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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Hierarchical Testing of a Hybrid Machine Learning‐Physics Global Atmosphere Model

Machine learning (ML)-based models have demonstrated high skill and computational efficiency, often outperforming conventional physics-based models in weather and subseasonal predictions. While prior studies have assessed their fidelity in capturing synoptic-scale atmospheric dynamics, their performance across timescales and under out-of-distribution forcing, such as +3K or +4K uniform-warming forcings, and the sources of biases remain elusive, to establish the model's reliability for Earth science. Here, we design three sets of experiments targeting synoptic-scale phenomena, interannual variability, and out-of-distribution uniform-warming forcings. We evaluate the Neural General Circulation Model (NeuralGCM), a hybrid model integrating a dynamical core with ML-based component, against observations and physics-based Earth system models (ESMs). At the synoptic scale, NeuralGCM captures the evolution and propagation of extratropical cyclones with performance comparable to ESMs. At the interannual scale, when forced by El Niño-Southern Oscillation sea surface temperature (SST) anomalies, NeuralGCM successfully reproduces associated teleconnection patterns but exhibits deficiencies in capturing nonlinear response. Under out-of-distribution uniform-warming forcings, NeuralGCM simulates similar responses in global-average temperature and precipitation and reproduces large-scale tropospheric circulation features similar to those in ESMs. Notable weaknesses include overestimating the tracks and spatial extent of extratropical cyclones, biases in the teleconnected wave train triggered by tropical SST anomalies, and differences in upper-level warming and stratospheric circulation responses to SST warming compared to physics-based ESMs. The causes of these weaknesses were explored. Despite the noted weaknesses, NeuralGCM reproduces responses across experiments reasonably and performs comparably to ESMs. By integrating a dynamical core with ML, NeuralGCM shows potential for developing ML-based ESMs.

global warming↗
DOE OSTI2025

Recent Warming of the Southern Hemisphere Subtropical Lower Stratosphere and Antarctic Ozone Healing

Observed temperature changes from 2002 to 2022 reveal a pronounced warming of the Southern Hemisphere (SH) subtropical lower stratosphere, and a cooling of the Antarctic lower stratosphere. In contrast, model simulations of 21st-century stratospheric temperature changes show widespread cooling driven by increasing greenhouse gases, with local warming in the Antarctic lower stratosphere due to ozone healing. We provide evidence that these discrepancies between observed and simulated stratospheric temperature changes are linked to a slowdown of the Brewer-Dobson Circulation, particularly in the SH. These changes in the stratospheric circulation are strongest from October through December. This altered circulation warms the SH subtropical lower stratosphere while cooling the Antarctic lower stratosphere, canceling and even reversing the Antarctic ozone recovery that would have occurred in its absence during this period. When circulation changes are accounted for, the SH subtropical lower-stratospheric warming is removed, and Antarctic lower-stratospheric warming is revealed with enhanced ozone healing, highlighting the crucial role of the stratospheric circulation in shaping temperature and ozone changes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Light absorption enhancement of black carbon in a pyrocumulonimbus cloud

Abstract Pyrocumulonimbus (pyroCb) firestorm systems have been shown to inject significant amounts of black carbon (BC) to the stratosphere with a residence time of several months. Injected BC warms the local stratospheric air, consequently perturbing transport and hence spatial distributions of ozone and water vapor. A distinguishing feature of BC-containing particles residing within pyroCb smoke is their thick surface coatings made of condensed organic matter. When coated with non-refractory materials, BC’s absorption is enhanced, yet the absorption enhancement factor ( E abs ) for pyroCb BC is not well constrained. Here, we perform particle-scale measurements of BC mass, morphology, and coating thickness from inside a pyroCb cloud and quantify E abs using an established particle-resolved BC optics model. We find that the population-averaged E abs for BC asymptotes to 2.0 with increasing coating thickness. This value denotes the upper limit of E abs for thickly coated BC in the atmosphere. Our results provide observationally constrained parameterizations of BC absorption for improved radiative transfer calculations of pyroCb events.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Robust Multiyear Climate Impacts of Volcanic Eruptions in Decadal Prediction Systems

Abstract Major tropical volcanic eruptions have a large impact on climate, but there have only been three major eruptions during the recent relatively well‐observed period. Models are therefore an important tool to understand and predict the impacts of an eruption. This study uses five state‐of‐the‐art decadal prediction systems that have been initialized with the observed state before volcanic aerosols are introduced. The impact of the volcanic aerosols is found by subtracting the results of a reference experiment where the volcanic aerosols are omitted. We look for the robust impact across models and volcanoes by combining all the experiments, which helps reveal a signal even if it is weak in the models. The models used in this study simulate realistic levels of warming in the stratosphere, but zonal winds are weaker than the observations. As a consequence, models can produce a pattern similar to the North Atlantic Oscillation in the first winter following the eruption, but the response and impact on surface temperatures are weaker than in observations. Reproducing the pattern, but not the amplitude, may be related to a known model error. There are also impacts in the Pacific and Atlantic Oceans. This work contributes toward improving the interpretation of decadal predictions in the case of a future large tropical volcanic eruption.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Identifying Northern Hemisphere Stratospheric and Surface Temperature Responses to the Mt. Pinatubo Eruption within E3SMv2-SPA

The Mt. Pinatubo eruption on 15 June 1991 is often associated with surface warming in the subsequent Northern Hemisphere winter. Employing E3SMv2 with prognostic aerosol modifications, we generated an ensemble of simulations initialized on 1 June 1991 to limit the intra-ensemble variability at the time of the eruption and a more traditional ensemble representing the full range of intra-ensemble variability. For each ensemble member we generated a paired counterfactual simulation with the Pinatub forcing removed allowing for isolation of the Pinatubo impact. In general, the limited variability ensemble has greater coherence in the Pinatubo impact across ensemble members which leads to more statistically robust signals compared to the full variability ensemble. Stratospheric warming patterns from Pinatubo were approximately zonally symmetric and confined between 30°S and 50°N. Isolating localized surface temperature impacts was more difficult, but the limited variability simulation did identify a preferential region of cooling between 20°S to 50°N.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Exceptional stratospheric contribution to human fingerprints on atmospheric temperature

In 1967, scientists used a simple climate model to predict that human-caused increases in atmospheric CO 2 should warm Earth’s troposphere and cool the stratosphere. This important signature of anthropogenic climate change has been documented in weather balloon and satellite temperature measurements extending from near-surface to the lower stratosphere. Stratospheric cooling has also been confirmed in the mid to upper stratosphere, a layer extending from roughly 25 to 50 km above the Earth’s surface (S 25 − 50 ). To date, however, S 25 − 50 temperatures have not been used in pattern-based attribution studies of anthropogenic climate change. Here, we perform such a “fingerprint” study with satellite-derived patterns of temperature change that extend from the lower troposphere to the upper stratosphere. Including S 25 − 50 information increases signal-to-noise ratios by a factor of five, markedly enhancing fingerprint detectability. Key features of this global-scale human fingerprint include stratospheric cooling and tropospheric warming at all latitudes, with stratospheric cooling amplifying with height. In contrast, the dominant modes of internal variability in S 25 − 50 have smaller-scale temperature changes and lack uniform sign. These pronounced spatial differences between S 25 − 50 signal and noise patterns are accompanied by large cooling of S 25 − 50 (1 to 2 ° C over 1986 to 2022) and low S 25 − 50 noise levels. Our results explain why extending “vertical fingerprinting” to the mid to upper stratosphere yields incontrovertible evidence of human effects on the thermal structure of Earth’s atmosphere.

climate modeling↗
DOE OSTI2021

Identifying the sources of uncertainty in climate model simulations of solar radiation modification with the G6sulfur and G6solar Geoengineering Model Intercomparison Project (GeoMIP) simulations

We present here results from the Geoengineering Model Intercomparison Project (GeoMIP) simulations for the experiments G6sulfur and G6solar for six Earth system models participating in the Climate Model Intercomparison Project (CMIP) Phase 6. The aim of the experiments is to reduce the warming that results from a high-tier emission scenario (Shared Socioeconomic Pathways SSP5-8.5) to that resulting from a medium-tier emission scenario (SSP2-4.5). These simulations aim to analyze the response of climate models to a reduction in incoming surface radiation as a means to reduce global surface temperatures, and they do so either by simulating a stratospheric sulfate aerosol layer or, in a more idealized way, through a uniform reduction in the solar constant in the model. We find that over the final two decades of this century there are considerable inter-model spreads in the needed injection amounts of sulfate (29 ± 9 Tg-SO 2 /yr between 2081 and 2100), in the latitudinal distribution of the aerosol cloud and in the stratospheric temperature changes resulting from the added aerosol layer. Even in the simpler G6solar experiment, there is a spread in the needed solar dimming to achieve the same global temperature target (1.91 ± 0.44 %). The analyzed models already show significant differences in the response to the increasing CO 2 concentrations for global mean temperatures and global mean precipitation (2.05 K ± 0.42 K and 2.28 ± 0.80 %, respectively, for SSP5-8.5 minus SSP2-4.5 averaged over 2081–2100). With aerosol injection, the differences in how the aerosols spread further change some of the underlying uncertainties, such as the global mean precipitation response (–3.79 ± 0.76 % for G6sulfur compared to –2.07 ± 0.40 % for G6solar against SSP2-4.5 between 2081 and 2100). These differences in the behavior of the aerosols also result in a larger uncertainty in the regional surface temperature response among models in the case of the G6sulfur simulations, suggesting the need to devise various, more specific experiments to single out and resolve particular sources of uncertainty. The spread in the modeled response suggests that a degree of caution is necessary when using these results for assessing specific impacts of geoengineering in various aspects of the Earth system. However, all models agree that compared to a scenario with unmitigated warming, stratospheric aerosol geoengineering has the potential to both globally and locally reduce the increase in surface temperatures.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Stratospheric aerosol injection can weaken the carbon dioxide greenhouse effect

Abstract Stratospheric aerosol injection is a proposed method for offsetting greenhouse gas-induced warming by introducing scattering aerosols into the lower stratosphere to reflect sunlight. Here we explore a potentially more efficient alternative: weakening the Earth’s greenhouse effect by deploying absorptive aerosols in the upper stratosphere (~10 hPa). These aerosols warm the carbon dioxide emission level—where outgoing longwave radiation is most sensitive to temperature—thereby enhancing top-of-atmosphere infrared emission without altering atmospheric carbon dioxide concentrations. Idealized climate model simulations indicate that this approach can reduce global temperatures an order of magnitude more efficiently per unit aerosol mass than conventional scattering-based interventions. Although based on simplified model experiments lacking interactive aerosol processes and operational constraints, our results identify a distinct physical mechanism for climate intervention, arguing for further research into the impacts—especially potential unintended side effects—of injecting absorptive aerosols into the upper stratosphere as an alternative solar radiation management strategy.

Environmental Sciences & Ecology↗
DOE OSTI2020

Sensitivity of the latitude of the westerly jet stream to climate forcing

The latitude of the westerly jet stream is influenced by a variety of climate forcings. Their effects often manifest as a tug-of-war between tropical forcing, characterized by tropical upper-tropospheric warming, and polar forcing, with a signature of Antarctic stratospheric cooling or Arctic amplification. Here we present a unified forcing-feedback frame work relating different climate forcings to their forced jet changes, in which the interactions between the westerly jet and synoptic storms are synthesized by a zonal advection feedback, analogous to the feedback framework for assessing climate sensitivity. This framework is supported by a prototype feedback analysis in the atmospheric dynamical core of a climate model with diverse thermal and mechanical forcings. Our analysis indicates that the latitude of a westerly jet is most sensitive to the thermally-induced jet speed changes near the tropopause. The jet shift also displays a larger sensitivity than linearity for the equatorward shift.

atmospheric dynamics, atmospheric variability, cli↗
DOE OSTI2025

Cold-air outbreaks in the continental US: Connections with stratospheric variations

Mid-latitude Northern Hemisphere extreme cold events continue to occur despite overall winter warming trends. These events have been linked to weakened stratospheric polar vortex (SPV) states. In this study, we analyze both the upper and lower polar stratosphere for links to extreme winter cold and snow in the continental US, finding two SPV variations of interest. The first features an upper-level vortex displaced toward western Canada and linked to northwestern US severe winter weather. The second features a weakened upper-level vortex displaced toward the North Atlantic and linked to central-eastern US severe winter weather. Both variations feature lower-level stretched vortices and stratospheric wave reflection. Since 2015, a northwestward shift in severe winter weather across the US is concurrent with an increase in the frequency of the westward-focused variation relative to the eastward-focused variation and a shift to more negative phases of the El Niño–Southern Oscillation.

Science & Technology - Other Topics↗
DOE OSTI2021

Nonlinear Response of Atmospheric Blocking to Early Winter Barents–Kara Seas Warming: An Idealized Model Study

Wintertime Ural blocking (UB) has been shown to play an important role in cold extremes over Eurasia, and thus it is useful to investigate the impact of warming over the Barents–Kara Seas (BKS) on the behavior of Ural blocking. In our study the response of UB to stepwise tropospheric warming over the BKS is examined using a dry dynamic core model. Nonlinear responses are found in the frequency and local persistence of UB. The frequency and local persistence of the UB increase with the strength of BKS warming in a less strong range and decrease with the further increase of BKS warming, which is linked to the UB propagation influenced by upstream background atmospheric circulation. For a weak BKS warming, the UB becomes more persistent due to its less westward movement associated with intensified upstream zonal wind and meridional potential vorticity gradient (PVy) in the North Atlantic mid-high latitudes, which corresponds to a negative height response over the North Atlantic high latitudes. When BKS warming is strong, a positive height response appears in the early winter stratosphere, and its subsequent downward propagation leads to a negative NAO response or increased Greenland blocking events, which reduces zonal wind and PVy in the high latitudes from North Atlantic to Europe, thus enhancing the westward propagation of UB and reducing its local persistence. The transition to the negative NAO phase and the retrogression of UB are not found when numerically suppressing the downward influence of weakened stratospheric polar vortex, suggesting a crucial role of the stratospheric pathway in nonlinear responses of UB to the early winter BKS warming.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

High-Latitude Stratospheric Aerosol Geoengineering Can Be More Effective if Injection Is Limited to Spring

Stratospheric aerosol geoengineering focused on the Arctic could substantially reduce local and worldwide impacts of anthropogenic global warming. Because the Arctic receives little sunlight during the winter, stratospheric aerosols present in the winter at high latitudes have little impact on the climate, whereas stratospheric aerosols present during the summer achieve larger changes in radiative forcing. Injecting SO 2 in the spring leads to peak aerosol optical depth (AOD) in the summer. We demonstrate that spring injection produces approximately twice as much summer AOD as year-round injection and restores approximately twice as much September sea ice, resulting in less increase in stratospheric sulfur burden, stratospheric heating, and stratospheric ozone depletion per unit of sea ice restored. Furthermore, we also find that differences in AOD between different seasonal injection strategies are small compared to the difference between annual and spring injection.

58 GEOSCIENCES↗
DOE OSTI2022

Variability of Water Vapor in the Tropical Middle Atmosphere Observed From Satellites and Interpreted Using SD-WACCM Simulations

Water vapor in the middle atmosphere plays an essential role in global warming, ozone depletion, and the formation of polar stratospheric and mesospheric clouds. We show that tropical middle atmospheric water vapor simulated with the specified-dynamics version of the Whole Atmosphere Community Climate Model (SD-WACCM) is consistent with changes observed in a merged satellite data set, which encompasses the period 1993–2020. Consistent with previous work, we find no significant trend in the stratosphere in either the observations or the simulation; in the mesosphere, we find a long-term trend of 0.1 ppmv per decade, but only in the observations. We also analyze an SD-WACCM simulation for the longer period 1980–2019 to quantify the contribution of various factors to the decadal variation of middle atmospheric water vapor. Over 1980–1995, the simulated water vapor in the upper stratosphere and mesosphere, averaged zonally and over ±30° latitude, increases by 0.30 ppmv per decade due to increasing methane emissions. After 1995, a significant abrupt decrease of water vapor of 0.37 ppmv per decade and then a gradual increase of 0.33 ppmv per decade result from changes in stratospheric cold point temperature. The cold-point temperature is strongly influenced by the strength of the Brewer-Dobson circulation. The acceleration of the Brewer-Dobson circulation before about 2003 leads to a cooler tropical tropopause and a decrease of water vapor, and the deceleration thereafter leads to corresponding warming of the tropopause and an increase in water vapor.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes

There is now substantial literature on climate model studies of equatorial or tropical stratospheric SO 2 injections that aim to counteract the surface warming produced by rising concentrations of greenhouse gases. Here we present the results from the first systematic intercomparison of climate responses in three Earth system models wherein the injection of SO 2 occurs at different latitudes in the lower stratosphere: CESM2-WACCM6, UKESM1.0 and GISS-E2.1-G. The first two use a modal aerosol microphysics scheme, while two versions of GISS-E2.1-G use a bulk aerosol (One-Moment Aerosol, OMA) and a two-moment (Multiconfiguration Aerosol TRacker of mIXing state, MATRIX) microphysics approach, respectively. Our aim in this work is to determine commonalities and differences between the climate model responses in terms of the distribution of the optically reflective sulfate aerosols produced from the oxidation of SO 2 and in terms of the surface response to the resulting reduction in solar radiation. A focus on understanding the contribution of characteristics of models transport alongside their microphysical and chemical schemes, and on evaluating the resulting stratospheric responses in different models, is given in the companion paper (Bednarz et al., 2023). The goal of this exercise is not to evaluate these single-point injection simulations as stand-alone proposed strategies to counteract global warming; instead we determine sources and areas of agreement and uncertainty in the simulated responses and, ultimately, the possibility of designing a comprehensive intervention strategy capable of managing multiple simultaneous climate goals through the combination of different injection locations. We find large disagreements between GISS-E2.1-G and the CESM2-WACCM6 and UKESM1.0 models regarding the magnitude of cooling per unit of aerosol optical depth (AOD) produced, which varies from 4.7 K per unit of AOD in CESM2-WACCM6 to 16.7 K in the GISS-E2.1-G version with two-moment aerosol microphysics. By normalizing the results with the global mean response in each of the models and thus assuming that the amount of SO 2 injected is a free parameter that can be managed independently, we highlight some commonalities in the overall distributions of the aerosols, in the inter-hemispheric surface temperature response and in shifts to the Intertropical Convergence Zone, as well as some areas of disagreement, such as the extent of the aerosol confinement in the equatorial region and the efficiency of the transport to polar latitudes. In conclusion, we demonstrate that it is possible to use these simulations to produce more comprehensive injection strategies in multiple climate models. However, large differences in the injection magnitudes can be expected, potentially increasing inter-model spreads in some stratospheric quantities (such as aerosol distribution) while reducing the spread in the surface response in terms of temperature and precipitation; furthermore, the selection of the injection locations may be dependent on the models' specific stratospheric transport.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

What goes up must come down: impacts of deposition in a sulfate geoengineering scenario

The problem of reducing the impacts of rising anthropogenic greenhouse gas on warming temperatures has led to the proposal of using stratospheric aerosols to reflect some of the incoming solar radiation back to space. The deliberate injection of sulfur into the stratosphere to form stratospheric sulfate aerosols, emulating volcanoes, will result in sulfate deposition to the surface. We consider here an extreme sulfate geoengineering scenario necessary to maintain temperatures at 2020 levels while greenhouse gas emissions continue to grow unabated. We show that the amount of stratospheric sulfate needed could be globally balanced by the predicted decrease in tropospheric anthropogenic SO 2 emissions, but the spatial distribution would move from industrialized regions to pristine areas. We show how these changes would affect ecosystems differently depending on present day observations of soil pH, which we use to infer the potential for acid-induced aluminum toxicity across the planet.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Stratosphere-Troposphere Coupling of Extreme Stratospheric Wave Activity in CMIP6 Models

Extreme stratospheric wave activity has been suggested to be connected to surface temperature anomalies, but some key processes are not well understood. Using observations, we show that the stratospheric events featuring weaker-than-normal wave activity are associated with increased North American (NA) cold extreme risks before and near the event onset, accompanied by less frequent atmospheric river (AR) events on the west coast of the United States. Strong stratospheric wave events, on the other hand, exhibit a tropospheric weather regime transition. Further, they are preceded by NA warm anomalies and increased AR frequency over the west coast, followed by increased risks of NA cold extremes and north-shifted ARs over the Atlantic. Moreover, these links between the stratosphere and troposphere are attributed to the vertical structure of wave coupling. Weak wave events show a wave structure of westward tilt with increasing altitudes, while strong wave events feature a shift from westward tilt to eastward tilt during their life cycle. This wave phase shift indicates vertical wave coupling and likely regional planetary wave reflection. Further examinations of CMIP6 models show that models with a degraded representation of stratospheric wave structure exhibit biases in the troposphere during strong wave events. Specifically, models with a stratospheric ridge weaker than the reanalysis exhibit a weaker tropospheric signal. Our findings suggest that the vertical coupling of extreme stratospheric wave activity should be evaluated in the model representation of stratosphere-troposphere coupling.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

A Multivariate Space‐Time Dynamic Model for Characterizing the Atmospheric Impacts Following the Mt. Pinatubo Eruption

The June 1991 Mt. Pinatubo eruption resulted in a massive increase of sulfate aerosols in the atmosphere, absorbing radiation and leading to global changes in surface and stratospheric temperatures. A volcanic eruption of this magnitude serves as a natural analog for stratospheric aerosol injection, a proposed solar radiation modification method to combat a warming climate. The impacts of such an event are multifaceted and region-specific. Our goal is to characterize the multivariate and dynamic nature of the atmospheric impacts following the Mt. Pinatubo eruption. We developed a multivariate space-time dynamic linear model to understand the full extent of the spatially- and temporally-varying impacts. Specifically, spatial variation is modeled using a flexible set of basis functions for which the basis coefficients are allowed to vary in time through a vector autoregressive (VAR) structure. This novel model is cast in a Dynamic Linear Model (DLM) framework and estimated via a customized MCMC approach. We demonstrate how the model quantifies the relationships between key atmospheric parameters prior to and following the Mt. Pinatubo eruption with reanalysis data from MERRA-2 and highlight when such a model is advantageous over univariate models.

Dynamic Linear Model↗
DOE OSTI2025

Assessing the performance of solar radiation management geoengineering simulations

Offsetting the global warming caused by anthropogenic increases in atmospheric greenhouse gases by deliberate injection of aerosols into the stratosphere is the most studied of solar radiation management geoengineering schemes. The long-term success or failure of such schemes in achieving their stated goals is assessed by comparing simulated geoengineered temperature, precipitation and tropical cyclones metrics to equivalent fields in the simulated targeted climate simulations. Results using available data sets from three single model stabilized climate target experiments and three multimodel climate change reduction experiments are presented and compared against a measure of internal variability. While all but one experimental scheme is successful in achieving their targeted global mean annual surface temperature, their success at regional scales varies significantly and is often larger than the internal variability metric used here.

climate model evaluation↗