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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Characterizing sample degradation from synchrotron based X-ray measurements of ultra-thin exfoliated flakes

It is undeniable that novel 2D devices and heterostructures will have a lasting impact on the advancement of future technologies. However, the inherent instability of many exfoliated van der Waals (vdW) materials is a well-known hurdle yet to be overcome. Thus, the sustained interest in exfoliated vdW materials underscores the importance of understanding the mechanisms of sample degradation to establish proactive protective measures. Here, the impact of prolonged synchrotron-based X-ray beam exposure on exfoliated flakes of two contemporary vdW materials, NiPS 3 and α-RuCl 3 , is explored using resonant inelastic X-ray scattering (RIXS) and total fluorescence yield X-ray absorption spectroscopy (XAS). In NiPS 3 , the resulting RIXS and XAS spectra show a suppression, then vanishing, of NiS 6 multiplet excitations coupled with an upward shift of the peak energy of the XAS as a function of X-ray dose. In α-RuCl 3 , the signs of beam damage from the RIXS spectra are less evident. However, the post-experiment characterization of both materials using Raman spectroscopy exhibits signals of an amorphous and disordered system compared to pristine flakes; in addition, energy-dispersive X-ray spectroscopy of NiPS 3 shows evidence of ligand vacancies. As synchrotron radiation is fast becoming a required probe to study 2D vdW materials, these findings lay the groundwork for the development of future protective measures for synchrotron-based prolonged X-ray beam exposure, as well as for X-ray free electron laser.

2D magnetism↗
NASA NTRS2001

A Broad-Band X-Ray Study of the Geminga Pulsar

We present a comprehensive study of the Geminga pulsar at energies 0.1-10 keV using data from the ASCA, ROSAT, and EUVE satellites. The bulk of the soft X-ray flux can be parameterized as a blackbody of T = (5.6 +/- 0.6) x 10(exp 5) K, occupying a fraction 0. 10 - 0.64 of the surface area of the neutron star at the parallax distance of 160 pc. The ASCA detection of Geminga resolves the nature of the harder X-ray component previously discovered by ROSAT in favor of nonthermal emission, rather than thermal emission from a heated polar cap. The hard X-ray spectrum can be fitted by a power-law of energy index 1.0 +/- 0.5. The hard X-ray light curve has a strong main peak and a weak secondary peak; its total pulsed fraction is = 55%. Three ROSAT PSPC observations show significant variability of Geminga's light curve. In particular, a peculiar energy dependence of the modulation in the soft X-ray component, dubbed the "Geminga effect" in the original PSPC data, is not present in later observations. In addition, fine structure in the soft X-ray light curve, interpreted as eclipses due to cyclotron resonance scattering by a plasma screen on the closed magnetic field lines, almost disappeared in the most recent observations. All of the variable properties of Geminga can probably be associated with the nonthermal process that supplies e(sup +, sup -) pairs to its inner magnetosphere.

Halpern, Jules P.↗
DOE OSTI2025

Coupling of electronic transition to ferroelectric order in a 2D semiconductor

A ferroelectric material often exhibits a soft transverse optical (TO) phonon mode which governs its phase transition. Charge coupling to this ferroelectric soft mode may further mediate emergent physical properties, including superconductivity and defect tolerance in semiconductors. However, direct experimental evidence for such coupling is scarce. Here we show that a photogenerated coherent phonon couples strongly to the electronic transition above the bandgap in the van der Waals (vdW) two-dimensional (2D) ferroelectric semiconductor NbOI 2 . Using terahertz time-domain spectroscopy and first-principles calculations, we identify this mode as the TO phonon responsible for ferroelectric order. This exclusive coupling occurs only with the above-gap electronic transition and is absent in the valence band as revealed by resonant inelastic X-ray scattering. Our findings suggest a new role of the soft TO phonon mode in electronic and optical properties of ferroelectric semiconductors.

36 MATERIALS SCIENCE↗
NASA NTRS1992

Resonance scattering of Fe XVII - A density diagnostic

Resonance scattering of the 15.01 A Fe XVII line, found to be important by Rugge & McKenzie, provides a new density diagnostic for solar active regions that is not subject to the lower density limit of the competing diagnostic. For a 'typical' active region, over 50 percent of the photons for this resonance line could be scattered out of the line of sight. The effect is much stronger for this line than for any other line in the soft X-ray part of the spectrum used routinely to determine active region electron temperatures, emission measures, or densities. Once understood and accounted for in the analysis, the resonance scattering of the 15.01 A Fe XVII line leads to a direct measurement of the density of the active region plasma. In the four active regions studied here, the derived densities range is 1-4 x 10 exp 9/cu cm.

Schmelz, J. T.↗
NASA NTRS1974

A study of X-ray emission from galactic and extragalactic sources with emphasis on soft and ultra-soft wavelengths

A Black Brant VC rocket was used to scan the Coma and Virgo clusters in order to measure structure in the X-ray sources. The rocket also made measurements of soft X-ray spectra, soft X-ray background flux during a 50 deg scan of the sky, soft X-rays from De Voucoulers 50, set limits to the energy dependence of soft X-ray background spectra, and the flux of solar 584 A radiation resonantly scattered by interstellar He flowing through the solar system.

Bowyer, C. S.↗
NASA NTRS2022

High-energy Photon Opacity in the Twisted Magnetospheres of Magnetars

Magnetars are neutron stars characterized by strong surface magnetic fields generally exceeding the quantum critical value of 44.1 TG. High-energy photons propagating in their magnetospheres can be attenuated by QED processes like photon splitting and magnetic pair creation. In this paper, we compute the opacities due to photon splitting and pair creation by photons emitted anywhere in the magnetosphere of a magnetar. Axisymmetric, twisted dipole field configurations embedded in the Schwarzschild metric are treated. The paper computes the maximum energies for photon transparency that permit propagation to infinity in curved spacetime. Special emphasis is given to cases where photons are generated along magnetic field loops and/or in polar regions; these cases directly relate to resonant inverse Compton scattering models for the hard X-ray emission from magnetars and Comptonized soft gamma-ray emission from giant flares. We find that increases in magnetospheric twists raise or lower photon opacities, depending on both the emission locale and the competition between field-line straightening and field strength enhancement. Consequently, given the implicit spectral transparency of hard X-ray bursts and persistent "tail" emission of magnetars, photon splitting considerations constrain their emission region locales and the twist angle of the magnetosphere; these constraints can be probed by future soft gamma-ray telescopes such as COSI and AMEGO. The inclusion of twists generally increases the opaque volume of pair creation by photons above its threshold, except when photons are emitted in polar regions and approximately parallel to the field.

radiation mechanisms: non-thermal↗
DOE OSTI2025

X-Ray Polarization of the Magnetar 1E 1841−045

We report on IXPE and NuSTAR observations beginning 40 days after the 2024 outburst onset of magnetar 1E 1841−045, marking the first IXPE observation of a magnetar in an enhanced state. Our spectropolarimetric analysis indicates that both a blackbody (BB) plus double power-law (PL) and a double blackbody plus power-law spectral model fit the phase-averaged intensity data well, with a hard PL tail (Γ = 1.19 and 1.35, respectively) dominating above ≈5 keV. For the former model, we find the soft PL (the dominant component at soft energies) exhibits a polarization degree (PD) of ≈30% while the hard PL displays a PD of ≈40%. Similarly, the cool BB of the 2BB+PL model possesses a PD of ≈15% and a hard PL PD of ≈57%. For both models, each component has a polarization angle (PA) compatible with celestial north. Model-independent polarization analysis supports these results, wherein the PD increases from ≈15% to ≈70% in the 2–3 keV and 6–8 keV ranges, respectively, while the PA remains nearly constant. We find marginal evidence for phase-dependent variability of the polarization properties, namely a higher PD at phases coinciding with the hard X-ray pulse peak. We compare the hard X-ray PL to the expectation from resonant inverse Compton scattering (RICS) and secondary pair cascade synchrotron radiation from primary high-energy RICS photons; both present reasonable spectropolarimetric agreement with the data, albeit the latter does so more naturally. We suggest that the soft PL X-ray component may originate from a Comptonized corona in the inner magnetosphere.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2004

Chandra X-ray Observations of Jovian Low-latitude Emissions: Morphological, Temporal, and Spectral Characteristics

Chandra observed X-rays from Jupiter during 24-26 February 2003 for about 40 hours with the ACIS-S and HRC-I instruments. The analysis of Jovian low-latitude "disk" Xray emissions are presented and compared with the high-latitude "auroral" emissions. We report the first Chandra ACIS-S measured X-ray spectrum (0.3-2 keV) of Jupiter's low-latitude disk The disk X-ray emission is harder and extends to higher energies than the auroral spectrum. The temporal variation in the Jovian disk X-rays is on an average consistent with those in the solar X-rays observed by GOES, and TIMED/SSE. Contrary to the auroral X-rays, the disk emissions are uniformly distributed over Jupiter; no indication of longitudinal dependence or correlation with surface magneh field strength is visible. Also, unlike the approx. 40 +/- 20 min periodic oscillations seen in the auroral X-ray emissions, the disk emissions do not show any periodic oscillations. The disk spectrum seems to be consistent with resonant and fluorescent scattering of solar X-rays by the Jovian upper atmosphere. Jupiter's disk is found to be about 50% dimmer in soft X-rays in February 2003 compared that in December 2000, which is consistent with the decrease in solar activity. No evidence of lightning-induced X-rays is seen in the Chandra X-ray data. The Jovian disk spectra observed with Chandra-ACIS is stronger than that observed with XMM-Newton two months later during April 28-29, 2003. The XMM-Newton Xray image of Jupiter shows evidence of limb darkening on the anti-sunward side as seen from Earth, as well as an asymmetry with respect to the subsolar point: suggesting a solar driven process.

Bhardwaj, Anil↗
NASA NTRS1996

The Geminga Pulsar: Soft X-Ray Variability and an EUVE Observation

We observed the Geminga pulsar with the EUVE satellite, detecting pulsed emission in the Deep Survey imager. Joint spectral fits of the EUVE flux with ROSAT PSPC data are consistent with thermal plus power-law models in which the thermal component makes the dominant contribution to the soft X-ray flux seen by EUVE and ROSAT. The data are consistent with blackbody emission of T = (4-6) x 10(exp 5) K over most of the surface of the star at the measured parallax distance of 160 pc. Although model atmospheres are more realistic, and can fit the data with effective temperatures a factor of 2 lower, current data would not discriminate between these and blackbody models. We also find evidence for variability of Geminga's soft X-ray pulse shape. Narrow dips in the light curve that were present in 1991 had largely disappeared in 1993/1994, causing the pulsed fraction to decline from 32% to 18%. If the dips are attributed to cyclotron resonance scattering by an e(+/-) plasma on closed magnetic field lines, then the process that resupplies that plasma must be variable.

Halpern, Jules P.↗
NASA NTRS2001

The Geminga Pulsar: Soft X-Ray Variability and an EUVE Observation

We observed the Geminga pulsar with the EUVE satellite, detecting pulsed emission in the Deep Survey imager. Joint spectral fits of the EUVE flux with ROSAT PSPC data are consistent with thermal plus power-law models in which the thermal component makes the dominant contribution to the soft X-ray flux seen by EUVE and ROSAT. The data are consistent with blackbody emission of T = (4 - 6) x 10(exp 5) K over most of the surface of the star at the measured parallax distance of 160 pc. Although model atmospheres are more realistic, and can fit the data with effective temperatures a factor of 2 lower, current data would not discriminate between these and blackbody models. We also find evidence for variability of Geminga's soft X-ray pulse shape. Narrow dips in the light curve that were present in 1991 had largely disappeared in 1993/1994, causing the pulsed fraction to decline from 32% to 18%. If the dips are attributed to cyclotron resonance scattering by an e1 plasma on closed magnetic field lines, then the process that resupplies that plasma must be variable.

Halpern, Jules P.↗
DOE OSTI2024

Attosecond delays in X-ray molecular ionization

The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization. Accordingly, the past decade has produced a large volume of work on photoionization delays following single photon absorption of an extreme ultraviolet (XUV) photon. However, the measurement of time-resolved core-level photoionization remained out of reach. The required x-ray photon energies needed for core-level photoionization were not available with attosecond tabletop sources. We have now measured the x-ray photoemission delay of core-level electrons, and here report unexpectedly large delays, ranging up to 700 attoseconds in NO near the oxygen K-shell threshold. These measurements exploit attosecond soft x-ray pulses from a free-electron laser (XFEL) to scan across the entire region near the K-shell threshold. Furthermore, we find the delay spectrum is richly modulated, suggesting several contributions including transient trapping of the photoelectron due to shape resonances, collisions with the Auger-Meitner electron that is emitted in the rapid non-radiative relaxation of the molecule, and multi-electron scattering effects. Finally, the results demonstrate how x-ray attosecond experiments, supported by comprehensive theoretical modelling, can unravel the complex correlated dynamics of core-level photoionization.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1994

The composition of a coronal active region

The relative abundances of iron, oxygen, magnesium, and neon in a coronal active region are determined from measurements of soft X-ray line and broadband intensities. The emission measure, temperature, and column density are derived from these measured intensities and are used to place a constraint on the abundances of the heavier elements relative to hydrogen in the corona. The intensity measurements were made on 1987 December 11, when an active region was observed jointly by the American Science and Engineering (AS&E) High Resolution Soft X-Ray Imaging Sounding-Rocket Payload and the X-Ray Polychromator Flat Crystal Spectrometer (FCS) onboard the Solar Maximum Mission spacecraft. The coordinated observations include images through two broadband filters (8 to 29 A and 8 to 39, 44 to 60 A) and profiles of six emission lines: Fe XVII (15.01 A), FE VIII (15.26 A), O VIII (18.97 A), Mg XI (9.17 A), Ne IX (13.44 A), and Fe XVIII (14.21 A). The effects of resonance scattering are considered in the interpretation of the FCS line intensities. We calculated the expected intensity ratio of the two Fe XVII lines as a function of optical depth and compared this ratio with the observed intensity ratio to obtain the optical depths of each of the lines and the column density. The line intensities and the broadband filtered images are consistent with the emission from a thermal plasma where Fe, O, Mg, and Ne have the 'adopted coronal' abundances of Meyer (1985b) relative to one another, but are not consistent with the emission from a plasma having photospheric abundances: The ratios of the abundances of the low first ionization potential (FIP) elements (Fe and Mg) to the abundances of the high-FIP elements (Ne and O) are higher than the ratios seen in the photosphere by a factor of about 3.5. This conclusion is independent of the assumption of either an isothermal or a multithermal plasma. The column densities derived from the Fe XVII line ratio and the geometry of the active region provide a diagnostic of the abundance of hydrogen relative to the heavier elements. We find that the abundance of iron with respect to hydrogen in the corona is higher than the value given Meyer (1985b) by a factor of 8.2(-5.4, +5.1). This means that, for the observed active region, the absolute abundances of the low-FIP elements (Fe and Mg) are enhanced in the corona relative to the photosphere, while the abundances of the high-FIP elements (Ne and O) are either slightly enhanced in the corona or nearly the same in the photosphere and the corona.

Waljeski, K.↗
NASA NTRS2021

X-ray Emission from Magnetized Neutron Star Atmospheres at Low Mass Accretion Rates

Recent observations of X-ray pulsars at low luminosities allow, for the first time, to compare theoretical models for the emission from highly magnetized neutron star atmospheres at low mass accretion rates ( M ≲ 10(exp 15) g s(exp -1)) with the broadband X-ray data. The purpose of this paper is to investigate the spectral formation in the neutron star atmosphere at low M and to conduct a parameter study of physical properties of the emitting region. We obtain the structure of the static atmosphere, assuming that Coulomb collisions are the dominant deceleration process. The upper part of the atmosphere is strongly heated by the braking plasma, reaching temperatures of 30–40 keV, while its denser isothermal interior is much cooler (~2 keV). We numerically solve the polarized radiative transfer in the atmosphere with magnetic Compton scattering, free-free processes, and non-thermal cyclotron emission due to possible collisional excitations of electrons. The strongly polarized emitted spectrum has a double-hump shape that is observed in low-luminosity X-ray pulsars. A low-energy “thermal” component is dominated by extraordinary photons that can leave the atmosphere from deeper layers due to their long mean free path at soft energies. We find that a high-energy component is formed due to resonant Comptonization in the heated non-isothermal part of the atmosphere even in the absence of collisional excitations. The latter, however, affect the ratio of the two components. A strong cyclotron line originates from the optically thin, uppermost zone. A fit of the model to NuSTAR and Swift/XRT observations of GX304􀀀1 provides an accurate description of the data with reasonable parameters. The model can thus reproduce the characteristic double-hump spectrum observed in low-luminosity X-ray pulsars and provides insights into spectral formation.

X-Ray binaries↗
NASA NTRS1992

Coronal abundances in solar active regions measured by the Solar Maximum Mission flat crystal spectrometer

High resolution soft X-ray spectra acquired by the Flat Crystal Spectrometer (FCS) on solar Maximum Mission provide an excellent data base to study the relative abundances of O, Ne, Mg, and Fe in solar active regions. The FCS data show significant variability for all combinations of these elements. The largest variation occurs for Fe:Ne, which shows region to region changes of up to a factor of 7, and frequent factor of 2 variations in day to day samples of a given region. The atomic data and the ionization balance calculations used to interpret the line ratios affect the actual abundance values obtained, but have little effect on the magnitude of the total range of variation inferred. Resonance scattering of Fe XVII could cause a systematic offset in the abundances determined, but cannot be responsbile for the bulk of the observed variability. While abundance variability complicates the derivation of plasma parameters from spectroscopic measurements, it should offer exciting new clues to the processes which form and heat the corona.

Saba, Julia L. R.↗
NASA NTRS1985

Photoionization models for the wind from TW Vir

Line profiles are examined for the resonance doublets of the ions C IV, Si IV, and N V in the spectrum of the dwarf nova TW Virginis as observed by Cordova and Mason (1982). Line strengths depend on the abundances of the scattering ions and hence on the physical characteristics in the stellar wind. Results of the study show that the observed UV line ratios from TW Vir cannot be produced by photoionization by either an unattenuated single bremsstrahlung or by a single blackbody spectrum. Satisfactory values of the abundance ratios can be produced by bremsstrahlung spectra extending into the X-ray region which have low-energy cutoffs near the N IV threshold energy at 77 eV and have fluxes corresponding to an ionization parameter xi-sub-br of about 10. A finding that the flux in the soft X-ray bremsstrahlung component must exceed the EUV blackbody flux by at least an order of magnitude has implications for theories of the continuum emission from cataclysmic variables.

Kallman, T.↗
NASA NTRS2013

Suzaku View of the Neutron Star in the Dipping Source 4U 1822-37

The dipping X-ray source 4U 1822−37 was observed by Suzaku on 2006 Octrober 20 for a net exposure of 37 ks. The source was detected with the XIS at a 1-10 keV flux of 5.5 ×10(exp −10) erg per square centimeter per second, and with the HXD (HXD-PIN) at a 10-50 keV flux of 8.9 ×10(exp −10) erg per square centimeter per second. With HXD-PIN, the pulsation was detected at a barycentric period of 0.592437 seconds, and its change rate was reconfirmed as −2.43 × 10(exp −12) seconds per second. The 1-50 keV spectra of 4U 1822-37 were found to be very similar to those of Her X- 1 in the slopes, cutoff and iron lines. Three iron lines (Fe Kalpha, Fe XXV, and Fe XXVI) were detected, on top of a 1-50 keV continuum that is described by an NPEX model plus a soft blackbody. In addition, a cyclotron resonance scattering feature was detected significantly ( greater than 99% confidence), at an energy of 33+/-2 keV with a depth of 0.4(sup +0.6)/(sub −0.3). Therefore, the neutron star in this source is concluded to have a strong magnetic field of 2.8 × 10(exp 12) G. Further assuming that the source has a relatively high intrinsic luminosity of several times 10(exp 37) erg per second, its spectral and timing properties are consistently explained.

Stars: magnetic field↗
DOE OSTI2025

Pair Cascades in Magnetar Magnetospheres

Resonant inverse Compton scattering (RICS) of soft thermal photons by relativistic particles on closed magnetic field loops has been proposed to explain the hard emission observed up to and beyond 200 keV from magnetars. If particles injected at the base of the loops have Lorentz factors ≳10 2 , the RICS spectra will be attenuated by both one-photon pair production and photon splitting in the ultrastrong magnetar fields, producing additional spectral components from pair synchrotron radiation and split photons that produce further generations of pairs and split photons. We investigate such cascades initiated by the primary injected electrons through a Monte Carlo simulation, and study the cascade spectra and pair distributions. For most observer angles, the pair synchrotron and split-photon spectra dominate the RICS primary spectra and produce complex polarization signals. In particular, the synchrotron spectra are highly polarized with degree 40%–80%, are softer than the RICS spectra, and may account for the high polarization of some magnetar spectra observed by the Imaging X-ray Polarimetry Explorer above 3 keV.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1995

The soft gamma-ray spectrum of A0535+26: Detection of an absorption feature at 110 keV by OSSE

We present soft gamma-ray observations by the Oriented Scintillation Spectrometer Experiment (OSSE) on the Compton Gamma Ray Observatory (GRO) of the transient X-ray binary pulsar A0535+26. The observations were made 1994 February 8-17, immediately prior to the peak of a giant outburst. The phase averaged spectrum is complex and cannot be described by a single-component model. We find that structure in the spectrum above 100 keV can best be modeled by an absorption feature near 110 keV, which we interepret as the signature of cyclotron resonant scattering. Because of OSSE's 45 keV threshold, we are unable to make a definitive statement on the presence of a 55 keV absorption line; however, we can conclude that if this line does exist, it must have a smaller optical depth than the line at 110 keV. A first harmonic (=fundamental) cyclotron resonance at 110 keV corresponds to a magnetic field strength at the surface of the neutron star of approximately 1 x 10(exp 13) G (approximately 5 x 10(exp 12) G if the first harmonic is at 55 keV).

Grove, J. E.↗