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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
NASA NTRS1990

Life cycles of persistent anomalies. II - The development of persistent negative height anomalies over the North Pacific Ocean

Consideration is given to the potential sources for the development of cases defined by strong and persistent negative height anomalies over the central North Pacific. The analyses of Dole (1986) are extended by providing a more complete synoptic description of the developments and additional diagnostic analysis to identify dynamical mechanisms responsible for the developments. The synoptic characteristics of the developments are reviewed and the barotropic and baroclinic processes of the developments are analyzed. The reproducibility and representativeness of the results are examined. The observed characteristics suggest that the large-scale flow anomalies develop as a result of an instability of three-dimensional wintertime mean flow.

Dole, Randall M.↗
DOE OSTI2020

Explaining persistent incomplete mixing in multicomponent reactive transport with Eulerian stochastic model

We present an Eulerian stochastic advection–diffusion–reaction (SADR) model and use it to explain incomplete mixing typically observed in transport experiments with bimolecular reactions. Unlike traditional advection– dispersion–reaction (ADR) models, the SADR model describes mechanical and diffusive mixing as two separate processes. In the SADR model, mechanical mixing is driven by random advective velocity whose variance is given by the coefficient of mechanical dispersion. The diffusive mixing is modeled as a Fickian diffusion process with the effective diffusion coefficient. We demonstrate that the sum of the two coefficients is equal to the dispersion coefficient, but only the effective diffusion coefficient contributes to the mixing-controlled reactions. We use experimental results of Gramling et al. * * to show that for transport and bimolecular reactions in porous media, the SADR model is significantly more accurate than the ADR model, which overestimates the concentration of the reaction product by as much as 60%. We also show that the SADR model predicts an experimentally observed bell- shaped spatial distribution of the reactive product concentration, while the ADR model results in a concentration distribution with an unphysical kink.

Bimolecular reactions, incomplete mixing, Stochast↗
DOE OSTI2014

Persistent Subdiffusive Proton Transport in Perfluorosulfonic Acid Membranes

Proton transport (PT) in solutions of small amphiphiles in water has previously been shown to be subdiffusive for long times. The present study analyzes simulations of hydrated perfluorosulfonic acid (PFSA) membranes in order to determine whether PT is also subdiffusive in these important amphiphilic systems. Here, we show that PT is indeed subdiffusive for several hundred picoseconds for all hydration levels examined, and the subdiffusive behavior is highly dependent on water concentration. We also investigate the caging of the excess proton using a recently developed technique and show that the excess proton exhibits caging effects up to at least 1 ns in PFSA systems. In order to fully characterize the long-time behavior of PT in PFSAs, these results demonstrate that multiple nanosecond trajectories are needed, well beyond the current capabilities of ab initio molecular dynamics.

25 ENERGY STORAGE↗
DOE OSTI2014

Interaction of light with the ZnO surface: Photon induced oxygen “breathing,” oxygen vacancies, persistent photoconductivity, and persistent photovoltage

ZnO surfaces adsorb oxygen in the dark and emit CO{sub 2} when exposed to white light, reminiscent of the lungs of living creatures. We find that this exchange of oxygen with the ambient affects the integrity of the ZnO surface. Thus, it forms a basis for several interesting surface phenomena in ZnO, such as photoconductivity, photovoltage, and gas sensing, and has a role in ZnO electrical conduction. Using x-ray photoelectron spectroscopy on ZnO nanowires, we observed a decomposition of ZnO under white light and formation of oxygen-depleted surface, which explains photoconductivity by the electron donation of oxygen vacancies. Our findings suggest that the observed decomposition of the ZnO lattice may only take place due to photon-induced reduction of ZnO by carbon containing molecules (or carbo-photonic reduction), possibly from the ambient gas, accounting in a consistent way for both the reduced demands on the energy required for decomposition and for the observed emission of lattice oxygen in the form of CO{sub 2}. The formation of oxygen-vacancy rich surface is suggested to induce surface delta doping, causing accumulation of electrons at the surface, which accounts for both the increase in conductivity and the flattening of the energy bands. Using surface photovoltage spectroscopy in ultra high vacuum, we monitored changes in the deep level spectrum. We observe a wide optical transition from a deep acceptor to the conduction band, which energy position coincides with the position of the so called “green luminescence” in ZnO. This green transition disappears with the formation of surface oxygen vacancies. Since the oxygen vacancies are donors, while the green transition involves surface acceptors, the results suggest that the initial emission of oxygen originates at the defect sites of the latter, thereby eliminating each other. This suggests that the green transition originates at surface Zn vacancy acceptors. Removing an oxygen atom from a Zn vacancy completes the vacancy to become a full ZnO molecule vacancy, which does not produce deep levels. Our results explain why ZnO finds use as an electrical detector for oxygen and for carbon containing gas molecules. They may also shed new light on photocatalytic uses of ZnO. It is suggested that similar surface phenomena may affect other semiconducting oxides.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Far infrared edge photoresponse and persistent edge transport in an inverted InAs/GaSb heterostructure

Direct current (DC) transport and far infrared photoresponse were studied an InAs/GaSb double quantum well with an inverted band structure. The DC transport depends systematically upon the DC bias configuration and operating temperature. Surprisingly, it reveals robust edge conduction despite prevalent bulk transport in our device of macroscopic size. Under 180 GHz far infrared illumination at oblique incidence, we measured a strong photovoltaic response. We conclude that quantum spin Hall edge transport produces the observed transverse photovoltages. Overall, our experimental results support a hypothesis that the photoresponse arises from direct coupling of the incident radiation field to edge states.

Dyer, G. C.↗
DOE OSTI2014

X-ray-induced persistent photoconductivity in vanadium dioxide

The resistivity of vanadium dioxide (VO2) decreased by over one order of magnitude upon localized illumination with x rays at room temperature. Despite this reduction, the structure remained in the monoclinic phase and had no signature of the high-temperature tetragonal phase that is usually associated with the lower resistance. Once illumination ceased, relaxation to the insulating state took tens of hours near room temperature. However, a full recovery of the insulating state was achieved within minutes by thermal cycling. We show that this behavior is consistent with random local-potential fluctuations and random distribution of discrete recombination sites used to model residual photoconductivity.

Dietze, S. H.↗
DOE OSTI2022

3D Simulations Capture the Persistent Low-Mode Asymmetries Evident in Laser-Direct-Drive Implosions on OMEGA

Spherical implosions in Inertial Confinement Fusion (ICF) are inherently sensitive to perturbations that may arise from experimental constraints and errors. Control and mitigation of low-mode (long wavelengths) perturbations is a key milestone to improving implosion performances. Here, we present the first 3-D radiation-hydrodynamic simulations of directly driven ICF implosions with an inline package for polarized Crossed-Beam Energy Transfer (CBET). Simulations match bang times, yields (separately accounting for laser-induced high modes and fuel age), hot spot flow velocities and direction, for which polarized CBET contributes to the systematic flow orientation evident in the OMEGA implosion database. Current levels of beam mispointing, imbalance, target offset and asymmetry from polarized CBET degrade yields by more than 40%. The effectiveness of two mitigation strategies for low-modes is explored.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Identification and Characterization of Persistent Cold Pool Events from Temperature and Wind Profilers in the Columbia River Basin

Cold pool events occur when deep layers of stable, cold air remain trapped in a valley or basin for multiple days, without mixing out from daytime heating. With large impacts on air quality, freezing events, and es-pecially on wind energy production, they are often poorly forecast by modern mesoscale numerical weather prediction (NWP) models. Understanding the characteristics of cold pools is, therefore, important to provide more accurate forecasts. This study analyzes cold pool characteristics with data collected during the Second Wind Forecast Improvement Project (WFIP2), which took place in the Columbia River basin and Gorge of Oregon and Washington from fall 2015 until spring 2017. A subset of the instrumentation included three microwave radiometer pro?lers, six radar wind pro?lers with radio acoustic sounding systems, and seven sodars, which together provided seven sites with collocated vertical pro?les of temperature, humidity, wind speed, and wind direction. Using these collocated observations, we developed a set of criteria to determine if a cold pool was present based on stability, wind speed, direction, and temporal continuity, and then developed an automated algorithm based on these criteria to identify all cold pool events over the 18 months of the ?eld project. Characteristics of these events are described, including statistics of the wind speed distributions and pro?les, stability conditions, cold pool depths, and descent rates of the cold pool top. The goal of this study is a better understanding of these characteristics and their processes to ultimately lead to improved physical parameterizations in NWP models, and consequently improve forecasts of cold pool events in the study region as well at other locations that experiences similar events.

McCaffrey, Katherine L.↗