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At least 37 records · Page 2

TRACER Radar b1 Data Processing: Corrections, Calibrations, and Processing Report

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility deployed the first ARM Mobile Facility (AMF1) to Houston, Texas for the Tracking Aerosol Convection Interactions Experiment (TRACER) field campaign. The TRACER campaign was conducted from October 1, 2021 to September 30, 2022, with an intensive operational period (IOP) from June 1 to September 30, 2022. To investigate the life cycles of convective cells in the polluted and humid urban environment of Houston, ARM deployed cloud and precipitation radars, including the C-band Scanning ARM Precipitation Radar (CSAPR2), the X/Ka-band Scanning ARM Cloud Radar (SACR), and the Ka-band ARM Zenith cloud Radar (KAZR), as shown in Figure 1. This report presents an analysis of radar data quality, hardware calibrations, and radar data corrections.

54 ENVIRONMENTAL SCIENCES↗

Characterization of carbonaceous aerosols during TRACER-CAT

Absorbing aerosols (AA) have an important impact on the global radiation budget and cloud properties. The composition and properties of AA can vary substantially throughout the atmosphere, depending on the particle source and the influence of chemical aging. Uncertainties associated with the radiative effects of AA remain substantial. A key contributor to this uncertainty is understanding the extent to which coatings in general, and water uptake especially, alters absorption by AA particles and how this depends on particle composition. We deployed new and existing experimental tools during the Tracking Aerosol Convection Interactions Experiment (TRACER) campaign in Houston, TX as part of the Carbonaceous Aerosols Thrust (CAT) to provide detailed characterization of aerosol optical, chemical, and physical properties. Our TRACER-CAT measurements complemented and expanded on the planned TRACER instrumentation, allowing for more detailed characterization of aerosol properties of relevance to cloud development (a core focus of TRACER), such as the composition of particles that can act as cloud condensation nuclei, than would otherwise be available. Our measurements have allowed for assessment of the relationship(s) between AA optical properties (with a focus on absorption) and the chemical and physical characteristics (including the mixing state of black carbon (BC) containing particles). These field observations occurred in collaboration with Los Alamos National Laboratory in summer 2022 during the TRACER intensive operating period. The instrumentation we co-deployed provided for measurement of (i) multi-wavelength dry aerosol absorption, scattering, and extinction, (ii) the size-dependent composition and abundance of sub-micron aerosol, differentiating between those particles that do and do not contain BC, (iii) BC-specific concentrations and size distributions, (iv) particle size, and (v) the first field measurements at an ARM site of the influence of RH on multi-wavelength absorption by ambient AA. We have leveraged the natural variability of the atmosphere and of aerosol sources in the Houston region to (i) specifically disentangle contributions to light absorption from BC, absorbing organic carbon (brown carbon), and coatings on BC, (ii) characterize the mixing state of BC and assess the factors that give rise to compositional differences between BC-containing and BC-free aerosol, and (iii) establish how water uptake influences absorption and how any such effect depends on particle composition and BC mixing state. Overall, our study contributed to the mission of the Atmospheric System Research program in multiple ways. Through the deployment of complementary, advanced instrumentation for characterization of a wide range of aerosol properties our work helped to maximize the scientific impact of the TRACER campaign. Our work also allowed for development of new insights into the relationship(s) between aerosol composition, hygroscopicity, and the mixing state of BC with aerosol optical properties. Through this, our work has provided knowledge that can improve understanding and model representation of aerosol processes as they affect the Earth’s radiation budget.

54 ENVIRONMENTAL SCIENCES↗

TRACER-MAP Field Campaign Report

During July-August 2022, the U.S. Department of Energy (DOE) Atmospheric System Research (ASR)-funded Tracking Aerosol Convection Interactions Experiment (TRACER)-MAP campaign completed an Atmospheric Radiation Measurement (ARM) user facility field study to measure and map aerosol, volatile organic compounds (VOC), trace gas, and select meteorological observations across Houston, Texas. That ASR project and ARM field campaign, TRACER-MAP, was designed to complement measurements made at the first ARM Mobile Facility (AMF1) by the Aerosol Observing System (AOS) during the TRACER campaign. In this manner, TRACER-MAP effectively extended aerosol measurements from the TRACER AMF deployment, increasing the spatial coverage across the Houston metropolitan area, characterizing a greater diversity of source mixtures (e.g., industrial, traffic, residential, and biogenic) and capturing air masses with differential aging of urban source emissions (e.g., downtown versus downwind). That rich data set now offers many possibilities for in-depth analysis that align with the ASR mission to “research aerosol processes that affect Earth’s radiative balance and hydrological cycle.”

54 ENVIRONMENTAL SCIENCES↗

Test Flights of NOAA Ozone Photometer for Uncrewed Aerial Systems (UAS)/Balloon-Based Studies (OPUS) during TRACER (Field Campaign Report)

We proposed to integrate and fly the National Oceanic and Atmospheric Administration (NOAA) Ozone Photometer for Uncrewed Aerial Systems (UAS)/Balloon-Based Studies (OPUS) on the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility’s tethered balloon system (TBS) during the second phase (August 1-15) of the 2022 Tracking Aerosol Convection Interactions Experiment (TRACER) in southwest Houston, Texas. The two main goals were: 1) Test fly the sensor to discover and address any potential problems such as interface and communication with other instruments, interferences with other instruments and radio, and 2) If OPUS performs well, then inter-compare OPUS with the EN-SCI ozonesondes that will also be flown on the TBS. The collaborating institutions are DOE Sandia National Laboratories TBS team, the University of Houston, and St. Edward's University.

47 OTHER INSTRUMENTATION↗

Pinned Clouds over Industrial Sources of Heat during TRACER

An analysis of stereo-camera data from the Tracking Aerosol Convection Interactions Experiment (TRACER) campaign in Houston, Texas, reveals the existence of pinned clouds sitting atop industrial heat sources. These are not plumes of vapor and condensate emanating from stacks: The pinned shallow cumuli have cloud bases at about the lifting condensation of near-surface air. On many mornings, the pinned clouds are the only shallow cumuli in the field of view of the stereo cameras, persisting by themselves for at least an hour. On those mornings, the lower atmosphere straddles the boundary between stable and unstable, and the waste heat from industrial facilities is able to pin moist convection overhead. When solar heating of the surface becomes sufficient later in the morning, those mornings transition to having widespread shallow moist convection. Occurring within the field of view of the stereo cameras and other TRACER instruments, these pinned clouds represent steady plume-like moist convection triggered by known heat sources in a well-characterized atmosphere, making them a rich target for further study. Significance Statement This article introduces steady-state cumulus clouds observed during the Tracking Aerosol Convection Interactions Experiment (TRACER) campaign that were pinned to industrial heat sources. These pinned clouds were present in the early morning only when conditions were primed for moist convection, but for which there was not yet enough solar heating to trigger widespread convection. They persist in a statistical steady state and therefore provide a natural setting to explore the mechanisms controlling convective dynamics, which play a central role in Earth’s atmospheric circulation and radiative balance.

Atmosphere↗

TRACER Radar b1 Data Processing: Corrections, Calibrations, and Processing Report

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility deployed the first ARM Mobile Facility (AMF1) to Houston, Texas for the Tracking Aerosol Convection Interactions Experiment (TRACER) field campaign. The TRACER campaign was conducted from October 1, 2021 to September 30, 2022, with an intensive operational period (IOP) from June 1 to September 30, 2022.

54 ENVIRONMENTAL SCIENCES↗

Aerosol Hygroscopic Growth, Mixing State, and Cloud Condensation Nuclei Activity during TRACER (Field Campaign Report)

Convective clouds play a critical role in the Earth’s climate system. Recent research has shown that a realistic representation of convective processes is critical to constraining climate sensitivity in global climate models. Theoretical and modeling studies showed that aerosols could have strong dynamic feedback to convection in warm and humid environments through enhancing ice-related processes and condensational growth. A few observation-based studies also suggested the influence of aerosols on convective cloud and precipitation properties. However, robust observational quantification of an aerosol effect on convective clouds isolated from other factors remains elusive. Understanding the impact of aerosol on convective clouds requires knowledge of the cloud condensation nuclei (CCN) spectrum, which represents the number of particles that uptake water and form cloud droplets as a function of supersaturation. The water uptake by aerosol is also of critical importance for the direct interaction of aerosol with radiation (i.e., aerosol direct effect) due to light scattering and absorption by aerosol. While both droplet activation under supersaturated conditions (i.e., relative humidity RH > 100%) and the hygroscopic growth under sub-saturated conditions (i.e., RH < 100%) are strongly influenced by particle hygroscopicity, the thermodynamic regimes and measurement methods are quite different. Aerosol particles, especially organic particles, can exhibit higher hygroscopicity for droplet activation than that for hygroscopic growth. In the subsaturated regime, the hygroscopicity of organic particles can also vary strongly with RH. However, global climate models usually treat organic species in aerosols with a constant hygroscopicity, potentially introducing substantial uncertainties in the quantification of aerosol radiative effects.

54 ENVIRONMENTAL SCIENCES↗

TRACER-iso Field Campaign Report

The TRACER-iso project took place from June 1 to September 30, 2022, as part of the intensive operational period (IOP) of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s TRacking Aerosol Convection interactions ExpeRiment (TRACER) at the main project site at the La Porte, Texas, municipal airport. The project sought to use measurements of the stable isotopic composition of water vapor to better understand cloud-aerosol interactions in deep convection in a polluted urban setting.

54 ENVIRONMENTAL SCIENCES↗

CSAPR2 cell-tracking data collected during TRACER

One of the challenges of analyzing convective cell properties is quick evolution of the individual convective cells. While the operational radar data provide great a data set to analyze the evolution of radar observables of convective precipitation clouds statistically, previous studies also suggested that, because of the quick evolution of cell life cycle, conventional radar volume scan strategies taking ~5-7 minutes might not capture the detailed evolution. The TRACER campaign deployed CSAPR2, which performed frequent update of RHI and sector PPI scans to track convective cells every < 2 minutes guided by a new cell-tracking framework, Multisensor Agile Adaptive Sampling (MAAS; Kollias et al. 2020). This allows for capturing fast-evolving radar observables. The submitted data files are CSAPR2 data in CfRadial format collected during the TRACER field campaign from June to September 2020. The data files include processed radar variables including: noise-masked reflectivity and differential reflectivity corrected for rain attenuation and systematic biases, noise-masked dealiased radial velocity, specific differential phase, locations of target cells (latitude, longitude, radar range), and radar-echo classification.

54 ENVIRONMENTAL SCIENCES↗

CSAPR2 Optimized Convective Cell Tracking Data during TRACER

One of the challenges in analyzing convective cell properties is to observe the quick evolution of individual convective cells. While the operational radar data provide a volumetric data set to analyze radar observables of convective precipitation clouds, previous studies also suggested the quick evolution of cell life cycle that might not be captured by conventional radar volume scan strategies that take ~5-7 minutes. Aiming at enhancing our understanding of the links between convective cloud kinematic and microphysical processes as well as life cycles, the Tracking Aerosol Convection Interactions ExpeRiment (TRACER; Jensen et al. 2019) was conducted at Houston, Texas, in 2022. The TRACER campaign deployed the 2nd generation C-band Scanning ARM Precipitation Radar (CSAPR2), which performed frequent updates of range height indicator (RHI) and sector plan position indicator (PPI) scans to track individual convective cells every < 2 minutes, guided by a new cell tracking framework, Multisensor Agile Adaptive Sampling (MAAS; Kollias et al. 2020). This allows for capturing fast-evolving radar observables. We provide the processed CSAPR2 cell tracking data in CfRadial format collected during the TRACER field campaign from June to September 2022. The data files include processed radar variables: noise-masked reflectivity and differential reflectivity corrected for rain attenuation and systematic biases, noise-masked dealiased radial velocity, specific differential phase, locations of target cells (latitude, longitude, radar range), and radar-echo classification. Figure 1 provides an example of a 3D image of CSAPR2 reflectivity from the lowest PPI scan and an RHI scan after data processing.

54 ENVIRONMENTAL SCIENCES↗

Spectro-Microscopic Investigation of the Aerosol Impact on Hydrological Processes

This project investigated physico-chemical characteristics of atmospheric particles collected during DOE ARM field campaigns and how they are involved in the hydrological cycle. Our efforts were focused on multi-modal chemical imaging and molecular characterization of atmospheric particles and snow samples collected during the Surface-Atmosphere Integrated Field Laboratory (SAIL) campaign and particle samples from the Tracking Aerosol Convection Interactions ExpeRiment (TRACER) campaign.

54 ENVIRONMENTAL SCIENCES↗

Results of Multiple Tracer Injections into Fractures in the EGS Collab Testbed-1

The EGS Collab project constructed an intermediate scale (~10-20 m) testbed at the 4850 level of the Stanford Underground Research Facility (SURF) in South Dakota for testing and validating fracture stimulation and flow/transport models. This testbed consists of eight ~200 ft (~60 m) HQ-diameter (9.6 cm) boreholes that are drilled into the crystalline rocks of the Poorman Formation from the West Access Drift tunnel. Of the eight boreholes, one borehole is used as an injection/stimulation well, while another sub-parallel borehole located about 10 m away from the injection well is used as a production well, and rest of the other boreholes are used as geophysical/fluid sampling monitoring wells. Hydraulic stimulation activities were conducted at three locations along the injection hole in an attempt to create direct fracture connections to the production hole. A flow system has been established between injection and production boreholes through a set of hydraulically stimulated fractures propagated from a notch located at 164 ft in the injection hole. Although we planned for a single production well, a set of natural fractures in the testbed is believed to have intersected the stimulated hydraulic fractures and provided additional flow paths for water to be transported to the drift through multiple monitoring boreholes and weep zones. As the flow tests continued after stimulation activities, single or a combination of two or three producers become dominant producers at different times, mostly as a response to intersection of hydraulic fracture and testbed wells, activation of natural fractures and making new leak points to the monitoring wells, resealing of leaky wells, and so on. Since late October 2018, multiple tracers were injected into the fracture system at the 164 ft location that involves both stimulated and natural fractures, and tracers were recovered from multiple locations in nearby wells and weep. The cumulative water recoveries over the time have ranged from 50 to 90%; however, the injected tracer recoveries from various production sources are much less (ranging from a few percentages to 38%). Changes in water/tracer recoveries, shifting of major producing wells from one well to the others, and other observations (e.g., microseismic, electric resistivity tomography, etc.) indicate a testbed that has undergone several changes since October 2018. In this paper, we present tracer recovery data accumulated during several tracer campaigns, provide conceptual testbed flow pathways, and provide observations that suggest a evolutionary nature of fracture volume and fracture geometry in the testbed.

15 GEOTHERMAL ENERGY↗

A Closed Bay-Breeze Circulation and Its Lifecycle From TRACER With a New Orienteering Tape Recorder Diagram

A closed bay-breeze circulation (BBC) followed by a gulf-breeze front (GBF) was observed on 10 September 2022 during the Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) TRACER campaign. Using high-resolution X-band Scanning Cloud Radar (XSACR) and a newly developed orienteering tape recorder diagram, the study analyzed radar reflectivity and Doppler velocity to identify anomalies and track the evolution of these circulations. The BBC, a mesoscale system approximately 30-km long, 30-km wide, and 2-km deep, formed from enhanced horizontal convective rolls along the Galveston Bay coast, progressing northwestward under a 6 m s−1 onshore flow anomaly and reaching 1.5 km depth with return flow aloft. The inland penetration speed was 2 m s−1, driven by an observed 6-9 K land-water temperature contrast. The GBF, coupled to the BBC, intensified with additional southerly flow, penetrating further inland after the BBC collapsed. Passing over the TRACER field site, both fronts significantly impacted boundary layer thermodynamics, dynamics, and aerosol concentration. The BBC event exhibited four lifecycle stages-formation, development, maturation, and dissipation-driven by solar heating, wind field rotation, and interactions with convective eddies and the GBF. This study provides insights into the inland evolution of coastal breeze circulations and their interactions with environmental processes.

54 ENVIRONMENTAL SCIENCES↗

Evaluating E3SM Global Storm‐Resolving Model Simulations of Deep Convection: Insights From DP‐SCREAM During TRACER

Global Storm-Resolving Models (GSRMs) are becoming increasingly vital for advancing climate modeling and improving the prediction of extreme weather events. Houston, a coastal region frequently affected by deep convective storms, offers an ideal setting to evaluate the ability of GSRMs to simulate deep convection. This study assesses the performance of the Doubly Periodic Simple Cloud-Resolving E3SM (Energy Exascale Earth System Model) Atmosphere Model (DP-SCREAM) using observations from the TRacking Aerosol Convection interactions ExpeRiment (TRACER) campaign. DP-SCREAM effectively reproduces the diurnal cycles of clouds and precipitation, demonstrating much greater skill than the E3SM single column model. The DP-SCREAM is demonstrated to be applicable to coastal regions, partially due to the forcing data sets already capturing the influence of breezes. DP-SCREAM also replicates biases persistent in the global version of SCREAM: the underrepresentation of boundary layer shallow clouds, a lack of mid-level congestus clouds, and the popcorn convection, characterized by small and disorganized convective cells generating the strongest precipitation. To investigate these issues, two sensitivity experiments were conducted: increasing the mixing length and scaling up the buoyancy flux within the Simplified Higher Order Closure scheme. Increasing the mixing length improved mid-level congestus representation and reduced unrealistic early morning fog occurrence. Enhancing buoyancy flux only marginally improved the bias of underproduced big convective cells. In conclusion, an additional resolution sensitivity test at 0.5 km grid spacing demonstrated that a refined horizontal resolution alone is insufficient to resolve these biases.

54 ENVIRONMENTAL SCIENCES↗

Variability in Ice Nucleating Particles Across Greater Houston Texas

The concentration and cloud-forming potential of a region's ice nucleating particle (INP) population have uncertain impacts on deep convective clouds. Specifically, ice nucleating particles (INPs) may affect various cloud properties related to the formation, lifetime, and precipitation of deep convective clouds. As part of the U.S. Department of Energy's TRacking Aerosol and Convection interaction ExpeRiment (TRACER) campaign, researchers from Texas A&M University deployed three Davis Rotating-drum Universal-size-cut Monitoring (DRUM) samplers throughout Greater Houston, Texas from June through September 2022. Ambient particles, collected at the surface with the DRUM samplers in four aerodynamic diameter size ranges (>3, 3–1.2, 1.2–0.34, and 0.34–0.15 μm), were analyzed in offline cold-stage ice nucleation experiments. The INP population in Greater Houston is complex, varying by site and day, but can be generalized by a weak to moderately efficient mode of INPs at −24°C and an efficient mode at −15°C. Analysis reveals that supermicron particles are largely responsible for ice nucleation warmer than −20°C across the region while submicron particles dominate at temperatures colder than −20°C. Additionally, significant spatial diversity in the INP population was observed, with differences in mean nucleation temperature between sites for nearly every size cut. Although INP concentrations were typically ∼0.08 L −1 at −20°C throughout the campaign, a notable region-wide increase in INP concentration for particles freezing at temperatures warmer than −20°C occurred from mid-August to mid-September. This comprehensive characterization of Greater Houston's INP population, including spatial, temporal, and particle size variations, can help constrain ice microphysics parameterizations in weather and climate models.

Thompson, Seth A. [Texas A & M Univ., College Stat↗

Coastal Urban Boundary-layer Interactions with Convection (CUBIC)

The CUBIC project added three extra weather‑profiling stations across Houston during the 2021 TRACER campaign to better understand how sea breezes, urban heat, and local circulations affect air quality and help trigger storms. These observations, combined with drone data and model simulations, give a clearer picture of how the boundary layer behaves in a coastal city.

54 ENVIRONMENTAL SCIENCES↗