickel, and chromium) levels using laser fluorescence, Raman scattering, and ultraviolet–visible–near-infrared absorption spectra. In this paper, an efficient approach to developing and evaluating tens of thousands of partial least-squares regression (PLSR) models, built from fused optical spectra or multimodal acquisitions, is discussed. Each PLSR model was optimized with unique preprocessing combinations, and features were selected using genetic algorithm filters. The 7-factor D-optimal design training set contained just 55 samples to minimize the number of samples. The performance of PLSR models was evaluated by using an automated latent variable selection script. PLS1 regression models tailored to each species outperformed a global PLS2 model. PLS1 models built using fused spectra data and a multimodal (i.e., analyzed separately) approach yielded similar information, resulting in percent root-mean-square error of prediction values of 0.9–5.7% for the seven factors. Further, the optical techniques and data processing strategies established in this study allow for the direct analysis of numerous species without measuring luminescence lifetimes or relying on a standard addition approach, making it optimal for near-real-time, in situ measurements. Nuclear reactor modeling helped bound training set conditions and identified elemental ratios of lanthanide fission products to characterize the burnup of irradiated nuclear fuel. Leveraging fluorescence, spectrophotometry, experimental design, and chemometrics can enable the remote quantification and characterization of complex systems with numerous species, monitor system performance, help identify the source of materials, and enable rapid high-throughput experiments in a variety of industrial processes and fundamental studies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Estimation of sensor measurement errors in reactor coolant systems using multi-sensor fusion

A nuclear power plant is typically instrumented with a variety of sensors to continually monitor its variables, and their sensor’s measurements may be used to assess the plant state and initiate safety actions, if needed. Errors in sensor measurements, due to factors such as calibration drifts, critically affect such state assessments. Here, we address a problem of estimating sensor errors using physics-informed machine learning methods that use measurements collected under known plant conditions. For a given sensor, we propose an information fusion method that uses measurements from other sensors to estimate its output assuming it is error-free and provides its difference from an actual measurement as an error estimate. We present the ensemble of trees and support vector machine fusers, and evaluate their performance using measurements collected over an emulated test loop of a pressurized water reactor. The plant variables are related to each other through the underlying physical laws under inertial constraints that place bounds on their derivatives, which analytically justify the applicability of machine learning methods for computing these fusers. Under twenty scenarios, we assess their sensor error estimates for pressure sensors of the heat exchanger of a reactor’s primary coolant system. Multiple types of errors are captured by both fusers under externally induced calibration drifts, blockages, minor leaks and air gaps in sensing lines, and electromagnetic interference; the root mean square error of the estimation of error is under 2.2% percent of the maximum measurement. We present generalization equations, in the framework of statistical learning theory, for these methods that characterize the confidence probability that the estimation error is bounded by a specified parameter in future test scenarios.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Additive Manufacturing of Miniaturized Peak Temperature Monitors for In-Pile Applications

Passive monitoring techniques have been used for peak temperature measurements during irradiation tests by exploiting the melting point of well-characterized materials. Recent efforts to expand the capabilities of such peak temperature detection instrumentation include the development and testing of additively manufactured (AM) melt wires. In an effort to demonstrate and benchmark the performance and reliability of AM melt wires, we conducted a study to compare prototypical standard melt wires to an AM melt wire capsule, composed of printed aluminum, zinc, and tin melt wires. The lowest melting-point material used was Sn, with a melting point of approximately 230 °C, Zn melts at approximately 420 °C, and the high melting-point material was aluminum, with an approximate melting point of 660 °C. Through differential scanning calorimetry and furnace testing we show that the performance of our AM melt wire capsule was consistent with that of the standard melt-wire capsule, highlighting a path towards miniaturized peak-temperature sensors for in-pile sensor applications.

36 MATERIALS SCIENCE↗