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At least 37 records · Page 2

RaDIATE Collaboration for Material Studies

In the recent past, major accelerator facilities have been limited in beam power not by their accelerators, but by the beam intercepting device survivability. As next-generation accelerator target facilities (High Energy Physics, Spallation Sources, …) become increasingly more powerful and intense, high power target systems face key technical challenges. Beam-intercepting devices such as beam windows and secondary particle-production targets are continuously bombarded by high-energy high-intensity pulsed proton beams to produce secondary particles. Energy deposition from the primary beam induces near instantaneous heating (thermal shock) and microstructural changes (radiation damage) in the beam-intercepting materials. Both thermal shock and radiation damage ultimately degrade the performance and lifetime of targets and have been identified as the leading cross-cutting challenges of high-power target facilities. In order to operate reliable beam-intercepting devices in the framework of energy and intensity increase for next generation accelerators, the RaDIATE collaboration (Radiation Damage In Accelerator Target Environment) managed by Fermilab, brings together existing expertise in nuclear material and accelerator targets from 20 international institutions to execute a coordinated strategy for high power targetry R&D. This collaboration is generating new and useful materials data for application within the accelerator and the fission/fusion communities. I will give an overview of the RaDIATE R&D program and the achievement in the last few years on material studies in support of High Power Targetry development, including results obtained from irradiation test, development of novel materials and the prospective towards future irradiation campaign. A highlight will be given to the results in collaboration with our colleagues from J-PARC.

Pellemoine, Frederique↗

Molten Salt Targets for Future High-Power Accelerator Facilities

This talk will give an overview of will give an overview of recent work that began to examine the feasibility of molten salts as a target material for very high power beams as a potential solution for some of the present and future challenges of high power targetry at Fermilab, anchored by the F2D2 conceptual design study. This will include discussion of target and beam dump applications as well as likely challenges, potential for future R&D, projects, and synergy with existing high-power targetry research.

Williams, Jonathan K. [Fermilab]↗

Novel Materials and Concepts for Next-Generation High Power Target Applications

Novel beam-intercepting materials and targetry concepts are essential to improve the performance, reliability and operation lifetimes of next generation multi-megawatt (multi-MW) accelerator target facilities. The beam-intercepting materials and components must sustain an order-of-magnitude increase in particle beam intensities and are beyond the current state-of-the-art. With conventional materials already limiting the scope of experiments, it is crucial to investigate novel target materials, technologies and concepts that will satisfy the requirements and maximize the physics benefits of future energy and intensity frontier experiments. This paper provides an overview of the related targetry R&D required over the next 10 years to support and enable future high-power accelerator target facilities.

43 PARTICLE ACCELERATORS↗

Versatile tape-drive target for high-repetition-rate laser-driven proton acceleration

We present the development and characterization of a high-stability, multi-material, multi-thickness tape-drive target for laser-driven acceleration at repetition rates of up to 100 Hz. The tape surface position was measured to be stable on the sub-micrometre scale, compatible with the high-numerical aperture focusing geometries required to achieve relativistic intensity interactions with the pulse energy available in current multi-Hz and near-future higher repetition-rate lasers ( > kHz). Long-term drift was characterized at 100 Hz demonstrating suitability for operation over extended periods. The target was continuously operated at up to 5 Hz in a recent experiment for 70,000 shots without intervention by the experimental team, with the exception of tape replacement, producing the largest data-set of relativistically intense laser–solid foil measurements to date. This tape drive provides robust targetry for the generation and study of high-repetition-rate ion beams using next-generation high-power laser systems, also enabling wider applications of laser-driven proton sources.

47 OTHER INSTRUMENTATION↗

Flexible tape-drive target system for secondary high-intensity laser-driven sources

Here, we present the development of a flexible tape-drive target system to generate and control secondary high-intensity laser-plasma sources. Its adjustable design permits the generation of relativistic MeV particles and x rays at high-intensity (i.e., ≥1 × 10 18 W cm —2 ) laser facilities, at high repetition rates (>1 Hz). The compact and robust structure shows good mechanical stability and a high target placement accuracy (<4 μm RMS). Its compact and flexible design allows for mounting in both the horizontal and vertical planes, which makes it practical for use in cluttered laser-plasma experimental setups. The design permits ~170° of access on the laser-driver side and 120° of diagnostic access at the rear. A range of adapted apertures have been designed and tested to be easily implemented to the targetry system. The design and performance testing of the tape-drive system in the context of two experiments performed at the COMET laser facility at the Lawrence Livermore National Laboratory and at the Advanced Lasers and Extreme Photonics (ALEPH) facility at Colorado State University are discussed. Experimental data showing that the designed prototype is also able to both generate and focus high-intensity laser-driven protons at high repetition rates are also presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A customizable data management framework for high-repetition-rate high-energy-density science

The high-energy-density (HED) physics community is moving toward a new paradigm of high-repetition-rate (HRR) operation. To fully leverage the scientific power of HRR HED facilities, all of the components of each subsystem (laser, targetry, and performance diagnostics) must be connected and synchronized in a reliable and robust manner while the data acquired are tagged and archived in real time. To this end, GA has begun developing a generalized NoSQL-database framework, the MongoDB repository for information and archiving. An organizational strategy has been developed that shifts HED data organization from a shot-based to a diagnostic-based approach in order to increase archival and retrieval efficiency that lends itself to optimization applications. This work is a first step in pushing HRR HED science toward data management solutions that emphasize machine actionability and aim to stimulate community engagement to define data standards in HED science.

Instruments & Instrumentation↗

Accelerating the rate of discovery: toward high-repetition-rate HED science

As high-intensity short-pulse lasers that can operate at high-repetition-rate (HRR) (>10 H z ) come online around the world, the high energy density (HED) science they enable will experience a radical paradigm shift. The >10 3 increase in shot rate over today's shot-per-hour drivers translates into dramatically faster data acquisition, more experiments, and the ability to exploit machine learning, and thus the potential to significantly accelerate the advancement of HED science. A wide range of HED experiments, from opacity investigations to secondary source generation to plasma nuclear physics, will benefit from the increased statistics, precision, and exploration of phase space. Besides increasing the rate at which scientific experiments can be performed, HRR also allows for the rapid delivery of optimal experiments supported by simulations and modeling augmented by close coupling to empirical data. To fully realize such an HRR framework, numerous subsystems must be developed and brought together, including feedback laser control loops, high-throughput targetry and diagnostics, cognitive simulation, enhanced HED codes, and advanced data analytics. This paper describes the vision for an integrated HRR laser experimental HED system and outlines some of the major considerations and challenges for realizing it.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser-driven ion and electron acceleration from near-critical density gas targets: Towards high-repetition rate operation in the 1 PW, sub-100 fs laser interaction regime

Ion acceleration from gaseous targets driven by relativistic-intensity lasers was demonstrated as early as the late 1990s, yet most of the experiments conducted to date have involved picosecond-duration, Nd:glass lasers operating at low repetition rate. Here, we present measurements on the interaction of ultraintense ( ≈ 10 20 W cm − 2 , 1 PW ) , ultrashort ( ≈ 70 fs ) Ti:Sa laser pulses with near-critical ( ≈ 10 20 cm − 3 ) helium gas jets, a debris-free targetry with the potential for future compatibility with high ( ≈ 1 Hz ) repetition rate operation. We provide evidence of α particles being forward accelerated up to ≈ 2.7 − MeV energy with a total flux of ≈ 10 11 sr − 1 as integrated over > 0.1 − MeV energies and detected within a 0.5 − mrad solid angle. We also report on on-axis emission of relativistic electrons with an exponentially decaying spectrum characterized by a ≈ 10 − MeV slope, i.e., five times larger than the standard ponderomotive scaling. The total charge of these electrons with energy above 2 MeV is estimated to be of ≈ 1 nC , corresponding to ≈ 0.1 % of the laser drive energy. In addition, we observe the formation of a plasma channel, extending longitudinally across the gas density maximum and expanding radially with time. These results are well captured by large-scale particle-in-cell simulations, which reveal that the detected fast ions most likely originate from reflection off the rapidly expanding channel walls. The latter process is predicted to yield ion energies in the MeV range, which compare well with the measurements. Finally, direct laser acceleration is shown to be the dominant mechanism behind the observed electron energization. Published by the American Physical Society 2024

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

FRIB Beam Power Ramp-up: Status and Plans

After project completion on scope, on cost, and ahead of schedule, the Facility for Rare Isotope Beams began operations for scientific users in May of 2022. The ramp-up to a beam power of 400 kW is planned over a six-year period; 1 kW was delivered for initial user runs from in 2022, and 5 kW was delivered as of February 2023. Test runs with 10 kW 36Ar and 48Ca beams were conducted in July 2023. Upgrade plans include doubling the primary-beam energy to 400 MeV/nucleon for enhanced discovery potential (¿FRIB 400¿). This talk reports on the strategic plans towards high power operations emphasizing challenges and resolutions in beam-interception devices and targetry systems, radiation protection and controls, and legacy system renovation and integration.

43 PARTICLE ACCELERATORS↗

Multiphysics Simulations of Thermal Shock Testing of Nanofibrous High Power Targets

Increase of primary beam power for neutrino beam-lines leads to a reduced lifespan for production targets. New concepts for robust targets are emerging from the field of High Power Targetry (HPT); one idea being investigated by the HPT R&D Group at Fermilab is an electrospun nanofiber target. As part of their evaluation, samples with different densities were sent to the HiRadMat facility at CERN for thermal shock tests. The samples with the higher density, irradiated under a high intensity beam pulse, exhibit major damage at the impact site whereas those with the lower density show no apparent damage. The exact cause of this failure was unclear at the time. In this paper, we present the results of multiphysics simulations of the thermal shock experienced by the nanofiber targets that suggest the failure originates from the reduced permeability of the high density sample to air flow. The air present in the porous target expands due to heating from the beam, but is unable to flow freely in the high density sample, resulting in a larger back pressure that blows apart the nanofiber mat. We close with a discussion on how to further validate this hypothesis.

43 PARTICLE ACCELERATORS↗

Bayesian optimization scheme for the design of a nanofibrous high power target

High Power Targetry (HPT) R&D is critical in the context of increasing beam intensity and energy for next generation accelerators. Many target concepts and novel materials are being developed and tested for their ability to withstand extreme beam environments; the HPT R&D Group at Fermilab is developing an electrospun nanofiber material for this purpose. The performance of these nanofiber targets is sensitive to their construction parameters, such as the packing density of the fibers. Lowering the density improves the survival of the target, but reduces the secondary particle yield. Optimizing the lifetime and production efficiency of the target poses an interesting design problem, and in this paper we study the applicability of Bayesian optimization to its solution. We first describe how to encode the nanofiber target design problem as the optimization of an objective function, and how to evaluate that function with computer simulations. We then explain the optimization loop setup. Thereafter, we present the optimal design parameters suggested by the algorithm, and close with discussions of limitations and future refinements.

43 PARTICLE ACCELERATORS↗

Production of the Medically Important Radionuclides 52 Mn and 90 Nb

This collaborative proposal will create an integrated program of radionuclide production and research activities aimed toward the efficient isolation and characterization of the medically-relevant nuclides 52Mn and 90Nb. These two metallo-radionuclides were selected based on their emerging importance to the nuclide and medical communities but general lack of availability. The research described in this proposal will develop parameters and procedures for delivering clinical-grade, high specific-activity 52Mn and 90Nb for preclinical and translational applications by optimizing the cyclotron targetry and separation chemistry of 52Mn and 90Nb for use in basic positron-emission tomography (PET) radiotracer experiments. In addition the infrastructure that will be put in place through this project will enable a long term research partnership, with broader impact, between the three participating institutions. This proposal was submitted in 2012 under DE-FOA-0000743 and we have revised the present proposal significantly by addressing all of the previous Reviewers’ comments. Moreover, we have included newly acquired pilot data towards the production and characterization of these radionuclides.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Production of Medically Important Radionuclides 52 Mn and 90 Nb

Over the final reporting period of this project, we at MGH finalized our effort on Project 2: Production and Characterization of 90 Nb which, as per our previous report led us to an interesting application of mass spectrometry in radiometal chemistry. Overall, our research has developed parameters and procedures for delivering high 90 Nb for preclinical and translational applications by initializing the cyclotron targetry and separation chemistry for delivering 90 Nb in a chemical form suitable for subsequent development of 90 Nb-based PET radiotracers, and most recently we have published on the mass spectrometry applications described in the present report. We have been working with MSKCC (PI Jason Lewis) on the 90 Nb methodology and have had input from UAB (PI Suzy Lapi). An in-person meeting was held during the upcoming funding period with 2 PIs who are co-organizing the Radiochemistry Symposium (Lapi and Vasdev) and Program Director Dr. Ethan Balkin, during the ACS National Meeting in March 2018, and 2 PIs (Lewis and Vasdev) co presented in at the World Federation of Nuclear Medicine and Biology at a symposium sponsored by the Australian Nuclear Sciences and Technology Organisation, where they are both collaborating, in Melbourne, Australia in April 2018. Future projects and collaborations are under discussion with the Lapi lab to focus on new applications of 76 Br chemistry, and a new collaboration has already resulted with the Lewis lab on 18 F radiochemistry that employ iodonium ylide based precursors developed in the Vasdev lab, for clinical production of [ 18 F]MFBG. It is noteworthy that the PI has now relocated to the University of Toronto and has 2 cyclotrons (IBA Cyclone and Scanditronix MC-17) that will also be used to explore new 11 C-radiochemistry including [ 11 C]CO.

07 ISOTOPE AND RADIATION SOURCES↗

Snowmass2021 Topical Group Report from AF07: Targets and Sources

For the next multi-megawatt accelerator generation, targets and other beam-intercepting components will face even more severe challenges due to the higher power densities, higher energy, and higher radiation. A comprehensive research and development program must be implemented to address the challenges. International collaborations such as RaDIATE or High Power Targetry Workshop should be leveraged and expanded to accelerate knowledge gain and avoid duplicated efforts. The next generation of high power targets will need novel designs allowing better high heat flux cooling methods, novel materials, advanced simulations, and better instrumentation. Four main R&D tracks were identified and discussed for targets. For electron sources, current state of art and challenges we are facing for key components such as cathodes, guns and injector design for sources R&D are presented for highly polarized electrons and unpolarized high current high brightness beams. For ion sources such as electron cyclotron resonance ion source (ECRIS), laser ion source (LIS), charge breeders, status of development are reviewed, and areas require investment for future R&D are discussed separately. Facilities critical for various source development are recommended.

43 PARTICLE ACCELERATORS↗

The Status and Ambitions of the US Heavy Element Program

The aim of this whitepaper is to highlight the current capabilities and priorities of the US Heavy Element community and to provide the framework for a coordinated advancement of nuclear science from these studies. This is an organized effort to reflect on what has been achieved in the field given the recommendations and initiatives of the 2015 NSAC Long Range Plan, and on what can be realized in the next decade given current and possibly expanded investments. Current investments have positioned the US community to be among the world leaders in studies of the nuclear and chemical properties of the heaviest elements. These include studies of reaction mechanisms, moving us ever closer to the “island of stability”, in spectroscopy, allowing us to better understand nuclear structure at these extreme proton numbers, in chemical behavior, looking to determine how these elements should be placed on the Periodic Table, in performing the first measurements where isotopes are directly identified by their mass numbers, and in laying the foundation for a potential US-led new element discovery experiment. At present, the highest priority of the US Heavy Element community is to capitalize on the current investments by supporting the operations of US facilities at optimal values. These facilities include the Argonne Tandem Linac Accelerator System at Argonne National Laboratory and other Department of Energy facilities such as the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory, which has a dedicated superheavy element program, as well as university laboratories, including Texas A&M University. The High Flux Isotope Reactor at Oak Ridge National Laboratory is crucial to providing the radioactive isotopes required for heavy element science targets. This facility should be supported to provide the actinide materials that are essential for US-based science. Production of stable, rare isotopes for beam material, including 48 Ca, 50 Ti, 54 Cr and 58 Fe, at the Stable Isotope Production and Research Center is critical to continued research in heavy element science and should be a priority. The continued development of targets for heavy element science and retaining US-based expertise is critical for the heavy element community. This is an area that is currently under pressure. For example, the target laboratory at Argonne National Laboratory serves a broad community and is currently under threat due to loss of critical personnel. The skills needed to make targets for nuclear science and develop new targetry methods need to be supported long term at Argonne, Oak Ridge and Lawrence Livermore National Laboratories as well as maintaining the programs at Oregon State University and San José State University as vital pipelines for training students. Advances in theory are the foundation to understand how nuclei behave and to predict those behaviors in new circumstances. Progress in these studies will necessitate continued and new investment and access to high-performance computing. The future health of the heavy element field is dependent on the continuous support of talented early-career professionals at all levels. It is critical that opportunities continue to be created for the next generation to become established in heavy element research so that we can ensure the field is attracting and retaining the best minds for continued success. It is also clear that to ensure diversity of ideas, perspectives and techniques, we need to recruit diverse personnel that are trained at the best facilities. The heavy element community is in support of continued investment to programs with initiatives in diversity, equity, and inclusion. Looking to the next decade of research, support needs to maintain and grow US leadership in heavy element science. Specifically, new investments in state-of-the-art instrumentation will be essential to scientific development of the field and in expanding scientific knowledge. Advances in the next generation of electron cyclotron resonance ion sources, multi-reflection time-of-flight devices, laser spectroscopy, trapping methods and next generation alpha and gamma spectroscopy systems should be prioritized.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Production and Separations for High Specific Activity 186 Re, 189 Re and 47 Sc for Research and Clinical Applications: effective design of targets and recycling of targets and radioisotope separation

This grant involved three objectives for producing high specific activity radionuclides using reactor and accelerator technologies that would find use in medical, industrial and research applications. There was a strong emphasis in all projects to develop and train staff and students in all aspects of targetry, reactor and accelerator production, separation of radionuclides from enriched target material, and evaluating the specific activity of the product radionuclides. An additional objective was training of students (undergraduate, graduate, postdoctoral) in all aspects of radiochemistry.

07 ISOTOPE AND RADIATION SOURCES↗

ACE: Proton beam upgrade plan at Fermilab

aFor Snowmass and P5, Fermilab recently proposed a new upgrade plan known as Accelerator Complex Evolution (ACE) to occur after PIP-II upgrade in tandem with DUNE/LBNF operation. The first phase of ACE, ACE-MIRT, is the ACE Main Injector Ramp and Targetry upgrade, which would raise the LBNF beam power from 1.2 MW to 2 MW by shortening the Main Injector cycle time to around 0.65s. The second phase of ACE, AC-BR, is the ACE Booster Replacement, which would replace the Booster with a new machine and achieve 2.4 MW for DUNE/LBNF. The implications for the Fermilab neutrino program and future experiments hosted at Fermilab will be discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Accelerator challenges in the Fermilab Neutrino Program

In Fermilab's 2022-2023 proton complex run, Fermilab recovered from an unexpected failure in the neutrino focusing horn to achieve a record beam power of 960 kW. For Snowmass and P5, Fermilab recently proposed a new upgrade plan known as Accelerator Complex Evolution (ACE) to occur after PIP-II upgrade in tandem with DUNE/LBNF operation. The first phase of ACE, is the ACE Main Injector Ramp and Targetry upgrade, would raise the LBNF beam power from 1.2 MW to 2 MW by shortening the Main Injector cycle time to around 0.65s. The second phase of ACE, the ACE Booster Replacement, would replace the Booster with a new machine and achieve 2.4 MW for DUNE/LBNF. The core accelerator challenges, present and future, for operating intense neutrino beams at Fermilab will be highlighted.

43 PARTICLE ACCELERATORS↗