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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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34 records · Page 2

Toward the Discovery of New Elements: Production of Livermorium (𝑍 = 116) with 50 Ti

The 244 Pu ⁢(50 Ti ,𝑥⁢𝑛)⁢ 294−𝑥 Lv reaction was investigated at Lawrence Berkeley National Laboratory’s 88-Inch Cyclotron. The experiment was aimed at the production of a superheavy element with 𝑍 ≥114 by irradiating an actinide target with a beam heavier than 48 Ca. Produced Lv ions were separated from the unwanted beam and nuclear reaction products using the Berkeley Gas-filled Separator and implanted into a newly commissioned focal-plane detector system. Two decay chains were observed and assigned to the decay of 290 Lv . The production cross section was measured to be 𝜎 prod = 0.44($^{+0.58}_{−0.28}$) pb at a center-of-target center-of-mass energy of 220(3) MeV. Furthermore, this represents the first published measurement of the production of a superheavy element near the “island of stability,” with a beam of 50 Ti and is an essential precursor in the pursuit of searching for new elements beyond 𝑍 =118.

36 MATERIALS SCIENCE↗

Advancements in nuclear data evaluations in the unresolved resonance region [Slides]

Minimal updates to current capabilities (SAMMY/AMPX) and to the ENDF format are proposed to include threshold reaction for outgoing charged-particle channels in the URR formalism. If average resonance parameters are reported, probability tables for newly defined reactions channels may be needed, implemented, and tested. Nuclear data evaluation of n+ 35 Cl reactions can be considered the best case to apply the proposed updates.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterization of the Multi-Coincident Bismuth Germanate Oxide Spectrometer at the Nuclear Counting Facility

A multi-detector γ-ray spectroscopy system including 3 high-purity germanium (HPGe) detectors has been developed at the Nuclear Counting Facility at Lawrence Livermore National Laboratory. This system operates not only in conventional singles γ-ray detection mode but also incorporates features like coincidence and anti-coincidence techniques. These advanced detection modes can significantly enhance the system’s sensitivity, making it a powerful tool for isotope identification and quantification, especially for complex samples with high background and overlapping peaks. In this re port, we present a comprehensive performance characterization of the Multi-Coincident Bismuth Oxide Spectrometer (MCBOS) using a variety of sample types, including 60 Co, 48 Sc, and mixed fission product samples. Each sample provides unique tests for the MCBOS capabilities. Additionally, a GEANT4 model of the MCBOS has been generated to aid with the characterization of the system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Joint Sample Analyses of Nuclear Forensic Materials Provided by the Republic of Kazakhstan: U. S. Laboratory Results

This document serves as an interim report to summarize sample analyses performed by Lawrence Livermore National Laboratory (LLNL) and Los Alamos National Laboratory (LANL) on a series of five nuclear forensics samples provided by the Institute of Nuclear Physics (INP) in the Republic of Kazakhstan. The sample set contains four uranium oxide powders and one low-enriched uranium fuel pellet. The samples were provided as part of a broader collaboration that involved a set of joint sample analyses conducted by INP and the US National Laboratories. The joint analyses are being conducted using well-developed analytical plans. These activities are designed to support the advancement of nuclear forensic science and capacity building in all three institutes in both countries. This report builds upon an earlier preliminary summary of the joint interactions and will be augmented by a final report. The final report will summarize the results and value of all sample analyses performed at the three institutes (INP, LLNL, and LANL). The final report will also provide an intercomparison of the results, analytical methods and best practices employed, as well as outline future collaborative nuclear forensics activities that are being developed in the Kazakhstan region.

and nuclear chemistry↗

Using radiochemistry to diagnose fuel-ablator mix in inertial confinement fusion studies at the National Ignition Facility: measurement of Tc/Mo isotopic ratios for the Pushered Single Shell campaign

The development of radiochemical measurement techniques as a diagnostic for fusion experiments at the National Ignition Facility enables a new method for assessing fuel-ablator mix and the impact of this mix on capsule performance. Diagnosing capsule mix in internal confinement fusion studies is difficult due to the small spatial scales (10s of µm) and short-time frames (100s of ps) over which the mix typically evolves in these experiments. For the Pushered Single Shell campaign, radiochemical measurements on debris collected from fusion experiments can be used to determine isotopic ratios of activation products, particularly 96g Tc/ 99 Mo and 95g Tc/ 99 Mo, to provide vital information on nuclear reactions in the burning plasma that can inform simulations that seek to understand the degree of capsule-fuel mix and the impact on the capsule performance. These radiochemical measurements have been conducted regularly since November 2023 providing data on a range of capsule designs and neutron yields. Data from eight NIF experiments is presented, the measured 96g Tc/ 99 Mo and 95g Tc/ 99 Mo range from (0.5–5) × 10 –4 to (0.3–3) × 10 –4 , respectively. The development of radiochemical diagnostics aids in understanding and optimizing the design of fusion experiments, providing unique and valuable insights into capsule behavior and directly measuring fuel-ablator mix.

and nuclear chemistry↗

Assessment of rare earth element fractionation in NIF implosions with radiochemically doped capsules

An ongoing experimental campaign at the National Ignition Facility (NIF) aims to measure neutron induced nuclear reaction cross–sections using radiochemically doped target capsules. Critical to this campaign is the ability to collect a representative sample of the reaction products using Solid Radiochemical Collectors (SRCs) fielded around the NIF chamber. The shot presented in this paper used a doped target capsule with a neopentane gas fill was to investigate the ratio of isotopes collected at three chamber angles. It was found that SRC samples of rare earth elements collected from NIF are representative of the ingoing dopant mix, thereby concluding that fractionation does not occur during a NIF implosion. This validates the doped capsule method for use in measuring neutron induced reaction cross-sections.

Capsule Doping↗

Unlocking the Path to Decarbonized Building Thermal Systems: Strategies for Designers and Contractors: Preprint

The design and construction community plays a pivotal role in facilitating the transition to decarbonized thermal systems that maintain human comfort while reducing building emissions. Through the U.S. Department of Energy Better Buildings initiative's Design and Construction Allies, a cohort of leading architecture, engineering, and construction firms have identified top ranked barriers that designers and contractors face when implementing solutions for building owners. These barriers to decarbonizing thermal - especially heating - systems include equipment availability; electrical capacity constraints; space allocations; complex system configurations; and lack of experience in designing, installing, and maintaining heat pumps. These impediments significantly amplify the risk and financial burden associated with the adoption of decarbonized solutions. The barriers also decrease the likelihood that designers, contractors, and owners will adopt decarbonization strategies without clear plans and guidance on how to implement these solutions, mitigate risk, and overcome the identified barriers. The National Renewable Energy Laboratory, the Design and Construction Allies, and the American Society of Heating, Refrigerating, and Air-Conditioning Engineers have developed "how to" thermal decarbonization guidance based on best practices. The subjects covered range from the role of energy efficiency in facilitating decarbonized heating solutions to strategies for decarbonizing new and existing heating, ventilating, and air-conditioning systems. The focus is on overcoming barriers so that energy-efficient, electrified buildings - both new and retrofit - become the industry standard. This paper outlines 1) the method used to collect and organize this guidance, 2) industry barriers to decarbonization, and 3) decarbonization techniques that have broad market applicability.

building heating↗

From Chills to Thrills: Revolutionizing Energy Efficiency and Load Flexibility in Supermarket Refrigeration

Open-vertical medium-temperature refrigerated display cases comprise nearly 50% of total case lineups in a typical supermarket, with more than 80% of their cooling load attributed to infiltration of warm and moist air from the surrounding space. The infiltration takes place across the air curtain system of the display case. While the air curtain acts as a thermal shield and as a cooling mechanism to maintain product temperature, it also entrains large amounts of heat and moisture from the adjacent space. Additionally, from food safety and quality standpoints, these fixtures are vulnerable to electric outages and traditionally cannot participate in load flexibility events. This paper describes key features of an innovative design of a self-contained, water-cooled, medium-temperature, open-vertical display case. The novel concept will eliminate the inefficient air curtain system and incorporate a hybrid radiant and low-airflow convective cooling design with a thermal-energy-storage-coupled heat exchanger integrated into the refrigeration circuit. The focus of this paper is on evaluating the thermal performance of the novel hybrid design in maintaining target product temperature. It presents thermal performance findings from thermo-fluid system modeling and robust state-of-the-art laboratory experiments used to validate those models. Load flexibility attributes from thermal energy storage are not discussed. A controlled-environment chamber at the National Renewable Energy Laboratory was leveraged to validate the thermal performance of the novel technology. Final results from bench-scale experiments indicate the proposed design maintained mean product temperatures within food safety guidelines.

commercial refrigeration↗

Decarbonizing Building Thermal Systems: A How-to Guide for Heat Pump Systems and Beyond

Buildings account for a substantial portion of carbon emissions, primarily due to the widespread use of fossil fuels in heating systems. Decarbonization of heating is essential to meet climate targets and reduce the environmental impact of buildings. Heat pumps are capable of leveraging renewable energy sources and can provide heating and cooling in an energy-efficient manner. By leveraging heat pump technology, buildings can significantly reduce their carbon footprint, minimize energy consumption, and decrease their reliance on fossil fuels. The design and construction community plays a pivotal role in facilitating the transition to heat pump systems for heating and cooling. However, this transition requires specialized knowledge and expertise. This resource was developed for architects, engineers, and contractors in response to an industry need for a comprehensive technical resource that guides them through the intricacies of heat pump system design, installation, and maintenance. This resource provides detailed information on system sizing, selection of appropriate heat systems, heat sources, and integration with existing building systems. Moreover, it emphasizes best practices for ensuring operational efficiency, system longevity, and reliability. The development of this recourse was a collaborative effort between NREL/DOE Better Buildings Design and Construction Allies and ASHRAE Task Force for Building Decarbonization. This resource is composed of two complimentary portions that will be completed and released on separate time frames. The first portion will be completed and released in 2023, while the second portion will be released in 2024.

building thermal systems↗

From Chills to Thrills: Revolutionizing Energy Efficiency and Load Flexibility in Supermarket Refrigeration: Preprint

Open-vertical medium-temperature refrigerated display cases comprise nearly 50% of total case lineups in a typical supermarket, with more than 80% of their cooling load attributed to infiltration of warm and moist air from the surrounding space. The infiltration takes place across the air curtain system of the display case. While the air curtain acts as a thermal shield and as a cooling mechanism to maintain product temperature, it also entrains large amounts of heat and moisture from the adjacent space. Additionally, from food safety and quality standpoints, these fixtures are vulnerable to electric outages and traditionally cannot participate in load flexibility events. This paper describes key features of an innovative design of a self-contained, water-cooled, medium-temperature, open-vertical display case. The novel concept will eliminate the inefficient air curtain system and incorporate a hybrid radiant and low-airflow convective cooling design with a thermal-energy-storage-coupled heat exchanger integrated into the refrigeration circuit. The focus of this paper is on evaluating the thermal performance of the novel hybrid design in maintaining target product temperature. It presents thermal performance findings from thermo-fluid system modeling and robust state-of-the-art laboratory experiments used to validate those models. Load flexibility attributes from thermal energy storage are not discussed. A controlled-environment chamber at the National Renewable Energy Laboratory was leveraged to validate the thermal performance of the novel technology. Final results from bench-scale experiments indicate the proposed design maintained mean product temperatures within food safety guidelines.

commercial refrigeration↗

R-matrix evaluation of the 15 N Compound System for Criticality Safety Analyses [Abstract]

The evaluation of the 15 N compound system was selected by the Nuclear Criticality Safety Program (NCSP) due to the importance of nitrogen in criticality benchmarks and in actinide chemistry encountered during fuel reprocessing. For improved accuracy in transport calculations, it is recommended to obtain and distribute resonance parameters to describe n + 14 N reactions.

AZURE↗

Automated Direct Perturbation Calculations with SCALE TSUNAMI [Abstract]

In nuclear criticality safety analysis, the sensitivity of the eigenvalue keff to uncertainties in nuclear data and its evaluation are crucial. The TSUNAMI sequences within the SCALE code system offer users various options with both multigroup (MG) and continuous-energy (CE) 3D Monte Carlo (MC) transport capabilities for calculating keff sensitivity coefficients and storing them in a sensitivity data file (SDF). Each methodology available in TSUNAMI offers distinct advantages and limitations, and its effectiveness can vary based on the specific problem being solved. As a best practice, practitioners typically use the direct perturbation (DP) method as a confirmatory step alongside their sensitivity calculations to verify the accuracy of the sensitivity data generated. In this process, DP calculations are usually performed on select nuclides, those considered most important for validating their total sensitivities. However, because of code limitations, analysts use a workaround method when conducting DP calculations for a single nuclide: rather than perturbing the nuclide's microscopic cross section, an equivalent number density for this nuclide is calculated to reflect the effect of a change in the macroscopic cross section due to a perturbation in the microscopic cross section. The current approach requires rerunning the CSAS criticality calculation several times with model changes. Although this method can yield results with acceptable accuracy, it is labor-intensive and prone to errors.

AZURE: SAMMY↗

Revisiting Source Convergence Diagnostics in the KENO Monte Carlo Neutron Transport Codes [Abstract]

Monte Carlo criticality transport codes, which rely on the power iteration procedure, are a fundamental tool for nuclear criticality safety practitioners in assessing the neutron multiplication factor (k eff ) for problems involving fissile material. In these calculations, ensuring the convergence of both the fission source distributions and the k eff estimate for accurate results is crucial. However, a converged k eff estimate does not necessarily mean the fission source distribution is also converged because the fission source and flux distribution may continue to evolve even after k eff convergence. Therefore, most Monte Carlo transport criticality codes now offer various diagnostic tests to assess fission source convergence in addition to the k eff convergence by analyzing the trends of these quantities over multiple generations.

AZURE↗