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Pulsed Airborne Lidar Measurements of Atmospheric CO2 Column Absorption and Line Shapes from 3-13 km Altitudes

We have developed a lidar technique for measuring the tropospheric C02 concentrations as a candidate for NASA's planned ASCENDS mission. Our technique uses two pulsed laser transmitters allowing simultaneous measurement of a C02 absorption line in the 1570 nm band, 02 extinction in the Oxygen A-band and surface height and backscatter. The lidar measures the energy and time of flight of the laser echoes reflected from the atmosphere and surface. The lasers are stepped in wavelength across the C02 line and an 02 line region during the measurement. The receiver uses a telescope and photon counting detectors, and measures the background light and energies of the laser echoes from the surface along with scattering from any aerosols in the path. The gas extinction and column densities for the C02 and 02 gases are estimated from the ratio of the on- and off- line signals via the DIAL technique. Time gating is used to isolate the laser echo signals from the surface, and to reject laser photons scattered in the atmosphere. We have developed an airborne lidar to demonstrate the C02 measurement from the NASA Glenn Lear 25 aircraft. The airborne lidar steps the pulsed laser's wavelength across a selected C02 line with 20 steps per scan. The line scan rate is 450 Hz and laser pulse widths are I usec. The time resolved laser backscatter is collected by a 20 cm telescope, detected by a photomultiplier and is recorded by a photon counting system. We made initial airborne measurements on flights during October and December 2008. Laser backscatter and absorption measurements were made over a variety of land and water surfaces and through thin and broken clouds. Atmospheric C02 column measurements using the 1571.4, 1572.02 and 1572.33 nm C02 lines. Two flights were made above the DOE SGP ARM site at altitudes from 3-8 km. These nights were coordinated with DOE investigators who Hew an in-situ C02 sensor on a Cessna aircraft under the path. The increasing C02 line absorptions with altitudes were evident and comparison with in-situ measurements showed agreements to 6 ppm. This spring we improved the aircraft's nadir window. During July and August 2009 we made 9 additional 2 hour long flights and measured the atmospheric C02 absorption and line shapes using the 1572.33 nm C02 line. Measurements were made at stepped altitudes from 3-13 km over a variety of surface types in Nebraska, Illinois, the SGP ARM site, and near and over the Chesapeake Bay in North Carolina and Virginia. Strong laser signals and clear line shapes were observed at all altitudes, and some measurements were made through thin clouds. The flights over the ARM site were underflown with in-situ measurements made from the DOE Cessna. The Oklahoma and east coast t1ights were coordinated with a LaRC/ITT C02 lidar on the LaRC UC-12 aircraft, a LaRC in~situ C02 sensor, and the Oklahoma flights also included a JPL C02 lidar on a Twin Otter aircraft. Ed Browell and Gary Spiers led the LaRC and JPL teams. More details of the t1ights, measurements and analysis will be described in the presentation.

Abshire, J. B.↗

Analysis of Pulsed Airborne Lidar Measurements of Atmospheric CO2 Column Absorption from 3-13 km Altitudes

We have developed a pulsed lidar technique for measuring the tropospheric CO2 concentrations as a candidate for NASA's ASCENDS space mission [1]. It uses two pulsed laser transmitters allowing simultaneous measurement of a CO2 absorption line in the 1575 nm band, O2 extinction in the Oxygen A-band, surface height and backscatter profile. The lasers are precisely stepped in wavelength across the CO2 line and an O2 line region during the measurement. The direct detection receiver measures the energies of the laser echoes from the surface along with the range profile of scattering in the path. The column densities for the CO2 and O2 gases are estimated from the ratio of the on- and off-line signals via the integrated path differential absorption (IPDA) technique. The time of flight of the laser pulses is used to estimate the height of the scattering surface and to reject laser photons scattered in the atmosphere. We developed an airborne lidar to demonstrate an early version of the CO2 measurement from the NASA Glenn Lear-25 aircraft. The airborne lidar stepped the pulsed laser's wavelength across the selected CO2 line with 20 wavelength steps per scan. The line scan rate is 450 Hz, the laser pulse widths are 1 usec, and laser pulse energy is 24 uJ. The time resolved laser backscatter is collected by a 20 cm telescope, detected by a NIR photomultiplier and is recorded on every other reading by a photon counting system [2]. During August 2009 we made a series of 2.5 hour long flights and measured the atmospheric CO2 absorption and line shapes using the 1572.33 nm CO2 line. Measurements were made at stepped altitudes from 3-13 km over locations in the US, including the SGP ARM site in Oklahoma, central Illinois, north-eastern North Carolina, and over the Chesapeake Bay and the eastern shore of Virginia. Although the received signal energies were weaker than expected for ASCENDS, clear CO2 line shapes were observed at all altitudes, and some measurements were made through thin clouds. The Oklahoma and east coast flights were coordinated with a LaRC/ITT CO2 lidar on the LaRC UC-12 aircraft, and in-situ measurements were made using its CO2 sensor and radiosondes. We have conducted an analysis of the ranging and IPDA lidar measurements from these four flights. Most flights had 5-6 altitude steps with 200-300 seconds of recorded measurements per step. We used a cross-correlation approach to process the laser echo records. This was used to estimate the range to the scattering surface, to define the edges of the laser pulses and to determine echo pulse energy at each wavelength. We used a minimum mean square approach to fit an instrument response function and to solve for the best-fit CO2 absorption line shape. We then calculated the differential optical depth (DOD) of the fitted CO2 line. We computed its statistics at the various altitude steps, and compare them to the DODs calculated from spectroscopy based on HITRAN 2008 and the column conditions calculated from the airborne in-situ readings. The results show the lidar and in-situ measurements have very similar DOD change with altitude and greater than 10 segments per flight where the scatter in the lidar measurements are less than or equal to 1ppm. We also present the results from subsequent CO2 column absorption measurements, which were made with stronger detected signals during three flights on the NASA DC-8 over the southwestern US in during July 2010.

Abshire, James B.↗

Pulsed Airborne Lidar Measurements of Atmospheric CO2 Column Absorption and Line Shapes from 3-13 km Altitudes

We have developed a pulsed lidar technique for measuring the tropospheric CO2 concentrations as a candidate for NASA's planned ASCENDS space mission. Our technique uses two pulsed laser transmitters allowing simultaneous measurement of a CO2 absorption line in the 1570 nm band, O2 extinction in the Oxygen A-band and surface height and backscatter. The lidar measures the energy and time of flight of the laser echoes reflected from the atmosphere and surface. The lasers are rapidly and precisely stepped in wavelength across the CO2 line and an O2 line region during the measurement. The direct detection receiver uses a telescope and photon counting detectors, and measures the background light and energies of the laser echoes from the surface along with scattering from any aerosols in the path. The gas extinction and column densities for the CO2 and O2 gases are estimated from the ratio of the on- and off- line signals via the DIAL technique. Time gating is used to isolate the laser echo signals from the surface, and to reject laser photons scattered in the atmosphere. The time of flight of the laser pulses are also used to estimate the height of the scattering surface and to identify cases of mixed cloud and ground scattering. We have developed an airborne lidar to demonstrate the CO2 measurement from the NASA Glenn Lear-25 aircraft. The airborne lidar steps the pulsed laser's wavelength across the selected CO2 line with 20 steps per scan. The line scan rate is 450 Hz, the laser pulse widths are 1 usec, and laser pulse energy is 24 uJ. The time resolved laser backscatter is collected by a 20 cm telescope, detected by a photomultiplier and is recorded by a photon counting system. We made initial airborne measurements on flights during fall 2008. Laser backscatter and absorption measurements were made over a variety of land and water surfaces and through thin clouds. The atmospheric CO2 column measurements using the 1572.33 nm CO2 lines. Two flights were made above the US Department of Energy's (DOE) SGP ARM site at altitudes from 3-8 km. These flights were coordinated with DOE investigators who flew an in-situ CO2 sensor on a Cessna aircraft under the path. The increasing CO2 line absorptions with altitudes were evident and comparison with in-situ measurements showed agreements to 6 ppm. In spring 2009 we improved the aircraft's nadir window and during July and August we made 9 additional 2 hour long flights and measured the atmospheric CO2 absorption and line shapes using the 1572.33 nm CO2 line. Measurements were made at stepped altitudes from 3-13 km over a variety of surface types in Nebraska, Illinois, the SGP ARM site, and near and over the Chesapeake Bay in North Carolina and eastern Virginia. Strong laser signals and clear CO2 line shapes were observed at all altitudes, and some measurements were made through thin clouds. The flights over the ARM site were underflown with in-situ measurements made from the DOE Cessna. Analysis shows that the average signal levels follow predicted values, the altimetry measurements had an uncertainty of about 4 m, and that the average optical line depths follow the number density calculated from in-situ sensor readings. The Oklahoma and east coast flights were coordinated with a LaRC/ITT CO2 lidar on the LaRC UC-12 aircraft, a LaRC in-situ CO2 sensor, and the Oklahoma flights also included a JPL CO2 lidar on a Twin Otter aircraft. More details of the flights, measurements, analysis and scaling to space will be described in the presentation.

Abshire, James↗

Efficient Extraction Of Building Elevation Attributes For Flood Risk Management Using Airborne LiDAR Data

In this paper, we address the need for extracting two key building elevation attributes—Lowest Adjacent Grade (LAG) and Highest Adjacent Grade (HAG)—which are crucial for effective flood risk management. Conventional methods, involving onsite surveying or the use of optical imagery-derived building footprints combined with Digital Elevation Models (DEMs), often face misalignment and time discrepancy issues due to varied remote sensing sources. We introduce a new, scalable method that exclusively relies on airborne LiDAR data to overcome these challenges. Our approach employs an object-based ground filtering technique, and the results were evaluated using two different DEMs and building footprint sets. The findings demonstrate that our single-source method, utilizing only airborne LiDAR data, significantly improves the accuracy of LAG and HAG calculations compared to traditional methods that use hand-digitized building footprints. The proposed approach offers a solution for comprehensive flood risk management endeavors.

Song, Hunsoo↗

Airborne lidar mapping of vertical ozone distributions in support of the 1990 Clean Air Act Amendments

The 1990 Clean Air Act Amendments mandated attainment of the ozone standard established by the U.S. Environmental Protection Agency. Improved photochemical models validated by experimental data are needed to develop strategies for reducing near surface ozone concentrations downwind of urban and industrial centers. For more than 10 years, lidar has been used on large aircraft to provide unique information on ozone distributions in the atmosphere. However, compact airborne lidar systems are needed for operation on small aircraft of the type typically used on regional air quality investigations to collect data with which to develop and validate air quality models. Data presented in this paper will consist of a comparison between airborne differential absorption lidar (DIAL) and airborne in-situ ozone measurements. Also discussed are future plans to improve the airborne ultraviolet-DIAL for ozone and other gas observations and addition of a Fourier Transform Infrared (FTIR) emission spectrometer to investigate the effects of other gas species on vertical ozone distribution.

Uthe, Edward E.↗

Improving Carbon Estimation of Large Tropical Trees by Linking Airborne Lidar Crown Size to Field Inventory

Quantifying tropical aboveground biomass (agb) is an outstanding challenge that requires knowledge on the 3D structure of forests. Recent studies suggest that the uncertainty in estimating agb of large trees is significantly reduced if tree height and crown size are accounted for in addition to the traditional trunk diameter and wood density. Due to the fact that field inventory techniques are not adapted to characterize the 3D forest structure, crown size metrics (e.g. height and radius) are commonly estimated as a function of trunk diameter using allometric models with limitations in explaining crown variability. Airborne lidar techniques have the potential for characterizing tree height and crown size but are not adapted to estimate trunk diameter, which is a strong predictor of agb. Here, we investigate the synergy of field inventory and airborne lidar techniques to characterize the forest structure by assessing the uncertainty introduced by the field-based allometric models in the estimation of agb at the tree-level. We focus in 1454 large individual trees (trunk diameter > 60 cm) located within the La Selva Biological Station for which we dispose of field observations (trunk diameter and wood density) and lidar derived metrics (tree height and crown radius). We show that the field-based allometric models overestimate tree height and underestimate crown radius. As a result, the allometric approach overestimates the tree-level agb in 0.8 Mg when considering the 1454 individuals and the errors can reach more than 50% of the agb of individual trees. These errors on the large trees agb highly impact on the plot-level results and then propagate to the estimation of carbon stocks at the regional and national-levels.

Clark, David↗

Airborne lidar observations of long-range transport in the free troposphere

Airborne lidar measurements of ozone and aerosols in the lower troposphere show the presence of pollutant layers above the mixed layer. Two case studies are analyzed to identify probable source regions and mechanisms for material injection into the free troposphere above local mixed layers. An elevated haze/oxidant layer observed over South Carolina on Aug. 2, 1980, was found to originate in cumulus convection over Georgia on Aug. 1, 1980. An extensive haze/oxidant layer observed over southeastern Virginia on July 31, 1981, is shown to have been in contact with the New England mixed layer on July 30, 1981. This transported air mass is estimated to contribute approximately 30 percent of the ozone maximum measured at the surface in the Norfolk, VA, area on July 31, 1981. Such elevated 'reservoir' layers are transported over long ranges and are not detected by sensors which are confined to the surface.

Shipley, S. T.↗

Airborne lidar experiments at the Savannah River Plant

The results of remote sensing experiments at the Department of Energy (DOE) Savannah River Nuclear Facility utilizing the NASA Airborne Oceanographic Lidar (AOL) are presented. The flights were conducted in support of the numerous environmental monitoring requirements associated with the operation of the facility and for the purpose of furthering research and development of airborne lidar technology. Areas of application include airborne laser topographic mapping, hydrologic studies using fluorescent tracer dye, timber volume estimation, baseline characterization of wetlands, and aquatic chlorophyll and photopigment measurements. Conclusions relative to the usability of airborne lidar technology for the DOE for each of these remote sensing applications are discussed.

Krabill, William B.↗

Tropopause fold structure determined from airborne lidar and in situ measurements

Airborne differential absorption lidar and in situ data obtained during the April 20, 1984 flight experiment conducted over Nevada and California are analyzed. The O3 and aerosols profiles and in situ measurements reveal a 2.0-km-deep layer (with high O3 concentrations and enhanced aerosol backscattering) and a correlation of 0.8 between O3 and aerosol backscatter (with both values decreasing about 25 percent along the central axis of the fold). It is observed that the cold boundary of the fold has weaker gradients, larger-scale undulations, and more irregularity than the warm boundary. The potential vorticity distribution along the flight path was derived from radiosonde data. A positive correlation between the O3 mixing ratio and the potential vorticity values in the fold is detected; the average ratio between O3 and potential vorticity is 50.2 ppbv/10 to the -5th sq cm deg per g s.

Browell, E. V.↗

Airborne lidar observations in the wintertime Arctic stratosphere - Ozone

Large-scale distributions of ozone (O3) were measured with an airborne lidar system as part of the 1989 Airborne Arctic Stratospheric Expedition. Measurements of O3 distributions were obtained between January 6 and February 15, 1989, on 15 long-range flights into the polar vortex from the Solar Air Station, Norway. The observed O3 distribution was found to clearly indicate the edge of the polar vortex and to be an effective tracer of dynamical processes in the lower stratosphere. On the last two flights of the expedition, large regions with reduced O3 levels were observed by the lidar inside the polar vortex. Ozone had decreased by as much as 17 percent in the center of these areas, and using the in situ measurements made on the ER-2 aircraft, it was concluded that this decline was due to chemical O3 destruction.

Browell, E. V.↗

Airborne lidar observations of Arctic polar stratospheric clouds - Indications of two distinct growth stages

Airborne lidar observations of Arctic polar stratospheric clouds (PSCs) during January 1984 and January 1986 show contrast suggestive of two distinct PSC growth stages delineated by the frost-point temperature. Results obtained at temperatures 2-6 K above the frost point indicate a stage of significant, but limited, particle growth such as proposed in recent models of PSC formation by co-deposition of HNO3 and H2O vapors. Results obtained at a temperature near the frost point indicate the formation of somewhat larger crystalline particles.

Poole, Lamont R↗

Measurement of Atmospheric CO2 Column Concentrations to Cloud Tops With a Pulsed Multi-Wavelength Airborne Lidar

We have measured the column-averaged atmospheric CO2 mixing ratio to a variety of cloud tops by using an airborne pulsed multi-wavelength integrated-path differential absorption (IPDA) lidar. Airborne measurements were made at altitudes up to 13 km during the 2011, 2013 and 2014 NASA Active Sensing of CO2 Emissions over Nights, Days, and Seasons (ASCENDS) science campaigns flown in the United States West and Midwest and were compared to those from an in situ sensor. Analysis of the lidar backscatter profiles shows the average cloud top reflectance was approx. 5% for the CO2 measurement at 1572.335 nm except to cirrus clouds, which had lower reflectance. The energies for 1 micro-s wide laser pulses reflected from cloud tops were sufficient to allow clear identification of CO2 absorption line shape and then to allow retrievals of atmospheric column CO2 from the aircraft to cloud tops more than 90% of the time. Retrievals from the CO2 measurements to cloud tops had minimal bias but larger standard deviations when compared to those made to the ground, depending on cloud top roughness and reflectance. The measurements show this new capability helps resolve CO2 horizontal and vertical gradients in the atmosphere. When used with nearby full-column measurements to ground, the CO2 measurements to cloud tops can be used to estimate the partial-column CO2 concentration below clouds, which should lead to better estimates of surface carbon sources and sinks. This additional capability of the range-resolved CO2 IPDA lidar technique provides a new benefit for studying the carbon cycle in future airborne and space-based CO2 missions.

atmospheric↗

Pulsed Doppler lidar airborne scanner

This report covers the work accomplished during the reporting period on Pulsed Doppler Lidar Airborne Scanner and describes plans for the next reporting period. The objectives during the current phase of the contract are divided into four phases. Phase 1 includes ground testing of the system and analysis of data from the 1981 Severe Storms Test Flights. Phase 2 consists of preflight preparation and planning for the 1983 flight series. The flight test itself will be performed during Phase 3, and Phase 4 consists of post-flight analysis and operation of the system after that flight test. The range profile from five samples taken during Flight 10, around 1700 Z is given. The lowest curve is taken from data collected upwind of Mt. Shasta at about 10,000 feet of altitude, in a clear atmosphere, where no signals were observed. It thus is a good representation of the noise level as a function of range. The next curve was taken downwind of the mountain, and shows evidence of atmospheric returns. There is some question as to whether the data are valid at all ranges, or some ranges are contaminated by the others.

Dimarzio, C. A.↗

High-Rate Data-Capture for an Airborne Lidar System

A high-rate data system was required to capture the data for an airborne lidar system. A data system was developed that achieved up to 22 million (64-bit) events per second sustained data rate (1408 million bits per second), as well as short bursts (less than 4 s) at higher rates. All hardware used for the system was off the shelf, but carefully selected to achieve these rates. The system was used to capture laser fire, single-photon detection, and GPS data for the Slope Imaging Multi-polarization Photo-counting Lidar (SIMPL). However, the system has applications for other laser altimeter systems (waveform-recording), mass spectroscopy, xray radiometry imaging, high-background- rate ranging lidar, and other similar areas where very high-speed data capture is needed. The data capture software was used for the SIMPL instrument that employs a micropulse, single-photon ranging measurement approach and has 16 data channels. The detected single photons are from two sources those reflected from the target and solar background photons. The instrument is non-gated, so background photons are acquired for a range window of 13 km and can comprise many times the number of target photons. The highest background rate occurs when the atmosphere is clear, the Sun is high, and the target is a highly reflective surface such as snow. Under these conditions, the total data rate for the 16 channels combined is expected to be approximately 22 million events per second. For each photon detection event, the data capture software reads the relative time of receipt, with respect to a one-per-second absolute time pulse from a GPS receiver, from an event timer card with 0.1-ns precision, and records that information to a RAID (Redundant Array of Independent Disks) storage device. The relative time of laser pulse firings must also be read and recorded with the same precision. Each of the four event timer cards handles the throughput from four of the channels. For each detection event, a flag is recorded that indicates the source channel. To accommodate the expected maximum count rate and also handle the other extreme of very low rates occurring during nighttime operations, the software requests a set amount of data from each of the event timer cards and buffers the data. The software notes if any of the cards did not return all the data requested and then accommodates that lower rate. The data is buffered to minimize the I/O overhead of writing the data to storage. Care was taken to optimize the reads from the cards, the speed of the I/O bus, and RAID configuration.

Valett, Susan↗

Aerosol Wind Profiler (AWP) Doppler Wind Lidar Airborne Observations During the NOAA Joint Venture 3-D Wind Measurement Demonstration and NASA Active-Passive Profiling Experiment (APEX)

The NASA Langley Research Center (LaRC) has recently completed development of the Aerosol Wind Profiler (AWP) airborne Doppler wind lidar (DWL) instrument. AWP was supported by the NASA Earth Science Technology Office and the Earth Science Division, a project that adapted the Wind-Space Pathfinder (Wind-SP) DWL transceiver onto a structure for flight aboard a variety of NASA research aircraft. AWP demonstrates many technologies required for a space DWL mission, including a coherent-detection, optical heterodyne laser transmitter with high pulse energy (up to ~55 mJ) and repetition rate (200 Hz), electronic control of the beam path allowing for multiple viewing angles (allowing vector wind measurements) with no moving parts, compact highly-stable and tunable reference lasers allowing for high-precision measurement of velocity at long ranges while mitigating the impact of satellite platform velocity, and many others. AWP represents NASA’s only currently operational airborne 3-D wind profiling sensor. NASA LaRC was selected by the NOAA Joint Venture (JV) program to conduct a suborbital 3-D Wind measurement campaign demonstrate how data from a coherent-detection DWL like AWP could serve NOAA’s weather analysis and forecasting needs. The NOAA JV program is designed to work with the private sector, academia and other federal agencies to explore the feasibility and capability of emerging technologies spacecraft and other mission-specific tools to meet NOAA’s mission requirements. AWP was initially demonstrated on the NASA DC-8 within this JV program in October 2023, piggybacking on the NASA EcoDemonstrator mission focused on in-situ sampling of jet aircraft emissions and contrail formation from Everett, Washington. The in-situ sampling resulted in very frequent and rapid aircraft attitude changes which unfortunately degraded AWP data quality. But, during times with level flight and AVAPS dropsonde operations, AWP demonstrated excellent precision (< 2 m/s RMS) with high vertical (< 100 meter) resolution and 2 km spacing between profiles. AWP will be flown again on the NASA LaRC Gulfstream-3 from mid-September to mid-October 2024 out of Hampton, VA to complete the NOAA JV 3-D wind demonstration. Additional AWP flights will occur in early November from southern California during the NASA Active-Passive Profiling Experiment (APEX), focused on underflights of the NASA ER-2 equipped with many atmospheric profiling sensors. This presentation will summarize AWP measurements collected during these two fall 2024 flight campaigns, and how the AWP data compares with AVAPS dropsonde, NOAA weather prediction model, and GOES atmospheric motion vector data.

Kristopher Bedka↗

Airborne lidar observations in the wintertime Arctic stratosphere - Polar stratospheric clouds

Polar stratospheric cloud (PSC) distributions in the wintertime Arctic stratosphere and their optical characteristics were measured with a multiwavelength airborne lidar system as part of the 1989 Airborne Arctic Stratospheric Expedition. PSCs were observed on 10 flights between January 6 and February 2, 1989, into the polar vortex. The PSCs were found in the 14-27 km altitude range in regions where the temperatures were less than 195 K. Two types of aerosols with different optical characteristics (Types 1a and 1b) were observed in PSCs thought to be composed of nitric acid trihydrate. Water ice PSCs (Type 2) were observed to have high scattering ratios (greater than 10) and high aerosol depolarizations (greater than 10 percent) at temperatures less than 190 K.

Browell, E. V.↗

Airborne Lidar Measurements of XCO 2 in Synoptically Active Environment and Associated Comparisons With Numerical Simulations

Frontal boundaries have been shown to cause large changes in CO 2 mole-fractions, but clouds and the complex vertical structure of fronts make these gradients difficult to observe. It remains unclear how the column average CO 2 dry air mole-fraction (XCO 2 ) changes spatially across fronts, and how well airborne lidar observations, data assimilation systems, and numerical models without assimilation capture XCO 2 frontal contrasts (ΔXCO 2 , i.e., warm minus cold sector average of XCO 2 ). We demonstrated the potential of airborne Multifunctional Fiber Laser Lidar (MFLL) measurements in heterogeneous weather conditions (i.e., frontal environment) to investigate the ΔXCO 2 during four seasonal field campaigns of the Atmospheric Carbon and Transport-America (ACT-America) mission. Most frontal cases in summer (winter) reveal higher (lower) XCO 2 in the warm (cold) sector than in the cold (warm) sector. During the transitional seasons (spring and fall), no clear signal in ΔXCO 2 was observed. Intercomparison among the MFLL, assimilated fields from NASA's Global Modeling and Assimilation Office (GMAO), and simulations from the Weather Research and Forecasting-—Chemistry (WRF-Chem) showed that (a) all products had a similar sign of ΔXCO 2 though with different levels of agreement in ΔXCO 2 magnitudes among seasons; (b) ΔXCO 2 in summer decreases with altitude; and (c) significant challenges remain in observing and simulating XCO 2 frontal contrasts. A linear regression analyses between ΔXCO 2 for MFLL versus GMAO, and MFLL versus WRF-Chem for summer-2016 cases yielded a correlation coefficient of 0.95 and 0.88, respectively. The reported ΔXCO 2 variability among four seasons provide guidance to the spatial structures of XCO 2 transport errors in models and satellite measurements of XCO 2 in synoptically-active weather systems.

54 ENVIRONMENTAL SCIENCES↗