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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2

Dynamic Radioactive Source for Evaluating and Demonstrating Time-dependent Performance of Continuous Air Monitors

Evaluation of continuous air monitors in the presence of a plutonium aerosol is time intensive, expensive, and requires a specialized facility. The Radiation Protection Services Group at Los Alamos National Laboratory has designed a Dynamic Radioactive Source, intended to replace plutonium aerosol challenge testing. Furthermore, the Dynamic Radioactive Source is small enough to be inserted into the sampler filter chamber of a typical continuous air monitor. Time-dependent radioactivity is introduced from electroplated sources for real-time testing of a continuous air monitor where a mechanical wristwatch motor rotates a mask above an alpha-emitting electroplated disk source. The mask is attached to the watch’s minute hand, and as it rotates, more of the underlying source is revealed. The alpha activity we measured increases with time, simulating the arrival of airborne radioactive particulates at the air sampler inlet. The Dynamic Radioactive Source allows the temporal behavior of puff and chronic release conditions to be mimicked without the need for radioactive aerosols. The new system is configurable to different continuous air monitor designs and provides an in-house testing capability (benchtop compatible). It is a repeatable and reusable system and does not contaminate the tested air monitor. Test benefits include direct user control, realistic (plutonium) aerosol spectra, and iterative development of continuous air monitor alarm algorithms. We also used data obtained using the Dynamic Radioactive Source to elucidate alarm algorithms and to compare the response time of two commercial continuous air monitors.

07 ISOTOPE AND RADIATION SOURCES↗

A Comparison of Cs-137 γ Rays and 320-kV X-Rays in a Mouse Bone Marrow Transplantation Model

US homeland security concerns regarding the potential misuse of some radiation sources used in radiobiological research, for example, cesium-137 ( 137 Cs), have resulted in recommendations by the National Research Council to conduct studies into replacing these sources with suitable X-ray instruments. The objective of this research is to compare the effectiveness of an X-RAD 320 irradiator (PXINC 2010) with a 137 Cs irradiator (Gammacell-1000 Unit) using an established bone marrow chimeric model. Using measured radiation doses for each instrument, we characterized the dose–response relationships for bone marrow and splenocyte ablation, using a cytotoxicity-hazard model. Our results show that the X-RAD 320 photon energy spectrum was suitable for ablating bone marrow at the 3 exposure levels used, similar to that of 137 Cs photons. However, the 320-kV X-rays were not as effective as the much higher energy γ rays at depleting mouse splenocytes. Furthermore, the 3 X-ray levels used were less effective than the higher energy γ rays in allowing the successful engraftment of donor bone marrow, potentially as a result of the incomplete depletion of the spleen cells. More defined studies are warranted for determining whether bone marrow transplantation in mice can be successfully achieved using 320-kV X-rays. A higher X-ray dose then used is likely needed for transplantation success.

320-kV X-rays↗

High Power UV LED Industrial Curing Systems

UV curing is a green technology that is largely underutilized because UV radiation sources like Hg Lamps are unreliable and difficult to use. High Power UV LEDs are now efficient enough to replace Hg Lamps, and offer significantly improved performance relative to Hg Lamps. In this study, a modular, scalable high power UV LED curing system was designed and tested, performing well in industrial coating evaluations. In order to achieve mechanical form factors similar to commercial Hg Lamp systems, a new patent pending design was employed enabling high irradiance at long working distances. While high power UV LEDs are currently only available at longer UVA wavelengths, rapid progress on UVC LEDs and the development of new formulations designed specifically for use with UV LED sources will converge to drive more rapid adoption of UV curing technology. An assessment of the environmental impact of replacing Hg Lamp systems with UV LED systems was performed. Since UV curing is used in only a small portion of the industrial printing, painting and coating markets, the ease of use of UV LED systems should increase the use of UV curing technology. Even a small penetration of the significant number of industrial applications still using oven curing and drying will lead to significant reductions in energy consumption and reductions in the emission of green house gases and solvent emissions.

42 ENGINEERING↗

Analyses of Dose Rates for Second Inner Reflector Plug Replacement at Spallation Neutron Source

The Inner Reflector Plug (IRP) is a central component of the Spallation Neutron Source (SNS) target monolith, which houses the liquid mercury target and four liter-sized neutron moderator units. It is exposed to high-level radiation fields during routine operation and builds up significant activity. The IRP needs to be replaced due to moderator neutron poison and decoupler burn-out, which is used for shaping neutron pulses. The first IRP exchange took place in March 2018 and next one, which is IRP2, is planned to be replaced during the facility maintenance period in the end of December 2025, beginning of January 2026 calendar year. The replacement of IRP is a complex task due to its location in the area receiving high irradiation, being under significant amount of shielding, and size, which requires removal in segments. For planning the replacement workflow to help to reduce radiation exposure to workers dose rates for each stage of extraction/replacement operation are predicted.

42 ENGINEERING↗

Normetex Pump Alternatives Study

A mainstay pump for tritium systems, the Normetex scroll pump, is currently unavailable because the Normetex company went out of business. This pump was an all-metal scroll pump that served tritium processing facilities very well. Current tritium system operators are evaluating replacement pumps for the Normetex pump and for general used in tritium service. An all-metal equivalent alternative to the Normetex pump has not yet been identified. 1. The ideal replacement tritium pump would be hermetically sealed and contain no polymer components or oils. Polymers and oils degrade over time when they contact ionizing radiation. 2. Halogenated polymers (containing fluorine, chlorine, or both) and oils are commonly found in pumps. These materials have many properties that surpass those of hydrocarbon-based polymers and oils, including thermal stability (higher operating temperature) and better chemical resistance. Unfortunately, they are less resistant to degradation from ionizing radiation than hydrocarbon-based materials (in general). 3. Polymers and oils can form gaseous, condensable (HF, TF), liquid, and solid species when exposed to ionizing radiation. For example, halogenated polymers form HF and HCl, which are extremely corrosive upon reaction with water. If a pump containing polymers or oils must be used in a tritium system, the system must be designed to be able to process the unwanted by-products. Design features to mitigate degradation products include filters and chemical or physical traps (eg. cold traps, oil traps). 4. Polymer components can work in tritium systems, but must be replaced regularly. Polymer components performance should be monitored or be regularly tested, and regular replacement of components should be viewed as an expected normal event. A radioactive waste stream must be established to dispose of used polymer components and oil with an approved disposal plan developed based on the facility location and its regulators. Polymers have varying resistances to ionizing radiation - aromatic polymers such as polyimide Vespel (TM) and the elastomer EPDM (ethylene propylene diene monomer) have been found to be more resistant to degradation in tritium than other polymers. This report presents information to help select replacement pumps for Normetex pumps in tritium systems. Several pumps being considered as Normetex replacement pumps are discussed.

07 ISOTOPE AND RADIATION SOURCES↗

Modeling Cell Survival Fraction and Other Dose-Response Relationships for Immunodeficient C.B-17 SCID Mice Exposed to 320-kV X Rays

US homeland security concerns related to potential misuse of γ-ray-emitting radiation sources employed in radiobiological research (eg, shielded cesium-137 irradiators) led to recommendations by the National Research Council to conduct studies into possibly replacing γ-ray irradiators used in research involving small rodent and other models with X-ray instruments. A limiting factor is suitability of the X-ray photon energy spectra. The objective of our research was to demonstrate the suitability of the radiation energy spectrum of 320-kV X rays after filtration (HVL = 4 mm Cu) for in-vivo cytotoxicity studies in immunodeficient C.B-17 SCID mice. By using a previously-published Hazard Function (HF) model to characterize dose-response relationships for in vivo bone marrow and spleen cell survival fractions and also to characterize the acute lethality risk (hematopoietic syndrome mode) we demonstrate that the filtered 320-kV X-ray beam appears suitable for such studies. A key finding for C.B-17 SCID mice when compared to results previously obtained for immunocompetent C.B-17 mice is that the immunodeficient mice appear to be more radioresistant, implicating a possible role of the immune system capacity in radiosensitivity of mammals.

Scott, Bobby R.↗

The Langley Parameterized Shortwave Algorithm (LPSA) for Surface Radiation Budget Studies

An efficient algorithm was developed during the late 1980's and early 1990's by W. F. Staylor at NASA/LaRC for the purpose of deriving shortwave surface radiation budget parameters on a global scale. While the algorithm produced results in good agreement with observations, the lack of proper documentation resulted in a weak acceptance by the science community. The primary purpose of this report is to develop detailed documentation of the algorithm. In the process, the algorithm was modified whenever discrepancies were found between the algorithm and its referenced literature sources. In some instances, assumptions made in the algorithm could not be justified and were replaced with those that were justifiable. The algorithm uses satellite and operational meteorological data for inputs. Most of the original data sources have been replaced by more recent, higher quality data sources, and fluxes are now computed on a higher spatial resolution. Many more changes to the basic radiation scheme and meteorological inputs have been proposed to improve the algorithm and make the product more useful for new research projects. Because of the many changes already in place and more planned for the future, the algorithm has been renamed the Langley Parameterized Shortwave Algorithm (LPSA).

Gupta, Shashi K.↗

Search for heavy Majorana neutrinos in pp collisions at √s = 8 TeV with the CMS detector & photodetector and calorimeter R&D for particle colliders

This thesis contains both physics analysis and hardware studies. It consists of two primary sections: the results of a search for heavy Majorana mass neutrinos, using the event signature of same (like) sign charged electron pairs ($e^{\pm} e^{\pm}$ ) and two jets, and the results of studies to upgrade the Hadronic Forward (HF) and Hadronic Endcap (HE) subdetectors in the Compact Muon Solenoid (CMS) detector in response to the high intensity proton-proton collisions generated at the Large Hadron Collider (LHC) at European Organization for Nuclear Research (CERN, Conseil Europ\'{e}en pour la Recherche Nucl\'{e}aire). In this search for Majorana mass neutrinos, same sign dielectron ($e^{\pm} e^{\pm}$) + dijet events in the final state have been considered as a signature for neutrino particles. The analyzed data corresponds to an integrated luminosity of 19.7 fb\textsuperscript{-1} of proton-proton collisions at a center of mass energy of $\sqrt{s} = 8 \text{TeV}$, collected using the CMS detector during the 2012 operation at the LHC. Monte Carlo simulations accounting for the theoretical expectations of the Standard Model (SM) and the detector limitations are used to prototype the experiment and to test proposed analysis steps. No excess of events is observed in the data beyond the expected SM background. Upper limits are set on the mixing element squared, $|{V}_{eN}|^{2}$, of the heavy Majorana neutrino with standard model neutrinos, as a function of Majorana neutrino mass for masses in the range of 40-500 $GeV/c^2$. The detector upgrade search comprises three sections of this thesis. The first section describes the test results of 1785 multianode Hamamatsu R7600U-200-M4 photomultiplier tubes (PMT) in numerous parameters such as gain, dark current, and timing characteristics, which provide insights on the expected performance of the upgraded CMS-HF detector. These PMTs replaced the previous single anode R7525 PMTs because the glass windows of previous PMTs are the source of Cherenkov radiation, which causes a background noise in the experiment. The second section reports characterization results of two types of PMTs in a novel operation mode for Secondary Emission (SE) Ionization Calorimetry, which is a novel technique to measure electromagnetic shower particles in extreme radiation environments. The third section presents the test results of novel scintillating materials for CMS experiment in specific and future particle accelerators in general. These materials are Polyethylene Naphthalate (PEN), Polyethylene Terephthalate (PET), high efficiency mirror (HEM) and quartz plates with various organic and inorganic coating materials such as p-Terphenyl (pTp), Anthracene and Gallium-doped Zinc Oxide (ZnO:Ga). We have investigated them for radiation hardness, light yield, timing characteristics, and scintillation and transmission properties.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Summary of Analytical Services for the Hanford Site Radionuclide NESHAP Program

This document is a summary of the point source analytical requirements used to demonstrate compliance for the Department of Energy (DOE) Hanford Site operations with 40 Code of Federal Regulations (CFR) Part 61, “National Emission Standards for Hazardous Air Pollutants,” (NESHAP) Subpart H, “National Emission Standards for Emissions of Radionuclides Other Than Radon From Department of Energy Facilities,” and the Washington Administrative Code (WAC) 246-247, “Radiation Protection – Air Emissions.” This reference collects information from multiple source documents and is not intended to create, supersede, replace or over-ride any existing contractual, DOE, federal or state statutes, regulations, compliance agreements, orders, permits, licenses or other requirements. The requirement source document governs where any difference may exist. The Hanford Mission Integration Solutions (HMIS) Environmental organization has been contracted by DOE to manage and report data collected from the sampling and monitoring of radioactive air emissions point sources, colloquially called stacks. The Environmental organization coordinates the analyses and reporting of samples collected at various facilities across the Hanford Site. These facilities operate approximately 52 stacks that require sampling, monitoring or estimating radioactive air emissions. The stacks are operated by Bechtel National, Inc. (BNI), Central Plateau Cleanup Company (CPCCo), Hanford Tank Waste Operations & Closure (H2C), Hanford Laboratory Management and Integration (HLMI), and Pacific Northwest National Laboratory (PNNL). Stack samples from CPCCo, HLMI and H2C facilities are collected by the operating contractor staff, delivered to HMIS, and then shipped to an offsite contracted laboratory for analyses. The field and laboratory sample data uploaded into the Sample Management and Analytical Results Tracking (SMART) database are used to calculate sample volumes and concentrations. Sample concentrations are evaluated for compliance with federal and state regulations, permits, and license requirements. The SMART database also calculates total curies released for sampled point sources and stacks. Point source effluent concentrations and releases are published annually in publicly available reports. The BNI and PNNL operate several DOE-Hanford Field Office (HFO) stacks subject to the requirements of 40 CFR 61, Subpart H and WAC 246-247. The concentrations, curies released and dose modeling evaluation for these stacks are included in the DOE-HFO annual radionuclide NESHAP report. The sample collection, analyses and emissions estimates for these stacks are outside the scope of HMIS contracted responsibilities and not addressed further in this document.

54 ENVIRONMENTAL SCIENCES↗

Complete time-resolved X-ray shape capability for a 10 MJ implosion: Milestone Report for MRT 8818

This report documents completion of MRT 8818, which established an upgraded equatorial time-resolved X-ray imaging capability for high-yield inertial confinement fusion experiments at the National Ignition Facility (NIF) using the equatorial Dilation X-ray Imager (DIXI). The need for this work arose from the sustained increase in fusion yield at NIF, which progressively intensified the neutron and gamma-ray environment experienced by target diagnostics. Although the existing polar imaging capability, particularly the Polar Dilation X-ray Imager (PDIXI), remained viable at high yields, the equatorial capability became inadequate because of radiation-induced failure of electronic readout hardware and increasing background levels that degraded image quality and ultimately caused saturation. The work performed under MRT 8818 addressed this limitation through a combination of hardware replacement, background characterization, and targeted mitigation. The DIXI backend was converted from CCD-based electronic readout to photographic film, and the principal sources of internally generated background were investigated using prior analyses, dedicated tests, and comparison with PDIXI performance on high-yield shots. This effort led to implementation of two principal improvements: a multilayer optical coating to suppress broadband radiation-induced background generated in the fiber-optic extension cylinder, and replacement of Kodak TMAX 400 film with Agfa Copex Rapid to reduce background generated directly in the film. These upgrades were completed in 2025 and performance assessment based on DT shot data since then, comparing with Polar DIXI and scaling of these experiments to 10 MJ indicates an expected signal-to-background ratio of approximately 34 for a single pinhole image, substantially exceeding the MRT 8818 completion criterion of SNR > 5.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Modeling of Am-241 as an alternative fuel source in a radioisotope thermoelectric generator

Radioisotope thermoelectric generators (RTGs) have been utilized in the USA to power satellites and space exploration equipment for over half a century. In our preceding paper, Dustin and Borrelli (2021), we assessed the performance of 241 Am as an alternative to 238 Pu by modeling the specific decay-heat and gamma spectra of several potential radioisotopes in SCALE-ORIGEN, and comparing these with 238 Pu An analysis of heat output, heat stability, safety, availability and required mass showed that of the isotopes reviewed, 241 Am had the greatest potential for replacing 238 Pu, with additional design considerations. In our current work, we have assessed radiation transport for two configurations of an 241 Am powered Multi-Mission Radioisotope Thermoelectric Generator (MMRTG), due to the potential health effects for operators, fabricators, and others with the potential to be exposed to neutrons and lower energy gamma rays. We have modeled the use of americium as a fuel source replacement for plutonium in current MMRTG designs. The assessment has been performed using MCNP6, in terms of neutron and gamma emissions that might interfere with sensitive equipment and power system production. The radiation transport behavior in terms of dose rate of the 241 Am fueled models is compared with that of a 238 Pu fueled model. Finally, additional work was performed to validate modeling simplifications with regards to thermocouple material configurations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Characterizing the radiation response of Cherenkov glass detectors with isotopic sources

Abstract Cherenkov detectors are widely used for particle identification and threshold detectors in high-energy physics. Glass Cherenkov detectors that are sensitive to beta emissions originating from neutron activation have been demonstrated recently as a potential replacement for activation foils. In this work, we set the groundwork to evaluate large Cherenkov glass detectors for sensitivity to MeV photons through first understanding the measured response of small Cherenkov glass detectors to isotopic gamma-ray sources. Counting and pulse height measurements are acquired with reflected glass Cherenkov detectors read out with a photomultiplier tube. Simulation was used to inform our understanding of the measured results. This simulation included radioactive source decay, radiation interaction, Cherenkov light generation, optical ray tracing, and photoelectron production. Implications for the use of Cherenkov glass detectors to measure low energy gammaray response are discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Comparative Effects of Radiation Sterilization Modality on Medical PVC Tubing

As the production volume of single-use, polymer-based medical devices increases each year, so does the need for throughput capacity to sterilize the devices. Around 80% of radiation-sterilized devices are processed using gamma-ray radiation from industrial cobalt-60 sources. Supply chain, security, and disposal concerns are prompting manufacturers and contract sterilizers to explore alternatives to irradiation using cobalt-60 gamma-rays, such as electron beam (E-beam) and X-ray radiation. Advantages of these ‘machine’ sources over radioisotope-based sources are that they do not decay, a characteristic that requires cobalt-60 to be replaced over time, they can be turned off when not in use, and they do not represent the same level of concern regarding misuse. One of the barriers to direct transition from gamma-ray sterilization to E-beam or X-ray sterilization is concern over the relatively unknown effects of sterilization dose of these alternative modalities on the performance of medical device polymers. Commercially available medical devices sterilized with gamma-ray irradiation exhibit acceptable device function, acceptable mechanical performance, and acceptable discoloration. To be viable, alternate sterilization methods must not only achieve acceptable sterilization, but the process must also result in a product with functional, mechanical, and visual effects acceptable to customers and the regulator. Flexible polyvinyl chloride (PVC) is a plastic material that is commonly found in single-use medical devices and is known for its sensitivity to radiation processing. For instance, transparent PVC is known to yellow upon irradiation. To encouraging sterilization alternatives to cobalt-60 gamma-ray, we directly compared the effects of gamma-ray, E-beam, and X-ray radiation exposure at similar sterilization-relevant doses on key properties of medical grade PVC tubing.

cobalt-60↗

Experimental Results From a 2kW Brayton Power Conversion Unit

This paper presents experimental test results from operation of a 2 kWe Brayton power conversion unit. The Brayton converter was developed for a solar dynamic power system flight experiment planned for the Mir Space Station in 1997. The flight experiment was cancelled, but the converter was tested at Glenn Research Center as part of the Solar Dynamic Ground Test Demonstration system which included a solar concentrator, heat receiver, and space radiator. In preparation for the current testing, the heat receiver was removed and replaced with an electrical resistance heater, simulating the thermal input of a steady-state nuclear source. The converter was operated over a full range of thermal input power levels and rotor speeds to generate an overall performance map. The converter unit will serve as the centerpiece of a Nuclear Electric Propulsion Testbed at Glenn. Future potential uses for the Testbed include high voltage electrical controller development, integrated electric thruster testing and advanced radiator demonstration testing to help guide high power Brayton technology development for Nuclear Electric Propulsion (NEP).

Hervol, David↗

Summary of Analytical Services for the Hanford Site Radionuclide NESHAP Program

This document serves as a summary of the analytical requirements used to demonstrate compliance on the Department of Energy (DOE) Hanford Site to 40 CFR 61, “National Emission Standards for Hazardous Air Pollutants,” (NESHAP) Subpart H, “National Emission Standards for Emissions of Radionuclides Other Than Radon From Department of Energy Facilities,” and WAC 246-247, “Radiation Protection – Air Emissions.” This document is a reference summarizing information from multiple existing requirement source documents and does not create, supersede, replace or over-ride any existing contractual, DOE, federal, state, permit or license requirement. The requirement source documents govern where any differences may exist.

54 ENVIRONMENTAL SCIENCES↗

Diffusion model for lightning radiative transfer

A one-speed Boltzmann transport theory, with diffusion approximations, is applied to study the radiative transfer properties of lightning in optically thick thunderclouds. Near-infrared (lambda = 0.7774 micrometers) photons associated with a prominent oxygen emission triplet in the lightning spectrum are considered. Transient and spatially complex lightning radiation sources are placed inside a rectangular parallelepiped thundercloud geometry and the effects of multiple scattering are studied. The cloud is assumed to be composed of a homogeneous collection of identical spherical water droplets, each droplet a nearly conservative, anisotropic scatterer. Conceptually, we treat the thundercloud like a nuclear reactor, with photons replaced by neutrons, and utilize standard one-speed neutron diffusion techniques common in nuclear reactor analyses. Valid analytic results for the intensity distribution (expanded in spherical harmonics) are obtained for regions sufficiently far from sources. Model estimates of the arrival-time delay and pulse width broadening of lightning signals radiated from within the cloud are determined and the results are in good agreement with both experimental data and previous Monte Carlo estimates. Additional model studies of this kind will be used to study the general information content of cloud top lightning radiation signatures.

Koshak, William J.↗

Dose received by occupationally exposed workers at a nuclear medicine department

Personal Dose Equivalent (PDE) values were determined for occupational exposed workers (OEW) at the Nuclear Medicine Department (NMD) of 'Instituto Nacional de Cancerologia' (INCan), Mexico, using TLD-100 thermoluminescent dosemeters. OEW at NMD, INCan make use of radiopharmaceuticals for diagnosis and treatment of diseases. Radionuclides associated to a pharmaceutical compound used at this Department are {sup 131}I, {sup 18}F, {sup 68}Ga, {sup 99m}Tc, {sup 111}In and {sup 11}C with main gamma emission energies between 140 and 511 keV. Dosemeter calibration was performed at the metrology department of 'Instituto Nacional de Investigaciones Nucleares' (ININ), Mexico. Every occupational worker used dark containers with three dosimeters which were replaced monthly for a total of 5 periods. Additionally, control dosemeters were also placed at a site free of radioactive sources in order to determine the background radiation. Results were adjusted to find PDE/day and estimating annual PDE values in the range between 2 mSv (background) and 9 mSv. The mean annual value is 3.51 mSv and the standard deviation SD is 0.78 mSv. Four of the 16 OEW received annual doses higher than the average +1 SD (4.29 mSv). Results depend on OEW daily activities and were consistent for each OEW for the 5 studied periods as well as with PDE values reported by the firm that performs the monthly service. All obtained values are well within the established annual OEW dose limit stated in the {sup R}eglamento General de Seguridad Radiologica{sup ,} Mexico (50 mSv), as well as within the lower limit recommended by the 'International Commission on Radiation Protection' (ICRP), report no.60 (20 mSv). These results verify the adequate compliance of the NMD at INCan, Mexico with the norms given by the national regulatory commission.

61 RADIATION PROTECTION AND DOSIMETRY↗