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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Raising the Bar in High Performance Laboratory Design

Laboratory facilities are expensive to build and operate, they consume energy at high rates compared to other types of buildings, and modifications are frequently required to accommodate ever-changing research activities. PNNL sought ways to address these issues in the design and construction of a 14,700 sq. ft. new laboratory building. To improve adaptability to change a high roof structure was used that allows raising the ceiling when needed with minimal disruption to installed HVAC and electrical utilities. Also, HVAC equipment was located on a mezzanine above the central corridor rather than above ceilings. This eliminates the need for maintenance personnel to routinely access lab spaces, reducing disruption to research staff and improving maintenance access. To improve the reliability of operations while reducing energy consumption, heat pipe heat recovery with evaporative cooling, zoned heating/cooling coils, high-efficiency condensing boilers, district cooling, VAV fume hoods, DDC controls, energy use monitoring, and implementation of the US Department of Energy’s Guiding Principles for Federal Leadership in Sustainable Buildings were all used. The energy model developed during design projected energy use at 2,840 MBtu/yr, a 13.5% savings over ASHRAE Standard 90.1-2010. The first full year of operation resulted in actual energy use of 2,661 MBtu, a savings of 19% over Standard 90.1. As a result of the project design’s demonstrated success, these strategies will be incorporated into a significantly larger (125,000 sq ft), $65 million lab facility to be constructed on the PNNL campus in 2020.

Scott, Jeffery M.↗
DOE OSTI2025

Experimental targets for dark photon dark matter

Ultralight dark photon dark matter features distinctive cosmological and astrophysical signatures and is also supported by a burgeoning direct-detection program searching for its kinetic mixing with the ordinary photon over a wide mass range. Dark photons, however, cannot necessarily constitute the dark matter in all of this parameter space. In minimal models where the dark photon mass arises from a dark Higgs mechanism, early-Universe dynamics can easily breach the regime of validity of the low-energy effective theory for a massive vector field. In the process, the dark sector can collapse into a cosmic string network, precluding dark photons as viable dark matter. We establish the general conditions under which dark photon production avoids significant backreaction on the dark Higgs and identify regions of parameter space that naturally circumvent these constraints. After surveying implications for known dark photon production mechanisms, we propose novel models that set well-motivated experimental targets across much of the accessible parameter space. We also discuss complementary cosmological and astrophysical signatures that can probe the dark sector physics responsible for dark photon production.

Dark matter↗
DOE OSTI2023

DarkNESS: Characterization of Space Multi-Chip Module Skipper-CCDs and Readout Electronics

The DarkNESS mission has the goal of deploying a 6U CubeSat fitted with an array of skipper-CCDs in Low Earth Orbit (~400 km). The new instrument will take measurements of diffuse x-rays and look for signatures of dark matter decay in the spectrum. DarkNESS will also perform a direct search for strongly interacting sub-GeV dark matter in regions of the parameter space not accessible to ground based experiments [1]. Skipper-CCDs allow for low-noise astronomical observations which can extend the discovery reach for direct dark matter search experiments. This paper will discuss the laboratory characterization of the two key components of the scientific payload: the space Multi-Chip Module (sMCM), and their readout electronics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

CubeSats for Gamma-Ray Astronomy [Book Chapter]

After many years of flying in space primarily for educational purposes, CubeSats – tiny satellites with form factors corresponding to arrangements of “1U” units, or cubes, each 10 cm on a side – have come into their own as valuable platforms for technology advancement and scientific investigations. CubeSats offer comparatively rapid, low-cost access to space for payloads that can be built, tested, and operated by relatively small teams, with substantial contributions from students and early career researchers. Continuing advances in compact, low-power detectors, readout electronics, and flight computers have now enabled X-ray and gamma-ray sensing payloads that can fit within the constraints of CubeSat missions, permitting in-orbit demonstrations of new techniques and innovative high-energy astronomy observations. Gamma-ray-sensing CubeSats are certain to make an important contribution in the new era of multi-messenger, time-domain astronomy by detecting and localizing bright transients such as gamma-ray bursts, solar flares, and terrestrial gamma-ray flashes; however, other astrophysical science areas requiring long observations in a low-background environment, including gamma-ray polarimetry, studies of nuclear lines, and measurement of diffuse backgrounds, will likely benefit as well. Here we present the primary benefits of CubeSats for high-energy astronomy, highlight the scientific areas currently or soon to be studied, and review the missions that are currently operating, under development, or proposed. A rich portfolio of CubeSats for gamma-ray astronomy already exists, and the potential for a broad range of creative and scientifically productive missions in the near future is very high.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Perturbative instability of nonergodic phases in non-Abelian quantum chains

An important challenge in the field of many-body quantum dynamics is to identify nonergodic states of matter beyond many-body localization (MBL). Strongly disordered spin chains with non-Abelian symmetry and chains of non-Abelian anyons are natural candidates, as they are incompatible with standard MBL. In such chains, real space renormalization group methods predict a partially localized, nonergodic regime known as a quantum critical glass (a critical variant of MBL). Here, this regime features a treelike hierarchy of integrals of motion and symmetric eigenstates with entanglement entropy that scales as a logarithmically enhanced area law. We argue that such tentative nonergodic states are perturbatively unstable using an analytic computation of the scaling of off-diagonal matrix elements and accessible level spacing of local perturbations. Our results indicate that strongly disordered chains with non-Abelian symmetry display either spontaneous symmetry breaking or ergodic thermal behavior at long times. We identify the relevant length and timescales for thermalization: Even if such chains eventually thermalize, they can exhibit nonergodic dynamics up to parametrically long timescales with a nonanalytic dependence on disorder strength.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Low Repetition-Rate, High-Resolution Femtosecond Transmission Electron Microscopy

Spatial and energy resolutions of state-of-the-art transmission electron microscopes (TEMs) have surpassed 50 pm and 5 meV. However, with respect to the time domain, even the fastest detectors combined with the brightest sources may only be able to reach the microsecond timescale. Thus, conventional methods are incapable of resolving myriad fundamental ultrafast (i.e., attosecond to picosecond) atomic-scale dynamics. The successful demonstration of femtosecond (fs) laser-based (LB) ultrafast transmission electron microscopy (UEM) nearly 20 years ago provided a means to span this nearly 10-order-of-magnitude temporal gap. While nanometer-picosecond UEM studies of dynamics are now well established, ultrafast Å-scale imaging has gone largely unrealized. Further, while instrument development has rightly been an emphasis, and while new modalities and uses of pulsed-beam TEM continue to emerge, the overall chemical and materials application space has been only modestly explored to date. In this Perspectives article, we argue that these apparent shortfalls can be attributed to a simple lack of data and detail. We speculate that present work and continued growth of the field will ultimately lead to the realization that Å-scale fs dynamics can indeed be imaged with minimally modified UEM instrumentation and with repetition rates (f rep ) below - and perhaps even well below - 1 MHz. We further argue that use of low f rep , whether for LB UEM or for chopped/bunched beams, significantly expands the accessible application space. Furthermore, this calls for systematically establishing modality-specific limits so that especially promising technologies can be pursued, thus ultimately facilitating broader adoption as individual instrument capabilities expand.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Non‐Equilibrium Synthesis Methods to Create Metastable and High‐Entropy Nanomaterials

Stabilizing multiple elements within a single phase enables the creation of advanced materials with exceptional properties arising from their complex composition. However, under equilibrium conditions, the Hume–Rothery rules impose strict limitations on solid-state miscibility, restricting combinations of elements with mismatched crystal structures, atomic radii, valence states, or electronegativities. This severely narrows the accessible compositional space for creating new inorganic materials. In this review, we highlight how non-equilibrium synthesis methods, featuring ultrafast heating and quenching, can overcome these thermodynamic barriers, enabling integration of immiscible elements into metastable and high-entropy nanostructures. The resulting materials benefit from both kinetic trapping and stabilization by high configurational entropy, leading to enhanced phase stability. These materials can exhibit unique structural and functional properties that are needed for advancing catalysis, energy storage, thermoelectrics, and sensing. Furthermore, the ability of non-equilibrium methods to generate unconventional compositions and structures expands the material design space dramatically, offering rich datasets for AI-guided materials discovery. When combined with their inherent high-throughput and scalable characteristics, these approaches enable rapid, iterative optimization and accelerate the development and industrial production of next-generation inorganic materials.

high-entropy materials↗
DOE OSTI2020

On the ATLAS top mass measurements and the potential for stealth stop contamination

The discovery of the stop — the Supersymmetric partner of the top quark — is a key goal of the physics program enabled by the Large Hadron Collider. Although much of the accessible parameter space has already been probed, all current searches assume the top mass is known. This is relevant for the “stealth stop” regime, which is characterized by decay kinematics that force the final state top quark off its mass shell; such decays would contaminate the top mass measurements. We investigate the resulting bias imparted to the template method based ATLAS approach. A careful recasting of these results shows that effect can be as large as 2.0 GeV, comparable to the current quoted uncertainty on the top mass. Thus, a robust exploration of the stealth stop splinter requires the simultaneous consideration of the impact on the top mass. Additionally, we explore the robustness of the template technique, and point out a simple strategy for improving the methodology implemented for the semi-leptonic channel.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

High-Entropy Oxides in the Mullite-Type Structure

High-entropy materials (HEMs) represent a new class of solid solutions containing at least five different elements. Their compositional diversity makes them promising as platforms for the development of functional materials. We synthesized new HEMs in a mullite-type structure and present five compounds, i.e., Bi 2 (Al 0.25 Ga 0.25 Fe 0.25 Mn 0.25 ) 4 O 9 and A 2 Mn 4 O 10 with variations of A = Nd, Sm, Y, Er, Eu, Ce, and Bi, demonstrating the vast accessible composition space. By combining scattering, microscopy, and spectroscopy techniques, we show that our materials are mixed solid solutions. Remarkably, when following their crystallization in situ using X-ray diffraction and X-ray absorption spectroscopy, we find that the HEMs form through a metastable amorphous phase without the formation of any crystalline intermediates. We expect that our synthesis is excellently suited to synthesizing diverse HEMs and therefore will have a significant impact on their future exploration.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Unconventional colloidal aggregation in chiral bacterial baths

Abstract When in equilibrium, thermal forces agitate molecules, which then diffuse, collide and bind to form materials. However, the space of accessible structures in which micron-scale particles can be organized by thermal forces is limited, owing to the slow dynamics and metastable states. Active agents in a passive fluid generate forces and flows, forming a bath with active fluctuations. Two unanswered questions are whether those active agents can drive the assembly of passive components into unconventional states and which material properties they will exhibit. Here we show that passive, sticky beads immersed in a bath of swimmingEscherichia colibacteria aggregate into unconventional clusters and gels that are controlled by the activity of the bath. We observe a slow but persistent rotation of the aggregates that originates in the chirality of theE. coliflagella and directs aggregation into structures that are not accessible thermally. We elucidate the aggregation mechanism with a numerical model of spinning, sticky beads and reproduce quantitatively the experimental results. We show that internal activity controls the phase diagram and the structure of the aggregates. Overall, our results highlight the promising role of active baths in designing the structural and mechanical properties of materials with unconventional phases.

Physics↗
DOE OSTI2025

Engineering modular enzyme assembly: synthetic interface strategies for natural products biosynthesis applications

Covering: 2020 to 2025Natural products remain indispensable sources of therapeutic and bioactive compounds, yet traditional discovery strategies are constrained by compound rediscovery. Modular biosynthetic enzymes, such as type I polyketide synthases (PKSs) and type A non-ribosomal peptide synthetases (NRPSs), offer promising platforms for combinatorial biosynthesis owing to their programmable architectures. However, practical implementation is frequently limited by inter-modular incompatibility and domain-specific interactions. This review highlights recent advances in modular enzyme assembly enabled by synthetic interfaces-including cognate docking domains, synthetic coiled-coils, SpyTag/SpyCatcher, and split inteins-which function as orthogonal, standardized connectors to facilitate post-translational complex formation. These interfaces support rational investigations into substrate specificity, module compatibility, and pathway derivatization as well as general enzyme clustering applications beyond PKS and NRPS systems. Synthetic interfaces can be integrated with computational tools to support a more systematic and scalable framework for modular enzyme engineering by providing predictive insights into domain compatibility and interface design. These approaches within iterative design-build-test-learn workflows can accelerate the programmable assembly of biosynthetic systems and expand the accessible chemical space for natural products.

Kim, Gahyeon↗
DOE OSTI2020

Excited state dynamics of cis,cis-1,3-cyclooctadiene: Non-adiabatic trajectory surface hopping

We have performed trajectory surface hopping dynamics for cis,cis-1,3-cyclooctadiene to investigate the photochemical pathways involved after being excited to the S 1 state. Our calculations reveal ultrafast decay to the ground state, facilitated by conical intersections involving distortions around the double bonds. The main distortions are localized on one double bond, involving twisting and pyramidalization of one of the carbons of that double bond (similar to ethylene), while a limited number of trajectories decay via delocalized (non-local) twisting of both double bonds. The interplay between local and non-local distortions is important in our understanding of photoisomerization in conjugated systems. The calculations show that a broad range of the conical intersection seam space is accessed during the non-adiabatic events. Several products formed on the ground state have also been observed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Kinetic-ballooning-bifurcation in tokamak pedestals across shaping and aspect-ratio

We use a new gyrokinetic threshold model to predict a bifurcation in tokamak pedestal width-height scalings that depends strongly on plasma shaping and aspect-ratio. The bifurcation arises from the first and second stability properties of kinetic-ballooning-modes that yields wide and narrow pedestal branches, expanding the space of accessible pedestal widths and heights. The wide branch offers potential for edge-localized-mode-free pedestals with high core pressure. For negative triangularity, low-aspect-ratio configurations are predicted to give steeper pedestals than conventional-aspect-ratio. Both wide and narrow branches have been attained in tokamak experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Probing the dynamics and bottleneck of the key atmospheric SO 2 oxidation reaction by the hydroxyl radical

SO 2 (Sulfur dioxide) is the major precursor to the production of sulfuric acid (H 2 SO 4 ), contributing to acid rain and atmospheric aerosols. Sulfuric acid formed from SO 2 generates light-reflecting sulfate aerosol particles in the atmosphere. This property has prompted recent geoengineering proposals to inject sulfuric acid or its precursors into the Earth’s atmosphere to increase the planetary albedo to counteract global warming. SO 2 oxidation in the atmosphere by the hydroxyl radical HO to form HOSO 2 is a key rate-limiting step in the mechanism for forming acid rain. However, the dynamics of the HO + SO 2 → HOSO 2 reaction and its slow rate in the atmosphere are poorly understood to date. Herein, we use photoelectron spectroscopy of cryogenically cooled HOSO 2 – anion to access the neutral HOSO 2 radical near the transition state of the HO + SO 2 reaction. Spectroscopic and dynamic calculations are conducted on the first ab initio-based full-dimensional potential energy surface to interpret the photoelectron spectra of HOSO 2 – and to probe the dynamics of the HO + SO 2 reaction. In addition to the finding of a unique pre-reaction complex (HO⋯SO 2 ) directly connected to the transition state, dynamic calculations reveal that the accessible phase space for the HO + SO 2 → HOSO 2 reaction is extremely narrow, forming a key reaction bottleneck and slowing the reaction rate in the atmosphere, despite the low reaction barrier. This study underlines the importance of understanding the full multidimensional potential energy surface to elucidate the dynamics of complex bimolecular reactions involving polyatomic reactants.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Piecewise Omnigenous Stellarators

In omnigenous magnetic fields, charged particles are perfectly confined in the absence of collisions and turbulence. For this reason, the magnetic configuration is optimized to be close to omnigenity in any candidate for a stellarator fusion reactor. However, approaching omnigenity imposes severe constraints on the spatial variation of the magnetic field. In particular, the topology of the contours of constant magnetic field strength on each magnetic surface must be such that there are no particles transitioning between different types of wells. This, in turn, usually leads to complicated plasma shapes and coils. This Letter presents a new family of optimized fields that display tokamak-like collisional energy transport while having transitioning particles. This result radically broadens the space of accessible reactor-relevant configurations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

Bounds on Lorentz Invariance Violation from Muon Fluctuations at the Pierre Auger Observatory

Quantum gravity theories often modify spacetime symmetries. In particular, Lorentz invariance may be violated when approaching the Planck scale. Although the scales at which interactions occur in extensive air showers induced by ultra-high-energy cosmic rays in the atmosphere are many orders of magnitude below the Planck scale, these violations might still be observable. In this Letter, the fluctuations in the number of muons in the extensive air showers measured at the Pierre Auger Observatory are exploited, for the first time, to constrain Lorentz invariance violations. The bounds derived in the hadronic sector are the strongest ever obtained, and do not rely on assumptions about the mass composition of ultra-high-energy cosmic rays. The fluctuations in the number of muons constitute a new and powerful observable to further explore Lorentz invariance in a region of the parameter space not accessible to other observables.

Abdul Halim, A. [Adelaide U.] (ORCID:0000000312181↗
DOE OSTI2021

White Box Access to Quantum Testbeds for Co-Design

At Lawrence Livermore National Laboratory (LLNL), we operate and maintain the Quantum Device and Integration Testbed (QuDIT) facility, a small quantum testbed that supports about 10 active research teams (including our own) and over 50 internal and external collaborators. This testbed is designed to give remote white box access to users for research, training, and outreach. A guiding principle behind the development of our testbed infrastructure, software and user interfaces is to empower users to perform experiments at the cutting edge of quantum information science at any level of abstraction, from materials studies, device physics and control and characterization techniques to algorithm development and quantum operating system design. Our testbed targets a multilevel quantum system (qudit) to expand the accessible Hilbert space of a simple-to-manufacture quantum device and focuses on quantum simulation, typically implemented through custom gates designed with quantum optimal control methods, rather than on a universal computing framework with a fixed gate set. We leverage the Lab’s high-performance computing (HPC) program and related expertise to simulate quantum systems, develop hybrid algorithms, and generate gates optimized for given simulations. Additionally, we have adopted a co-design philosophy from the HPC community in designing new hardware, so that the systems we develop are optimized for the specific physics simulations we plan to use them for.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗