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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS2018

Retrieval of H2O Abundance in Titan's Stratosphere: A (Re)Analysis of CIRS/Cassini and PACS/Herschel Observations

Since its first measurement 20 years ago by the Infrared Space Observatory (ISO), the water (H2O) mole fraction in Titan’s stratosphere remains uncertain due to large differences between the determinations from available measurements. More particularly, the recent measurements made from the Herschel observatory (PACS (Photodetector Array Camera and Spectrometer) and HIFI (Heterodyne Instrument for the Far Infrared)) estimated the H2O mole fraction to be 0.023 parts per billion at 12.1 millibars. A mixing ratio of 0.14 parts per billion at 10.7 millibars was, however, retrieved from nadir spatially-resolved observations of Cassini/CIRS (Composite Infrared Spectrometer). At the same pressure level (10.7 millibars), this makes a difference of a factor of 5.5 between PACS and CIRS measurements, and this has notably prevented current models from fully constraining the oxygen flux flowing into Titan’s atmosphere. In this work, we try to understand the differences between the H2O mole fractions estimated from Herschel/PACS and Cassini/CIRS observations. The strategy for this is to 1) analyse recent disc-averaged observations of CIRS to investigate if the observation geometry could explain the previous observed differences, and 2) (re)analyse the three types of observation with the same retrieval scheme to assess if previous differences in retrieval codes/methodology could be responsible for the previous discrepancies. With this analysis, we show that using the same retrieval method better reconcile the previous measurements of these instruments. However, the addition of the disc-averaged CIRS observations, instead of confirming the consistency between the different datasets, reveals discrepancies between one of the CIRS disc-averaged set of observations and PACS measurements. This raises new questions regarding the possibility of latitudinal variations of H2O, which could be triggered by seasonal changes of the meridional circulation. As it has already been shown for nitriles and hydrocarbons, this circulation could potentially impact the latitudinal distribution of H2O through the subsidence or up- welling of air rich in H2O. The possible influence of spatial/time variations of the OH/H2O input flux in Titan’s atmosphere is also discussed. The analysis of more observations will be needed in future work to address the questions arising from this work and to improve the understanding of the sources of H2O in Titan’s atmosphere.

Bauduin, S.↗
NASA NTRS1976

Planetary spectra for anisotropic scattering

Some effects on planetary spectra that would be produced by departures from isotropic scattering are examined. The phase function is the simplest departure to handle analytically and the only phase function, other than the isotropic one, that can be incorporated into a Chandrasekhar first approximation. This approach has the advantage of illustrating effects resulting from anisotropies while retaining the simplicity that yields analytic solutions. The curve of growth is the sine qua non of planetary spectroscopy. The discussion emphasizes the difficulties and importance of ascertaining curves of growth as functions of observing geometry. A plea is made to observers to analyze their empirical curves of growth, whenever it seems feasible, in terms of coefficients of which are the leading terms in radiative-transfer analysis. An algebraic solution to the two sets of anisotropic H functions is developed which gives emergent intensities accurate to 0.3%.

Chamberlain, J. W.↗
NASA NTRS2016

SPICE Tools Supporting Planetary Remote Sensing

NASA's "SPICE" ancillary information system has gradually become the de facto international standard for providing scientists the fundamental observation geometry needed to perform photogrammetry, map making and other kinds of planetary science data analysis. SPICE provides position and orientation ephemerides of both the robotic spacecraft and the target body; target body size and shape data; instrument mounting alignment and field-of-view geometry; reference frame specifications; and underlying time system conversions.

Observation geometry↗
NASA NTRS2017

Angular Normalization of GOME-2 Sun-Induced Chlorophyll Fluorescence Observation as a Better Proxy of Vegetation Productivity

Sun-induced chlorophyll fluorescence (SIF) has been regarded as a promising proxy for gross primary productivity (GPP) over land. Considerable uncertainties in GPP estimation using remotely sensed SIF exist due to variations in the Sun-satellite view observation geometry that could induce unwanted variations in SIF observation. In this study, we normalize the far-red Global Ozone Monitoring Experiment-2 SIF observations on sunny days to hot spot direction (SIF(h)) to represent sunlit leaves and compute a weighted sum of SIF (SIF(t)) from sunlit and shaded leaves to represent the canopy. We found that SIF(h) is better correlated with sunlit GPP simulated by a process-based ecosystem model and SIF(t) is better correlated with the simulated total GPP than the original SIF observations. The coefficient of determination (R(exp 2)) are increased by 0.04 +/- 0.03, and 0.07 +/- 0.04 on a global average using SIF(h) and SIF(t), respectively. The most significant increases of the R(exp 2) (0.09 +/- 0.04 for SIF(t) and 0.05 +/- 0.03 for SIF(h)) appear in deciduous broadleaf forests.

Australia↗
NASA NTRS1997

Pair Production and Gamma-Ray Emission in the Outer Magnetospheres of Rapidly Spinning Young Pulsars

Electron-positron pair production and acceleration in the outer magnetosphere may be crucial for a young rapidly spinning canonical pulsar to be a strong Gamma-ray emitter. Collision between curvature radiated GeV photons and soft X-ray photons seems to be the only efficient pair production mechanism. For Crib-like pulsars, the magnetic field near the light cylinder is so strong, such that the synchrotron radiation of secondary pairs will be in the needed X-ray range. However, for majority of the known Gamma-ray pulsars, surface emitted X-rays seem to work as the matches and fuels for a gamma-ray generation fireball in the outer magnetosphere. The needed X-rays could come from thermal emission of a cooling neutron star or could be the heat generated by bombardment of the polar cap by energetic particles generated in the outer magnetosphere. With detection of more Gamma-ray pulsars, it is becoming evident that the neutron star's intrisic geometry (the inclination angle between the rotation and magnetic axes) and observational geometry (the viewing angle with respect to the rotation axis) are crucial to the understanding of varieties of observational properties exhibited by these pulsars. Inclination angles for many known high energy Gamma-ray pulsars appear to be large and the distribution seems to be consistent with random orientation. However, all of them except Geminga are pre-selected from known radio pulsars. The viewing angles are thus limited to be around the respective inclination angles for beamed radio emission, which may induce strong selection effect. The viewing angles as well as the inclination angles of PSR 1509-58 and PSB 0656+14 may be small such that most of the high energy Gamma-rays produced in the outer accelerators may not reach the observer's direction. The observed Gamma-rays below 5 MeV from this pulsar may be synchrotron radiation of secondary electron-positron pairs produced outside the accelerating regions.

Ruderman, Malvin↗
NASA NTRS1986

Application of the Baseline Rotonet system to the prediction of helicopter tone noise

The capabilities of the baseline Rotonet system designed to predict helicopter noise are analyzed. The modules of the system utilized for main and tail rotor geometry and blade section aerodynamic characteristics, for analyses, and for source-to-observer geometry, and atmospheric and ground effects calculations are described; a diagram of the system is provided. The Rotonet system produces axial force, tone noise, and sound pressure level information and a one third octave spectrum related to rotor tone noise and broadband noise sources. Main rotor noise predictions are compared with flight data. It is observed that both sets of data reveal increase loading on the advancing side and decrease loading on the retreating side. The tone noise and sound pressure levels for the first and second harmonics correlate well with the flight data; however, there is only fair agreement for the third harmonics of the sound pressure level. Analysis of the spectra display lower noise levels for higher altitudes and lower speeds. It is noted that the baseline Rotonet system is applicable for predicting performance and noise signatures for the lower harmonics. A phase II Rotonet system for evaluating higher harmonics is being developed.

Golub, R. A.↗
NASA NTRS1998

F/NAS/ Pressure Temperature Retrieval Techniques

The purpose of this investigation is to study methods and ways for rapid inversion programs involving the correlated k-method, and to modify the existing programs so that the rapid analysis of data can be accomplished. The earth's atmosphere as well as those around the planets consist of gases which emit radiation in the infrared spectral region, providing wealth of information about chemical and physical processes in the atmosphere. The atmospheric molecular constituents absorb and radiate by vibrational and rotational transitions, and the observed spectra exhibit characteristic spectral features in the region of the electromagnetic spectrum. The observed absorption or thermal emission spectra may be obtained with space-borne high resolution infrared spectrometers the 50-1000 micrometers spectral region. A detailed analysis of the observed spectra leads to information about the atmospheric thermal structure, composition, and the physical and chemical processes. The analytic techniques involve the development of radiative transfer models for the calculation of the observed radiance and transmittances for realistic atmospheric conditions and observational geometries, and the development of inversion methods for retrieval of atmospheric parameters from the observations.

Poularikas, Alexander↗
NASA NTRS1979

Simultaneous H/1216 A/ and He/584 A/ observations of the interstellar wind by Mariner 10

In late 1973 and early 1974 the Mariner 10 spacecraft performed four roll calibration maneuvers (RCM). The Ultraviolet Spectrometer (UVS) measured the intensity of both He(584 A) and H(1216 A) emissions from interplanetary gas. The data and the observational geometry have been described by Broadfoot and Kumar (1978). Analysis of these 4 sets of observations is extremely important since they are the first simultaneous intensity measurements of H and He emissions free of geocoronal contamination to be recorded in one day, thus precluding significant variations in the solar fluxes.

Ajello, J. M.↗
NASA NTRS1995

The 16-45 micron observations of the Galactic Center

Existing observations of the Galactic Center at infrared and radio wavelengths challenge our understanding of the detailed morphology and energy balance of the inner few parsec, including the Galactic Center and the infrared torus. The distribution and nature of the sources heating this region are still not well understood; existing determinations of dust temperature and ionization do not provide us with consistent pictures of the relative important of the central source and the embedded stars in this dusty region. The composite IR emission of the Galactic Center can be crudely divided into three categories: (1) hot dust heated directly by an incident UV field along the inner region of the Galactic Center torus; (2) warm dust heated by te non-ionizing radiation of the embedded stars and re-radiated NIR dust emission; (3) cooler absorbing dust located along the galactic line of sight. The apparent inconsistencies between the observations and theoretical expectations may stem from the interplay of various physical process and source-cloud geometries. Observations with increased spatial and spectral resolution are clearly needed to provide the information necessary to address the various problems. Therefore, we made 15-45 micron spectrophotometric observations of the inner 80 min (3 pc) regions surrounding the Galactic Center with the 20 min aperture of Goddard Cryogenic Grating Spectrometer No. 2 in May 1994 from the KAO. We measured nine points, including the 50 and 90 micron peaks of Davidson et al. and points between them and SgrA,. The wavelength coverage of our instrument ensures sensitivity to the hot dust component, silicate emission and/or absorption features, and cooler dust at longer wavelengths. Our observations will be used to set limits on the luminosity of any central sources, or give an independent estimate of central luminosity, and to set limits on the range of acceptable dust parameters for this region.

Chan, Kin-Wing↗
NASA NTRS1984

Vibrational and rotational excitation of CO in comets. Part 1: Non-equilibrium calculations. Part 2: Results of the calculation for standard bright comet, comet Iras-Araki-Alcock and comet Halley

The vibrational and rotational excitation of the CO molecule in cometary comae were investigated using a model which includes IR vibrational pumping by the solar flux, vibrational and rotational radiative decay, and collisional coupling among rotational states. Steady state was not assumed in solving the rate equations. The evolution of a shell of CO gas was monitored as it expanded from the nucleus into the outer coma. Collisional effects were treated using a kinetic temperature profile derived from theoretical work on the coma energy balance. The kinetic temperature was assumed to be extremely cold in the inner coma; this has significant consequences for the CO excitation. If optical depth effects are ignored, only low J transitions will be significantly excited in comets observed at high spatial resolution. Ground-based observations of CO co-vibrational and rotational transitions will be extremely difficult due to lack of sensitivity and/or terrestrial absorption. However, CO should be detectable from a large comet with favorable observing geometry if the CO is a parent molecule present at the 10% level (or greater) relative to H2O. Observations using cooled, spaceborne instruments should be capable of detecting CO emission from even moderately bright comets.

Chin, G.↗
NASA NTRS2017

Effects of Surface BRDF on the OMI Cloud and NO2 Retrievals: A New Approach Based on Geometry-Dependent Lambertian Equivalent Reflectivity (GLER) Derived from MODIS

The Ozone Monitoring Instrument (OMI) cloud and NO2 algorithms use a monthly gridded surface reflectivity climatology that does not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (GLER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. GLER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from MODIS over land and the Cox Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare GLER and climatological LER at 466 nm, which is used in the OMI O2-O2cloud algorithm to derive effective cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and GLERs is carried out. GLER and corresponding retrieved cloud products are then used as input to the OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with GLERs can increase NO2 vertical columns by up to 50 % in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

MODIS BRDF OMI clouds NO2 GLER↗
NASA NTRS2016

Consistent Evaluation of ACOS-GOSAT, BESD-SCIAMACHY, CarbonTracker, and MACC Through Comparisons to TCCON

Consistent validation of satellite CO2 estimates is a prerequisite for using multiple satellite CO2 measurements for joint flux inversion, and for establishing an accurate long-term atmospheric CO2 data record. Harmonizing satellite CO2 measurements is particularly important since the differences in instruments, observing geometries, sampling strategies, etc. imbue different measurement characteristics in the various satellite CO2 data products. We focus on validating model and satellite observation attributes that impact flux estimates and CO2 assimilation, including accurate error estimates, correlated and random errors, overall biases, biases by season and latitude, the impact of coincidence criteria, validation of seasonal cycle phase and amplitude, yearly growth, and daily variability. We evaluate dry-air mole fraction (X(sub CO2)) for Greenhouse gases Observing SATellite (GOSAT) (Atmospheric CO2 Observations from Space, ACOS b3.5) and SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) (Bremen Optimal Estimation DOAS, BESD v2.00.08) as well as the CarbonTracker (CT2013b) simulated CO2 mole fraction fields and the Monitoring Atmospheric Composition and Climate (MACC) CO2 inversion system (v13.1) and compare these to Total Carbon Column Observing Network (TCCON) observations (GGG2012/2014). We find standard deviations of 0.9, 0.9, 1.7, and 2.1 parts per million vs. TCCON for CT2013b, MACC, GOSAT, and SCIAMACHY, respectively, with the single observation errors 1.9 and 0.9 times the predicted errors for GOSAT and SCIAMACHY, respectively. We quantify how satellite error drops with data averaging by interpreting according to (error(sup 2) equals a(sup 2) plus b(sup 2) divided by n (with n being the number of observations averaged, a the systematic (correlated) errors, and b the random (uncorrelated) errors). a and b are estimated by satellites, coincidence criteria, and hemisphere. Biases at individual stations have year-to-year variability of 0.3 parts per million, with biases larger than the TCCON predicted bias uncertainty of 0.4 parts per million at many stations. We find that GOSAT and CT2013b under-predict the seasonal cycle amplitude in the Northern Hemisphere (NH) between 46 and 53 degrees North latitude, MACC over-predicts between 26 and 37 degrees North latitude, and CT2013b under-predicts the seasonal cycle amplitude in the Southern Hemisphere (SH). The seasonal cycle phase indicates whether a data set or model lags another data set in time. We find that the GOSAT measurements improve the seasonal cycle phase substantially over the prior while SCIAMACHY measurements improve the phase significantly for just two of seven sites. The models reproduce the measured seasonal cycle phase well except for at Lauder_125HR (CT2013b) and Darwin (MACC). We compare the variability within 1 day between TCCON and models in June-July-August; there is correlation between 0.2 and 0.8 in the NH, with models showing 10-50 percent the variability of TCCON at different stations and CT2013b showing more variability than MACC. This paper highlights findings that provide inputs to estimate flux errors in model assimilations, and places where models and satellites need further investigation, e.g., the SH for models and 45-67 degrees North latitude for GOSAT and CT2013b.

ACOS-GOSAT↗
NASA NTRS1996

Analysis of Cumulus Solar Irradiance Reflectance (CSIR) Events

Clouds are extremely important with regard to the transfer of solar radiation at the earth's surface. This study investigates Cumulus Solar Irradiance Reflection (CSIR) using ground-based pyranometers. CSIR events are short-term increases in solar radiation observed at the surface as a result of reflection off the sides of convective clouds. When sun-cloud observer geometry is favorable, these occurrences produce characteristic spikes in the pyranometer traces and solar irradiance values may exceed expected clear-sky values. Ultraviolet CSIR events were investigated during the summer of 1995 using Yankee Environmental Systems UVA-1 and UVB-1 pyranometers. Observed data were compared to clear-sky curves which were generated using a third degree polynomial best-fit line technique. Periods during which the observed data exceeded this clear-sky curve were identified as CSIR events. The magnitude of a CSIR event was determined by two different quantitative calculations. The MAC (magnitude above clear-sky) is an absolute measure of the difference between the observed and clear-sky irradiances. Maximum MAC values of 3.4 Wm(exp -2) and 0.069 Wm(exp -2) were observed at the UV-A and UV-B wavelengths, respectively. The second calculation determined the percentage above clear-sky (PAC) which indicated the relative magnitude of a CSIR event. Maximum UV-A and UV-B PAC magnitudes of 10.1% and 7.8%, respectively, were observed during the study. Also of interest was the duration of the CSIR events which is a function of sun-cloud-sensor geometry and the speed of cloud propagation over the measuring site. In both the UV-A and UV-B wavelengths, significant CSIR durations of up to 30 minutes were observed.

Laird, John L.↗
NASA NTRS2017

Absence of a Detectable Lunar Nanodust Exosphere During a Search with LRO's LAMP UV Imaging Spectrograph

The Lyman-Alpha Mapping Project (LAMP) UV spectrograph on board the Lunar Reconnaissance Orbiter (LRO) performed a campaign to observe the Moon's nanodust exosphere, evidence for which was provided by the Lunar Atmosphere and Dust Environment Explorer (LADEE) Ultraviolet and Visible Spectrometer (UVS) during the 2014 Quadrantid meteoroid stream. These LADEE/UVS observations were consistent with a nanodust exosphere modulated by meteoroid impacts. LRO performed off-nadir maneuvers around the peak of the 2016 Quadrantids, in order to reproduce, as closely as possible, the active meteoroid environment and observing geometry of LADEE/UVS. We analyzed LAMP spectra to search for sunlight backscattering from nanodust. No brightness enhancement attributable to dust, of any size, was observed. We determine an upper limit for dust column concentration of ~10(^ 5) sq. cm for grains of radius ~25 nm, and an upper limit for dust column mass of ~10 11 g sq. cm, nearly independent of grain size for radii <100 nm.

Spectrograph↗
NASA NTRS1985

Convective Oscillations at Crystal/Melt Interface

Oscillatory instability in shape of solid/liquid interface geometry observed in heat-transfer experiments in long, thin vertical cylinder filled with succinonitrile. Novel fluid flow configuration with cylindrical symmetry developed to permit detailed heat flow experiments in geometry also mathematically tractable.

Glicksman, M.↗
NASA NTRS2017

Cloud and Sun-Glint Statistics Derived from GOES and MODIS Observations Over the Intra-Americas Sea for GEO-CAPE Mission Planning

Knowledge of cloud cover, frequency, and duration is not only important to study cloud dynamics, but also critical in determining when and where to take ocean measurements from geostationary orbits such as the Geostationary Coastal and Air Pollution Events (GEO-CAPE) mission due to the challenges in achieving complete hemispheric coverage of coastal oceans, estuaries, and inland waters at hourly frequency. Using GOES hourly measurements at 4 km nadir resolution between 2006 and 2011, the number of cloud-free hourly observations per day (N(sub cf)) for solar zenith angle Theta(sub 0) less than 80 degrees was estimated for each 0.1 degree location of the Intra-Americas Sea. The number of Sun-glint-affected hourly observations per day [Ns(sub sg)] was also calculated based on the planned GEO-CAPE observation geometry and realistic wind speed. High-latitude and equatorial oceans showed the lowest N(sub cf) (less than 2.4) in all climatological months, and highest N(sub cf) was observed in the Gulf of Mexico (GoM) and Caribbean (greater than 4.5). Different regions showed differences in seasonality of cloud-free conditions and also showed differences in the hour of a day at which the satellite observations would have the maximal cloud-free and glint-free probability (Temperature maximum). Cloud cover from Moderate Resolution Imaging Spectroradiometer (MODIS) 1 km measurements are greater than 10 degrees higher than those from the MODIS 250 m measurements, supporting ocean color missions at subkilometer resolutions to enhance both spatial coverage and temporal frequency. These findings provide valuable information for GEO-CAPE mission planning to maximize its science value through minimizing the impacts of clouds and Sun glint.

Feng, Lian↗
NASA NTRS1993

Observation of pressure ridges in SAR images of sea ice: Scattering theory and comparison with observations

Ridges and keels (hummocks and bummocks) in sea ice flows are important in sea ice research for both scientific and practical reasons. Sea ice movement and deformation is driven by internal and external stresses on the ice. Ridges and keels play important roles in both cases because they determine the external wind and current stresses via drag coefficients. For example, the drag coefficient over sea ice can vary by a factor of several depending on the fluid mechanical roughness length of the surface. This roughness length is thought to be strongly dependent on the ridge structures present. Thus, variations in ridge and keel structure can cause gradients in external stresses which must be balanced by internal stresses and possibly fracture of the ice. Ridging in sea ice is also a sign of fracture. In a practical sense, large ridges form the biggest impediment to surface travel over the ice or penetration through sea ice by ice-strengthened ships. Ridges also play an important role in the damage caused by sea ice to off-shore structures. Hence, observation and measurement of sea ice ridges is an important component of sea ice remote sensing. The research reported here builds on previous work, estimating the characteristics of ridges and leads in sea ice from SAR images. Our objective is to develop methods for quantitative measurement of sea ice ridges from SAR images. To make further progress, in particular, to estimate ridge height, a scattering model for ridges is needed. Our research approach for a ridge scattering model begins with a survey of the geometrical properties of ridges and a comparison with the characteristics of the surrounding ice. For this purpose we have used airborne optical laser (AOL) data collected during the 1987 Greenland Sea Experiment. These data were used to generate a spatial wavenumber spectrum for height variance for a typical ridge - the typical ridge is the average over 10 large ridges. Our first-order model radar scattering includes both the quasi-specular and Bragg resonant scatter mechanisms. This model is extended to include contributions from volume scatter and scatter from discrete objects. Geometrical characteristics from the AOL survey and model calculations imply that for radar wavelengths and observation geometries that are dominated by the quasi-specular scattering mechanism radar backscatter from a ridge is a measure of peak ridge height. We present scattering model results and compare them with ridges observed during the LEADEX experiment of March-April 1992 when both X, C, and L-band aircraft SAR and the ERS-1 satellite SAR observed a region in the Beaufort Sea near 86 deg N, 10 deg W. Data were also collected documenting ridge characteristics on the surface. The surface data are used to generate a SAR signature via the scattering model described above. The predicted SAR signatures compare well with the SAR observations.

Vesecky, J. F.↗
NASA NTRS2017

Accounting for the Effects of Surface BRDF on Satellite Cloud and Trace-Gas Retrievals: A New Approach Based on Geometry-Dependent Lambertian-Equivalent Reflectivity Applied to OMI Algorithms

Most satellite nadir ultraviolet and visible cloud, aerosol, and trace-gas algorithms make use of climatological surface reflectivity databases. For example, cloud and NO2 retrievals for the Ozone Monitoring Instrument (OMI) use monthly gridded surface reflectivity climatologies that do not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun-sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (LER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. The geometry-dependent LER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from the Moderate Resolution Imaging Spectroradiometer (MODIS) over land and the Cox-Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare the geometry-dependent and climatological LERs for two wavelengths, 354 and 466 nm, that are used in OMI cloud algorithms to derive cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and geometry-dependent LERs is carried out. Geometry-dependent LER and corresponding retrieved cloud products are then used as inputs to our OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with geometry-dependent LERs can increase NO2 vertical columns by up to 50% in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

Lambert-equivalent reflectivity↗