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At least 37 records · Page 2

A New Method to Grow SiC: Solvent-Laser Heated Floating Zone

The solvent-laser heated floating zone (solvent-LHFZ) growth method is being developed to grow long single crystal SiC fibers. The technique combines the single crystal fiber growth ability of laser heated floating zone with solvent based growth techniques (e.g. traveling solvent method) ability to grow SiC from the liquid phase. Initial investigations reported in this paper show that the solvent-LHFZ method readily grows single crystal SiC (retains polytype and orientation), but has a significant amount of inhomogeneous strain and solvent rich inclusions.

Woodworth, Andrew A.↗

A New Method to Grow SiC: Solvent-Laser Heated Floating Zone

The solvent-laser heated floating zone (solvent-LHFZ) growth method is being developed to grow long single crystal SiC fibers. The technique combines the single crystal fiber growth ability of laser heated floating zone with solvent based growth techniques (e.g. traveling solvent method) ability to grow SiC from the liquid phase. Initial investigations reported in this paper show that the solvent-LHFZ method readily grows single crystal SiC (retains polytype and orientation), but has a significant amount of inhomogeneous strain and solvent rich inclusions.

Woodworth, A. A.↗

Fabrication of silicon-tipped fiber-optic temperature sensors using aerogel-assisted glass soldering with precise laser heating

We demonstrate the fabrication of fiber-optic Fabry–Perot interferometer (FPI) temperature sensors by bonding a small silicon diaphragm to the tip of an optical fiber using low melting point glass powders heated by a 980 nm laser on an aerogel substrate. The heating laser is delivered to the silicon FPI using an optical fiber, while the silicon temperature is being monitored using a 1550 nm white-light system, providing localized heating with precise temperature control. The use of an aerogel substrate greatly improves the heating efficiency by reducing the thermal loss of the bonding parts to the ambient environment. A desirable temperature for bonding can be achieved with relatively small heating laser power. The bonding process is carried out in an open space at room temperature for convenient optical alignment. The precise temperature control ensures minimum perturbation to the optical alignment and no induced thermal damage to the optical parts during the bonding process. For demonstration, we fabricated a low-finesse and high-finesse silicon FPI sensor and characterized their measurement resolution and temperature capability. The results show that the fabrication method has a good potential for high-precision fabrication of fiber-optic sensors.

Sheng, Qiwen↗

Laser-heated thruster

The development of computer codes for the thrust chamber of a rocket of which the propellant gas is heated by a CW laser beam was investigated. The following results are presented: (1) simplified models of laser heated thrusters for approximate parametric studies and performance mapping; (3) computer programs for thrust chamber design; and (3) shock tube experiment to measure absorption coefficients. Two thrust chamber design programs are outlined: (1) for seeded hydrogen, with both low temperature and high temperature seeds, which absorbs the laser radiation continuously, starting at the inlet gas temperature; and (2) for hydrogen seeded with cesium, in which a laser supported combustion wave stands near the gas inlet, and heats the gas up to a temperature at which the gas can absorb the laser energy.

Kemp, N. H.↗

Laser heating system at the Extreme Conditions Beamline, P02.2, $\mathrm{PETRA III}$

A laser heating system for samples confined in diamond anvil cells paired with in situ X-ray diffraction measurements at the Extreme Conditions Beamline of PETRA III is presented. The system features two independent laser configurations (on-axis and off-axis of the X-ray path) allowing for a broad range of experiments using different designs of diamond anvil cells. The power of the continuous laser source can be modulated for use in various pulsed laser heating or flash heating applications. An example of such an application is illustrated here on the melting curve of iron at megabar pressures. The optical path of the spectroradiometry measurements is simulated with ray-tracing methods in order to assess the level of present aberrations in the system and the results are compared with other systems, that are using simpler lens optics. Based on the ray-tracing the choice of the first achromatic lens and other aspects for accurate temperature measurements are evaluated.

47 OTHER INSTRUMENTATION↗

Stability of laser heated flows

A local stability analysis is utilized to determine the stability of disturbances generated at each point along a nozzle of variable area ratio for a one-dimensional flow heated by laser radiation entering from the upstream direction. The governing equations for the quasi-one-dimensional flow without viscous dissipation, diffusion, and thermal conduction but including radiative heat transfer are given. The governing equations are combined to yield a relationship which governs the Mach number variation through the nozzle. The complete steady-state solution can be calculated from knowledge of the Mach number profile, the inlet conditions, and the laser power. The local stability analysis permits obtaining contour (or contours) of neutral stability. Solutions have been obtained for various nozzle configurations, but only one set of example calculations is presented. The results obtained indicate that the analysis serves as an important indicator as to where potential absorption wave phenomena may be initiated.

Wu, P. K. S.↗

Laser heating and evaporation of a single droplet

The laser technology is being abundantly studied for controlled energy deposition for a range of applications in aerodynamic flow control, material processing, ignition, and combustion. The absorption of laser radiation by liquid droplets affects further propagation of laser in the atmosphere and causes bleaching of suspended droplets while the ignition and combustion characteristics in combustors are influenced by the evaporation rate of the sprayed fuel. In this work, we present a multi-dimensional mathematical model built on OpenFOAM for laser heating and evaporation of a single droplet in the diffusion dominated regime taking into account absorption of the laser radiation, evaporation process and vapor flow dynamics. The developed solver is validated against available experimental and numerical data for the ethanol and water droplet heating and evaporation. For continuous heating the peak temperature is established by the balance of cooling, evaporation and heating and results in high temperature for larger droplets. It has been shown that for heating by a single laser pulse the maximum temperature of droplets depends only on the peak intensity of the laser radiation. Furthermore, for the peak irradiance close to the transition to the boiling regime, temporal dynamics of the droplet temperature is independent of the droplet size. With proper normalization of time, the dynamics of the droplet shrinkage and cooling is shown to be independent of droplet sizes and peak laser intensities. The influence of cooling and evaporation processes on droplet heating was found to be controlled by the pulse repetition rate for repeated pulse operation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

SiC growth by Solvent-Laser Heated Floating Zone

In an effort to grow single crystal SiC fibers for seed crystals the following two growth methods have been coupled in this work: traveling solvent and laser heated floating zone to create the solvent-laser heated floating zone (Solvent-LHFZ) crystal growth method. This paper discusses the results of these initial experiments, which includes: source material, laser heating, and analysis of the first ever Solvent-LHFZ SiC crystals (synchrotron white beam x-ray topography confirmed).

Woodworth, Andrew A.↗

Experimental and calculational investigation of laser-heated additive manufactured foams

Foam materials are starting to find application in laser-heated Hohlraums used to drive inertial confinement fusion implosions. Foams made using additive manufacturing (AM) techniques are now available and may have advantages over traditional chemical (aerogel) foams. Here, we present new experimental data on laser-heated AM foams. Samples of four different types of printed AM foams were heated using a single 527 nm laser beam at the Jupiter Laser Facility. The laser pulse was ∼180 J square pulse with an FWHM of 1.6 ns and a peak intensity of 3–4 × 1014 W/cm2. The foam densities ranged from 12 to 93 mg/cc (all supercritical for 527 nm light). We measured the backscattered light (power and spectrum), the transmitted light, side-on x-ray images, and the Ti K-shell emission that was used to infer the time-integrated temperature. The fraction of backscattered light was 6%–15% of the input laser energy. The pure carbon foam sample had less backscatter than a C8H9O3 foam of similar density, which was consistent with multi-fluid calculations that predicted less ion heating for the C8H9O3 foam. The level of backscatter and the thermal front speeds for the AM foams were similar to values measured for stochastic (aerogel) foams under similar conditions.

36 MATERIALS SCIENCE↗

Design of a double-sided laser heating compatible piezoelectrically driven dynamic diamond anvil cell

Piezoelectrically driven dynamic diamond anvil cells are generally limited to use at room temperature due to spatial conflicts with the optical components necessary for double-sided laser heating. Here, this work describes the design of a double-sided laser-heating-compatible, piezoelectrically driven dynamic diamond anvil cell (LH-dDAC) that expands the range of experimentally accessible compression rate/temperature space. By developing a spatially in-parallel design, in which the diamond anvils and the piezo actuators lie alongside each other, the total length of the apparatus is reduced to 66.5 mm. The new LH-dDAC is capable of probing both overpressure and compression-rate effects on the kinetics of phase transitions. We illustrate the capability of the new LH-dDAC using the following cases: (1) a simultaneous pressure and temperature jump from 19.5 GPa and room temperature to 40 GPa and ≈1550 K and (2) a controlled compression ramp at ≈1850 K and ≈100 GPa/s. By pairing rapid compression with laser heating, the new LH-dDAC opens the door to studies of diffusionally controlled transformations at high pressures and temperatures.

Copley, J. A. [Princeton Univ., NJ (United States)↗

Characterizing laser-heated polymer foams with simultaneous x-ray fluorescence spectroscopy and Thomson scattering at the Matter in Extreme Conditions Endstation at LCLS

Understanding the behavior of polymer foams at high energy density conditions is crucial to advance inertial fusion energy research. Here, we present a new experimental platform designed to measure the thermodynamic state of these materials at megabar pressures. At the Matter in Extreme Conditions Endstation of the Linac Coherent Light Source, we heat samples using an optical, high-intensity, femtosecond laser and dynamically probe them with ultra-short, coherent x-ray pulses of high peak brightness. We perform x-ray Thomson scattering measurements in forward and backward scattering geometries to capture both collective and non-collective electron behavior in the sample. Simultaneously, x-ray fluorescence spectroscopy is used to measure the emission from a mid-Z dopant, providing complementary information on the plasma conditions. By combining these techniques, we obtain temporally resolved temperature measurements of the transient warm dense matter states. Our initial experiments designed to benchmark the platform with carbon samples yielded data resolving the ultrafast response to laser heating with sub-picosecond resolution, measuring plasma temperatures exceeding 50 eV. These findings lay the foundation for precision studies of the dynamic evolution of laser-heated polymer foams.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Kinetic corrections to heat-flow and Nernst advection for laser heated plasmas

Reduced models for approximating the impact of kinetic electron behavior on the transport of thermal energy and magnetic field are investigated. The thermal flux limiter has improved agreement with Vlasov–Fokker–Planck data when a harmonic form is used that adjusts the electron mean free path to account for electron–electron collisions; these results apply to both unmagnetized and magnetized plasmas. Once a magnetic field is incorporated, the mean free path should also be modified using the electron gyroradius. A flux limiter on Nernst advection of magnetic fields is also required; a form that limits Nernst by the same fraction as the thermal heat-flow best reproduces kinetic simulations. A flux limiter form for the cross terms (Righi–Leduc and cross-gradient-Nernst) is also suggested. Hohlraum simulations relevant to fusion experiments on the National Ignition Facility are found to be sensitive to all of these details.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Volatiles in the deep Earth: An experimental study using the laser-heated diamond cell

Experiments with the laser-heated diamond cell show that H2O and CO2 can be stabilized within crystalline mineral structures of the lower-mantle, and hence can be present at relatively non-volatile components of the Earth's deep interior. Samples quenched from high pressures and temperatures document that the MgCO3-FeCO3 magnesite-siderite solid-solution is stable and coexists with (Mg,Fe)SiO3 perovskite at 30-40 GPa and approximately 1500-2000 K. In contrast, H2O combines with the silicate to form (Mg,Fe)SiH2O4 phase D, coexisting with (Mg,Fe)SiO3 perovskite at these conditions. If enough water is present, phase D can become the predominant phase in the MgSiO3-H2O system at lower-mantle conditions. Our work extends previous studies to Fe-bearing compositions and to the pressures of the mid-lower mantle. Thus, the results of high-pressure experiments suggest that both H2O and CO2 can be abundant in the Earth's lower mantle, being present in stable hydroxisilicate and carbonate phases.

Li, Xiaoyuan↗

Thermal Conductivity Change Kinetics of Ceramic Thermal Barrier Coatings Determined by the Steady-State Laser Heat Flux Technique

A steady-state laser heat flux technique has been developed at the NASA Glenn Research Center at Lewis Field to obtain critical thermal conductivity data of ceramic thermal barrier coatings under the temperature and thermal gradients that are realistically expected to be encountered in advanced engine systems. In this study, thermal conductivity change kinetics of a plasma-sprayed, 254-mm-thick ZrO2-8 wt % Y2O3 ceramic coating were obtained at high temperatures. During the testing, the temperature gradients across the coating system were carefully measured by the surface and back pyrometers and an embedded miniature thermocouple in the substrate. The actual heat flux passing through the coating system was determined from the metal substrate temperature drop (measured by the embedded miniature thermocouple and the back pyrometer) combined with one-dimensional heat transfer models.

Zhu, Dongming↗

Synthesis of ceramic powders and surface films from laser heated gases

Two new processes have been developed that are based on laser-heated gases. Both permit unusually precise levels of process control and, thereby, materials having superior properties. The power process yields Si, Si3N4 and SiC powders that are uniform in size, nonagglomerated, small diameter, spherically shaped and high purity. Manufacturing cost analyses show that submicron powders can be made with an energy cost of approximately 2 kWhr/kg and a dollar cost of 2-3.30 $/kg, exclusive of the costs of feed materials. The laser-induced chemical vapor deposition process (LICVD) causes reactant gases to be heated by absorbing IR light from a laser beam that passes parallel to the substrate surface. Laser heating permits independent control of gas and substrate temperatures while operating in a conventional, thermally activated chemical vapor deposition mode. Spin density, hydrogen content, electrical conductivity and mobility gap properties show the LICVD process capable of producing very high quality films.

Haggerty, J. S.↗

Laser-heated capillary discharge plasma waveguides for electron acceleration to 8 GeV

A plasma channel created by the combination of a capillary discharge and inverse Bremsstrahlung laser heating enabled the generation of electron bunches with energy up to 7.8 GeV in a laser-driven plasma accelerator. The capillary discharge created an initial plasma channel and was used to tune the plasma temperature, which optimized laser heating. Although optimized colder initial plasma temperatures reduced the ionization degree, subsequent ionization from the heater pulse created a fully ionized plasma on-axis. The heater pulse duration was chosen to be longer than the hydrodynamic timescale of ≈ 1 ns, such that later temporal slices were more efficiently guided by the channel created by the front of the pulse. Here, simulations are presented which show that this thermal self-guiding of the heater pulse enabled channel formation over 20 cm. The post-heated channel had lower on-axis density and increased focusing strength compared to relying on the discharge alone, which allowed for guiding of relativistically intense laser pulses with a peak power of 0.85 PW and wakefield acceleration over 15 diffraction lengths. Electrons were injected into the wake in multiple buckets and times, leading to several electron bunches with different peak energies. To create single electron bunches with low energy spread, experiments using localized ionization injection inside a capillary discharge waveguide were performed. A single injected bunch with energy 1.6 GeV, charge 38 pC, divergence 1 mrad, and relative energy spread below 2% full-width half-maximum was produced in a 3.3 cm-long capillary discharge waveguide. This development shows promise for mitigation of energy spread and future high efficiency staged acceleration experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗