Positron annihilation in helium - Theory and experiment
Positron annihilation in helium
Drachman, R. J.↗
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Positron annihilation in helium.
Modified adiabatic scattering function applied to positron annihilation in helium
SCATTERING FUNCTION↗
Positron annihilation in the interstellar medium
Positronium formation and annihilation are studied in a model for the interstellar medium consisting of cold cloud cores, warm partially ionized cloud envelopes, and hot intercloud gas. The gamma-ray spectra resulting from positron annihilation in these components of the interstellar medium are calculated. The spectra from the individual components are then combined, using two limiting assumptions for the propagation of the positrons, namely, that the positrons propagate freely throughout the interstellar medium, and that the positrons are excluded from the cold cloud cores. In the first case, the bulk of the positrons annihilate in the cloud cores and the annihilation line exhibits broad wings resulting from the annihilation of positronium formed by charge exchange in flight. In the second case, the positrons annihilate mainly in the warm envelopes, and the line wings are suppressed.
Guessoum, Nidhal↗
On the origin of the positron annihilation radiation from the direction of the galactic center
Physical constraints on the possible configuration of the positron annihilation region observed at the galactic center with gamma ray instrumentation focused on 511 keV emission are discussed. The line width is less than 2.5 keV, implying that the positrons annihilate in a gas that features some ionization. The line width also limits velocities to less than 700 km/sec, while the line center indicated a bulk velocity along the line of sight of between -90 to 200 km/sec. Data from emissions less than 511 keV suggest a production of 511 keV photons/positron ratio of 0.65 to account for the continuum emission detected. The annihilation region requires a temperature of at least 50,000 K and an ionization fraction of at least 10 percent, a density near 100,000 H/cu cm, and a diameter less than 10 to the 18th cm. Relativitistic considerations support pair production around an accreting black hole or the collision of collimated photon beams as possible sources of the emissions.
Lingenfelter, R. E.↗
Positron annihilation processes update
The present knowledge concerning the positron annihilation processes is reviewed, with emphasis on the data of the cross sections of the various processes of interest in astrophysical applications. Recent results are presented including results on reaction rates and line widths, the validity of which is verified.
Guessoum, Nidhal↗
Free-positron annihilation mean life in diatomic and rare gases in liquid and solid states.
Free-positron annihilation mean life in diatomic and rare gases as a function of first electron ionization potential and outermost electron density
DIATOMIC GAS↗
OSSE observations of Galactic 511 keV positron annihilation radiation - Initial phase 1 results
The Oriented Scintillation Spectrometer Experiment (OSSE) on the Compton Gamma-Ray Observatory (GRO) has performed numerous observations of the Galactic plane and Galactic center region to measure the distribution of Galactic 511 keV positron annihilation radiation and to search for time variability of the emission. The initial 511 keV line fluxes for the observations performed during the first 18 months of the GRO mission are presented. The 511 keV line flux for a typical Galactic center observation is (2.5 +/- 0.3) x 10 exp -4 gamma/sq cm per sec, where the quoted uncertainty represents the 1 sigma statistical uncertainty. No statistically significant time variability of the line flux has been observed; the 3 sigma upper limit to daily variations from the mean is 3 x 10 exp -4 gamma/sq cm per sec. The distribution of Galactic 511 keV positron annihilation radiation implied by the OSSE observations is discussed and compared with observations by other instruments.
Purcell, W. R.↗
Hydrated doped-BaZrO 3 proton conductors studied by positron annihilation lifetime spectroscopy
The study of defect chemistry for doped BaZrO 3 proton conductors is of particular interest because of defect interactions that can affect the proton conductivity of the material. Protons incorporated due to the material's hydration can be trapped by negatively charged immobile dopants, reducing proton mobility. The reduction of the proton conduction impedes using BaZrO 3 materials in energy conversion applications at intermediate temperatures (300°C – 600°C). The probing of proton trapping in doped BaZrO 3 is hindered by the limited availability of techniques sensitive to defect chemistries. In this work, we used positron annihilation lifetime spectroscopy (PALS) to study the defect chemistry of Y-doped and Sc-doped BaZrO 3 . Using a two-state positron trapping model we showed that PALS can be used to study the defect chemistry of hydrated dense proton conductors. Positron trapping rates and lifetimes were correlated with doping levels of the materials. Probability significance t-tests were carried out for PALS parameters to verify whether there are differences/similarities for various populations: non-doped/doped, level and type of doping, high temperature, and surface effects. Further, the results revealed that the initial doping generates a significant number of traps available for positrons. Doping in yttrium increased the positron trapping rate, while this effect was not observed with scandium. Low-temperature hydration affects specimens significantly inhibiting positron trapping at undoped BaZrO 3 material and highly doped specimens. Positronium formation in rough surface layers, and highly doped specimens was detected but does not exceed 1%.
36 MATERIALS SCIENCE↗
Positron annihilation spectroscopy of defects in nuclear and irradiated materials- a review
Positron is the only probe that can detect individual atomic vacancies and small and large vacancy clusters induced by irradiation with remarkable sensitivity, providing information about their size, concentration, and chemical environment. The focus of this review article is to provide guidance to facilitate applications of positron annihilation spectroscopy (PAS) in irradiation-induced defect studies to advance the development of new radiation-tolerant materials. The principle of PAS, its techniques, and data analysis methods are described. PAS studies of defects in nuclear and irradiated materials are reviewed and discussed in depth. Future developments to advance PAS applications in nuclear materials research and studies of materials under extreme environments are presented.
Atomic scale defects↗
Positron annihilation induced Auger electron spectroscopy
Recently, Weiss et al. have demonstrated that it is possible to excite Auger transitions by annihilating core electrons using a low energy (less than 30eV) beam of positrons. This mechanism makes possible a new electron spectroscopy, Positron annihilation induced Auger Electron Spectroscopy (PAES). The probability of exciting an Auger transition is proportional to the overlap of the positron wavefunction with atomic core levels. Since the Auger electron energy provides a signature of the atomic species making the transition, PAES makes it possible to determine the overlap of the positron wavefunction with a particular element. PAES may therefore provide a means of detecting positron-atom complexes. Measurements of PAES intensities from clean and adsorbate covered Cu surfaces are presented which indicate that approx. 5 percent of positrons injected into CU at 25eV produce core annihilations that result in Auger transitions.
Weiss, Alex↗
Positron annihilation in gamma-ray bursts
Emission features appear at energies of 350 to 450 keV in the spectra of a number of gamma ray burst sources. These features were interpreted as electron-positron annihilation lines, redshifted by the gravitational field near the surface of a neutron star. Evidence that gamma ray bursts originate at neutron stars with magnetic field strengths of approx. 10(exp 12) Gauss came from recent observations of cyclotron scattering harmonics in the spectra of two bursts. Positrons could be produced in gamma ray burst sources either by photon-photon pair production or by one-photon pair production in a strong magnetic field. The annihilation of positrons is affected by the presence of a strong neutron star magnetic field in several ways. The relaxation of transverse momentum conservation causes an intrinsic broadening of the two-photon annihilation line and there is a decrease in the annihilation cross section below the free-space value. An additional channel for one-photon annihilation also becomes possible in high magnetic fields. The physics of pair production and annihilation near strongly magnetized neutron stars will be reviewed. Results from a self-consistent model for non-thermal synchrotron radiation and pair annihilation are beginning to identify the conditions required to produce observable annihilation features from strongly magnetized plasmas.
Harding, Alice K.↗
Direct positron annihilation and positronium formation in thermal plasmas
In the present evaluation of the rate of direct positron annihilation with electrons in the nonrelativistic limit, general analytic expressions are given for the radiative recombination of positrons to form positronium. Formulae are derived for the radiative capture to bound states of atomic hydrogen, and the connection between the two problems is demonstrated. Annihilation from excited states of positronium is considered, and it is estimated that 90 percent of the annihilations occur from the ground 1s state for both ortho and para positronium following radiative capture and cascade. A convenient form is given for the photodissociation cross section of positronium.
Gould, Robert J.↗
Defect Characterization Using Positron Annihilation Spectroscopy on Laser-Ablated Surfaces
In recent years, short, pulsed laser ablation has been gaining popularity for machining small-scale test geometries from bulk samples and for efficient serial sectioning. These laser-based techniques are being added to the toolbox in material science, which makes it necessary to understand the changes in the material that occur from the laser–material interaction. Positron annihilation spectroscopy is a unique, nondestructive technique to investigate small defects in materials difficult to investigate by other tools. In this work, Doppler broadening and positron lifetime annihilation spectroscopy are utilized to help quantify the damage in materials treated with short, pulsed lasers. Using a femtosecond laser on single crystal silicon, this manuscript shows that clusters of vacancy-like defects and small voids increase systematically with laser power. Lastly, the damage induced by the laser can also reach to micrometer depths.
36 MATERIALS SCIENCE↗
An interpretation of the narrow positron annihilation feature from X-ray nova Muscae 1991
The physical mechanism responsible for the narrow redshifted positron annihilation gamma-ray line from the X-ray nova Muscae 1991 is studied. The orbital inclination angle of the system is estimated and its black hole mass is constrained under the assumptions that the annihilation line centroid redshift is purely gravitational and that the line width is due to the combined effect of temperature broadening and disk rotation. The large black hole mass lower limit of 8 solar and the high binary mass ratio it implies raise a serious challenge to theoretical models of the formation and evolution of massive binaries.
Chen, Wan↗
Are mildly active galaxies sources of electron-positron annihilation radiation?
Mildly active galaxies are examined as possible sources of 511-keV line radiation resulting from electron-positron annihilations. Observations of seven galaxies of various types are made using an HEAO-3 gamma-ray spectrometer. It is shown that none of the galaxies are detected in the 511 keV line and therefore the proposed scaling law for 511-keV line emission from the galactic nuclei is not valid. The results indicate that the scaling overestimates the 511-keV line flux by a factor of 3 or more. Possible causes of this discrepancy are considered. The expected values of and the observed 2.3-sigma upper limits to the 511-keV line flux for each source and the Galactic Center are presented in a table.
Marscher, A. P.↗
Diffuse 0.511 MeV line emission and the distribution of positron annihilation in the galaxy
We model the distribution in the Galaxy of 0.511 MeV line emission and the implied positron annihilation using plausible distributions based on observations at other photon energies. We use 0.511 MeV line observations from the Galactic center and from directions away from the Galactic center to normalize the two-dimensional 0.511 MeV sky maps. We find that in order to understand all of the available data it is necessary to invoke the presence of a time-variable component of 0.511 MeV line emission in addition to an underlying diffuse component. The large 0.511 MeV fluxes observed with broad field of view detectors, such as the SMM gamma-ray spectrometer, can be reconciled with the small fluxes seen with narrow field-of-view instruments (GRIS and OSSE) from directions away from the Galactic center if the diffuse emission follows the distribution of Galactic novae for which the recently detected 0.511 MeV line emission from the Galactic center with OSSE is predominantly of diffuse origin. For future GRIS and HEXAGONE observations from the direction of the Galactic center we predict a minimum 0.511 MeV line flux of (6.0 +/- 0.9) x 10 exp -4 photons/sq cm/s.
Skibo, J. G.↗
Evaluation of adsorption and mechanical strength of 13X zeolite mixtures with phyllosilicate binders using molecular dynamics simulation and positron annihilation spectroscopy
There is growing interest in developing zeolites with novel internal structures that have optimal adsorptive capacity and high mechanical strength, while offering advantages, such as being light weight. We integrate computational and experimental methods to explore the effect of binder/zeolite types, and weight percentages on the mechanical strength of 13X zeolite and adsorption capacities of N 2 , H 2 O, and CO 2 for additive manufacturing (AM) applications with the goal of maximizing both adsorption and strength. Zeolite 13X mixtures and phyllosilicate binders (either bentonite or kaolin) are combined using molecular dynamics (MD) simulations to create structures with various binder/zeolite weight percentages. Further, adsorption capabilities and mechanical strength are assessed using the grand canonical Monte Carlo (GCMC) and ReaxFF modules, respectively. Our modeling shows that an optimized zeolite/binder ratio for N 2 adsorption is around 15 wt% for kaolin and roughly 10 wt% for bentonite. The resulting parameters can be applied to facilitate macro-scale computational fluid dynamics (CFD) and finite element method (FEM) simulations of an AM zeolite structure. We also performed Positron Annihilation Lifetime Spectroscopy (PALS) measurements on zeolite samples to explore the effect of changes in the internal volume. The results show an inverse relationship between the free volume and the solid loading and adding a binder changes the morphology of the zeolite-binder compound and decreases open-volume area significantly.
36 MATERIALS SCIENCE↗
Variable positron annihilation radiation from the galactic center region
HEAO 3 Cosmic Gamma-Ray Spectrometer evidence is presented for the existence of a time-varying, unshifted, narrow 511 keV line emission from the vicinity of the galactic center. Although uncertainties exist regarding the spatial extent of the features as well as its centroid, all data are consistent with emission from a single point source located at the galactic center. This interpretation would require a source luminosity of 2 x 10 to the 37th ergs/sec, and a positron annihilation rate of about 10 to the 43rd/sec. It is concluded that a variable source of positrons which could generate such an annihilation figure might be a massive black hole at the galactic center, as has been suggested by IR observations.
Riegler, G. R.↗