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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2

Photoelectric conversion on Earth’s surface via widespread Fe- and Mn-mineral coatings

Sunlight drives photosynthesis and associated biological processes, and also influences inorganic processes that shape Earth’s climate and geochemistry. Bacterial solar-to-chemical energy conversion on this planet evolved to use an intricate intracellular process of phototrophy. However, a natural nonbiological counterpart to phototrophy has yet to be recognized. In this work, we reveal the inherent “phototrophic-like” behavior of vast expanses of natural rock/soil surfaces from deserts, red soils and karst environments, all of which can drive photon-to-electron conversions. Using scanning electron microscopy, transmission electron microscopy, micro-Raman spectroscopy and X-ray absorption spectroscopy, Fe and Mn (oxyhydr)oxide-rich coatings were found in rock varnishes, as were Fe (oxyhydr)oxides on red soil surfaces and minute amounts of Mn oxides on karst rock surfaces. By directly fabricating a photoelectric detection device on the thin section of a rock varnish sample, we have recorded the first in situ photocurrent micromapping of the coatings, which behave as highly sensitive and stable photoelectric systems. Additional measurements of red soil and powder separated from the outermost surface of karst rocks yielded photocurrents that are also sensitive to irradiation. The prominent solar-responsive capability of the phototrophic-like rocks/soils is ascribed to the semiconducting Fe and Mn (oxyhydr)oxide mineral coatings. The native semiconducting Fe/Mn-rich coatings may play a role similar in part to photosynthetic systems and thus provide a distinctive driving force for redox (bio)geochemistry on Earth’s surfaces.

Lu, Anhuai↗

Fourier Spectroscopy as a Method of Investigation of Photoelectric Properties of Organic Systems

A new method of investigation of photoelectric properties of layered thin-film structures based on broadband Fourier spectroscopy exhibiting a harmonically modulated optical delay is proposed. In contrast to traditional approaches to study photoelectric properties, which are based on application of dispersive spectral devices, the proposed method allows not only simultaneously covering the ultraviolet, visible, and infrared spectral ranges, while demonstrating a wide dynamic range and high spectral resolution, but also easily varying low-frequency modulation of the action of light. The capabilities of the method are demonstrated using a polycrystalline organic heterostructure as an example. Its spectral sensitivity, speed, and specific detectivity are measured. A model and an equivalent electric circuit are proposed for explanation of the results of the measurements.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

X-Ray Spectro-polarimetry with Photoelectric Polarimeters

We derive a generalization of forward fitting for X-ray spectroscopy to include linear polarization of X-ray sources, appropriate for the anticipated next generation of space-based photoelectric polarimeters. We show that the inclusion of polarization sensitivity requires joint fitting to three observed spectra, one for each of the Stokes parameters, I(E), U(E), and Q(E). The equations for Stokes’ I(E) (the total intensity spectrum) are identical to the familiar case with no polarization sensitivity, and for which the model-predicted spectrum is obtained by a convolution of the source spectrum, F(E′), with the familiar energy response function, ϵ(E′) R(E′, E), where ϵ(E′) and R(E′, E) are the effective area and energy redistribution matrix, respectively. In addition to the energy spectrum, the two new relations for U(E) and Q(E) include the source polarization fraction and position angle versus energy, a(E′), and ψ{sub 0}{sup ′}(E{sup ′}), respectively, and the model-predicted spectra for these relations are obtained by a convolution with the “modulated” energy response function, μ(E′) ϵ (E′)R(E, E′), where μ(E′) is the energy-dependent modulation fraction that quantifies a polarimeter’s angular response to 100% polarized radiation. We present results of simulations with response parameters appropriate for the proposed PRAXyS Small Explorer observatory to illustrate the procedures and methods, and we discuss some aspects of photoelectric polarimeters with relevance to understanding their calibration and operation.

79 ASTRONOMY AND ASTROPHYSICS↗

Methods of photoelectric observations

Photoelectric detectors and their operation are described, with emphasis on photomultipliers, infrared radiation detectors, and photoelectric photometers.

Chugaynov, P. F.↗

Photoelectric array detectors for use at XUV wavelengths

The characteristics of photoelectric detector systems for use at visible-light, ultraviolet, and X-ray wavelengths are briefly reviewed in the context of the needs of the Spacelab solar-physics facilities. Photoelectric array detectors for use at XUV wavelengths between 90 and 1500 A are described, and their use in the ESA Grazing-Incidence Solar Telescope (GRIST) facility is discussed.

Timothy, J. G.↗

Coronal transients in FE XIV 5303A: First two-dimensional photoelectric ground-based observations

An observational program was undertaken at Sacramento Peak Observatory to photoelectrically detect coronal transients. Continuous observations are made in the Fe XIV 5303A green line, utilizing the 40 cm coronagraph and the Photoelectric Coronal Photometer. Scans at three heights above the limb are combined to form a low resolution picture of the greenline corona every 20 to 30 minutes. Difference pictures, relative to an initial scan, are generated to search for sudden changes in the corona. The first few days of operation of this program have yielded three low-lying events ( 1.55 solar radii) following minor chromospheric activity (a surge and eruptive prominences), which propagated up through the corona with velocities on the order of 100 km/s.

Altrock, R. C.↗

Radar and photoelectric observations of asteroid 2100 Ra-Shalom

Asteroid Ra-Shalom was subjected to 13-cm wavelength radar and V-filter photoelectric observations during its August-September 1981 apparition; the radar data yield echoes in the same sense of circular polarization as transmitted (SC) as well as in the opposite sense (OC). SC-to-OC echo power ratio estimates indicate that most of the backscattering is due to single reflections from surface elements that are relatively smooth at decimeter scales. The photoelectric data suggest a value of 19.79 hours for the synodic rotation period.

Ostro, S. J.↗

The photoelectric effect from CsI by polarized soft X-rays

Studies of the polarization dependence of the photoelectric effect produced by soft X-rays from CsI indicate that the geometrical effects in these experiments can often mimic the polarization signature. This paper presents a detailed calculation of these geometrical effects that are produced when the X-ray beam is not precisely aligned on a rotatable plane photocathode. The experimentally observed geometrical effects were used to precisely determine the realignment of the incident beam of polarized X-rays on a rotatable photocathode. The results allow determinations of the true polarization dependence of the photoemission from CsI. It is shown that the photoelectric effect in CsI depends on the polarization state of the X-rays.

Shaw, Ping S.↗

Exploiting the Photoelectric effect for X-ray Polarimetry using Time Projection Chamber

The promise of photoelectric X-ray polarimetry has now been realized in laboratory demonstrations and may soon be used for astrophysical observations. Photoelectric polarimetry in gas filled proportional counters achieves high sensitivity through a combination of broad band width and good modulation. The band can be tuned by careful choice of gas composition and pressure. The measurements rely on imaging the tracks of photoelectrons. The initial direction of each track carries information about the electric field of the X-ray photon, and an ensemble of such measurements thus measures the net polarization of the source. A novel readout geometry using time projection chambers (TPC) allows deep (i.e. high efficiency) detectors, albeit without the ability to image the sky. Polarimeters which exploit the TPC geometry can be optimized for use behind telescopes, to study faint persistent sources, or as wide field of view instruments, designed to study bright transient events such as gamma-ray bursts or solar flares. We present the conceptual design of both types of TPC polarimeter. Recent laboratory results demonstrate that these polarimeters can achieve substantial gains in the polarization sensitivity achievable in experiments of modest size.

Jahoda, Keith↗

Electrostatic Charging of Lunar Dust by UV Photoelectric Emissions and Solar Wind Electrons

The ubiquitous presence of dust in the lunar environment with its high adhesive characteristics has been recognized to be a major safety issue that must be addressed in view of its hazardous effects on robotic and human exploration of the Moon. The reported observations of a horizon glow and streamers at the lunar terminator during the Apollo missions are attributed to the sunlight scattered by the levitated lunar dust. The lunar surface and the dust grains are predominantly charged positively by the incident UV solar radiation on the dayside and negatively by the solar wind electrons on the night-side. The charged dust grains are levitated and transported over long distances by the established electric fields. A quantitative understanding of the lunar dust phenomena requires development of global dust distribution models, based on an accurate knowledge of lunar dust charging properties. Currently available data of lunar dust charging is based on bulk materials, although it is well recognized that measurements on individual dust grains are expected to be substantially different from the bulk measurements. In this paper we present laboratory measurements of charging properties of Apollo 11 & 17 dust grains by UV photoelectric emissions and by electron impact. These measurements indicate substantial differences of both qualitative and quantitative nature between dust charging properties of individual micron/submicron sized dust grains and of bulk materials. In addition, there are no viable theoretical models available as yet for calculation of dust charging properties of individual dust grains for both photoelectric emissions and electron impact. It is thus of paramount importance to conduct comprehensive measurements for charging properties of individual dust grains in order to develop realistic models of dust processes in the lunar atmosphere, and address the hazardous issues of dust on lunar robotic and human missions.

Abbas, Mian M.↗

X-Ray Spectro-Polarimetry with Photoelectric Polarimeters

We derive a generalization of forward fitting for X-ray spectroscopy to include linear polarization of X-ray sources, appropriate for the anticipated next generation of space-based photoelectric polarimeters. We show that the inclusion of polarization sensitivity requires joint fitting to three observed spectra, one for each of the Stokes parameters, I(E), U(E), and Q(E). The equations for StokesI (E) (the total intensity spectrum) are identical to the familiar case with no polarization sensitivity, and for which the model-predicted spectrum is obtained by a convolution of the source spectrum, F (E), with the familiar energy response function,(E) R(E,E), where (E) and R(E,E) are the effective area and energy redistribution matrix, respectively. In addition to the energy spectrum, the two new relations for U(E) and Q(E) include the source polarization fraction and position angle versus energy, a(E), and 0(E), respectively, and the model-predicted spectra for these relations are obtained by a convolution with the modulated energy response function, (E)(E) R(E,E), where(E) is the energy-dependent modulation fraction that quantifies a polarimeters angular response to 100 polarized radiation. We present results of simulations with response parameters appropriate for the proposed PRAXyS Small Explorer observatory to illustrate the procedures and methods, and we discuss some aspects of photoelectric polarimeters with relevance to understanding their calibration and operation.

polarization↗

Disentangling Planets from Photoelectric Instability in Gas-rich Optically Thin Dusty Disks

Structures in circumstellar disks such as gaps and rings are often attributed to planets. This connection has been difficult to show unequivocally, as other processes may also produce these features. In particular, a photoelectric instability (PEI) has been proposed, operating in gas-rich optically thin disks, that generates structures predicted by planet–disk interactions. We examine the question of how to disentangle the planetary effects on disk structure from the effects of the PEI. We use the Pencil Code to perform 2D global hydrodynamical models of the dynamics of gas and dust in a thin disk with and without planetary perturbers. Photoelectric heating is modeled with an equation of state where pressure is proportional to dust surface density. The drag force on grains and its backreaction on the gas are included. Analyzing the situation without PEI, we find that gas–dust interactions alter the shape of the planetary gap from the dust-free case when the local dust-to-gas ratio ε approaches unity. This result also applies to primordial disks, because dust drifting inward accumulates at the edge of the planetary gap, and any initial dust-to-gas ratio eventually achieves ε = 1 if the dust reservoir is sufficient. We find a result particular to high dust-to-gas ratio disks as well: as dust drifts inward, the dust front becomes a sharp transition, and the backreaction triggers the Rossby wave instability. When PEI is included, we find that it obscures structures induced by planets unless the planet's mass is sufficiently large to carve a noticeable gap. Specifically, the instability generates arcs and rings of regular spacing: a planet is discernible when it carves a dust gap wider than the wavelength of the PEI.

Areli Castrejon↗

A New Search for Low-mass Dark Matter and an Examination and Reduction of the Uncertainty due to the Photoelectric Absorption Cross Section using a Cryogenic Silicon Detector with Single-charge Sensitivity

Many astrophysical observations point to the abundant existence of dark matter (DM) in the universe composed of particles beyond the Standard Model. However despite numerous experiments using different techniques, DM particles have yet to be directly observed. The Super Cryogenic Dark Matter Search (SuperCDMS) SNOLAB experiment will employ silicon and germanium crystal detectors operated at temperatures as low as 15~mK to probe DM interactions using phonon and ionization signals. Recently, R\&D; facilities have developed gram-sized high-voltage eV-scale (HVeV) silicon detectors that achieve single-electron-hole-pair resolution. By probing effective DM-electron interactions, these devices can be used for searches of low-mass DM candidates.This dissertation presents a DM search experiment known as HVeV Run~2 that employs a second-generation HVeV detector operated in an above-ground laboratory at Northwestern University (IL, USA). Energy spectra are obtained from a blind analysis with 0.39 and 1.2\,g-days of exposure with the detector biased at 60 and 100\,V, respectively. The 0.93~gram detector achieves a 3\,eV phonon energy resolution, corresponding to a world-leading charge resolution of 3\,\% of a single electron-hole pair for a detector bias of 100\,V. With charge carrier trapping and impact ionization effects incorporated into the DM signal models, the resulting exclusion limits are reported for inelastic DM-electron scattering for DM masses from 0.5--$10^{4}$\,MeV$/c^{2}$; in the mass range from 1.2--50\,eV$/c^{2}$ the limits for dark photon and axion-like particle absorption are reported.Several DM search experiments, including HVeV Run~2, are sensitive to low-mass DM candidates that rely on the temperature-dependent photoelectric absorption cross section of silicon. However discrepancies in the underlying literature data result in dominating systematic uncertainties on the DM exclusion limits. In order to reduce these systematic uncertainties, this dissertation presents a novel method of making a direct, low-temperature measurement of the photoelectric absorption cross section of silicon at energies near the band gap (1.2--2.8\,eV).

Wilson, Matthew James↗

The Influence of EL2 Centers on the Photoelectric Response of an Array of Radial GaAs/AlGaAs Nanowires

We have studied the role of EL2 centers in formation of the photoelectric response of an array of radial n-type GaAs/Al{sub x}Ga{sub 1 –x}As (x = 0.3) nanowires (NWs) grown by molecular beam epitaxy on a p-type silicon substrate. Results revealed a significant decrease in the time of NW photoresponse recovery as compared to that in a bulk crystal upon the transition of EL2 centers from a metastable nonactive state to the normal ground state.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

CALiPER Report 22.1: Photoelectric Performance of LED MR16 Lamps

This report is a follow-up to CALiPER Application Summary Report 22, which investigated the photometric performance of LED MR16 lamps. The initial report found that many of the LED MR16 lamps did not perform as required by ENERGY STAR based on their equivalency claims, although they generally did provide substantial efficacy advantages compared to halogen MR16 lamps. All testing was completed using laboratory power supplies, with all but one product tested at 12 V AC. In contrast, this report examined the photoelectric performance of the same set of lamps, using commercially available transformers and dimmers as well as laboratory power supplies providing both AC and DC power.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

CALiPER Report 22.1: Photoelectric Performance of LED MR16 Lamps

This report looks at the photoelectric performance of the same set of lamps assessed in Report 22, using commercially available transformers and dimmers as well as laboratory power supplies providing either AC or DC. The investigation explores several issues related to the testing and use of MR16 lamps in lighting systems and examines the range of performance that is possible for a given lamp model, based on the system to which it is connected.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Tailoring Bandgap of Perovskite BaTiO 3 by Transition Metals Co-Doping for Visible-Light Photoelectrical Applications: A First-Principles Study

The physical and chemical properties of V-M" and Nb-M" (M" is 3d or 4d transition metal) co-doped BaTiO 3 were studied by first-principles calculation based on density functional theory. Our calculation results show that V-M" co-doping is more favorable than Nb-M" co-doping in terms of narrowing the bandgap and increasing the visible-light absorption. In pure BaTiO 3 , the bandgap depends on the energy levels of the Ti 3d and O 2p states. The appropriate co-doping can effectively manipulate the bandgap by introducing new energy levels interacting with those of the pure BaTiO 3 . The optimal co-doping effect comes from the V-Cr co-doping system, which not only has smaller impurity formation energy, but also significantly reduces the bandgap. Detailed analysis of the density of states, band structure, and charge-density distribution in the doping systems demonstrates the synergistic effect induced by the V and Cr co-doping. The results can provide not only useful insights into the understanding of the bandgap engineering by element doping, but also beneficial guidance to the experimental study of BaTiO 3 for visible-light photoelectrical applications.

36 MATERIALS SCIENCE↗