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30 records · Page 2

Nuclear Criticality Safety Integral Experiment Covariance Determination

Integral benchmarks for criticality safety and nuclear data validation require expensive uncertainty quantification studies. Commonly, the uncertainty quantification ignores correlations between experiments that share components. Experiments such as the TEX (Thermal/Epithermal eXperiments) campaigns consist of many shared parts, such as fuel, which create a strong correlation in their uncertainties. While these correlations are known to exist, they are often not estimated due to the complexity of such calculations. This paper describes a software package that uses an intuitive method of determining the covariance for each of the experimental components, providing a correlation matrix for each family of parts across the multiple cases examined within a benchmark. The code uses the TEX-HEU campaign as a proof of concept, and we show that the correlations can be calculated with information commonly found in ICSBEP (International Criticality Safety Benchmark Evaluation Project) benchmarks. The estimated covariances are used in χ 2 trending studies to evaluate their impact on nuclear data validation. Without covariances, χ 2 per degree of freedom was calculated as 2.203 and with covariances it was 1.179. The difference shows that omitting covariance information may cause overly pessimistic bias quantifications. The covariance determination code can be easily integrated into current benchmark evaluations as well as reevaluating legacy benchmark uncertainties. Uncertainty correlation calculations should become the baseline for criticality safety integral experiment benchmarks and can now be easily calculated with the described software package.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Progress Towards the Reality of Low-Temperature Critical Experiments with Low-Temperature TEX

Integral benchmarks for criticality safety do not exist below room temperature. Incredible support for below room temperature benchmarks is present across the international community. Validation of low-temperature neutron cross sections is necessary to verify any operation at temperatures below room temperature which is typically observed in environments far from the equator. For example, a fissile material transportation truck may routinely observe ambient temperatures down to -40°C, which is the lower temperature bound of the normal conditions of transportation defined in the United States Title 10 Code of Federal Regulations §71.71c2. Similarly, the IAEA, which contains 176 member states, has the same requirement for subcriticality for fissile material transportation. Additionally, sub-room temperature benchmarks can validate newly produced cross sections, that include novel thermal scattering laws, from North Carolina State University. A six-case experiment designed based off the TEX-HEU baseline experiments has been proposed utilizing a chilled vacuum chamber capable of cooling the HEU stack down to -50°C. The six proposed configurations span the entire neutron fission energy range and can be tested at intermediate temperatures between room temperature and -40°C. Of the six configurations, the fastest case utilizes nearly 135 kg of HEU. Understanding the system is required prior to critical experiment operations. In order to test the functionality of the system, testing with surrogate fuel materials has been conducted. The following discusses the design of the low temperature TEX (LT-TEX) experiment as well as the progress made via surrogate testing towards a reality in which low-temperature integral benchmarks exist in the International Criticality Safety Benchmark Evaluation Project (ICSBEP).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Integral Experiment Final Design for Thermal/Epithermal eXperiments (TEX) using Highly Enriched Uranium with Polyethylene at Low Temperature (IER-479 CED-2 Report)

The goal of IER-479 is to design uranium critical experiments that can be used to validate low temperature cross sections and criticality safety analyses over multiple neutron energy regimes. Currently, there are no benchmarks in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook at temperatures lower than room temperature (International Criticality Safety Benchmark Evaluation Project Handbook, 2019). However, there are many needs for validation of criticality safety analysis at lower temperatures, including meeting transportation requirements and operations conducted outside or in unheated facilities. Additionally, NCSP has funded North Carolina State (NCSU) to generate new thermal scattering laws, including at lower temperatures, and the lack of integral benchmarks impedes data testing of these new cross sections. To address these needs, this report will present a critical experiment design covering various fission energy regimes with a goal temperature of -40°C (-40°F), which is based on the lower bound of expected non-cryogenic operational temperatures. The goal of the U.S. Nuclear Criticality Safety Program’s (NCSP) Thermal/Epithermal eXperiments (TEX) is to design and conduct new critical experiments to address high priority nuclear data needs from the nuclear criticality safety and nuclear data communities. The TEX program includes two series of baseline experimental configurations, one based on plutonium fuel (plutonium-aluminum Zero Power Physics Reactor (ZPPR) plates) and the other based on uranium fuel (highly enriched uranium (HEU) plates), that are moderated with varying thickness of polyethylene to create assemblies which span the thermal, intermediate, and fast fission energy regimes. The configurations are designed to be easily modified (for example, to add diluent materials of interest) to allow for efficient generation of additional benchmark configurations and allow for added nuclear data testing utility when comparing modified configurations to baseline configurations. The goal of IER-479 is to use the TEX-HEU concept (stack of HEU plates and polyethylene moderators) to design a critical experiment that can be used to validate low temperature cross sections and criticality safety analyses.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

TEX-Hf: Integral Experiment Execution of Thermal/Epithermal eXperiments using Highly Enriched Uranium with Polyethylene and Hafnium (IER-532 CED-3b Report)

This report documents the experimental configurations and measurements for IER-532, Thermal/Epithermal eXperiments (TEX) with highly enriched uranium (HEU) fuel and interstitial hafnium (Hf), moderated and reflected by polyethylene. TEX-Hf is a variation of and based on the TEX-HEU (IER-297) design, with the inclusion of hafnium. These configurations provide integral experiments for validation of hafnium in the thermal, intermediate, and fast neutron energy regimes by maximizing the sensitivity in k eff to the hafnium isotope cross sections. The experiment campaign was completed over seven weeks during the end of FY22 and beginning of FY23 at the National Critical Experiments Research Center at the Nevada National Security Site. The campaign produced seven experimental configurations, four reproducibility measurements, and many additional dimensional measurements that will be of use to the future benchmark evaluation of this experiment and other experiments using the same HEU fuel. Table 1 summarizes the TEX-Hf experimental configurations, including their physical parameters, calculated fission fractions, and estimated excess reactivities.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Integral Experiment Final Design for Thermal/Epithermal eXperiments with 233U3O8 ZPR Fuel Elements and Polyethylene (IER-329 CED-2 Report)

This report documents the integral experiment final design for IER-329, Thermal/Epithermal eXperiments (TEX) with 233 U 3 O 8 Zero Power Reactor (ZPR) Fuel Elements and Polyethylene. IER-329 (TEX-23) is the third baseline design in the Thermal/Epithermal eXperiments (TEX) series led by Lawrence Livermore National Laboratory (LLNL) and funded by the DOE’s Nuclear Criticality Safety Program. This experiment was designed to address the existing 233U integral benchmark experiments over prediction in k eff by up to 2% for thermal systems and under-prediction in k eff by up to 4% for intermediate systems. The TEX-23 design utilizes assemblies of 233 U 3 O 8 Zero Power Reactor (ZPR) fuel elements moderated and reflected by high-density polyethylene. This design is similar to the existing TEX-Pu and TEX-HEU designs, utilizing an adjustable moderator to tune the neutron energy spectra and modular layers for the incorporation of diluent materials.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TEX-Cl: Integral Experiment Execution of Thermal/Epithermal eXperiments using Highly Enriched Uranium with Polyethylene and Chloride Absorbers

This report documents the experimental configurations and measurements performed for IER-499, TEX with chlorine (TEX-Cl). TEX-Cl is a variant of the TEX-HEU campaign and utilizes highly enriched uranium fuel, high-density polyethylene (HDPE) moderators and reflectors, and interstitial NaCl salt absorbers. These experiments probe the chlorine (from the sodium chloride) absorption cross section in the thermal and intermediate neutron energy regimes, with a small portion in the fast neutron energy regime. Three configurations were selected by maximizing the sensitivity in k eff to the needs of Y-12 for their electrorefining operations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TEX-Hf Assemblies: Highly Enriched Uranium Plates with Hafnium Using Polyethylene Moderator and Polyethylene Reflector

This report documents the integral experiment evaluation and publication for IER-532 (TEX-Hf), Thermal/Epithermal eXperiments (TEX) with highly enriched uranium (HEU) fuel and hafnium (Hf), moderated and reflected by polyethylene. The design of TEX-Hf is a variation of IER-297 (TEX-HEU), with the inclusion of hafnium as a diluent material. The experiment and evaluation include seven configurations, all of which were acceptable as benchmark cases. These benchmark cases provide validation for hafnium in the thermal, intermediate, and fast neutron energy regimes by maximizing the sensitivity in k eff to the hafnium cross sections. The evaluation was reviewed and accepted by the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Technical Review Group on April 17, 2024, and was submitted to the ICSBEP in August 2024 following subgroup approval.

42 ENGINEERING↗

TEX-Chlorine: Highly Enriched Uranium with Chloride Absorbers to Provide Validation Benchmarks for Y-12 Electrorefining Facility

This report documents the final benchmark of the TEX-Chlorine (IER-499) Thermal Epithermal eXperiments (TEX) with highly enriched uranium with chlorine absorbers and high-density polyethylene reflectors and moderators. TEX-Chlorine is a variation of the TEX-HEU baseline assembly with the addition of sodium chloride absorber plates. This evaluation contains three experimental configurations that were performed on Comet at NCERC between July and August 2024. The three configurations, which were acceptable as benchmark cases, spanned from thermal (first two configurations) to fast (third configuration). All three cases were reviewed and accepted by the ICSBEP TRG in April 2025 and was submitted to the ICSBEP in August 2025 after receiving subgroup approval.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TEX-Chlorine for TerraPower - Experimental Execution Report

This report describes the critical configurations of the TEX4TerraPower project that were performed in FY26Q4. Within this report, the configurations are presented along with physical measurements performed in support of benchmarking. TEX4TerraPower builds upon the TEX-Chlorine experiments, which in turn were based on the TEX-HEU experiments. Similar to TEX-Chlorine, the TEX4TerraPower configurations iteratively layered HEU fuel with sodium chloride (NaCl) absorbers. However, the main difference in the density achieved during the fabrication process of the sodium chloride absorbers. Unlike TEX-Chlorine, which was able to achieve ~70% theoretical density, the TEX4TerraPower salt plates achieved >90% theoretical density by hydraulically pressing the salt.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A Look Towards the Execution of the Low-Temperature TEX Experimental Campaign

To address the mounting need for below roomtemperature nuclear data validation, the Low-Temperature Thermal Epithermal eXperiments (LT-TEX) have been designed. Validation of low-temperature neutron cross sections is necessary to verify any operation at temperatures below room temperature which is typically observed in environments far from the equator. For example, a fissile material transportation truck may routinely observe ambient temperatures down to -40°C, which is the lower temperature bound of the normal conditions of transportation defined in the United States Title 10 Code of Federal Regulations §71.71c2. Additionally, sub-room temperature benchmarks can validate newly produced cross sections, that include novel thermal scattering laws, from North Carolina State University.

LT-TEX↗