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NASA NTRS2021

Retrieval of Stratospheric Aerosol Size Distribution Parameters Using Satellite Solar Occultation Measurements at Three Wavelengths

In this work, a novel approach for the determination of the particle size distribution (PSD) parameters of stratospheric sulfate aerosols is presented. For this, ratios of extinction coefficients obtained from SAGE III/ISS (Stratospheric Aerosol and Gas Experiment III on the International Space Station) solar occultation measurements at 449, 756 and 1544 nm were used to retrieve the mode width and median radius of a size distribution assumed to be monomodal lognormal. The estimated errors at the peak of the stratospheric aerosol layer, on average, lie between 20% and 25% for the median radius and 5% and 7% for the mode width. The results are consistent in magnitude with other retrieval results from the literature, but a robust comparison is difficult, mainly because of differences in temporal and spatial coverage. Other quantities like number density and effective radius were also calculated. A major advantage of the described method over other retrieval techniques is that both the median radius and the mode width can be retrieved simultaneously, without having to assume one of them. This is possible due to the broad wavelength spectrum covered by the SAGE III/ISS measurements. Also, the presented method – being based on the analysis of three wavelengths – allows unique solutions for the retrieval of PSD parameters for almost all of the observed extinction spectra, which is not the case when using only two spectral channels. In addition, the extinction coefficients from SAGE III/ISS solar occultation measurements, on which the retrieval is based, are calculated without a priori assumptions about the PSD. For those reasons, the data produced with the presented retrieval technique may be a valuable contribution for a better understanding of the variability of stratospheric aerosol size distributions, e.g. after volcanic eruptions. While this study focuses on describing the retrieval method, and a future study will discuss the PSD parameter data set produced in depth, some exemplary results for background conditions in June 2017 are shown.

Felix Wrana↗
NASA NTRS2003

Measuring Aerosol Size Distributions from the NASA DC-8 in SOLVE II

The University of Denver Focused Cavity Aerosol Spectrometer (FCAS 11) and Nucleation-Mode Aerosol Size Spectrometer (N-MASS) were successfully integrated and flown aboard NASA s DC-8 for the second SAGE I11 Ozone Loss and Validation Experiment (SOLVE 11). Both instruments performed well during SOLVE, with virtually complete data coverage for all mission and test flights. The few exceptions to this were the occasional simultaneous zero-check for the instruments, and some data loss for channel 4 of the N-MASS. The only consequence of the latter is reduced resolution in the 15 to 60 nm range for the affected size distributions.

Reeves, Michael↗
NASA NTRS2000

Volcanic Signatures in Estimates of Stratospheric Aerosol Size, Distribution Width, Surface Area, and Volume Deduced from Global Satellite-Based Observations

Volcanic signatures in the stratospheric aerosol layer are revealed by two independent techniques which retrieve aerosol information from global satellite-based observations of particulate extinction. Both techniques combine the 4-wavelength Stratospheric Aerosol and Gas Experiment (SAGE) II extinction measurements (0.385 <= lambda <= 1.02 microns) with the 7.96 micron and 12.82 micron extinction measurements from the Cryogenic Limb Array Etalon Spectrometer (CLAES) instrument. The algorithms use the SAGE II/CLAES composite extinction spectra in month-latitude-altitude bins to retrieve values and uncertainties of particle effective radius R(sub eff), surface area S, volume V and size distribution width sigma(sub R). The first technique is a multi-wavelength Look-Up-Table (LUT) algorithm which retrieves values and uncertainties of R(sub eff) by comparing ratios of extinctions from SAGE II and CLAES (e.g., E(sub lambda)/E(sub 1.02) to pre-computed extinction ratios which are based on a range of unimodal lognormal size distributions. The pre-computed ratios are presented as a function of R(sub eff) for a given sigma(sub g); thus the comparisons establish the range of R(sub eff) consistent with the measured spectra for that sigma(sub g). The fact that no solutions are found for certain sigma(sub g) values provides information on the acceptable range of sigma(sub g), which is found to evolve in response to volcanic injections and removal periods. Analogous comparisons using absolute extinction spectra and error bars establish the range of S and V. The second technique is a Parameter Search Technique (PST) which estimates R(sub eff) and sigma(sub g) within a month-latitude-altitude bin by minimizing the chi-squared values obtained by comparing the SAGE II/CLAES extinction spectra and error bars with spectra calculated by varying the lognormal fitting parameters: R(sub eff), sigma(sub g), and the total number of particles N(sub 0). For both techniques, possible biases in retrieved-parameters caused by assuming a unimodal functional form are removed using correction factors computed from representative in situ measurements of bimodal size distributions. Some interesting features revealed by the LUT and PST retrievals include: (1) Increases in S and V (but not R(sub eff)) after the Ruiz and Kelut injections, (2) Increases in S, V, R(sub eff) after Pinatubo, (3) Post-Pinatubo increases in S, V, and R(sub eff) that are more rapid in the tropics than elsewhere, (4) Mid-latitude post-Pinatubo increases in R(sub eff) that lag increases in S and V, (5) S and V returning to pre-Pinatubo values sooner than R(sub eff) does, (6) Sharp increases in sigma(sub g), after Pinatubo and slight increases in sigma(sub g) after Ruiz, Etna, Kelut, Spurr and Rabaul, and (7) Gradual declines in the heights at which R(sub eff), S and V peak after Pinatubo.

Bauman, J. J.↗
NASA NTRS1986

Retrieval of aerosol size distribution moments from multiwavelength particulate extinction data

An iterative method for deriving the particle size distribution from multiwavelength satellite remote sensing data is presented and its use illustrated with an application to SAGE II data. The compression size distribution method (CSD) features interpolation and look-up features for relating the coefficients of a least-squares fit as a function of wavelength to parameters of the compression function that have been obtained by Mie calculations. Results are reported of comparisons between particulate radii predicted for the El Chichon volcano aerosol based on SAGE II data and 14 radii measured with NASA flights through the aerosol with aircraft carrying wire impactors.

Livingston, J. M.↗
NASA NTRS1978

A technique for measuring in situ size distribution of aerosols

A multistage cascade impactor instrument employing piezoelectric crystals for real-time aerosol size distribution measurements is described in this paper. The instrument measures the aerosol mass concentration as a function of particle size in 10 size intervals ranging from 0.05 micrometers to 25 micrometers in diameter. The particles are then analyzed for elemental composition and morphology by means of scanning electron microscopy (SEM). Examples of particle size distributions in rocket motor exhaust plumes measured with the instrument are presented together with the elemental composition and morphology obtained by SEM.

Woods, D. C.↗
NASA NTRS1989

Observations of aerosol optical depth during the First ISLSCP Field Experiment (FIFE)

Solar radiation measurements were made with a multiwavelength airborne tracking sunphotometer during the First International Satellite Land Surface Climatology Project Field Experiment (FIFE). Data from June 6, and October 11, 1987 are analyzed. Atmospheric optical properties were derived from the data, including total optical depth, aerosol optical depth, aerosol size distribution, aerosol phase function, and aerosol single scattering albedo. The aerosol optical depths for June 6 exhibited a spectral dependence that peaked at short wavelengths, whereas those for October 11 decreased monotonically with wavelength and closely followed an Angstrom wavelength dependence. Also, a unimodal aerosol size distribution was found for the June 6 data, while the October 11 data exhibited a power law size distribution. It is suggested that these differences indicate the need for simultaneous sunphotometer measurements and remotely sensed data.

Spanner, Michael A.↗
NASA NTRS1989

SAGE II aerosol data validation based on retrieved aerosol model size distribution from SAGE II aerosol measurements

Consideration is given to aerosol correlative measurements experiments for the Stratospheric Aerosol and Gas Experiment (SAGE) II, conducted between November 1984 and July 1986. The correlative measurements were taken with an impactor/laser probe, a dustsonde, and an airborne 36-cm lidar system. The primary aerosol quantities measured by the ground-based instruments are compared with those calculated from the aerosol size distributions from SAGE II aerosol extinction measurements. Good agreement is found between the two sets of measurements.

Wang, Pi-Huan↗
NASA NTRS1984

Latitudinal and altitudinal variation of size distribution of stratospheric aerosols inferred from SAGE aerosol extinction coefficient measurements at two wavelengths

A method of retrieving aerosol size distribution from the measured extinction of solar radiation at wavelengths of 0.45 microns and 1.0 microns has recently been proposed. This method is utilized to obtain latitudinal and altitudinal variations of size distributions of stratospheric aerosols from the Stratospheric Aerosol and Gas Experiment data for March 1979. Small particles are found in the lower stratosphere of the tropical region, and large particles are found at higher altitudes and latitudes in both hemispheres. Results of this study are consistent with the suggestion that the upper troposphere in tropical regions is a source of condensation nuclei in the stratosphere, and they become mature as they move to higher altitudes and latitude.

Yue, G. K.↗
NASA NTRS1984

Characterization of Surface Reflectance Variation Effects on Remote Sensing

The use of Monte Carlo radiative transfer codes to simulate the effects on remote sensing in visible and infrared wavelengths of variables which affect classification is examined. These variables include detector viewing angle, atmospheric aerosol size distribution, aerosol vertical and horizontal distribution (e.g., finite clouds), the form of the bidirectional ground reflectance function, and horizontal variability of reflectance type and reflectivity (albedo). These simulations are used to characterize the sensitivity of observables (intensity and polarization) to variations in the underlying physical parameters both to improve algorithms for the removal of atmospheric effects and to identify techniques which can improve classification accuracy. It was necessary to revise and validate the simulation codes (CTRANS, ARTRAN, and the Mie scattering code) to improve efficiency and accommodate a new operational environment, and to build the basic software tools for acquisition and off-line manipulation of simulation results. Initial calculations compare cases in which increasing amounts of aerosol are shifted into the stratosphere, maintaining a constant optical depth. In the case of moderate aerosol optical depth, the effect on the spread function is to scale it linearly as would be expected from a single scattering model. Varying the viewing angle appears to provide the same qualitative effect as modifying the vertical optical depth (for Lambertian ground reflectance).

Pearce, W. A.↗
NASA NTRS1990

Optical depth measurements and atmospheric correction of remotely sensed data for FIFE

Data derived from an airborne tracking-sun photometer are used to provide quantitative corrections for atmospheric effects in remotely sensed data. The atmospheric correction involves the validation of radiometric and atmospheric measurements and the application of single scattering approximation which permits the separation of Rayleigh scattering from aerosol scattering. Sun-photometer data are used to generate plots of spectral optical depths, aerosol size distributions, aerosol phase functions, and aerosol single-scattering albedos. The atmospheric correction model and the atmospheric optical properties are incorporated into a program which is applied to two flightlines of data. Atmospheric corrections tested on remotely sensed data permitted the removal of limb brightening, although the results require verification by means of ground measurements.

Wrigley, R. C.↗
NASA NTRS1980

Investigation of multiple scattering effects in aerosols

The results are presented of investigations on the various aspects of multiple scattering effects on visible and infrared laser beams transversing dense fog oil aerosols contained in a chamber (4' x 4' x 9'). The report briefly describes: (1) the experimental details and measurements; (2) analytical representation of the aerosol size distribution data by two analytical models (the regularized power law distribution and the inverse modified gamma distribution); (3) retrieval of aerosol size distributions from multispectral optical depth measurements by two methods (the two and three parameter fast table search methods and the nonlinear least squares method); (4) modeling of the effects of aerosol microphysical (coagulation and evaporation) and dynamical processes (gravitational settling) on the temporal behavior of aerosol size distribution, and hence on the extinction of four laser beams with wavelengths 0.44, 0.6328, 1.15, and 3.39 micrometers; and (5) the exact and approximate formulations for four methods for computing the effects of multiple scattering on the transmittance of laser beams in dense aerosols, all of which are based on the solution of the radiative transfer equation under the small angle approximation.

Deepak, A.↗
NASA NTRS1973

Investigations of atmospheric extinction using direct solar radiation measurements made with a multiple wavelength radiometer.

A multiple wavelength solar radiometer designed for the purpose of measuring atmospheric optical depth at discrete wavelengths through the visible region is described. Experimental techniques, including sample observations, are presented for obtaining atmospheric optical depth from radiometer measurements. These techniques apply for conditions where the optical depth is either temporally variant or invariant during the course of a day. The influence of the aerosol size distribution on optical depth is investigated. Theoretical calculations of the wavelength dependency of the aerosol optical depth contribution are presented for several representative aerosol size distributions. Methods are also presented for estimating the aerosol size distribution and aerosol mass loading from multiwavelength optical depth measurements.

Shaw, G. E.↗
NASA NTRS2002

Evaluation of SAGE II and Balloon-Borne Stratospheric Aerosol Measurements: Evaluation of Aerosol Measurements from SAGE II, HALOE, and Balloonborne Optical Particle Counters

Stratospheric aerosol measurements from the University of Wyoming balloonborne optical particle counters (OPCs), the Stratospheric Aerosol and Gas Experiment (SAGE) II, and the Halogen Occultation Experiment (HALOE) were compared in the period 1982-2000, when measurements were available. The OPCs measure aerosol size distributions, and HALOE multiwavelength (2.45-5.26 micrometers) extinction measurements can be used to retrieve aerosol size distributions. Aerosol extinctions at the SAGE II wavelengths (0.386-1.02 micrometers) were computed from these size distributions and compared to SAGE II measurements. In addition, surface areas derived from all three experiments were compared. While the overall impression from these results is encouraging, the agreement can change with latitude, altitude, time, and parameter. In the broadest sense, these comparisons fall into two categories: high aerosol loading (volcanic periods) and low aerosol loading (background periods and altitudes above 25 km). When the aerosol amount was low, SAGE II and HALOE extinctions were higher than the OPC estimates, while the SAGE II surface areas were lower than HALOE and the OPCS. Under high loading conditions all three instruments mutually agree to within 50%.

Hervig, Mark↗
NASA NTRS2023

Large-Eddy Simulations of Marine Boundary Layer Clouds Associated with Cold-Air Outbreaks during the ACTIVATE Campaign. Part II: Aerosol–Meteorology–Cloud Interaction

Aerosol effects on micro/macrophysical properties of marine stratocumulus clouds over the western North Atlantic Ocean (WNAO) are investigated using in situ measurements and large-eddy simulations (LES) for two cold-air outbreak (CAO) cases (28 February and 1 March 2020) during the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE). The LES is able to reproduce the vertical profiles of liquid water content (LWC), effective radius reff and cloud droplet number concentration Nc from fast cloud droplet probe (FCDP) in situ measurements for both cases. Furthermore, we show that aerosols affect cloud properties (N c , r eff , and LWC) via the prescribed bulk hygroscopicity of aerosols (¯k) and aerosol size distribution characteristics. N c , r eff , and liquid water path (LWP) are positively correlated to ¯κ and aerosol number concentration (N a ) while cloud fractional cover (CFC) is insensitive to ¯κ and aerosol size distributions for the two cases. The realistic changes to aerosol size distribution (number concentration, width, and the geometrical diameter) with the same meteorology state allow us to investigate aerosol effects on cloud properties without meteorological feedback. We also use the LES results to evaluate cloud properties from two reanalysis products, ERA5 and MERRA-2. Compared to LES, the ERA5 is able to capture the time evolution of LWP and total cloud coverage within the study domain during both CAO cases while MERRA-2 underestimates them.

Cloud forcing↗