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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2

Investigation of boosted proton energies through proton radiography of target normal sheath acceleration fields in the multi-ps regime

Multi-kilojoule, multi-picosecond short-pulse lasers, such as the National Ignition Facility-Advanced Radiographic Capability laser and the OMEGA-Extended Performance laser, which have been constructed over the last two decades, enable exciting opportunities to produce high-brightness, high-energy laser-driven proton sources for applications in high-energy-density science like proton fast ignition for inertial fusion energy, particle radiography, and materials science studies. Results on these platforms have demonstrated enhanced accelerated proton energies and electron temperatures when compared to established scaling laws. Recent work has developed a new scaling for proton TNSA in the multi-ps regime. However, this new physics in the multi-ps regime motivates the need to understand the origin of the enhancement in proton energies. Toward this goal, here this work presents the first measurements of the TNSA accelerating sheath field in the multi-ps regime for pulse durations of 0.6, 5, and 10 ps. This measurement was achieved by using a separate TNSA proton source to radiograph the spatiotemporal profile of the accelerating sheath that is responsible for proton acceleration. The use of stacked radiochromic film detectors allows for a discrete time profile of the radiographs, thus enabling the measurement of the temporal and spatial evolution of the accelerating field. In performing this measurement, we extract quantities such as the sheath strength as a function of time and pulse duration, which shows that longer pulse durations sustain a stronger electric field for a longer duration when compared to sub-ps laser pulses, which may enable the observed boosted proton energies and proton conversion efficiencies.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Investigation of Proton Beam-Driven Fusion Reactions Generated by an Ultra-Short Petawatt-Scale Laser Pulse

We present results from a pitcher-catcher experiment utilizing a proton beam generated with nanostructured targets at a petawatt-class, short-pulse laser facility to induce proton-boron fusion reactions in a secondary target. A 45-fs laser pulse with either 400 nm wavelength and 7 J energy, or 800 nm and 14 J, and an intensity of up to 5 × 10 21 W/cm 2 was used to irradiate either thin foil targets or near-solid density, nanostructured targets made of boron nitride (BN) nanotubes. In particular, for 800 nm wavelength irradiation, a BN nanotube target created a proton beam with about five times higher maximum energy and about ten times more protons than a foil target. This proton beam was used to irradiate a thick plate made of boron nitride placed in close proximity to trigger 11 B (p, α) 2α fusion reactions. A suite of diagnostics consisting of Thomson parabola ion spectrometers, postshot nuclear activation measurements, neutron time-of-flight detectors, and differentially filtered solid-state nuclear track detectors were used to measure both the primary proton spectrum and the fusion products. From the primary proton spectrum, we calculated (p, n) and (α,n) reactions in the catcher and compare with our measurements. The nuclear activation results agree quantitatively and neutron signals agree qualitatively with the calculations, giving confidence that primary particle distributions can be obtained from such measurements. These results provide new insights for measuring the ion distributions inside of proton-boron fusion targets.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Three-dimensional modeling of electric-field enhancement in multilayer dielectric gratings arising from inadvertent flaws

Pulse-compression gratings for high-power, short-pulse laser systems are exposed to high electric fields that are further enhanced locally due to their 2D nanostructured surface. This makes them vulnerable to laser-induced damage. The present work considers the effect on electric-field modulation caused by an array of commonly found inadvertent flaws in gratings including fabrication defects, contamination particles, and laser-induced–damage initiation. These defects affect the laser-damage performance characteristics of the grating. To understand the local field-enhancement distribution due these imperfections, 3D modeling of the electric-field distribution is performed with a sufficiently high resolution of 1/74 of the laser wavelength ( λ ) while considering a volume of ≈489 λ 3 . The results provide estimates for the ensuing electric-field intensification and projected reduction of the laser-damage thresholds, as well as the anticipated pattern of damage growth initiation.

47 OTHER INSTRUMENTATION↗

Demonstration of thermal fracture limits of gas-cooled Nd:APG-1 and Tm:YLF slabs

High-energy short-pulse laser systems demonstrated to date have been limited to low repetition rates due to significant thermal management challenges associated with scaling these systems to high average power, including the need to understand the thermal fracture limits of laser gain media. In this paper, we demonstrate the thermal fracture limits of two high-average-power gain media in a realistic diode-pumped amplifier geometry: a 5 mm thick Nd:APG-1 slab and a 2 mm thick Tm:YLF slab, both cooled by room-temperature helium gas. Finite element analysis revealed maximum tensile stress at fracture of 25 ± 3 MPa for Nd:APG-1 and 30 ± 3 MPa for Tm:YLF. These stress levels correspond to average volumetric heat loads of 13 ± 1 W/cm 3 in Nd:APG-1 and 247 ± 12 W/cm 3 in Tm:YLF. Additional simulations show geometric scaling: thinner slabs tolerate higher heat loads before fracture, while larger pump spots reach the fracture stress at lower heat loads.

Lasers↗

Diagnostics for Short-Pulse Radiography

The Multi-Probe project is developing radiographic techniques using probe beams generated by short-pulse lasers. Shortcomings in present detectors and future capabilities in new devices are described.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Characterization of the upgraded single-line-of-sight time-resolved x-ray imager using short-pulse visible and UV lasers

The single-line-of-sight time-resolved x-ray imager (SLOS-TRXI), a fast-gated x-ray imager used for capturing x-ray self-emission in inertial confinement fusion experiments on OMEGA, has been upgraded and characterized. SLOS-TRXI combines an electron-dilation imager and a hybrid complementary metal–oxide–semiconductor (hCMOS) sensor to capture multiple gated frames on a single line of sight with a temporal resolution of ~40 ps and a spatial resolution of 10 µm. The original hCMOS sensor with four frames was replaced with a newer-generation hCMOS sensor having eight frames. Gate characterizations of both the sensor and the entire SLOS-TRXI diagnostic were performed using ~10-ps FWHM visible (2ω) and UV (4ω) short-pulse lasers, respectively. A stepped echelon was used to generate a train of five UV laser pulses having an interpulse separation of 30 ± 3 ps. Characterization results of the hCMOS gating (2.28 ± 0.02-ns FWHM on average) and a temporal resolution of the upgraded SLOS-TRXI (34 ± 4-ps FWHM on average) are presented. A temporal magnification for the electron-dilation imager between 40 and 60 was inferred from the characterization results. Furthermore, the spatial resolution of the upgraded SLOS-TRXI remains the same in light of this work.

47 OTHER INSTRUMENTATION↗

Remote detection of radioactive material using a short-pulse CO 2 laser

Detection of radioactive material at distances greater than the radiated particle range is an important goal with applications in areas such as national defense and disaster response. Here, we demonstrate avalanche-breakdown-based remote detection of a 3.6 mCi α-particle source at a standoff distance of 10 m, using 70 ps, long-wave infrared (λ = 9.2 µm) CO 2 laser pulses. This is ∼10 times longer than our previous results using a mid-IR laser. The primary detection method is direct backscatter from microplasmas generated in the laser focal volume. The backscatter signal is amplified as it propagates back through the CO 2 laser chain, enhancing sensitivity by >100 times. Here we also characterize breakdown plasmas with fluorescence imaging, and present a simple model to estimate backscattered signals as a function of the seed density profile in the laser focal volume. All of this is achieved with a relatively long-drive laser focal geometry (f/200) that is readily scalable to >100 m.

43 PARTICLE ACCELERATORS↗

Optimizing MeV photon dose generation in laser-solid interactions via stable beam propagation

Bremsstrahlung MeV x rays with high doses are essential for radiography of dense objects. Intense, short-pulse laser-driven MeV x-ray sources offer a promising solution, but understanding how the dose scales with laser intensity is crucial for their development. While theory predicts a square root scaling with laser intensity, experimental verification has been hindered by significant shot-to-shot variations, often exacerbated by long preplasma scale lengths from low laser contrast. Here, we demonstrate low shot-to-shot dose variation and confirm the theoretical scaling using high-contrast OMEGA EP laser interactions with millimeter-thick tantalum foils, achieving MeV x-ray doses up to 5.4 rad at 1 m for E photon > 500 keV. Simulations reveal that the unique focal spot of the OMEGA EP laser enables efficient x-ray generation and reduced variability by facilitating deeper laser penetration into dense plasma, even with shorter preplasma scale lengths. Published by the American Physical Society 2025

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A platform to measure isentropes from proton-heated warm dense matter on short pulse laser facilities

We describe the development of an experimental platform that measures the release isentrope of materials heated isochorically to temperatures of a few electron volts, using short-pulse laser-produced protons to heat the sample and long-pulse laser-produced x rays to perform streaked x-ray radiography. The density profiles derived from the radiography data are integrated to generate pressure–density isentropes, independent of prior knowledge of the equation of state of the sample material. In order to understand the sensitivities of isentrope extraction from radiography data, we analyze synthetic radiographs generated by a radiation hydrodynamics code. Noise reduction and high spatial resolution are critical for isentrope reconstruction, as demonstrated by the analysis of a proof-of-principle shot day on the OMEGA-EP facility. In conclusion, the data demonstrate the feasibility of the platform for characterizing isentropes, and we discuss the necessary improvements to enhance precision in differentiating between equation-of-state models.

Equations of state↗

Diagnostic x-ray source using electrons produced by a 100 J-class picosecond laser

Many laser-based high-energy-density science (HEDS) facilities have one or more short-pulse (sub- to few-picosecond) laser beams for diagnostics. For the past decade, we have been developing a novel x-ray probing capability using such picosecond lasers interacting with an underdense plasma to produce relativistic electrons. The ultimate goal of these experiments is to demonstrate a new type of x-ray backlighter using the short-pulse ARC laser at the National Ignition Facility (NIF). Before this diagnostic is fielded at the NIF, it is critical to demonstrate the viability and reproducibility of the x-ray source on comparable high-power short-pulse laser systems. We present experiments that were carried out with the OMEGA EP laser at the University of Rochester’s laboratory for laser energetics. In these experiments, high-energy electrons are produced through a combination of the self-modulation instability and direct laser acceleration in an underdense gas jet. These electrons generate directional x-rays with characteristic energies up to several tens of keV as they execute betatron motion in the ion channel, and the inverse Compton scattering process generates even harder x-rays, with characteristic photon energies of 60–240 keV. When implemented on the OMEGA EP laser(s), this x-ray source yields results that are comparable to those obtained recently on the short-pulse Titan laser at the Jupiter Laser Facility at Lawrence Livermore National Laboratory, after accounting for differences in laser energy, peak intensity, focusing f/#, and plasma source. Applications of such an x-ray source for HEDS experiments are discussed.

backlighter↗

Modeling the Interaction of Laser-Produced Proton Beams with Matter

A major goal of this project is to significantly increase our understanding of isochoric heating of matter using laser produced proton beams, and the associated high energy density (HED) and warm dense matter (WDM) regimes generated. This will benefit research fields such as planetary science, fusion energy, plasma physics, and material science. For example, it will enhance our understanding of WDM properties of iron and silica under conditions encountered in planetary interiors and diagnostic components in fusion devices exposed to high fluxes of energetic plasma ions. The project is motivated by recent experiments that irradiated Si targets with proton beams generated by the 20 TW-laser at the SLAC MEC end-station. The HED/WDM states are probed using the 50 fs hard X-rays available in the 3rd harmonic of the LCLS. As part of this project, results from the phase contrast X-ray imaging, which shows the generation of compression waves that produces rear surface spallation, are compared with results from the 3D multi-physics multi- material code, PISALE, that combines Arbitrary Lagrangian-Eulerian (ALE) hydrodynamics with Adaptive Mesh Refinement (AMR). This comparison required modifications to several physics models in the PISALE (Pacific Island Structured-AMR with ALE) code. An important aspect of this project is the continued training of graduate students in HED physics and in conducting complex multiphysics simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Characterization of a platform for the gas transport, collection, and identification of fission products in the high-intensity laser environment

Recent progress in the production of laser accelerated high flux proton beams opens new possibilities for the study of fission in unique environments. To this end, we are currently pursuing the development of a platform for the swift gas transport, collection, and identification of fission products. Fission is induced in targets fixed inside a sealed chamber through which a carrier gas flows, transporting fission products to a carbon filter for collection and online spectroscopy. This has been recently demonstrated using target normal sheath accelerated protons at the PHELIX laser facility. There were large discrepancies between measured rates and those expected based on established fission yields and measured beam parameters. These discrepancies prompted a large number of tests at the Idaho Accelerator Center (IAC), where fission in uranium is induced by bremsstrahlung photons generated by 21 MeV electrons from a linear electron accelerator. Here, the results are compared to a series of models that account for the slowing of energetic fission fragments in the carrier gas and the fluid dynamics of the gas flow that transports fission products to the collection filter. Characterization of the apparatus reveals a few mechanisms that together account for a portion of the previously observed discrepancies at the PHELIX laser facility. However, additional research is necessary before high-accuracy experiments can be performed with the apparatus. Work performed under the auspices of the U.S. Department of Energy by LLNL under contract DE-AC52-07NA27344.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Demonstration of active neutron interrogation of special nuclear materials using a high-intensity short-pulse-laser-driven neutron source

Detecting shielded special nuclear material, such as nuclear explosives, is a difficult challenge pursued by non-proliferation, anti-terrorism, and nuclear security programs worldwide. Interrogation with intense fast-neutron pulses is a promising method to characterize concealed nuclear material rapidly but is limited by suitable source availability and proven instrumentation. In this study we have pioneered a demonstration of such an interrogation method using a high-intensity, short-pulse, laser-driven neutron source that offers potential benefits compared to conventional neutron sources. The measurement results reported here represent the first experimental demonstration of this interrogation approach on enriched uranium items and demonstrate the feasibility of a precise measurement using realistic nuclear materials, representative of field scenarios, even with just a single laser-driven neutron pulse. Bright pulsed sources can overcome the nuisance background of items with strong internal neutron sources, improving analytical power, while single-shot assay is attractive in high-throughput situations where time is at a premium. The science and technology of this type of neutron production is developing rapidly, and we anticipate that practical mobile interrogation systems will become available based on the detection concepts demonstrated here to meet the growing measurement needs.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Electron-beam-based Compton scattering x-ray source for probing high-energy-density physics

The physics basis for an electron-beam-based Compton scattering x-ray source is investigated for single-shot experiments at the major high-energy-density facilities, such as the Omega Laser Facility, National Ignition Facility, and Z pulsed power facility. A source of monoenergetic ( δ ε / ε < 5 % ) 10- to 50-keV x rays can be produced by scattering of a short-pulse optical laser by a 23- to 53-MeV electron beam and collimating the scattered photons. The number and spectrum of scattered photons are calculated as a function of electron packet charge, electron and laser pulse duration, laser intensity, and collision geometry. A source delivering greater than 10 10 photons in a 1-mm-radius spot and 100-ps time resolution is plausible with the available electron gun and laser technology. Applications of this source for x-ray diffraction, x-ray imaging, x-ray absorption fine structure, and x-ray absorption spectroscopy in high-energy-density physics experiments are described, demonstrating significant advancements compared to the present state of the art. Published by the American Physical Society 2024

47 OTHER INSTRUMENTATION↗

Characterization of blast waves induced by femtosecond laser irradiation in solid targets

Blast waves have been produced in solid target by irradiation with short-pulse high-intensity lasers. The mechanism of production relies on energy deposition from the hot electrons produced by laser–matter interaction, producing a steep temperature gradient inside the target. Hot electrons also produce preheating of the material ahead of the blast wave and expansion of the target rear side, which results in a complex blast wave propagation dynamic. Several diagnostics have been used to characterize the hot electron source, the induced preheating and the velocity of the blast wave. Results are compared to numerical simulations. These show how blast wave pressure is initially very large (more than 100 Mbar), but it decreases very rapidly during propagation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Silicon x-ray backlighter improvement by targets with spike-like microstructures

In order to accurately probe high energy density matter states, it is vital to create powerful x-ray backlighters. One approach to create such x-ray sources is based on the usage of short-pulse, high-energy lasers, which greatly benefits from an optimization of the laser target coupling. Here, the spectral and temporal x-ray emission profiles of structured silicon targets with micron-sized spikes on the front surface are studied at laser intensities of 10 17 W cm -2 . The laser pulse length is varied between 1 and 20 ps with an energy of up to 1 kJ. The structured targets show an up to 13× enhancement of silicon He α emission compared to flat foils with a well-defined, sharp emission pulse profile. Furthermore, the performance of the microstructured targets is compared to targets with a CH shield as well as foils irradiated with a UV prepulse.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Striated composite layers of silica and hafnia offering advantageous properties for short-pulse optical coatings

Monolayers containing subnanometer striations of silica and hafnia to form composite materials at varying ratios are explored as a method to develop high-index dielectric layers with increased laser-induced–damage thresholds (LIDTs). These layers can then be used in multilayer dielectric coatings for short-pulse, high-peak-power laser applications, particularly in regions of the highest electric-field intensity. Fabrication is achieved by means of exposure to two different evaporant vapor plumes, where local exposure to each plume is controlled via shielding to prevent simultaneous exposure. The LIDT of the resulting layers has been evaluated at 1053 nm with 600-fs pulses. The results indicate that such hafnia/silica layers exhibit LIDTs similar to silica for a refractive index of ≤1.65. These results suggest that the use of these layers in locations subjected to high electric-field intensity within multilayer dielectric coatings may significantly improve the LIDT, with this deposition process providing particular benefit for scaling to large-aperture, high-fluence components.

36 MATERIALS SCIENCE↗