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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Novel Hybrid Current Limiter for Grid-Forming Inverter Control During Unbalanced Faults

Grid-forming (GFM) inverter controls have illustrated many desirable features to enable the bulk integration of renewable resources into the future power grid; however, the performance of GFM inverters during unbalanced faults remains underexplored. This paper proposes a novel current-limiting method for GFM inverters to handle unbalanced fault conditions while providing voltage support to the main grid. The proposed current limiter combines concepts of dynamic virtual-impedance and current-reference saturation limiting, all built in the stationary reference frame, to achieve improved current-limiting performance under unbalanced load/fault conditions. System-wide full-order transient simulations with multiple GFM inverters demonstrate the potential of the method and benchmark the performance against state-of-the-art current limiters. Simulation results portray improved voltage balancing performance of the proposed method compared to both current-reference saturation and virtual-impedance limiting.

controller anti windup↗
DOE OSTI2023

Novel Hybrid Current Limiter for Grid-Forming Inverter Control During Unbalanced Faults: Preprint

Grid-forming (GFM) inverter controls have illustrated many desirable features to enable bulk integration of renewable sources into the future power grid. However, the performance of GFM inverters during unbalanced faults remains under-explored. In this paper, a novel current-limiting method is proposed for GFM inverters to handle unbalanced fault conditions while providing voltage support to the main grid. The proposed current limiter combines concepts of dynamic virtual-impedance and current-reference saturation limiting, all built-up in the stationary reference frame to achieve improved current-limiting performance under unbalanced load/fault conditions. System-wide full-order transient simulations with multiple GFM inverters demonstrate the potential of the method and benchmark the performance against state-of-the-art current limiters. Simulation results portray improved voltage balancing performance of the proposed method compared to both current-reference saturation and virtual-impedance limiting.

controller anti windup↗
DOE OSTI2022

Comparing measurement of limiting current in block copolymer electrolytes as a function of salt concentration with theoretical predictions

Optimizing electrolyte performance is crucial for the widespread adoption of electrochemical energy storage. We demonstrate that limiting current provides a robust criterion for determining the optimum electrolyte. Experiments were conducted on rigid block copolymer electrolytes comprising mixtures of polystyrene-block-poly(ethylene oxide) copolymer (SEO) and lithium bis(trifluoromethanesulfonyl) imide salt (LiTFSI) over a salt concentration range from r av = 0.04 to r av = 0.20 (r av is the molar ratio of lithium ions to ethylene oxide). Here we show that the maximum limiting current density is 4.3 mA cm –2 at r av = 0.12. The dependence of limiting current on salt concentration is in good agreement with predictions from Newman's concentrated solution theory with no adjustable parameters.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Moderate pH changes alter the fluxes, selectivities and limiting currents in ion transport through polyelectrolyte multilayers deposited on membranes

Layer-by-layer (LBL) polyelectrolyte coatings on membranes are attractive for their high selectivities between monovalent and divalent ions. However, deposition of poly(4-styrenesulfonate) (PSS)/protonated poly(allylamine) (PAH) films on ion-exchange membranes leads to low ion fluxes that restrict productivity or current efficiency. This study shows that increasing the solution pH from 6.5 to 8.3 enhances cation fluxes and limiting currents through (PAH/PSS) 5 PAH-coated cation-exchange membranes while still achieving order of magnitude selectivity increases compared to bare membranes. In Donnan dialysis through (PAH/PSS) 5 PAH-coated Nafion, at pH 8.3 the K + /Mg 2+ selectivity is 100, and the K + flux is 22 times that at pH 6.5. Moreover, at the higher pH the electrodialysis limiting current through these membranes increases ~5-fold. This enables electrodialysis separation of K + and Mg 2+ with a current efficiency around 0.75, a selectivity of 18, and 50% K + recovery from the source phase. Transmembrane potential measurements and increases in Cl - /SO 4 2- selectivities (from 9.5 at pH 6.5 to ~70 at pH 8.3) for porous alumina membranes coated with (PSS/PAH) 5 PSS films suggest that the coating becomes cation-permselective at higher pH. Increased cation transference numbers in polyelectrolyte coatings likely lead to the enhanced limiting currents for coated Nafion at higher pH. Lastly, (PAH/PSS) 5 PAH-coated Nafion shows a Li + /Mg 2+ Donnan dialysis selectivity >700 at neutral pH and a selectivity of 10 at pH 8.3. However, the Li + flux is 6 times greater at pH 8.3, which might make operation at the higher pH desirable.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Simulation for the fault current limiting operation of REBCO CORC superconducting cables with different core materials

With high power density and low loss, CORC superconducting cables composed of RE- Ba 2 Cu 3 O 7–δ (REBCO) coated conductors are of great interest for power transmission applications. They can also effectively be designed to serve as fault current limiters, thanks to their sharp superconducting-to-normal transition. Coupled electromagnetic-thermal finite element (FE) simulations implemented in COMSOL Multiphysics were developed and validated against the published results for the fault current limiting performance of two CORC cables of REBCO coasted conductors wound on either copper or stainless steel cores. For improved accuracy, temperature dependencies of electrical and thermal properties of all component materials were considered in the simulations. The simulations were performed in the cross-sections of the cables for every individual layer of each REBCO tape to deliver comprehensive understanding of evolution of the current distribution and temperature rise in those layers. Furthermore, the studies can suggest approaches to optimize cable design for fault current limiting (FCL) applications by assessing the role of individual components. In the paper, possible computational errors, challenges and improvements are also discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

Universal Relationship between Limiting Current and Electrochemical Transport Properties in Malonate-Based Polymer Electrolytes

There is considerable interest in developing high-performance electrolytes for rechargeable lithium batteries. For practical applications, the electrolyte must support large dc currents. However, the parameters most often reported in the literature, conductivity, κ, and current fraction, ρ + , reflect ion transport in the limit of infinitesimal currents. In this limit, the efficacy of an electrolyte is given by the product κρ + . The limiting current density, i lim , is the maximum current density that can be applied across an electrolyte; the cell voltage diverges if the applied current density exceeds ilim. This parameter reflects ion transport in the limit of large dc currents and is therefore of practical interest. It would therefore be convenient if i lim could be predicted from measurements of κρ + . In order to explore this possibility, we studied six malonate-based polymers and PEO at a fixed salt concentration (r = 0.08) and temperature (90°C) using symmetric cells with planar electrodes. Unfortunately, there is no correlation between ilim and κρ + . When the applied current density, i, is less than ilim, the cell voltage approaches a stable plateau, ϕ plateau . Here, we found a linear dependence between i and thickness-normalized plateau potential, ϕ plateau L –1 , irrespective of the magnitude of the applied current. In all seven polymer electrolytes, we found a linear correlation between ilim and the slopes of these lines, σ. In other words, measurements of σ can be used to predict the limiting current.

Jana, Rounak [Lawrence Berkeley National Laborator↗
DOE OSTI2025

A Methodology for the Analysis of Water Oxidation Electrocatalysts in the Absence of Limiting Current that Avoids the Pitfalls of Existing Methods

Water oxidation is an important reaction studied as a way to generate electrons from water, to promote water splitting and the formation of green hydrogen. When using electrodes to drive homogeneous water oxidation catalysis, cyclic voltammograms are analyzed to provide catalytic rate constants. There are two main methods, foot-of-the-wave analysis (FOWA) and limiting current analysis. FOWA relies on approximations inherent to analyzing water oxidation catalysis, such as determining the formal potential of the catalytic intermediate, E 0 cat . Limiting current methods are the optimal way to analyze catalyst performance but rely on observable limiting current, which is virtually never seen in water oxidation. To avoid those issues, a method is proposed for analyzing nonideal cyclic voltammetry waveshapes in water oxidation: by analyzing rate data across a large range of potentials, an optimal potential, E 0 cat , can be obtained, where catalytic current, i cat , is nearly independent of scan rate and has a linear dependency on buffer concentration. Here, the method is applied to four homogeneous water oxidation catalysts with prior extensive electrochemical elucidation, all of which lack an ideal, purely kinetic waveshape in cyclic voltammetry. Application of the method avoids the biases of the other methods cited for the kinetic analyses of water oxidation catalysts.

14 SOLAR ENERGY↗
DOE OSTI2024

Adaptive Fault Current-Limiting Control of MMC for Protection of Multiterminal HVDC Systems: Preprint

For the development of multi-terminal high voltage DC (MTDC) transmission, it is critical to design the protection system that can selectively isolate the faulty area from the healthy part of the dc grid using DC circuit breakers (DCCBs) while ensuring continuous operation of converter stations in the healthy part. However, because of the lack of fault current blocking capability in half-bridge (HB) modular multilevel converters (MMCs), when a dc fault occurs, the rising fault currents can quickly reach the blocking threshold within a few milliseconds and disrupt the operation of MMCs in the healthy part. Large DC reactors are often considered in series with DCCBs to reduce the rate of rise of fault currents and prevent blocking of MMCs in the healthy part of the grid. However, large DC reactors can prohibitively increase the cost of the system, particularly when they are considered in an offshore environment, for instance in offshore wind projects. Large dc reactors can also introduce stability issues and create post-fault oscillations. This paper presents an adaptive fault current limiting control method for MMCs to avoid their blocking and enable continuous operation of MTDC systems. It contains two parts: The first part is based on circulating current feedforward control that emulates virtual reactors in each arm of an MMC, which is immediately activated when the fault current starts to increase, to reduce the rate of rise of the fault current; the second part is triggered when the fault current exceeds a preset threshold by temporarily bypassing the SMs, serving as a complement to the fault current limiting effect of the first part. Both parts do not require fault detection signal and they are activated automatically during faults. Simulation case studies of a four-terminal bipolar MMC-HVDC system are presented to demonstrate the effectiveness of the proposed control methods.

active fault current limiting↗
DOE OSTI2025

Transient Stability-Enhancing Method for Grid-Forming Inverters Under Current Limiting

The primary controller of a grid-forming (GFM) inverter governs the internal reference voltage and angle, which enables the inverter to naturally synchronize and share power with the connected grid; however, during disturbances on the grid caused by, e.g., line faults, overloading, or frequency and phase shifts, a GFM inverter can be pushed into a current-limited operation to protect the device against thermal damage. This can lead to a windup of the internal reference frequency generated by the primary controller and cause a total loss of synchronism with the grid. Here, to make the primary controller of GFM inverters more robust against transient instability, this paper proposes a method that manipulates the reference signals governed by the primary controller by introducing the concept of fictitious power. The fictitious power counteracts the integrator windup in the primary controller, which enables the current-limited inverter to conceive a stable operating point. This method is benchmarked against five state-of-the-art GFM inverter stabilization methods to evaluate its stability-enhancing performance. Full-order electromagnetic-transient simulations and experimental results of a hardware inverter test setup validate the benefits of the method to improve the transient stability of GFM inverters in the face of grid disturbances.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2024

Adaptive Fault Current-Limiting Control of MMC for Protection of Multiterminal HVDC Systems

A crucial requirement of the protection system for multi-terminal high-voltage DC (MTDC) transmission is that it is capable of selectively isolating the faulty area from the healthy part of the network using DC circuit breakers (DCCBs), while ensuring continuous operation of converter stations in the healthy part of the network. But in the half-bridge modular multilevel converters (HB-MMCs) based MTDC system, since HB-MMCs do not have fault current absorption capability, when a DC fault occurs, the rising fault currents can quickly reach the blocking threshold within a few milliseconds and disrupt the operation of the MMCs in the healthy part. To facilitate fault-ride-through capability of MTDC system, large DC reactors are often considered in series with DCCBs to reduce the rate of rise of the fault current and prevent blocking the MMCs in the healthy part of the DC networks; however, large DC reactors prohibitively increase the cost of the system, introduce stability issues and can create post-fault oscillations. This paper presents an adaptive fault current-limiting control method for MMCs to avoid their blocking and enable the continuous operation of the healthy part of MTDC systems. The method contains two parts: The first part is based on circulating current feedforward control, which emulates virtual reactors in each arm of an MMC, and is immediately activated when the fault current starts to increase to reduce the rate of rise of the fault current. The second part temporarily bypasses all the submodules when the fault current exceeds a preset threshold, complementing the fault current-limiting effect of the first part. Neither part requires fault detection signals, and they are automatically activated during faults. Simulation case studies of a four-terminal bipolar MMC-based high-voltage DC system are presented to demonstrate the effectiveness of the proposed control methods.

active fault current limiting↗
DOE OSTI2023

Active Fault Current Limiting Control for Half-Bridge MMC in HVDC Systems

DC faults of MMC can result in a significantly large fault current due to the discharge of submodule capacitors. The fault current not only risks damaging the MMC but also demands a considerable breaking capacity from the dc circuit breaker (DCCBs). This paper introduces two novel active fault current limiting methods (AFCLs), namely virtual impedance-based and energy control-based AFCL. The first method utilizes circulating current feedforward, which introduces a virtual arm impedance to suppress the rate of rise of the fault current. Meanwhile, the second method relies on the control of the internally stored energy of the MMC to automatically minimize the number of submodules that discharge during a dc-side fault. Therefore, both the dc-side current and the MMC arm current can be effectively suppressed after the occurrence of the fault. The proposed methods do not require fault detection and their response is proportional to the rate of rise in the fault current. Simulation case studies are presented to demonstrate the proposed methods.

active current limiting control↗
DOE OSTI2024

Improved Tensor Current Limit from 8 B 𝛽 Decay Including New Recoil-Order Calculations

A precision measurement of the 𝛽 + decay of 8 B was performed using the Beta-decay Paul Trap to determine the 𝛽−𝜈 angular correlation coefficient 𝑎 𝛽⁢𝜈 . The experimental results were combined with new ab initio symmetry-adapted no-core shell-model calculations to yield the second-most precise measurement from Gamow-Teller decays, 𝑎 𝛽⁢𝜈 = −0.3345 ± 0.001⁢9 stat ± 0.002⁢1 syst . This value agrees with the standard model value of −1/3 and improves uncertainties in 8 B by nearly a factor of 2. By combining results from 8 B and 8 Li , a tight limit on tensor current coupling to right-handed neutrinos was obtained. A recent global evaluation of all other precision 𝛽 decay studies suggested a nonzero value for right-handed neutrino coupling in contradiction with the standard model at just above 3⁢𝜎. Finally, the present results are of comparable sensitivity and do not support this finding.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Calculating the space-charge-limited current density for nonplanar geometries by simulating the charge-free electric field

Calculating the space-charge-limited-current density (SCLCD) for a complicated diode geometry often requires computationally expensive particle-in-cell (PIC) codes. Here, this paper addresses this issue by using the charge-free electric field $E_0$ calculated using COMSOL Multiphysics to determine local and global SCLCD. The SCLCD obtained by using the surface average of $|E_0|^2$ on the cathode recovers theoretical results for one-dimensional (1D) planar, cylindrical, and tip-to-tip geometries in appropriate limits. We next compared tip-to-tip calculations with the SCLCD obtained using the PIC code Empire. The SCLCD calculated using COMSOL agreed well with Empire for flatter 1D tip-to-tip geometries and diverged with increasing sharpness. Physically, Empire predicts lower SCLCD than COMSOL because the electrons spread due to concentrated space-charge at the tip, whereas theory assumes that the electrons follow the charge-free electric field lines. We further assess the behavior of the SCLCD for tips protruding from the centers of flat, circular plates of various areas. Larger plate areas with constant tip size recover the 1D planar SCLCD globally and 1D tip-to-tip SCLCD locally, while reducing the difference between Empire and COMSOL calculations since larger plates capture more of the emitted electrons, reducing SCLCD suppression due to beam spreading. These results show that charge-free electric field simulations can be used to determine the SCLCD without needing to simulate particle dynamics in PIC.

Wright, Jack K. [Purdue Univ., West Lafayette, IN ↗
DOE OSTI2025

Simulations of the fault current limiting operation of a long-length REBCO CORC ® superconducting cable cooled by helium gas

Conductor-on-round-core (CORC®) cables composed of rare-earth-barium-copper-oxide high-temperature superconducting (HTS) tapes are of great interest for power transmission applications due to their many advantages such as high power density, light weight, and low loss. Closed circulation loops of cryogenic helium gas can be used to cool HTS cables down to low temperatures to significantly improve their current-carrying capacity. Coupled circuit-electromagnetic-thermal finite element simulations implemented in the COMSOL Multiphysics package were developed, validated, and then used for simulating the fault current limiting (FCL) performance and the cooling processes of an 8-layer CORC® cable cooled with a flow of cryogenic helium gas. In the simulations, the temperature dependence of the electrical and thermal properties of all component materials is implemented for improved accuracy. To overcome computational challenges caused by the considerable difference in geometrical scales (i.e. few-µm-thick HTS layers versus 10 m-long HTS cable), the model is divided into two separate simulations. The first simulation is performed on the transverse cross-section of the cable to calculate the electric field, heating power and temperature rise in each component of a CORC® cable during FCL operation. The heating power calculated in the first simulation is transferred to the second model to simulate the cooling of a 10 m-long cable after the fault is cleared. The effect of the helium gas flow rate on the cooling process is also investigated to develop strategic approaches for optimizing cooling systems for HTS cables with FCL capability. The simulations indicated that a 40 ms fault with a voltage drop of 20 V m −1 along the cable can result in a temperature increase from 60 K to about 165 K inside the cable, and it takes about 500 s to cool the cable back to nearly 60 K with a flow of cold helium gas at a rate of 5 g s −1 .

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2020

A methodology to compute the critical current limit in Nb3Sn magnets

Numerous experiments have shown that the loads applied to Nb3Sn strands and cables can reduce their critical current. Experiments, performed on uniaxially loaded strands, allowed to define clear laws to describe the evolution of the critical surface as a function of the applied current, field, temperature and strain. It is, however, still unclear how these laws can be applied to superconducting magnets. The present paper proposes a methodology to estimate the critical current and temperature margin reduction on superconducting magnets due to stress on the superconducting material. The methodology is tested on the MQXF magnets, a quadrupole developed for the High Luminosity LHC project, and successfully validated by comparing computed strain with data from strain gauge measurements. Overall, results suggested that, because of the stresses arising in winding during assembly, cool-down and powering, the current limit of the magnet is lower than the expected short sample limit, and that the most critical region does not coincide with the peak field location.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Elucidating the impact of the ionomer equivalent weight on a platinum group metal-free PEMFC cathode via oxygen limiting current

Leveraging the interactions between ionomer and catalyst can increase the performance of proton exchange membrane fuel cells. The impacts of the equivalent weight (EW) of perfluorosulfonic acid–based ionomers on the platinum group metal-free electrode structure and fuel cell performance have not been fully explored. Four membrane electrode assemblies (MEAs) were prepared by using a commercial Fe–N–C catalyst, two perfluorosulfonic acid ionomers with different EWs, that is, Aquivion 720 (A720) and Nafion 1100 (N1100), and two ionomer-to-catalyst (I/C) ratios. The four MEAs were characterized to understand the impact of the ionomer EW and content on the capacitance, proton conductivity, and mass transport on the cathode. The mass transport resistance was measured for the first time using a new oxygen reduction reaction limiting current method enabling to couple the effects of oxygen diffusion with liquid water generation. Low EW ionomer combined with a moderate I/C results in improved performance due to its enhanced proton conductivity. However, when used at high I/C, it can cause severe water flooding at high current density due to the enhanced liquid water uptake, especially at high relative humidity, resulting in lower catalyst utilization and higher mass transport resistance.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Collisional space-charge-limited current with monoenergetic velocity: From Child–Langmuir to Mott–Gurney

All theories coupling electron emission theories ultimately approach the space-charge-limited current (SCLC) in vacuum, given by the Child–Langmuir (CL) law, for sufficiently high voltage, or the Mott–Gurney (MG) law for finite electron mobility and high (but not infinite) voltage. These analyses demonstrate the presence of an SCLC regime that cannot be described by either CL or MG. Here, we derive an exact solution for SCLC for general electron mobility and nonzero velocity. We recover the traditional CL with nonzero initial velocity at high voltage. For low mobility (or infinite collision frequency), we derive corrections to the MG law that depend on the ratio of initial velocity to the product of collision frequency and gap distance or initial velocity to drift velocity for low and high voltage, respectively. Increasing collisionality decreases the correction to SCLC for nonzero velocity, indicating that these corrections are less important for low-mobility materials (e.g., solids) than high-mobility materials (e.g., air or vacuum). For a given gap distance (collision frequency), increasing the collision frequency (gap distance) increases the voltage necessary to make the gap appear more like vacuum. These results provide a generalized SCLC for both collisionality and initial velocity when assessing the transitions between electron emission mechanisms.

Physics↗
DOE OSTI2024

Solid-State, Single-Ion Conducting, Polymer Blend Electrolytes with Enhanced Li + Conduction, Electrochemical Stability, and Limiting Current Density

The development of solid-state polymer electrolytes with high lithium conductivity is crucial to improve lithium-ion battery performance and ameliorate the safety challenges associated with current solvent-based electrolytes. Unfortunately, sluggish polymer segmental dynamics are known to constrain conductivity enhancements in solid-state polymer electrolyte systems, limiting overall performance. In this work, a glassy single-ion-conducting polymer, poly[lithium sulfonyl(trifluoromethane sulfonyl)imide methacrylate] (PLiMTFSI), was blended with a flexible polymer, poly(oligo-oxyethylene methyl ether methacrylate) (POEM), and the impact of PLiMTFSI molecular weight and ion concentration on the thermal and ion-conducting behavior of blend electrolytes was investigated. High ionic conductivities approaching 1 × 10 -2 S/cm at 150 °C were realized in this polymer blend electrolyte system as a result of decoupling Li + transport from polymer segmental dynamics. The decoupled ion transport was attributed to the packing frustration of the glassy PLiMTFSI – sufficient percolating free volume was generated to produce effective ion diffusion pathways. This decoupling was tunable as the ion transport could be altered from being closely coupled to the polymer segmental dynamics (Vogel–Tammann–Fulcher-like) to hopping (Arrhenius-like) by increasing the PLiMTFSI molecular weight and ion concentration. Moreover, the immobilized TFSI anion resulted in high Li + selectivity (Li + transference number = 0.9), high electrochemical stability (up to 4.7 V against Li + / Li), and limiting current density of 1.8 mA/cm 2 (electrolyte thickness = 0.05 cm). These features suggest that this single-ion-conducting, polymer blend electrolyte might be a promising alternative to a benchmark system – salt-doped polyethylene oxide. Moreover, the above characteristics can support the battery operation at higher voltages using energy-dense Li metal anodes, with faster charging rates and enhanced energy/power densities. Altogether, the results suggest that polymer chain packing frustration can be exploited to overcome the constraints of slow polymer segmental relaxations to achieve rapid and highly selective ion transport and enhanced performance in solid-state polymer electrolytes.

36 MATERIALS SCIENCE↗