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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
NASA NTRS2004

Nitric Acid Uptake on Subtropical Cirrus Cloud Particles

The redistribution of HNO3 via uptake and sedimentation by cirrus cloud particles is considered an important term in the upper tropospheric budget of reactive nitrogen. Numerous cirrus cloud encounters by the NASA WB-57F high-altitude research aircraft during the Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) were accompanied by the observation of condensed-phase HNO3 with the NOAA chemical ionization mass spectrometer. The instrument measures HNO3 with two independent channels of detection connected to separate forward and downward facing inlets that allow a determination of the amount of HNO3 condensed on ice particles. Subtropical cirrus clouds, as indicated by the presence of ice particles, were observed coincident with condensed-phase HNO3 at temperatures of 197-224 K and pressures of 122-224 hPa. Maximum levels of condensed-phase HNO3 approached the gas-phase equivalent of 0.8 ppbv. Ice particle surface coverages as high as 1.4 # 10(exp 14) molecules/ square cm were observed. A dissociative Langmuir adsorption model, when using an empirically derived HNO3 adsorption enthalpy of -11.0 kcal/mol, effectively describes the observed molecular coverages to within a factor of 5. The percentage of total HNO3 in the condensed phase ranged from near zero to 100% in the observed cirrus clouds. With volume-weighted mean particle diameters up to 700 ?m and particle fall velocities up to 10 m/s, some observed clouds have significant potential to redistribute HNO3 in the upper troposphere.

Popp, P. J.↗
NASA NTRS2019

Seasonal Variation in Martian Water Ice Cloud Particle Size

We employ the complete record of Mars limb-viewing observations by the Compact Reconnaissance Imaging Spectrometer, totaling 922 successful retrievals, to chart the seasonal variation in water ice cloud particle size. Low-latitude clouds exhibit particle size sorting with altitude at all seasons, with particles ranging from >3.0 m in effective radius to 1.01.5 m. However, at a given altitude, the ice particle size often varies through the year. Ice particle sizes in the tropics follow a different seasonal cycle than ice mixing ratio. North polar clouds have a complex seasonal cycle, with a sloped size profile with altitude as the polar hood cloud forms in early fall trending to a roughly uniform 1.5 m profile by the end of winter. These data are an important metric to validate and improve general circulation model microphysical routines and to better understand how martian water ice clouds influence the atmospheric radiative budget.

Scott D. Guzewich↗
NASA NTRS2019

The New NASA Ames Infrared Optical Constant Facility. Determinations for Titan Aerosol-, and Exoplanet and Brown Dwarf Cloud Particle Analogs

Here we present a new optical constant facility developed at NASA Ames that will allow the determination of optical constants in the infrared of various materials, analogs of hazes and cloud particles in (exo)planet atmospheres and brown dwarfs. Our facility is composed of a Fourier Transform Infrared (FTIR) spectrometer continuously covering the Near-IR, mid-IR and Far-IR range (from 0.74 to 200 µm), coupled to variable angle transmittance and reflectance accessories that allow the characterization of the scattering properties of nonhomogeneous samples (laboratory planetary aerosol analogs, films, slabs of material, crystals, powders...) over a wide incidence and emittance angle range (0-90 degrees). This permits the angular light distribution in both transmission and reflection measurements to be characterized, enabling the determination of the complex indices of refraction, n and k, over the full NIR-FIR range via modeling of the laboratory observations. The resulting refractive indices are critical input parameters in radiative transfer models, exoplanet and brown dwarf cloud models, protoplanetary disk simulations and other models used for the interpretation of observational data from past, current and future (exo)planetary NASA missions. We will present preliminary data obtained on Titan aerosol analogs produced in the Titan Haze Simulation (THS) experiment on COSmIC, a unique experimental platform developed at NASA Ames that allows the simulation of Titan's complex atmospheric chemistry at Titan-like temperature (200 K). We will also introduce a new study of the optical properties of ammonium-bearing phosphates, potential cloud particles forming in temperate exoplanets and brown dwarfs.

Planetary Science↗
NASA NTRS1993

Estimation of cirrus cloud particle fallspeeds from vertically pointing Doppler radar

The First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment 2 (FIRE 2) was conducted in Coffeyville, Kansas in late 1991 to study the microphysical and radiative properties of cirrus clouds. A variety of active and passive remote sensors were employed, including an 8-mm-wavelength cloud-sensing Doppler radar developed at the Wave Propagation Laboratory (WPL). The radar, having excellent sensitivity to cloud particles (-30 dBZ at 10 km), good spatial resolution (37 m), and velocity precision (.05 ms -1), is an excellent tool for observing cirrus clouds. Having this radar directed toward the zenith for long periods of time during FIRE 2 permitted the reflectivity-weighted particle fallspeed to be related to reflectivity which allowed a separation of ice particle fallspeeds from vertical air motions. Additionally, such relationships proved useful in other multi-sensor techniques for determining vertical profiles of ice particle characteristic size and ice water content in cirrus clouds. The analysis method and the results of applying it to cirrus cloud reflectivity and velocity data collected during FIRE 2 are discussed.

Orr, Brad W.↗
NASA NTRS1972

Cloud microstructure as determined by an optical cloud particle spectrometer.

Use of an improved single-particle light-scattering instrument for measurement of cloud microstructure in field studies. Cloud particle size and number information is measured over 12 sizing intervals, in the range from 4 to 85 microns in diameter. The microstructure can be observed in real time and with a spatial resolution not previously reported. The general features of water cloud droplet size and number distributions are consistent with previous direct capture and replication studies. The transition from water to ice phase regions in cumuliform clouds can be inferred from dramatic changes observed in the distribution features. Results are also presented for stratus and cirrus cloud penetrations.

Ryan, R. T.↗
NASA NTRS1992

Determining water cloud particle sizes from lidar depolarization measurements and time dependent multiple scattering coefficients

We present a technique of extracting water cloud particle size information from lidar measurements in conjunction with double scattering calculations. In this presentation, we describe the technique and give examples using data taken with the Air Force Phillips Laboratory's (Geophysics Directorate) low altitude Nd:YAG, elastic backscatter lidar. In a related presentation we describe the double scattering lidar model which we developed for this work. The technique uses simultaneous measurements of two orthogonal linear polarization components of lidar returns from water clouds or other media composed of spherical particles. Any depolarization of the incident lidar radiation backscattered by such a media can only be due to multiple scattering. The amount of depolarization is dependent on the extinction coefficient and the single scatter phase matrix, both of which are functions of position in the medium. The phase matrix is dependent on the index of refraction of the particles and the particle size distribution. Our technique is a modification of a procedure presented in Reference 1. There, particle sizes of water clouds are determined from double scattering calculations together with measurements of radiation scattered from volumes outside the lidar receiver's field of view (which can only be multiply scattered radiation). The methodology of our technique is similar but our 'probe' of the scattering phase function (and thus the particle size distribution) is different.

Garner, R. C.↗
NASA NTRS2019

Laboratory Investigations of Cloud Particle Formation and Sublimation on Titan, Mars, and Earth

Microphysical modeling of cloud formation and growth relies on fundamental measurements of the properties of condensable gases which form cloud particles. NASA's Ames Chemistry Laboratory has the capability to measure vapor pressures and heterogeneous nucleation conditions for a variety of gases found in the atmospheres of solar system bodies. Highlights from work for Earth, Mars, and Titan demonstrate the range of conditions and atmospheres studied to date.

Iraci, Laura T.↗
NASA NTRS1987

Particle cloud kinetics in microgravity

Data related to particle-particle agglomeration/deaglomeration and particle-wall attachment are discussed. Particle-cluster cloud interactions and particle-cluster agglomeration/deagglomeration kinetics are studied. An apparatus designed and constructed for examining the agglomeration/deagglomeration effects for lycopodium under the conditions of an acoustically energized mixing process and of alpha-particle-induced deagglomerative processes is described; characteristic features and applications for the apparatus are examined. Requirements for combustion experimentation are discussed.

Berlad, A. L.↗
NASA NTRS1990

Microgravity acoustic mixing for particle cloud combustors

Experimental and theoretical investigations of acoustic mixing procedures designed to uniformly distribute fuel particles in a combustion tube for application in the proposed Particle Cloud Combustion Experiment (PCCE) are described. Two acoustic mixing methods are investigated: mixing in a cylindrical tube using high frequency spinning modes generated by suitably phased, or quadrature speakers, and acoustic premixing in a sphere. Quadrature mixing leads to rapid circumferential circulation of the powder around the tube. Good mixing is observed in the circulating regions. However, because axial inhomogeneities are necessarily present in the acoustic field, this circulation does not extend throughout the tube. Simultaneous operation of the quadrature-speaker set and the axial-speaker was observed to produce considerably enhanced mixing compared to operation of the quadrature-speaker set alone. Mixing experiments using both types of speakers were free of the longitudinal powder drift observed using axial-speakers alone. Vigorous powder mixing was obtained in the sphere for many normal modes: however, in no case was the powder observed to fill the sphere entirely. Theoretical analysis indicated that mixing under steady conditions cannot fill more than a hemisphere except under very unusual conditions. Premixing in a hemisphere may be satisfactory; otherwise, complete mixing in microgravity might be possible by operating the speaker in short bursts. A general conclusion is that acoustic transients are more likely to produce good mixing than steady state conditions. The reason is that in steady conditions, flow structures like nodal planes are possible and often even unavoidable. These tend to separate the mixing region into cells across which powder cannot be transferred. In contrast, transients not only are free of such structures, they also have the characteristics, desirable for mixing, of randomness and disorder. This conclusion is corroborated by mixing experiments using axial waves.

Pla, Frederic↗
NASA NTRS1969

Particle cloud impingement damage

Single impact data considered ineffective in estimating target damage induced by micron-sized particle cloud impingement

Laderman, A. J.↗
NASA NTRS1986

Flame propagation and extinction in particle clouds

Two phase flame propagation and extinction theory required to support the corresponding experiments planned for the space shuttle is being developed. Also being planned are specialized collaborative, experimental and theoretical NASA UCSD studies needed to support the ongoing definition of needed experimental hardware, experimental procedures, data acquisition philosophy, and other ground based support activities required to assure the success of space shuttle based experiments concerned with combustion of clouds of particulates at reduced gravitational conditions. The further development of relations delineating premixed particle cloud and premixed gaseous systems as well as burner stabilized and freely propagating flame systems is considered.

Berlad, A. L.↗
NASA NTRS1988

Particle cloud combustion in reduced gravity

The prinicipal objectives of this microgravity experiment program are to obtain flame propagation rate and flame extinction limit data for several important premixed, quiescent particle cloud combustion systems under near zero-gravity conditions. The data resulting from these experiments are needed for utilization with currently available and tractable flame propagation and extinction theory. These data are also expected to provide standards for the evaluation of fire hazards in particle suspensions in both Earth-based and space-based applications. Both terrestrial and space-based fire safety criteria require the identification of the critical concentrations of particulate fuels and inerts at the flame extinction conditions.

Berlad, A. L.↗
NASA NTRS1978

The phase function of Venus cloud particles from Mariner 10 data

Mariner 10 images of Venus taken at several phase angles were photometrically reduced. The analysis shows that the phase function of the cloud particles is not isotropic, as had been deduced earlier from the brightness distribution on spacecraft images taken at a single phase angle, but has a broad minimum near 60 deg and is forward-scattering. The scattering properties are in quantitative agreement with previous deductions from earth-based polarization measurements by Hansen and his associates.

Hapke, B.↗
NASA NTRS2002

Homogenous Surface Nucleation of Solid Polar Stratospheric Cloud Particles

A general surface nucleation rate theory is presented for the homogeneous freezing of crystalline germs on the surfaces of aqueous particles. While nucleation rates in a standard classical homogeneous freezing rate theory scale with volume, the rates in a surface-based theory scale with surface area. The theory is used to convert volume-based information on laboratory freezing rates (in units of cu cm, seconds) of nitric acid trihydrate (NAT) and nitric acid dihydrate (NAD) aerosols into surface-based values (in units of sq cm, seconds). We show that a surface-based model is capable of reproducing measured nucleation rates of NAT and NAD aerosols from concentrated aqueous HNO3 solutions in the temperature range of 165 to 205 K. Laboratory measured nucleation rates are used to derive free energies for NAT and NAD germ formation in the stratosphere. NAD germ free energies range from about 23 to 26 kcal mole, allowing for fast and efficient homogeneous NAD particle production in the stratosphere. However, NAT germ formation energies are large (greater than 26 kcal mole) enough to prevent efficient NAT particle production in the stratosphere. We show that the atmospheric NAD particle production rates based on the surface rate theory are roughly 2 orders of magnitude larger than those obtained from a standard volume-based rate theory. Atmospheric volume and surface production of NAD particles will nearly cease in the stratosphere when denitrification in the air exceeds 40 and 78%, respectively. We show that a surface-based (volume-based) homogeneous freezing rate theory gives particle production rates, which are (not) consistent with both laboratory and atmospheric data on the nucleation of solid polar stratospheric cloud particles.

Tabazadeh, A.↗
NASA NTRS1993

The structure of particle cloud premixed flames

The aim of this study is to provide a numerical and asymptotic description of the structure of planar laminar flames, propagating in a medium containing a uniform cloud of fuel-particles premixed with air. Attention is restricted here to systems where the fuel-particles first vaporize to form a known gaseous fuel, which is then oxidized in the gas-phase. This program is supported for the period September 14, 1991 to September 13, 1992. Some results of the study is shown in Ref. 1. The work summarized in Ref. 1 was initiated prior to September 14, 1991 and was completed on February 1992. Research performed in addition to that described in Ref. 1 in collaboration with Professor A. Linan, is summarized here.

Seshadri, K.↗