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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
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NASA NTRS2002

Electronic Absorption Spectra of Neutral Perylene (C20H12), Terrylene (C30H16), and Quaterrylene (C40H20) and their Positive and Negative Ions: Ne Matrix-Isolation Spectroscopy and Time Dependent Density Functional Theory Calculations

We present a full experimental and theoretical study of an interesting series of polycyclic aromatic hydrocarbons, the oligorylenes. The absorption spectra of perylene, terrylene and quaterrylene in neutral, cationic and anionic charge states are obtained by matrix-isolation spectroscopy in Ne. The experimental spectra are dominated by a bright state that red shifts with growing molecular size. Excitation energies and state symmetry assignments are supported by calculations using time dependent density functional theory methods. These calculations also provide new insight into the observed trends in oscillator strength and excitation energy for the bright states: the oscillator strength per unit mass of carbon increases along the series.

Halasinski, Thomas M.↗
NASA NTRS1999

The BATSE Gamma-Ray Burst Spectral Catalog: High Time Resolution Spectroscopy of Bright Bursts Using High Energy Resolution Data - 1

This is the first in a series of gamma-ray burst spectroscopy catalogs from the Burst And Transient Source Experiment (BATSE) on the Compton Gamma Ray Abstract: Observatory, each covering a different aspect of burst phenomenology. In this paper, we present time-sequences of spectral fit parameters for 156 bursts selected either for their high peak flux or fluence.

Preece, Robert D.↗
NASA NTRS2017

Single Object & Time Series Spectroscopy with JWST NIRCam

JWST will enable high signal-to-noise spectroscopic observations of the atmospheres of transiting planets with high sensitivity at wavelengths that are inaccessible with HST or other existing facilities. We plan to exploit this by measuring abundances, chemical compositions, cloud properties, and temperature-pressure parameters of a set of mostly warm (T 600 - 1200 K) and low mass (14 -200 Earth mass) planets in our guaranteed time program. These planets are expected to have significant molecular absorptions of H2O, CH4, CO2, CO, and other molecules that are key for determining these parameters and illuminating how and where the planets formed. We describe how we will use the NIRCam grisms to observe slitless transmission and emission spectra of these planets over 2.4 - 5.0 microns wavelength and how well these observations can measure our desired parameters. This will include how we set integration times, exposure parameters, and obtain simultaneous shorter wavelength images to track telescope pointing and stellar variability. We will illustrate this with specific examples showing model spectra, simulated observations, expected information retrieval results, completed Astronomer's Proposal Tools observing templates, target visibility, and other considerations.

NIRCam↗
NASA NTRS2004

RXTE Timing and Spectroscopy of a Black Hole X-Ray Binary in Outburst

This program was executed primarily to observe the black hole transient GX339-4. Observations were made simultaneously with XMM-Newton in 2004 March, and observations simultaneous with Chandra will continue to be made in the fall of 2004. As the total data set has not yet been obtained, a great deal of work remains. Preliminary examination of the data has shown extremely exciting spectral features (Fe K-alpha emission lines) and timing features (strong QPOs and flaring variability) of exactly the sort we hoped to obtain. We expect that the results of these observations will be finalized over the next year. The results will be presented in 2-3 publications in refereed journals. We have requested a no-cost extension of this grant to analyze and report our findings.

Miller, Jon M.↗
NASA NTRS2003

Fe XXV and Fe XXVI Diagnostics of the Black Hole and Accretion Disk in Active Galaxies: Chandra Time-Resolved Spectroscopy of NGC 7314

We report the detection of Fe xxv and Fe XXVI Ka emission lines from a Chandra High Energy Grating Spectrometer (HETGS) observation of the narrow-line Seyfert 1 galaxy NGC 7314, made simultaneously with RXTE. The lines are redshifted (cz approximately 1500 kilometers per second) relative to the systemic velocity and unresolved by the gratings. We argue that the lines originate in a near face-on (less than 7 deg) disk having a radial line emissivity flatter than r(exp -2). Line emission from ionization states of Fe in the range approximately Fe I a up to Fe XXVI is observed. The ionization balance of Fe responds to continuum variations on timescales less than 12.5 ks, supporting an origin of the lines close to the X-ray source. We present additional, detailed diagnostics from this rich data set. These results identify NGC 7314 as a key source to study in the future if we are to pursue reverberation mapping of space-time near black-hole event horizons. This is because it is first necessary to understand the ionization structure of accretion disks and the relation between the X-ray continuum and Fe Ka line emission. However, we also describe how our results are suggestive of a means of measuring black-hole spin without a knowledge of the relation between the continuum and line emission. Finally, these data emphasize that one can study strong gravity with narrow (as opposed to very broad) disk lines. In fact narrow lines offer higher precision, given sufficient energy resolution.

Yaqoob, Tahir↗
NASA NTRS1982

Time-resolved spectroscopy of solid poly/1-vinyl naphthalene/ following electron beam pulse radiolysis - Pulse radiolytic studies on polymers

Transient emission studies following pulse radiolysis of solid poly(1-vinyl naphthalene) show existence of excited monomers and two excimers. Quenching experiments indicate that excimers are not formed directly by recombination of ions but probably by trapping of migrating monomeric excitation in preformed traps whose density is approximately one in 1000.

Coulter, D. R.↗
NASA NTRS2001

UV Timing and Spectroscopy of the Crab Nebula Pulsar

We have used the Hubble Space Telescope and Space Telescope Imaging Spectrograph to obtain Near Ultraviolet (NUV) (1600-3200 Angstroms) and Far Ultraviolet (FUV) (1140-1720 Angstroms) spectra and pulse profiles of the Crab Nebula's pulsar. The pulse period agrees well with the radio predictions. The NUV and FUV pulse profiles are little changed from the visible wavelength profile. Spectra obtained with the Nordic Optical Telescope were combined with the UV spectra for full coverage from 1140-9250Angstoms. Dereddening the spectrum with a standard extinction curve achieves a flat spectrum for E(B-V)=0.52, R=3.1. Lyman alpha absorption indicates a column density of 3.0=/-0.5 x 10(exp 21) cm -2, consistent with the E(B-V) of 0.52. The dereddened spectrum can be fitted by a power law with spectral index alpha=0.11+/-0.04. A broad, blueshifted absorption is seen in CIV (1550Angstroms), reaching a velocity of about 2500 kilometer per second.

Gull, Theodore R.↗
NASA NTRS2004

Time Resolved Spectroscopy of High Field Polars (FUSE 00)

The following work has been accomplished: 1) The emission lines of O VI1 and He II were used to produce Doppler tomograms of the plasma emission. 2) An improved interstellar absorption model is being developed for the CIAO spectral fitting program, Sherpa. Use of the earlier version of this model showed it to be inadequate for its purpose. Once this model is working, we intend to complete our analysis of V884 Her and those of other FUSE programs. In addition to the above work, this grant has helped support the following related work: 1) The publication of the paper "Periodicities in the X-ray intensity variations of TV Columbae: an Intermediate Polar" by Rana, V. R., Singh, K. P., Schlegel, E. M., & Barrett, P. 2004, AJ, 126,489, and 2) FUSE data of a possible nova-like variable Ret 1 has been analyzed and shown to contain a hot (37000 deg) white dwarf (WD 0334-6400). The FUV spectrum shows strong absorption lines of C III.

Barrett, Paul↗
NASA NTRS2005

Strong-field Gravitational Effects in the Timing and Spectroscopy of X-Ray Binaries

Using the ray-tracing code described, we developed additional features to the hot spot model to explain the broadening of the quasi-periodic oscillation (QPO) peaks as well as the damping of higher frequency harmonics in the power spectrum. We derived a number of analytic results that agree closely with more detailed numerical calculations. Three primary pieces are developed: the superposition of multiple hot spots with finite lifetimes and random phases, a width in the radial distribution of geodesic orbits, and the scattering of photons from the hot spot through a corona around the black hole. The complete model is used to fit the observed power spectra of both type A and type B QPOs seen in XTE 51550-564, giving confidence limits on each of the model parameters. These results were presented in a conference paper and in a refereed publication. We also explored the possibility of using higher-order statistics, particularly the bispectrum and bicoherence, to distinguish between competing QPO models. These methods were applied to the hot spot model and a method was proposed to map out the spacetime metric around Kerr black holes in Ref. 3 below.

Bertschinger, Edmund↗
NASA NTRS2005

High Resolution Spectroscopy And Timing Of The Isolated Neutron Star RBS 1774

The 2004 May 31 XMM-Newton observation was reprocessed using SASv6.0.0 and times of high background were filtered out. The net exposure time remaining was 23 ks. The source was clearly detected in MOS1, MOS2 and PN chips. We performed both timing and spectroscopic analysis on the data. We performed a spectral analysis by fitting data from the three EPIC detectors simultaneously, finding that the broadband spectrum can be represented by a single absorbed blackbody, with kT = 0.10 keV. The fitting revealed the presence of an absorption feature at 0:7 keV, but the data did have enough resolution to allow us to discriminate between an absorption line and an edge. We also tested magnetized models of Pavlov et a1 and Zavlin et al, but found that fits with these models were considerably worse than with a blackbody. For the timing analysis, we extracted the counts within a 3000 radius aperture in both PN and MOS 1 and MOS2 but with the aperture truncated by a chord where it approached the edge of the CCD window in each case: this maximized the counts while avoiding any edge effects. We analyzed PN, MOSl and MOS2 data both individually and combined using the Maximum Likelihood Periodogram technique of Zane et al. (2002) and Cropper et al. (2004). Periods from 10000 s to 30 ms were searched, ensuring that in each case the period grid was 2.5 times better sampled than the Nyquist frequency. The search revealed a significant period at 9.437s. Taken overall, we found the characteristics of RBS 1774 to be remarkably similar to those of another X-ray faint isolated neutron stars. These results were written up for the Astrophysical Journal, and the paper has recently been accepted for publication.

Mushotzky, Richard↗
NASA NTRS2005

Time Resolved Spectroscopy of Eclipsing Polars

No changes have been made since the last annual progress report was submitted in conjunction with a unilateral NCX. Dr. Barrett was affected by an STScI Reduction in Force (RIF). He is now employed by the Johns Hopkins University and plans to continue his research there. No expenses have been charged to this grant, however the FUSE data for the eclipsing polar V1432 Aql has been received and processed using CALFWSE v3.0.6. The resulting summed spectrum has been used for a preliminary analysis of the interstellar absorption towards V1432 Aql. We find a hydrogen column density of less than 1.5e21 cm^-2. We have used this result in the paper "X-Ray Emission and Optical Polarization of V1432 Aquilae: An Asynchronous Polar" to fix the hydrogen column density in the soft (<0.5 keV) X-ray band when analyzing the XMM-Newton spectra of this polar. This has enabled us to find an accurate temperature for the blackbody component of 88+/-2 eV, which is significantly higher than that of other polars (20 - 40 eV). We hope to complete our analysis of the phase-resolved emission line spectra of V1432 Aql and to prepare the results for publication in a refereed journal. We hope to begin work on this star within the next few months.

Barrett, Paul↗
NASA NTRS1991

LDEF impact craters formed by carbon-rich impactors

Two small craters (number 74, 119 microns, and number 31, 158 microns in diameter) with depth to diameter ratios of about 0.59 and 0.8, respectively, were found in Al from the Long Duration Exposure Facility (LDEF) experiment tray A11EOOF). Both craters have residues concentrated in the crater bottoms, along the walls, and on top of the overturned rims. Low voltage scanning electron electron microscopy, Auger electron spectroscopy, time of flight secondary ion mass spectroscopy and energy dispersive x-ray spectroscopy were used to obtain high resolution imagery and elemental analysis. Analyses indicate that the impactor for both craters was carbon-rich, as the residues contain mostly C. Silicon, S, and F in low concentrations are present on the Al surface away from the craters and may be, in part, contaminants.

Bunch, T. E.↗
NASA NTRS2021

Waveguiding and Dispersion Properties of Interband Cascade Laser Frequency Combs

Mid-infrared semiconductor lasers have emerged as indispensable compact coherent sources for military and commercial applications. While much of the historical emphasis has been on maximizing the output power and/or spectral purity, a recent new focus has been on engineering these lasers to operate as optical frequency combs (OFCs) for broadband real-time spectroscopy. In particular, the combination of low-drive-power and broad gain bandwidth has made interband cascade laser (ICL) OFCs an attractive complement to quantum cascade laser OFCs operating at longer wavelengths. Moreover, ICL combs can potentially be incorporated into fully-integrated dual-comb spectrometers that employ fast, room-temperature IC photodetectors processed on the same chip.However, the high refractive index of the ICL’s GaSb substrate poses some challenges to the optical waveguiding. Because the modal index is considerably lower than that of the substrate, the optical field can penetrate the bottom cladding layer and leak into the GaSb, inducing wavelength-dependent interference that modifies the gain and group velocity dispersion (GVD) profiles. Even when the effect on lasing threshold is small, the comb properties can be adversely affected. Using the sub-threshold Fourier transform technique, we studied ICL combs with various ridge widths, substrate thicknesses, and center wavelengths. This allowed us to evaluate the effects of modal leakage on the GVD. We find that the resonant nature of the substrate modes induces oscillations, which affect both the spectral bandwidth and the phase-locking properties above threshold. Strategies to mitigate the GVD’s undesired and unpredictable spectral variation will be presented.

Meyer, J. R↗
NASA NTRS2011

Frame-Transfer Gating Raman Spectroscopy for Time-Resolved Multiscalar Combustion Diagnostics

Accurate experimental measurement of spatially and temporally resolved variations in chemical composition (species concentrations) and temperature in turbulent flames is vital for characterizing the complex phenomena occurring in most practical combustion systems. These diagnostic measurements are called multiscalar because they are capable of acquiring multiple scalar quantities simultaneously. Multiscalar diagnostics also play a critical role in the area of computational code validation. In order to improve the design of combustion devices, computational codes for modeling turbulent combustion are often used to speed up and optimize the development process. The experimental validation of these codes is a critical step in accepting their predictions for engine performance in the absence of cost-prohibitive testing. One of the most critical aspects of setting up a time-resolved stimulated Raman scattering (SRS) diagnostic system is the temporal optical gating scheme. A short optical gate is necessary in order for weak SRS signals to be detected with a good signal- to-noise ratio (SNR) in the presence of strong background optical emissions. This time-synchronized optical gating is a classical problem even to other spectroscopic techniques such as laser-induced fluorescence (LIF) or laser-induced breakdown spectroscopy (LIBS). Traditionally, experimenters have had basically two options for gating: (1) an electronic means of gating using an image intensifier before the charge-coupled-device (CCD), or (2) a mechanical optical shutter (a rotary chopper/mechanical shutter combination). A new diagnostic technology has been developed at the NASA Glenn Research Center that utilizes a frame-transfer CCD sensor, in conjunction with a pulsed laser and multiplex optical fiber collection, to realize time-resolved Raman spectroscopy of turbulent flames that is free from optical background noise (interference). The technology permits not only shorter temporal optical gating (down to <1 s, in principle), but also higher optical throughput, thus resulting in a substantial increase in measurement SNR.

Nguyen, Quang-Viet↗