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NASA NTRS1990

Research on diabatic initialization

The objective of this research project is to contribute to improvement in the synoptic analyses in the tropics for numerical weather prediction and climate research. In addition to a prediction model, four dimensional data assimilation systems have two principal components. One is objective analysis and the other is initialization. Various methods of objective analysis are designed primarily to analyze the mass and rotational wind fields. Methods of initialization are developed to obtain the irrotational wind and its associated vertical velocity field which are balanced with the mass field and free from meteorological noise. There are essentially three approaches to the problem of initialization: quasi-geostrophic theory, bounded derivative method and nonlinear normal mode method. In the midlatitudes, these approaches generally produce satisfactory results even without diabatic effects for large-scale motions. In the tropics, the situation is quite different from that in the midlatitudes. Because of a small magnitude of the Coriolis parameter and a weak horizontal temperature gradient in the tropics, any method of initialization must incorporate diabatic effects. In fact, it can be said that understanding the problem of diabatic initialization is the key to improving the analysis and weather forecasting in the tropics.

Kasahara, Akira↗

NASA NTRS1994

Quasi-biennial oscillations of ozone and diabatic circulation in the equatorial stratosphere

The quasi-biennial oscillation (QBO) in ozone in the equatorial stratosphere is obtained by analyzing the Stratospheric Aerosol and Gas Experiment (SAGE) data from 1984 to 1989. The phase of the ozone QBO in the lower stratosphere is found to precede the zonal wind QBO by several months as opposed to the theoretically expected in-phase relationship between the two. A mechanistic model is developed to explore possible reasons for this disagreement. The model is capable of simulating the actual time evolution of the ozone QBO by introducing the observed zonal wind profile as input. The modeled results confirm the conventional view that the ozone QBO is generated by the vertical ozone advection that is driven to maintain the temperature structure against radiative damping. However, a series of experiments emphasizes the importance of the feedback of the ozone QBO to the diabatic heating through the absorption of solar radiation. Due to this effect, the phase of the ozone QBO shifts up to a quarter cycle ahead and approaches that of the temperature QBO. Because of this inphase relationship, the feedback of the ozone QBO to the diabatic heating acts to compensate for the radiative damping of the temperature structure, thus reducing the magnitude of the induced diabatic circulation. Because the reduction of the magnitude of the vertical motion facilitates downward transport of easterly momentum by the mean flow, this feedback process can help to resolve the insufficiency of the easterly momentum in driving the dynamical QBO in general circulation models (GCMs). It should be emphasized that more sophisticated models that allow for full interaction between the chemical species and radiative and dynamical processes should be developed to improve our understanding of both dynamical and ozone QBOs.

Hasebe, Fumio↗

NASA NTRS2011

Global Distribution of Cloud Droplet Number Concentration, Autoconversion Rate, and Aerosol Indirect Effect Under Diabatic Droplet Activation

This study presents a global assessment of the sensitivity of droplet number to diabatic activation (i.e., including effects from entrainment of dry air) and its first-order tendency on indirect forcing and autoconversion. Simulations were carried out with the NASA Global Modeling Initiative (GMI) atmospheric and transport model using climatological metereorological fields derived from the former NASA Data Assimilation Office (DAO), the NASA Finite volume GCM (FVGCM) and the Goddard Institute for Space Studies version II (GISS) GCM. Cloud droplet number concentration (CDNC) is calculated using a physically based prognostic parameterization that explicitly includes entrainment effects on droplet formation. Diabatic activation results in lower CDNC, compared to adiabatic treatment of the process. The largest decrease in CDNC (by up to 75 percent) was found in the tropics and in zones of moderate CCN concentration. This leads to a global mean effective radius increase between 0.2-0.5 micrometers (up to 3.5 micrometers over the tropics), a global mean autoconversion rate increase by a factor of 1.1 to 1.7 (up to a factor of 4 in the tropics), and a 0.2-0.4 W m(exp -2) decrease in indirect forcing. The spatial patterns of entrainment effects on droplet activation tend to reduce biases in effective radius (particularly in the tropics) when compared to satellite retrievals. Considering the diabatic nature of ambient clouds, entrainment effects on CDNC need to be considered in GCM studies of the aerosol indirect effect.

Barahona, Donifan↗

DOE OSTI2025

Evaluating the gradients of localized diabatic state energies and couplings at minimum cost

We calculate the gradients of Boys diabatic state energies and couplings when the electronic vector space is generated by configuration interaction singles. Our approach follows the Lagrangian approach of Paz and Glover (rather than direct differentiation of the adiabatic-to-diabatic approaches that have been published previously). The result is that we achieve a dramatic increase in savings over previous approaches, and the present approach should be immediately useful to scientists focused on electronic relaxation, especially chemists studying electron transfer who wish to go beyond the Condon approximation. Here, a future extension to time-dependent density functional theory in the Tamm–Dancoff approximation is clear.

Chemical physics↗

NASA NTRS1984

A diabatic circulation experiment in a two-dimensional photochemical model

A two-dimensional photochemical model based on diabatic circulation has been used to simulate the behavior of N2O, CFCl3(F-11) and CF2Cl2(F-12) The circulation is based on estimates of net heating from the ground to 60 km. Eddy diffusion has been reduced with respect to other model studies with Kzz = 2000 sq cm/s everywhere bove 100 mbar. Resulting tracer profiles show reasonable agreement with measured profiles in the tropics and fall off much more sharply with altitude than those produced by models using larger values of Kzz. The agreement obtained is at least as good as that obtained with adjustable, eddy diffusion parameters. The diabatic circulation treatment is more closely related to related to real physical processes and thus more easily interpreted. Diffusive mixing appears to be more important in determining the details of the tracer distributions than the basic morphology.

Guthrie, P. D.↗

NASA NTRS1985

Response of the mesoscale atmosphere to diabatic heating

A study was initiated to determine the influence of convective latent heat release/diabatic heating on the production of kinetic energy during AVE/SESAME I. The primary focus has been on the relative importance of thermally forced modification of the wind field through thickness and height gradient changes versus inertial-advective effects via the diabatic component of vertical motion. Preliminary results have shown that because of the strong vertical shear over the convective region, ageostrophic response is primarily caused by the latter process. The diagnostic parameterization of convective heating has been extended for use in conjunction with satellite precipitation estimates in data-poor oceanic regions. An initial application was made to a mesoscale convective system embedded in the South Pacific convergence zone. Comparison to the heating field diagnosed as a residual in the thermodynamic equation using the ECMWF III-b analyses showed that the methodology will be useful in explaining the observed heating fields and determining the relative contribution of moist processes to the total diabatic heating. Research activities are now concentrated in the following areas: (1) Determining the sensitivity of vertical heating profiles to partitioning of gridscale versus convective precipitation; (2) assessing the possible effects of incorrect analyzed gridscale vertical motions on residuals in the heat budgets computed with the ECMWF III-b data sets.

Robertson, F. R.↗

NASA NTRS1987

A computation of the stratospheric diabatic circulation using an accurate radiative transfer model

The global diabatic circulation is computed for the months of January, April, July and October over the altitude region 100 to 0.1 mb using an accurate troposphere-stratosphere radiative transfer model, SBUV and SME ozone data, and NMC temperatures. There is high correlation between the level of wave activity and the local departure of the atmosphere from radiative equilibrium. An excess in the globally averaged net stratospheric heating from 40 to 50 km is computed for all months, and a deficit from 50 to 60 km is computed during solstice. A 20 percent uniform reduction in ozone from 40 to 50 km, or a temperature perturbation with an increase of 5 K at 1 mb, will bring the atmosphere into global radiative equilibrium without significant impact on the diabatic circulation. In the transitional months of April and October, the net heating in the fall hemispheres are very similar, while substantial differences exist between the spring hemispheres.

Rosenfield, Joan E.↗

NASA NTRS1987

A comparison of adiabatic and diabatic forcing in an intense extratropical cyclone system

The roles of adiabatic and diabatic forcings in the development of a cyclone are examined. The two types of height tendency equations (classical quasi-geostrophic and extended forms) employed to solve for height tendency are described. The extended equation, in which geostrophic wind is replaced with observed wind, the effects of diabatic heating are added, and three-dimensional varying static stability is permitted, is utilized to analyze the evolution of the January 9-11, 1975 cyclone event. The analysis reveals that vorticity advection has a primary effect on the movement and propagation of the wave system; the differential thermal advection has a secondary, but significant role in wave development; latent heating effects are minimal; and the vertical advection of static stability slows the propagation and development of the wave.

Tsou, Chih-Hua↗

NASA NTRS1987

The stratosphere - Climatologies of the radiative heating and cooling rates and the diabatically diagnosed net circulation fields

Stratospheric solar, IR, and net radiative heating are calculated on a monthly basis using solar and IR radiative codes and satellite derived distributions of ozone, water vapor, and temperature. Divergence-free, zonally averaged, advective fields are diagnosed using the calculated diabatic heating; associated stream functions are derived. The stratospheric transport of inert tracers is studied. Analysis of the diagnosed advective fields reveal that: (1) entry into the mid- to upper stratosphere of tropospheric air is mainly from altitude regions of + or - 10 deg at the equatorial tropopause; (2) at latitudes poleward of + or - 15 deg, tracers transported from the troposphere into the stratosphere are transported toward the pole and then downward and out of the stratosphere; and (3) the presence of net cooling cells in the lower stratospheric polar regions is important. The interannual variability of the diabatic circulation is estimated using heating and advection fields derived from LIMS data.

Callis, Linwood B.↗

NASA NTRS1986

Diabatic heating fields and the generation of available potential energy during FGGE

Global diabatic heating is estimated using fields of directly computed heating components, in particular those due to shortwave radiation, longwave radiation, sensible heating, and latent heating produced every 6 hours. The role of average fields of diabatic heating in the generation of available potential energy is examined. It is observed that latent heating is most significant in generating available potential energy.

Salstein, David A.↗

NASA NTRS1993

Research on diabatic initialization

The objective of this research is to contribute to the improvement of the analyses of irrotational wind and moisture fields in the tropics through advancement in the technique of initialization, incorporating diabatic effects and use of satellite-derived, radiometric imagery data that are not used currently by operational centers. Significant accomplishments during the period of May 1991 - April 1992 in research involving the following are presented: impact of tropical initialization upon the spin-up of precipitation forecasts; and a unified approach to diabatic initialization for improvement in the analysis of divergence and water vapor fields in the tropics. Focus of current research and plans for next year are discussed with respect to the topics of controlling the precipitation over shoot during the early part of a numerical forecast and the use of satellite imagery data for improvement of the tropical analysis.

Kashara, Akira↗

NASA NTRS1993

Diabatic dynamic initialization

A version of the dynamical adjustment procedure is generalized in order to make the procedure applicable to a diabatic model. In this new initialization procedure, backward adiabatic model integration is followed by forward diabatic model integration, with a high-frequency (low-pass) time filter in the form of the Euler backward time-differencing scheme applied throughout the integration. The new procedure was applied to the Goddard Laboratory for Atmospheres 4D data-assimilation system. It was found that, right from the beginning of the forecast integration, the forecast tendencies (and fields) were free of any noise due to imbalance in initial conditions, and the shocks related to an initial imbalance between model physics and dynamics, or the initial spinup effect, were practically removed.

Fox-Rabinovitz, Michael S.↗

NASA NTRS1991

Scale interactions and diabatic processes during the development of an Atlantic blocking event

Results of a case study of the development of a major blocking event over the North Atlantic Ocean are reported with emphasis on the potential roles of interactions between synoptic-scale systems and diabatic processes in the large-scale development. The approach used here involves the analysis of the evolution of the potential temperature on a constant potential vorticity (PV) surface, where the value of PV is chosen to be representative of that of the tropopause. The approach is shown to provide a simple way to qualitatively identify significant features in the development of the block, including scale interactions and diabatic processes.

Morgan, Michael C.↗

NASA NTRS1994

An assessment of satellite temperature distributions used to derive the net diabatic transport for zonally averaged models of the middle atmosphere

Determinations of the zonally averaged and diabatically derived residual mean circulation (RMC) are particularly sensitive to the assumed zonal mean temperature distribution used as input. Several different middle atmosphere satellite temperature distributions have been employed in models and are compared here: a 4-year (late 1978 to early 1982) National Meteorological Center (NMC) climatology, the Barnett and Corney (or BC) climatology, and the 7 months of Nimbus 7 limb infrared monitor of the stratosphere (LIMS) temperatures. All three climatologies are generally accurate below the 10 hPa level, but there are systematic differences between them of up to +/-5 K in the upper stratosphere and lower mesosphere. The NMC/LIMS differences are evaluated using time series of rocketsonde and reconstructed satellite temperatures at station locations. Much of those biases can be explained by the differing vertical resolutions for the satellite-derived temperatures; the time series of reconstructed LIMS profiles have higher resolution and are more accurate. Because the LIMS temperatures are limited to just two full seasons, one cannot obtain monthly RMCs from them for an annual model calculation. Two alternate monthly climatologies are examined briefly: the 4-year Nimbus 7 stratospheric and mesospheric sounder (SAMS) temperatures and for the mesosphere the distribution from the Solar Mesosphere Explorer (SME), both of which are limb viewers of medium vertical resolution. There are also differences of the order of +/-5 K for those data sets. It is concluded that a major source of error in the determination of diabatic RMCs is a persistent pattern of temperature bias whose characteristics vary according to the vertical resolution of each individual climatology.

Remsberg, Ellis E.↗

NASA NTRS1997

The Effect of Enhanced Diabatic Heating on Stratospheric Circulation

The objective of this research focuses on the stratospheric dynamical response to the increase in aerosol loading and subsequent enhanced diabatic heating resulting from the eruption of Mt. Pinatubo. The Langley research Center three dimensional general circulation model and modifications made to that model for this study are described (addition of hydrogen fluoride tracer and diabatic heating enhancement). Unperturbed hydrogen fluoride distribution is compared to the hydrogen fluoride distribution measured by HALOE. A comparison of control and perturbed model runs is presented.

Kleb, Mary M.↗

NASA NTRS2003

Diabatic Initialization of Mesoscale Models in the Southeastern United States: Can 0 to 12h Warm Season QPF be Improved?

It is well known that numerical warm season quantitative precipitation forecasts lack significant skill for numerous reasons. Some are related to the model--it may lack physical processes required to realistically simulate convection or the numerical algorithms and dynamics employed may not be adequate. Others are related to initialization-mesoscale features play an important role in convective initialization and atmospheric observation systems are incapable of properly depicting the three-dimensional stability structure at the mesoscale. The purpose of this study is to determine if a mesoscale model initialized with a diabatic initialization scheme can improve short-term (0 to 12h) warm season quantitative precipitation forecasts in the Southeastern United States. The Local Analysis and Prediction System (LAPS) developed at the Forecast System Laboratory is used to diabatically initialize the Pennsylvania State University/National center for Atmospheric Research (PSUNCAR) Mesoscale Model version 5 (MM5). The SPORT Center runs LAPS operationally on an hourly cycle to produce analyses on a 15 km covering the eastern 2/3 of the United States. The 20 km National Centers for Environmental Prediction (NCEP) Rapid Update Cycle analyses are used for the background fields. Standard observational data are acquired from MADIS with GOES/CRAFT Nexrad data acquired from in-house feeds. The MM5 is configured on a 140 x 140 12 km grid centered on Huntsville Alabama. Preliminary results indicate that MM5 runs initialized with LAPS produce improved 6 and 12h QPF threat scores compared with those initialized with the NCEP RUC.

Lapenta, William M.↗

DOE OSTI2020

Diabatic visualization shows effects of micro-fins on evaporation of R410A: Smooth, axial micro-fin, and helical micro-fin tubes

A novel approach to visualize the flow boiling inside a clear micro-fin tube under diabatic conditions is presented. Transparent smooth, axial micro-fin, and helical micro-fin tubes are made by 3D printing. The 3D printed tube is placed inside a glass tube and heated by the transparent secondary fluid flowing between the two tubes for providing the evaporation conditions and transparency. R410A flow boiling and the flow patterns in the three geometries captured with a high speed camera are compared. The experimental results show that micro-fin geometry influences flow behavior. Bubbles are mainly generated in the groove region due to a higher superheat than the fin region. Some of the liquid refrigerant is trapped in the grooves of the upper part of the micro-fin tube when the slug flow is present, and bubbles are generated in this thin liquid layer. In addition, the bubbles in the helical micro-fin tube are easier to merge because of the obstacle of the fin geometry for the bubble flowing path. As the two bubble merge, the conversion of surface free energy causes the bubble to travel with a higher velocity.

3D printed↗

DOE OSTI2022

Semiclassical Trajectory Studies of Reactive and Nonreactive Scattering of OH( 2 Σ + ) by H 2 Based on an Improved Full-Dimensional Ab Initio Diabatic Potential Energy Matrix

Here we present a new full-dimensional diabatic potential energy matrix (DPEM) for electronically nonadiabatic collisions of OH(A 2 Σ + ) with H 2 , and we calculate the probabilities of electronically adiabatic inelastic collisions, nonreactive quenching, and reactive quenching to form H 2 O+H. The DPEM was fitted using a many-body expansion with permutationally invariant polynomials in bond-order functions to represent the many-body part. The dynamics calculations were carried out with the fewest-switches with time uncertainty and stochastic decoherence (FSTU/SD) semiclassical trajectory method. We present results both for head-on collisions (impact parameter b equal to zero) and for a full range of impact parameters. The results are compared to experiment and to earlier FSTU/SD and quantum dynamics calculations with a previously published DPEM. The various theoretical results all agree that nonreactive quenching dominates reactive quenching, but there are quantitative differences between the two DPEMs and between the b=0 results and the all-b results, especially for the probability of reactive quenching.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗