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Simple model for the reconstruction of radionuclide concentrations and radiation exposures along the Techa River

The Techa River (Southern Urals, Russia) was contaminated in 1949-1956 by liquid radioactive wastes from the Mayak complex, the first Russian facility for the production of plutonium. The measurements of environmental contamination were started in 1951. A simple model describing radionuclide transport along the free-flowing river and the accumulation of radionuclides by bottom sediments is presented. This model successfully correlates the rates of radionuclide releases as reconstructed by the Mayak experts, hydrological data, and available environmental monitoring data for the early period of contamination (1949-1951). The model was developed to reconstruct doses for people who lived in the riverside communities during the period of the releases and who were chronically exposed to external and internal irradiation. The model fills the data gaps and permits reconstruction of external gamma-exposure rates in air on the river bank and radionuclide concentrations in river water used for drinking and other household needs in 1949-1951.

Non-NASA Center↗

Dynamo generation in Mercury

Models of the interior and thermal evolution of Mercury calculated by Siegfried and Solomon (1974) using Lewis' (1972) cosmochemical calculations to constrain the composition are tested for four necessary conditions for MHD dynamo generation. It is shown that dynamo generation requires at least a partially fluid interior, an energy source that drives a flow of core fluid relative to the rigidly rotating planet, a magnetic-field diffusion time in excess of the characteristic fluid-flow time scale, and a fluid flow of sufficient complexity to satisfy Cowling's (1934) theorem. It is concluded that a literal interpretation of Lewis' calculations implies that dynamo generation in Mercury is improbable. Generation would be possible only if the metallic core were contaminated with substantial amounts of radioactive material.

Stevenson, D. J.↗

Calibration Results for the AXAF Flux Contamination Monitor

The Flux Contamination Monitor (FCM) on the Advanced X-ray Astrophysics Facility (AXAF) serves the purposes of transfering the absolute flux calibration from the ground calibration at the X-Ray Calibration Facility (XRCF) at Marshall Space Flight Center to operation on orbit and of detecting any changes in molecular contamination of the High Resolution Mirror Assembly (HRMA) between ground calibration and the post-launch activation phase. we describe the design, construction, and characterization of the FCM radioactive sources, and their placement on the Forward Contamination Cover (FCC). We present results from FCM measurements with the AXAF focal plane instruments, particularly the AXAF CCD Imaging Spectrometer (ACIS), during the ground calibration phase at XRCF in 1997. Finally, we describe the plans for FCM on-orbit measurements during observatory activation and the subsequent analysis.

Elsner, Ronald F.↗

Calibration Results for the AXAF Flux Contamination Monitor

The AXAF Flux Contamination Monitor (FCM) serves the purposes of transferring the absolute flux calibration from the ground calibration at the X-Ray Calibration Facility (XRCF) to operation on orbit and of detecting any changes in molecular contamination of the High-Resolution Mirror Assembly (HRMA) between ground calibration and the post-launch activation. We describe the design, construction, and characterization of the FCM radioactive sources, and their placement on the Forward Contamination Cover (FCC). We present results from FCM measurements with the AXAF focal-plane instruments, particularly the AXAF CCD Imaging Spectrometer (ACIS), during the ground calibration phase at the XRCF in 1997. Finally, we describe the plans for FCM on-orbit measurements during observatory activation and for the subsequent analysis.

Elsner, R. F.↗

Shuttle filter study. Volume 2: Contaminant generation and sensitivity studies

Contaminant generation studies were conducted at the component level using two different methods, radioactive tracer technique and gravimetric analysis test procedure. Both of these were reduced to practice during this program. In the first of these methods, radioactively tagged components typical of those used in spacecraft were studied to determine their contaminant generation characteristics under simulated operating conditions. Because the purpose of the work was: (1) to determine the types and quantities of contaminants generated; and (2) to evaluate improved monitoring and detection schemes, no attempt was made to evaluate or qualify specific components. The components used in this test program were therefore not flight hardware items. Some of them had been used in previous tests; some were obsolete; one was an experimental device. In addition to the component tests, various materials of interest to contaminant and filtration studies were irradiated and evaluated for use as autotracer materials. These included test dusts, plastics, valve seat materials, and bearing cage materials.

Source record↗

Radiological Control Manual

Objectives of the manual are to (1) ensure compliance with requirements of AEC and governmental health agencies, (2) ensure against excessive and unnecessary exposure of personnel to harmful radiation, and (3) prevent contamination of equipment, materials, and environment with radioactive materials.

Noblin, J. W.↗

Lead in Martian Meteorites-- Observations and Inconsistencies: I. Chassigny

The history of Pb isotope analyses of the martian meteorites (SNC) and their interpretations is laden with difficulties. Two different analytical groups have interpreted their ancient (≥ 4 Ga) shergottite Pb ages as primary [1-5]. A Nakhla age of approximately 4.3 Ga has been interpreted to be primary as well [2]. This is in stark contrast to the young (≤ 1.4 Ga) crystallization ages defined by the Rb-Sr, Sm-Nd, Lu-Hf, and KAr systems [6]. Possibly, a better interpretation for the ancient Pb ages is that they reflect the formation times of the various SNC source regions [7]. A difficulty in dealing with Pb is that terrestrial contamination is ubiquitous, unlike the other chronometer systems noted above. This issue is complicated by the fact that radioactive decay causes localized mineral damage. So washing and leaching to remove Pb contamination tends to remove in situ radiogenic Pb. This issue is further compounded because U and Th are often concentrated in phosphates and other minor phases, so the leaching process tends to remove these, especially phosphates. Another difficulty is that it is not clear whether the observed Pb isotopic variation in leachates, residues, and ion-microprobe analyses is due to terrestrial or to indigenous martian Pb contamination [e.g., 8]. A third difficulty is that the shergottites on the one hand, and the nakhlites and chassignites on the other, appear to have come from separate source regions with different chemical compositions [e.g., 7]. Thus, it is expected that their Pb isotopic characteristics would be different. And even if all these meteorite types came from the same source region, their igneous ages differ considerably. The nakhlites and chassignites are ~1.4 Ga and the shergottites are ≤ 600 Ma [e.g., 6]. This age difference alone should assure that the two distinct SNC groups have differing Pb isotopic signatures.

Jones, J. H.↗

Double gloves reduce contamination of dry box atmosphere

Pair of encased low permeability hand gloves between which an inert gas circulates reduces dry box contamination. This innovation is applicable to dry boxes using radioactive and alkali metal compounds, submicron powders, and liquid metals.

Herbell, T. P.↗

A local recent supernova - Evidence from X-rays, Al-26 radioactivity and cosmic rays

Possible ways in which cosmic rays could have been contaminated by a local recent supernova are discussed, and ways in which this contamination may be affecting interpretation of Al-26 gamma radiation and locally observed cosmic rays as samples of the average Galactic distribution are considered. Mass spectra of cosmic rays are examined to see whether there is enrichment by a population arising from supernova preacceleration. The reinterpretation of the anomalous component in terms of a local supernova model is addressed.

Clayton, Donald D.↗

Asymptotic Giant Branch stars as a source of short-lived radioactive nuclei in the solar nebula

We carried out a theoretical evaluation of the contribution of Asymptotic Giant Branch (AGB) stars to some short-lived (10(exp 6) less than or equal to Tau-bar less than or equal to 2 x 10(exp 7) yr) isotopes in the Interstellar Medium (ISM) and in the early solar system using stellar model calculations for thermally pulsing evolutionary phases of low-mass stars. The yields of s-process nuclei in the convective He-shell for different neutron exposures tau(sub 0) were obtained, and AGB stars were shown to produce several radioactive nuclei (especially Pd-107, Pb-205, Fe-60, Zr-93, Tc-99, Cs-135, and Hf-182) in diferent amounts. Assuming either contamination of the solar nebula from a single AGB star or models for continuous injection and mixing from many stars into the ISM, we calculate the ratios of radioactive to stable nuclei at the epoch of the Sun's formation. The dilution factor between the AGB ejecta and the early solar system matter is obtained by matching the observed Pd-107/Pd-108 and depends on the value of tau(sub 0). It is found that small masses M(sub He) of He-shell material (10(exp -4)-10(exp -7) solar mass) enriched in s-process nuclei are sufficient to contaminate 1 solar mass of the ISM to produce the Pd-107 found in the early solar system. Predictions are made for all of the other radioactive isotopes. The optimal model to explain several observed radioactive species at different states of the proto-solar nebula involves a single AGB star with a low neutron exposure (tau(sub 0) = 0.03 mbarn(sup -1)) which contaminated the cloud with a dilution factor of M(sub He)/solar mass approximately 1.5 x 10(exp -4). This will also contribute newly synthesized stable s-process nuclei in the amount of approximately 10(exp -4) of their abundances already present in the proto-solar cloud. Variations in the degree of homogenization (approximately 30%) of the injected material may account for some of the small general isotopic anomalies found in meteorites. It is also found that Fe-60 is produced in small but significant quantities that may be sufficient to explain the observations if the time elapsed delta from the contamination of the ISM to the formation of protoplanetary bodies is not higher than delta = 5 x 10(exp 6) yr. If delta is longer, up to 10 x 10(exp 6) yr, this would require the single AGB star to experience enhanced neutron densities (n(sub n) approximately 3 x 10(exp 9)n/cu cm) in the s-processing zone in order to compensate for the branching at Fe-59. The alternative model of long-term continuous ejection of matter from many AGB stars does not appear to match the observations. We also estimate the Al-26 production from the H-shell and find that the Al-26 abundance in the early solar system may be readily explained in a self-consistent manner. Moreover, Al-26 from AGB stars may contribute substantially to the galactic Al-26 gamma-source, while no significant gamma-flux from Co-60 (deriving from Fe-60 decay) is to be expected.

Wasserburg, G. J.↗

Development of Modeling Approaches for Nuclear Thermal Propulsion Test Facilities

High efficiency of rocket propul-sion systems is essential for humanity to venture be-yond the moon. Nuclear Thermal Propulsion (NTP) is a promising alternative to conventional chemical rock-ets with relatively high thrust and twice the efficiency of the Space Shuttle Main Engine. NASA is in the pro-cess of developing a new NTP engine, and is evaluat-ing ground test facility concepts that allow for the thor-ough testing of NTP devices. NTP engine exhaust, hot gaseous hydrogen, is nominally expected to be free of radioactive byproducts from the nuclear reactor; how-ever, it has the potential to be contaminated due to off-nominal engine reactor performance. Several options are being investigated to mitigate this hazard potential with one option in particular that completely contains the engine exhaust during engine test operations. The exhaust products are subsequently disposed of between engine tests. For this concept (see Figure 1), oxygen is injected into the high-temperature hydrogen exhaust that reacts to produce steam, excess oxygen and any trace amounts of radioactive noble gases released by off-nominal NTP engine reactor performance. Water is injected to condense the potentially contaminated steam into water. This water and the gaseous oxygen (GO2) are subsequently passed to a containment area where the water and GO2 are separated into separate containment tanks.

Jones, Daniel R.↗

Review of Nuclear Thermal Propulsion Ground Test Options

High efficiency rocket propulsion systems are essential for humanity to venture beyond the moon. Nuclear Thermal Propulsion (NTP) is a promising alternative to conventional chemical rockets with relatively high thrust and twice the efficiency of highest performing chemical propellant engines. NTP utilizes the coolant of a nuclear reactor to produce propulsive thrust. An NTP engine produces thrust by flowing hydrogen through a nuclear reactor to cool the reactor, heating the hydrogen and expelling it through a rocket nozzle. The hot gaseous hydrogen is nominally expected to be free of radioactive byproducts from the nuclear reactor; however, it has the potential to be contaminated due to off-nominal engine reactor performance. NTP ground testing is more difficult than chemical engine testing since current environmental regulations do not allow/permit open air testing of NTP as was done in the 1960's and 1970's for the Rover/NERVA program. A new and innovative approach to rocket engine ground test is required to mitigate the unique health and safety risks associated with the potential entrainment of radioactive waste from the NTP engine reactor core into the engine exhaust. Several studies have been conducted since the ROVER/NERVA program in the 1970's investigating NTP engine ground test options to understand the technical feasibility, identify technical challenges and associated risks and provide rough order of magnitude cost estimates for facility development and test operations. The options can be divided into two distinct schemes; (1) real-time filtering of the engine exhaust and its release to the environment or (2) capture and storage of engine exhaust for subsequent processing.

Coote, David J.↗

Advanced Filter Technology For Nuclear Thermal Propulsion

The Scrubber System focuses on using HEPA filters and carbon filtration to purify the exhaust of a Nuclear Thermal Propulsion engine of its aerosols and radioactive particles; however, new technology may lend itself to alternate filtration options, which may lead to reduction in cost while at the same time have the same filtering, if not greater, filtering capabilities, as its predecessors. Extensive research on various types of filtration methods was conducted with only four showing real promise: ionization, cyclonic separation, classic filtration, and host molecules. With the four methods defined, more research was needed to find the devices suitable for each method. Each filtration option was matched with a device: cyclonic separators for the method of the same name, electrostatic separators for ionization, HEGA filters, and carcerands for the host molecule method. Through many hours of research, the best alternative for aerosol filtration was determined to be the electrostatic precipitator because of its high durability against flow rate and its ability to cleanse up to 99.99% of contaminants as small as 0.001 micron. Carcerands, which are the only alternative to filtering radioactive particles, were found to be non-existent commercially because of their status as a "work in progress" at research institutions. Nevertheless, the conclusions after the research were that HEPA filters is recommended as the best option for filtering aerosols and carbon filtration is best for filtering radioactive particles.

Castillon, Erick↗

Radioactivities of Long Duration Exposure Facility (LDEF) materials: Baggage and bonanzas

Radioactivities in materials onboard the returned Long Duration Exposure Facility (LDEF) satellite were studied by a variety of techniques. Among the most powerful is low background Ge semiconductor detector gamma ray spectrometry. The observed radioactivities are of two origins: those radionuclides produced by nuclear reactions with the radiation field in orbit and radionuclides present initially as contaminants in materials used for construction of the spacecraft and experimental assemblies. In the first category are experiment related monitor foils and tomato seeds, and such spacecraft materials as Al, stainless steel, and Ti. In the second category are Al, Be, Ti, Va, and some special glasses. Consider that measured peak-area count rates from both categories range from a high value of about 1 count per minute down to less than 0.001 count per minute. Successful measurement of count rates toward the low end of this range can be achieved only through low background techniques, such as used to obtain the results presented here.

Smith, Alan R.↗

Radioactivities of Long Duration Exposure Facility (LDEF) materials: Baggage and bonanzas

Radioactivities in materials onboard the returned Long Duration Exposure Facility (LDEF) satellite were studied by a variety of techniques. Among the most powerful is low-background Ge-semiconductor detector gamma-ray spectrometry, illustrated here by results obtained at the Lawrence Berkeley Laboratory's (LBL) Low Background Facilities. The observed radioactivities are of two origins: those radionuclides produced by nuclear reactions with the radiation field in orbit, and radionuclides present initially as 'contaminants' in materials used for construction of the spacecraft and experimental assemblies. In the first category are experiment-related monitor foils and tomato seeds, and such spacecraft materials as aluminum, stainless steel, and titanium. In the second category are aluminum, beryllium, titanium, vanadium, and some special glasses.

Smith, Alan R.↗