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At least 37 records · Page 2

Space Launch System Base Heating Test: Tunable Diode Laser Absorption Spectroscopy

This paper describes the Tunable Diode Laser Absorption Spectroscopy (TDLAS) measurement of several water transitions that were interrogated during a hot-fire testing of the Space Launch Systems (SLS) sub-scale vehicle installed in LENS II. The temperature of the recirculating gas flow over the base plate was found to increase with altitude and is consistent with CFD results. It was also observed that the gas above the base plate has significant velocity along the optical path of the sensor at the higher altitudes. The line-by-line analysis of the H2O absorption features must include the effects of the Doppler shift phenomena particularly at high altitude. The TDLAS experimental measurements and the analysis procedure which incorporates the velocity dependent flow will be described.

Parker, Ron↗

Airborne Carbon Dioxide Laser Absorption Spectrometer for IPDA Measurements of Tropospheric CO2: Recent Results

The National Research Council's decadal survey on Earth Science and Applications from Space[1] recommended the Active Sensing of CO2 Emissions over Nights, Days, and Seasons (ASCENDS) mission for launch in 2013-2016 as a logical follow-on to the Orbiting Carbon Observatory (OCO) which is scheduled for launch in late 2008 [2]. The use of a laser absorption measurement technique provides the required ability to make day and night measurements of CO2 over all latitudes and seasons. As a demonstrator for an approach to meeting the instrument needs for the ASCENDS mission we have developed the airborne Carbon Dioxide Laser Absorption Spectrometer (CO2LAS) which uses the Integrated Path Differential Absorption (IPDA) Spectrometer [3] technique operating in the 2 micron wavelength region.. During 2006 a short engineering checkout flight of the CO2LAS was conducted and the results presented previously [4]. Several short flight campaigns were conducted during 2007 and we report results from these campaigns.

lidar↗

Absorption Laser Differential Interferometry for Simultaneous Colinear Flow Property and Fluctuation Measurements

An absorption laser differential interferometer (A-LDI) was constructed and tested in an effort to simultaneously and colinearly measure flow properties (pressure, temperature, concentration) and flow fluctuations (changes in optical path length). Whereas typical LDI and focused LDI (FLDI) systems use fixed wavelength lasers as the light source (often either green at approximately 532 nm or red at approximately 630 nm), a tunable 760 nm diode laser was used to probe the A-band absorption spectrum of molecular oxygen. The A-LDI system was used to measure O2 absorption and flow fluctuations in a sub-atmospheric pressure-controlled test cell, with absorption profiles from direct absorption and wavelength modulation absorption matching simulated results, while simultaneously being sensitive to high frequency fluctuations from jets of either compressed air or 100% O2 from a gas bottle. The A-LDI system was also installed at the NASA Langley Research Center Probe Calibration Tunnel to assess the freestream flow state in a Mach 3.5 flow. LDI measurements of the freestream indicated increasing amplitudes of flow fluctuations with increasing stagnation pressure at a fixed stagnation temperature, while absorption results demonstrated sensitivity to freestream pressure changes.

Joshua M. Weisberger↗

Methods for Retrievals of CO2 Mixing Ratios from JPL Laser Absorption Spectrometer Flights During a Summer 2011 Campaign

The JPL airborne Laser Absorption Spectrometer instrument has been flown several times in the 2007-2011 time frame for the purpose of measuring CO2 mixing ratios in the lower atmosphere. This instrument employs CW laser transmitters and coherent detection receivers in the 2.05- micro m spectral region. The Integrated Path Differential Absorption (IPDA) method is used to retrieve weighted CO2 column mixing ratios. We present key features of the evolving LAS signal processing and data analysis algorithms and the calibration/validation methodology. Results from 2011 flights in various U.S. locations include observed mid-day CO2 drawdown in the Midwest and high spatial resolution plume detection during a leg downwind of the Four Corners power plant in New Mexico.

laser remote sensing↗

Laser Absorption Measurements of Equivalence Ratios Studied Along With Their Coupling to Pressure Fluctuations in Lean Premixed Prevaporized (LPP) Combustion

Concerns about damaging the Earth's ozone layer as a result of high levels of nitrogen oxides (known collectively as NOx) from high-altitude, high-speed aircraft have prompted the study of lean premixed prevaporized (LPP) combustion in aircraft engines. LPP combustion reduces NOx emissions principally by reducing the peak flame temperatures inside an engine. Recent advances in LPP technologies have realized exceptional reductions in pollutant emissions (single-digit ppm NOx for example). However, LPP combustion also presents major challenges: combustion instability and dynamic coupling effects between fluctuations in heat-release rate, dynamic pressure, and fuel pressure. These challenges are formidable and can literally shake an engine apart if uncontrolled. To better understand this phenomenon so that it can be controlled, we obtained real-time laser absorption measurements of the fuel vapor concentration (and equivalence ratio) simultaneously with the dynamic pressure, flame luminosity, and time-averaged gaseous emissions measurements in a research-type jet-A-fueled LPP combustor. The measurements were obtained in NASA Glenn Research Center's CE-5B optically accessible flame tube facility. The CE-5B facility provides inlet air temperatures and pressures similar to the actual operating conditions of real aircraft engines. The laser absorption measurements were performed using an infrared 3.39 micron HeNe laser in conjunction with a visible HeNe laser for liquid droplet scattering compensation.

Nguyen, Quang-Viet↗

Laser absorption measurements of OH concentration and temperature in pulsed facilities

A laser absorption flow diagnostic application has been developed at the NASA Ames 16-inch Shock Tunnel for purposes of measuring the thermochemical state of OH in flow environments of interest. Research objectives include the investigation of high temperature, low pressure chemistry pertinent to scramjet combustors and high altitude flight. The system can be operated in either the fixed frequency mode or in the rapid wavelength scanning mode to measure species mole fraction and temperature. Emission diagnostics have been employed to determine shock tunnel flow quality and assist in the proper application of the diagnostic and its data interpretation. Rotational lines in the OH system were probed in the expanding facility nozzle flow, and time-resolved measurements of temperature and mole fraction are provided.

Cavolowsky, John A.↗

Miniaturized Laser Absorption Spectrometer for Combustion Calorimetry and Process Monitoring

A miniaturized tunable laser absorption spectrometer capable of measuring gas-phase concentrations of CO, CO2, and O2 has been developed for operation in spacecraft environments. As part of the Spacecraft Fire Safety Demonstration (Saffire) project, we previously demonstrated the Combustion Product Monitor (CPM) instrument to characterize pyrolysis of relevant test materials in low gravity aboard a transfer vehicle returning from low Earth orbit. Here, we adapted the CPM instrument design to achieve detection of CO, CO2, and O2 with improved minimum detection limits and dynamic range as well as reduced instrument size and power. The instrument can be operated in either an open or sealed configureation, allowing for ambient gas composition measuremnts or in-line monitoring of gas streams. By accurately monitoring CO, CO2, and O2 with broad pressure/temperature calibration and response time on the order of 1 s, the instrument can be used to characterize the dynamics of combustion reactions in a variety of environments.

Briggs, Ryan M.↗

The airborne Laser Absorption Spectrometer - A new instrument of remote measurement of atmospheric trace gases

The Laser Absorption Spectrometer is a portable instrument developed by JPL for remote measurement of trace gases from an aircraft platform. It contains two carbon dioxide lasers, two optical heterodyne receivers, appropriate optics to aim the lasers at the ground and detect the backscattered energy, and signal processing and recording electronics. Operating in the differential-absorption mode, it is possible to monitor one atmospheric gas at a time and record the data in real time. The system can presently measure ozone, ethylene, water vapor, and chlorofluoromethanes with high sensitivity. Airborne measurements were made in early 1977 from the NASA/JPL twin-engine Beechcraft and in May 1977 from the NASA Convair 990 during the ASSESS-II Shuttle Simulation Study. These flights resulted in measurements of ozone concentrations in the lower troposphere which were compared with ground-based values provided by the Air Pollution Control District. This paper describes the details of the instrument and results of the airborne measurements.

Shumate, M. S.↗

Carbon Dioxide Laser Absorption Spectrometer (CO2LAS) Aircraft Measurements of CO2

The Jet Propulsion Laboratory Carbon Dioxide Laser Absorption Spectrometer (CO2LAS) utilizes Integrated Path Differential Absorption (IPDA) at 2.05 microns to obtain CO2 column mixing ratios weighted heavily in the boundary layer. CO2LAS employs a coherent detection receiver and continuous-wave Th:Ho:YLF laser transmitters with output powers around 100 milliwatts. An offset frequency-locking scheme coupled to an absolute frequency reference enables the frequencies of the online and offline lasers to be held to within 200 kHz of desired values. We describe results from 2009 field campaigns when CO2LAS flew on the Twin Otter. We also describe spectroscopic studies aimed at uncovering potential biases in lidar CO2 retrievals at 2.05 microns.

Lidar↗

Laser absorption phenomena in flowing gas devices

A theoretical and experimental investigation is presented of inverse Bremsstrahlung absorption of CW CO2 laser radiation in flowing gases seeded with alkali metals. In order to motivate this development, some simple models are described of several space missions which could use laser powered rocket vehicles. Design considerations are given for a test call to be used with a welding laser, using a diamond window for admission of laser radiation at power levels in excess of 10 kW. A detailed analysis of absorption conditions in the test cell is included. The experimental apparatus and test setup are described and the results of experiments presented. Injection of alkali seedant and steady state absorption of the laser radiation were successfully demonstrated, but problems with the durability of the diamond windows at higher powers prevented operation of the test cell as an effective laser powered thruster.

Chapman, P. K.↗

Method and apparatus for enhancing laser absorption sensitivity

A simple optomechanical method and apparatus is described for substantially reducing the amplitude of unwanted multiple interference fringes which often limit the sensitivities of tunable laser absorption spectrometers. An exterior cavity is defined by partially transmissible surfaces such as a laser exit plate, a detector input, etc. That cavity is spoiled by placing an oscillating plate in the laser beam. For tunable diode laser spectroscopy in the mid-infrared region, a Brewster-plate spoiler allows the harmonic detection of absorptances of less than 10 to the -5 in a single laser scan. Improved operation is achieved without subtraction techniques, without complex laser frequency modulation, and without distortion of the molecular lineshape signal. The technique is applicable to tunable lasers operating from UV to IR wavelengths and in spectrometers which employ either short or long pathlengths, including the use of retroreflectors or multipass cells.

Webster, Christopher R.↗

Continuous wave laser absorption techniques for gasdynamic measurements in supersonic flows

Line-of-sight measurements of velocity, temperature, pressure, density, and mass flux were performed in a transient shock tube flow using three laser absorption schemes. All methods employed an intracavity-doubled ring dye laser tuned to an OH transition at 306 nm. In the first scheme, the gas was labeled by 193.3-nm excimer photolysis of H2O, and the passage of the generated OH was detected downstream. In the second method, the laser was tuned at a rate of 3 kHz over the R1(7) and R1(11) line pair, and absorption was simultaneously monitored at 90 and 60 deg with respect to the flow. Velocity was determined from the Doppler shift of the profiles and the temperature from the intensity ratio of the lines. Pressure was determined from both the magnitude of absorption and the collisional broadening. In the third method, the laser wavelength was fixed at a single frequency, and a continuous measurement of velocity and pressure was obtained using the signals from the two beam paths. All methods gave results which compare favorably to calculated values.

Davidson, David F.↗

Vibrational relaxation of the bending mode of shock-heated CO2 by laser-absorption measurements.

Study of the vibrational relaxation characteristics of shock-heated CO2 using a tuned CO2 laser absorption technique. Absorption-coefficient histories were obtained for a single rotational state in each of the -10 0- and -02 0- levels over the temperature range from 500 to 2000 K, and for 21 rotational states of the -10 0- level at 1000 K. These histories have been combined with translational-rotational temperature histories based on interferometer measurements to calculate vibrational relaxation times for the bending mode. The results verify the mutual equilibrium of the bending and symmetric-stretch modes due to Fermi resonance. The bending mode relaxation times are approximately 10% shorter than predicted from interferometer results using the ratio of specific heats. Furthermore, relaxation times based on measurements of different rotational states at 1000 K show a variation with quantum number J, indicating a possible rotational nonequilibrium during the vibration relaxation process.

Eckstrom, D. J.↗

Intracavity Dye-Laser Absorption Spectroscopy (IDLAS) for application to planetary molecules

Time-resolved, quasi-continuous wave, intracavity dye-laser absorption spectroscopy is applied to the investigation of absolute absorption coefficients for vibrational-rotational overtone bands of water at visible wavelengths. Emphasis is placed on critical factors affecting detection sensitivity and data analysis. Typical generation-time dependent absorption spectra are given.

Lang, Todd M.↗

Compact Multi-Channel Infrared Laser Absorption Spectrometer for Spacecraft Fire Safety Monitoring

We report on the design of a six-channel tunable laser absorption spectroscopy instrument for measuring ambient gas-phase concentrations of CO, HCl, HCN, HF, CO2, and O2 in spacecraft environments. Monitoring of these compounds can provide early warning detection of fire events while also indicating what materials have been exposed to heating. Continued post-fire monitoring of these hazardous gases can also facilitate safe and effective cleanup. The sensor is a miniaturized version of a five-channel prototype that was previously validated in ground-based oxidative pyrolysis tests. Here, we describe absorption line selection and theoretical detection limits for a sensor with reduced absorption pathlengths for each detection channel, which allows for a substantial reduction in overall instrument footprint. Ultimately, the new instrument is designed to be used in fire safety tests conducted by NASA, where various materials will undergo oxidative pyrolysis in an unmanned spacecraft returning from low Earth orbit.

Briggs, Ryan M.↗

Fast-response, high-precision carbon monoxide sensor using a tunable diode laser absorption technique

A tunable diode laser instrument, denoted as DACOM (Differential Absorption CO Measurement), has been developed to meet the fast-response, high-precision CO measurement needs of the GTE (Global Tropospheric Experiment) program. Under the GTE program, DACOM participated in the three field missions of CITE 1 (Chemical Instrumentation Test and Evaluation 1), a project involving the intercomparison of trace gas measurement techniques. DACOM performance, including analyses of measurement error sources, is discussed for the ground-based mission at Wallops Island, VA (summer 1983), and two missions on the NASA CV-990 (fall 1983 and spring 1984). Examples of fast-response (about 1 s), high-precision (+ or - 1 part per billion by volume, + or - 1.5 percent of reading) airborne data are included to illustrate the capability of this instrument.

Sachse, Glen W.↗

In situ ozone data for comparison with laser absorption remote sensor: 1980 PEPE/NEROS program

Several sets of in situ ozone (O3) measurements were made by a NASA aircraft in support of the laser absorption spectrometer (LAS) remote sensor. These measurements were designed to provide comparative O3 data for the LAS sensor. The LAS, which was flown on a second aircraft, remotely measured the vertical burden of O3 from the aircraft to the surface. In situ results of the air quality (O3 and B sub scat) and meteorological (temperature and dewpoint) parameters for three correlative missions are presented. The aircraft flight plans, in situ concentration profiles and vertical burdens, and measurement errors are summarized.

Mcdougal, D. S.↗