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PNNL Measurement Results for the 2018 FlatTop Criticality Nuclear Accident Dosimetry Exercise at the Nevada National Security Site (IER-253)

The Pacific Northwest National Laboratory (PNNL) participated in the FlatTop exercise IER-253 at the National Nuclear Security Site (NNSS) during the week of May 21, 2018. This report summarizes the measurements of the personal nuclear accident dosimeters (PNAD). Additionally, portable survey instrument readings and measurements of the simulated biological samples are included. The FlatTop exercise (IER-253) tested only PNADs and did not include fixed nuclear accident dosimeters (FNAD). Previous PNAD results obtained in 2016 at the Godiva-IV exercise IER-148 were summarized in PNNL Measurement Results for the 2016 Criticality Accident Dosimetry Exercise at the Nevada National Security Site IER-148 (PNNL-26497). The results clearly indicated that the previous dose conversions were a historical legacy of the Hanford Site and corresponded closer to kerma dose (or first collision dose, and not to Hp(10) dose). The technical basis for PNAD dose was based on the Godiva-IV exercise and documented in A New Dose Calculation Methodology for New PNAD and FNAD Designs at PNNL (PNNL-27023). The configuration of the PNAD was described in these two documents. The FlatTop exercise was the first time PNNL tested this new dose calculation methodology. Results were generally favorable with some results conservatively over reported that fell above the performance criteria. The reported gamma dose results fell non-conservatively low because only the default parameters obtained from the Godiva-IV exercise were used, and because the OSL gamma dosimeter has an energy dependency. The results from the simulated biological samples were also favorable, and in several cases conservatively over reported.

61 RADIATION PROTECTION AND DOSIMETRY↗

Update of the Nuclear Criticality Slide Rule Calculations: Plutonium systems – Delayed Fission Gamma

IRSN (France), LLNL (USA) and ORNL (USA) began a long-term collaboration effort in 2015 to update the nuclear criticality Slide Rule for the emergency response to a nuclear criticality accident. The Slide Rule permits the estimation of neutron and gamma dose rates and integrated doses based upon estimated fission yields, as a function of distance from the fission source, and time after criticality accidents for different critical systems. This paper presents results from the fourth phase of the current update of the Slide Rule project, in which delayed fission-product gamma (DFG) dose rates of unreflected plutonium critical systems were compared by several modern 3D radiation transport codes (MCNP, COG, SCALE), using updated flux-to-dose conversion factors. Dose rates are calculated for fissile material at five moderation ratios (H/Pu), at 1 m above the ground as a function of distance (between 30 cm and 1,200 m) from the external surface of the source to the center of the detector, and for periods between 1 s and 1,000 min after the critical instantaneous event. Further efforts have been devoted to the determination of the delayed gamma source, by comparing the time-dependent energy spectra obtained from several methods. Overall, DFG dose rates calculated by each participant led to consistent results. Extra effort is under way to identify the cause of the remaining differences, by comparing precisely the gamma source, and particularly nuclides inventories.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Experiment Design and Preparation for a Shielding Benchmark Utilizing Godiva-IV

An experiment is currently being designed to provide a high-quality shielding benchmark for Criticality Accident Alarm System (CAAS) modeling. Previous benchmarks have suffered from uncertainty primarily due to two factors. The first factor is radiation that is not directly coming from the source, also known as room return. Room return is notoriously difficult to account for in experimental data and to model in benchmarks. The second factor is uncertainty associated with the source term itself. In order to reduce these two sources of uncertainty, this experiment will utilize a room return shield [1] that will reduce the effect of room return and previous work performed to ensure the reproducibility of the source term. The experiment will use the Godiva IV [2] assembly located at the National Criticality Experiments Research Center (NCERC) to provide a neutron source representative of a criticality accident. Previous experiments [3]-[4] have shown that Godiva IV is capable of producing both bursts and steady-state emissions of equal magnitude which will allow for reduced uncertainty in the source term. The room return shield will house and isolate the shielding samples, neutron activation foils, and other detectors. Data collected will provide a comparison of the neutron and gamma dose for shielded and unshielded configurations. This data will be used to validate shielding data used for modeling criticality accident alarm systems. Shielding samples included in this benchmark are C, Fe, NaCl, Pb, high density polyethylene, and SiO 2 . This paper details the design of the room return shield, the experimental plan, challenges, and mitigation strategies.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Criticality Safety Fundamentals [Slides]

Objectives of this presentation are: 1. Explain the difference between radiation safety vs. criticality safety, 2. Define criticality, 3. Explain the three types of chain reactions, 4. Define two terms scientists use to characterize criticality, 5. Explain what occurs during a criticality accident, 6. Identify prevention measures for avoiding a criticality accident, and 7. Identify the parameters that effect criticality of a system.

61 RADIATION PROTECTION AND DOSIMETRY↗

Conduct of Operations and Nuclear Criticality Safety Standards

Since the beginning of the nuclear age in 1943, there have been 22 criticality accidents in process facilities worldwide in which fissionable materials were processed by hand for various purposes. Of these 22 process criticality accidents, 16 involved faulty or flawed conduct of operations. Most of these process accidents (17 of 22) occurred before 1970, mostly due to the implementation of formal conduct of operations—such as the use of operating procedures and training—and the use of consensus standards for nuclear criticality safety (NCS). Obviously, the nuclear facilities applied lessons learned from their accident history, and the rate of criticality accidents was significantly reduced as a result. Over the years, it has been emphasized in NCS training courses and other venues in the United States that the consensus standards, such as ASA N6.1-1964, were the key contributors to this reduction in accidents. The formality of operations required to implement and apply the standards at a facility is also a crucial prerequisite that must be sufficiently robust to ensure NCS. This prerequisite is crucial to success fully implement the NCS consensus and other safety standards at a site.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Domestic and International Standards for Nuclear Criticality Safety – Overview and Status

The domestic and international consensus standards for nuclear criticality safety (NCS) have provided guidance for staff performing hands-on work in operations with fissionable materials. These consensus standards have contributed directly to the significant reduction in the rate of criticality accidents in process facilities since the 1940s. The last known criticality accident inside the United States was in 1978 (nearly 43 years ago) at the Idaho Chemical Processing Plant, and outside the United States, an accident occurred at Tokai-mura, Japan, in 1999 (23 years ago). The domestic consensus standards for NCS include the American Nuclear Society (ANS) standards. The ANS Standards Board, the NCS Consensus Committee, and the ANS-8 Subcommittee oversee the development and maintenance of these standards. There are currently eighteen standards in the ANS-8 series. Currently, there are six ANS-8 standards in revision mode and eleven in a maintenance mode with one new standard under development. The international consensus standards for NCS calculations, procedures, and practices are maintained and developed within the International Organization for Standardization (ISO), Technical Committee 85 on Nuclear Energy, Subcommittee 5 on Nuclear Fuel Technology, and Working Group 8, “Nuclear Criticality Safety.” Eleven standards are currently available, three standards are in revision mode, and two standards are development. This paper provides the NCS community with an overview and status report of domestic and international NCS consensus standards to stimulate interest and to support their continued development.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Domestic and International Standards for Nuclear Criticality Safety - Overview & Status [Abstract]

The domestic and international consensus standards for nuclear criticality safety (NCS) have provided guidance for staff performing hands-on work in operations with fissionable materials. These consensus standards have contributed directly to the significant reduction in the rate of criticality accidents in process facilities since the 1940s. The last known criticality accident inside the United States was in 1978 (nearly 43 years ago) at the Idaho Chemical Processing Plant, and outside the United States, an accident occurred at Tokai-mura, Japan, in 1999 (22 years ago). The domestic consensus standards for NCS include the American Nuclear Society (ANS) standards. The ANS Standards Board, the NCS Consensus Committee, and the ANS-8 Subcommittee oversee the development and maintenance of these standards. There are currently eighteen standards in the ANS-8 series. Currently, there are six ANS-8 standards in re- vision mode and eleven in a maintenance mode with one new standard under development. The international consensus standards for NCS calculations, procedures, and practices are maintained and developed within the International Organization for Standardization, Technical Committee 85 on Nuclear Energy, Subcommittee 5 on Nuclear Fuel Technology, and Working Group 8, “Nuclear Criticality Safety.” Eleven standards are currently available, three standards are in revision mode, and two standards are development. This paper provides the NCS community with an overview and status report of domestic and international NCS consensus standards to stimulate interest and to support their continued development.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

Godiva Experiments for the Nuclear Criticality Safety Program (NCSP)

Godiva IV is a fast burst critical assembly constructed of approximately 65 kg of highly enriched uranium (HEU) fuel alloyed with 1.5 percent molybdenum for strength. Godiva is one of the last such critical assemblies in the United States, and can be used for studies of super-prompt critical behavior as well as irradiations and demonstrations. A demonstration of a Godiva burst is usually performed as a highlight of the hands-on portion of the Criticality Safety Training Classes taught at the National Criticality Experiment Research Center (NCERC). The Godiva burst is used to demonstrate the concept of super-prompt critical and the time-scale of a criticality accident. In addition, several NCSP projects have been conducted on Godiva IV over the past two years. One experiment focused on collecting data to support multiphysics simulations using Photo-Doppler Velocimetry (PDV) to measure surface movement and gamma detectors to measure the burst output as the burst develops from background to peak over ten orders of magnitude. Another experiment was performed to demonstrate the functionality of the Criticality Accident Alarm System (CAAS) system developed for installation in the Y-12 Uranium Processing Facility (UPF). The system must not only respond to a criticality event and alarm, but must also be shown to operate in a high dose environment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Criticality Safety at Los Alamos National Laboratory [Slides]

The agenda for the presentation is as follows: Critical Systems (Daghlian Accident, Criticality Safety); Nuclear Criticality Safety at Los Alamos National Laboratory (A day in the life); Los Alamos National Laboratory (History, Today, Mission); and, Los Alamos and Surrounding Areas.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A Review of the Lawrence Livermore Nuclear Accident Dosimeter 1980s-present

A Nuclear Accident Dosimetry program is a federal requirement for all facilities that have the potential to have a criticality accident. Personnel Nuclear Accident Dosimeter (PNAD) theory and analytical procedures are driven by various scientific needs and interacting regulations. A brief history of the status of USA Department of Energy (DOE) nuclear accident dosimetry regulations, recommendations, and performance testing criteria are given. Then, the history of the Lawrence Livermore National Laboratory (LLNL) PNAD is explored, including changes in the physical dosimeter and adjustments of the analysis method through the last four decades. Finally, the performance of LLNL’s PNAD at criticality accident intercomparison training exercises since 2009 is explored. In general, reported neutron doses have been within or close to DOE-STD-1098 performance criteria while reported gamma doses have been outside of DOE-STD-1098 performance criteria. Reported total absorbed doses have varied in meeting ANSI/HPS N13.3 and ANSI/HPS N13.3 (R2019) performance criteria. Dosimetry staff retirement and turnover have left historical knowledge gaps, yet provided opportunities within the NAD program at LLNL. This review paper serves as an overview of the history and status of the NAD program. Brief technical, procedural and programmatic recommendations to improve LLNL’s NAD program are given. Technical recommendations include investigating orientation factors through modeling or empirical experimentation, investigating gamma dosimetry methods for high-dose scenarios, and exploring other dosimetric methods for simpler, quicker NAD analysis. Procedural recommendations include better documentation of conversion factor (activity-to-fluence and fluence-to-dose) derivations and spectrum uses, and updated analysis spreadsheets or simple Graphic User Interfaces for dose calculations. In conclusion, programmatic recommendations include formalized training for NAD analysts, and having multiple SMEs trained on the NAD program.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Godiva-IV Dosimetry Exercise 2022 (IER-538 CED4A Report)

This report presents the final results of IER 538, The International Nuclear Accident Dosimeter (NAD) Intercomparison Exercise with Godiva-IV. The purpose of the exercise, held in August of 2022, was to test participants’ NADs and dosimetry personnel to the dose estimation requirements established by ANSI/HPS-N13.3 Dosimetry for Criticality Accidents and DOE-STD-1098-2017, Radiological Control. Two prompt critical bursts of the Godiva critical assembly were used to simulate criticality accidents, and NADs from participating laboratories were placed at known locations around Godiva, mounted on either BOttle Manikin ABsorptions (BOMABs) phantoms (to simulate doses received by people) or plates (to simulate doses in free air). Similar exercises have been held in 2016 and 2018 using National Criticality Experiments Research Center’s (NCERC’s) Flattop and Godiva assemblies.

61 RADIATION PROTECTION AND DOSIMETRY↗

Modeling Approach to Critical in the Upcoming CERBERUS Experiment

The planned Critical Experiment Reflected By coppEr to betteR Understand Scattering (CERBERUS) seeks to maximize sensitivity to elastic neutron scattering in the intermediate energy region (0.625 eV to 100 keV). It will be performed near the end of FY 2023 at the National Criticality Experiments Research Center (NCERC). Very few International Criticality Safety Benchmark Evaluation Project (ICSBEP) benchmarks are sensitive to copper in this region. Creating a benchmark sensitive in this area will make the Zeus benchmark series, an intermediate benchmark evaluation that uses a copper reflector, more useful for code and nuclear data validation. Approaching criticality in a safe manner is of utmost importance to avoid a criticality accident, which would present a safety concern and could cause damage to equipment. The two rules that are followed closely to ensure that a criticality accident does not occur are the 3/4 rule and the 1/2 rule. The 3/4 rule states that no more than 3/4 of a critical mass can be assembled by hand, and the 1/2 rule states that no more than 1/2 of the material expected to reach criticality, or 1/2 the distance needed to reach criticality, can be added before another measurement of the count rate has been taken. This work will discuss the approach to criticality as modeled in MCNP6® 1 particle transport code with the ENDF/B- VIII.0 cross-section library and the .00c data library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Human Factors and Nuclear Criticality Safety Accidents [Slides]

The agenda for the presentation is as follows: Human Factors; Accident Review (Tokai Mura, Siberian Chemical Combine); Procedures; Accident Review (Los Alamos Waste Recovery); Environmental Distractions; Accident Review (Idaho Fuel Reprocessing); and, Equipment Reliability.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TA-18-1 Slotin Building Restoration – Summary of Work to be Performed

The National Historic Preservation Act (NHPA) requires LANL to identify, evaluate, record, and protect eligible historic properties like TA-18-1 Slotin Building. The Environmental Protection and Compliance-Environmental Stewardship (EPC-ES) Cultural Resources program consults with the New Mexico State Historic Preservation Office (SHPO) on undertakings that may affect these properties. TA-18-1 Slotin Building is an exceptionally significant Manhattan Project Property that has been determined eligible for the National Register of Historic Places and is included within the boundary of the Manhattan Project National Historical Park. The building was constructed in 1946 and served as laboratory space for criticality testing. It is the location of the May 1946 criticality accident that resulted in the death of Louis Slotin. As a result of the accident, new procedures and designs for criticality experiments were implemented to prevent further accidents.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

Development of Shielding Benchmarks Using the Godiva IV Assembly

The Nuclear Criticality Safety Program (NCSP) is developing a shielding benchmark using the Godiva IV assembly as a source. Its present status is reviewed herein. Even eight decades into the nuclear era, substantial work remains to develop a database of shielding benchmarks to support future nuclear development. A nuclear simulation is only as good as its supporting data, inputs, and validation basis. Uncertainty in these areas is addressed using conservatism, which adds margin and, occasionally, cost. In many shielding situations, high accuracy is not necessary because additional material is not particularly expensive. After all, 1–2 cm of lead often reduces the gamma ray dose substantially. However, in certain areas, conservatism can add unnecessary cost. These areas include mobile shielding applications such as casks, ships, microreactors, and spacecraft, where weight and, thus, margin is expensive. Although these characteristics are side benefits for NCSP shielding benchmark development, the main driver is enabling more reliable placement of criticality accident alarm systems (CAASs) in nuclear material facilities, such as those dedicated to the production of advanced reactor fuels. CAAS placement relies on more than accurate data and code validation. It also relies on sufficiently accurate materials specifications, geometry specifications, and a well-defined, alarm-producing baseline accident. All these things require tacit knowledge and understanding of the problem being evaluated. Benchmarks can help ensure this understanding.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

NDCS Group Meeting Work overview: NCSP Task ORNL IP&D-5 [Slides]

The presentation discusses the primary goal of the NCSP Task IP&D-5 which is to use available data from HPRR operation to create a benchmark report for inclusion in the ICSBEP, as a Criticality Accident Alarm System (CAAS) shielding benchmark. The presentation elaborates on the HPRR operation and how it relates to the KENO VI model, sulfur pellets measurements, and calculation methodology between KENO and MAVRIC FW-CADIS. The presentation concludes by stating that some work is still needed to evaluate uncertainties and to explain the discrepancy computation/experiment.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗