Spontaneous radiofrequency emission from hot-electron plasmas
Spontaneous radio frequency emission from hot electron plasma, and enhanced cyclotron radiation from electron cyclotron resonance discharge
HOT ELECTRON↗
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Kinetic Scale Structure of Low-Frequency Waves and Fluctuations
The dissipation of solar wind turbulence at kinetic scales is believed to be important for the heating of the corona and for accelerating the wind. The linear Vlasov kinetic theory is a useful tool for identifying various wave modes, including kinetic Alfven, fast magnetosonic/whistler, and ion-acoustic (or kinetic slow), and their possible roles in the dissipation. However, the kinetic mode structure in the vicinity of ion-cyclotron modes is not clearly understood. The present paper aims to further elucidate the structure of these low-frequency waves by introducing discrete particle effects through hybrid simulations and Klimontovich formalism of spontaneous emission theory. The theory and simulation of spontaneously emitted low-frequency fluctuations are employed to identify and distinguish the detailed mode structures associated with ion-Bernstein modes versus quasi-modes. The spontaneous emission theory and simulation also confirm the findings of the Vlasov theory in that the kinetic Alfven waves can be defined over a wide range of frequencies, including the proton cyclotron frequency and its harmonics, especially for high-beta plasmas. This implies that these low-frequency modes may play predominant roles even in the fully kinetic description of kinetic scale turbulence and dissipation despite the fact that cyclotron harmonic and Bernstein modes may also play important roles in wave-particle interactions.
waves↗
Nuclear pumped laser II
The first direct nuclear pumped laser using the He-2-(n,p) H-3 reaction is reported. Lasing took place on the 1.79 microns Ar I transition in a mixture of He-3-Ar at approximately 600 Torr total pressure. It was found that the electrically pulsed afterglow He-Ar laser had the same concentration profile as the nuclear pumped laser. As a result, nuclear lasing was also achieved in He-3-Xe (2.027 micron) and He-3-Kr (2.52 micron). Scaling of laser output with both thermal flux and total pressure as well as minority concentration has been completed. A peak output (He-3-Ar) of 3.7 watts has been achieved at a total pressure of 4 atm. Direct nuclear pumping of He-3-Ne has also been achieved. Nuclear pumping of a He-3-NF3 mixture was attempted, lasing in FI at approximately 7000 A, without success, although the potential lasing transitions appeared in spontaneous emission. Both NF3 and 238UF6 appear to quench spontaneous emission when they constitute more than 1% of the gas mixture.
Deyoung, R. J.↗
Saturation Phenomena in LIF Measurements, Appendix B
Optical saturation is the phenomenon in which the laser-induced rates of absorption and spontaneous emission between two levels, induced by a laser, become comparable to or greater than the spontaneous emission and collision rates connecting these levels. This results in the excited state population N(u) acquiring a value of similar magnitude to that of the ground state, N(e). Under these conditions the observed fluorescence signal, which is proportional to N(u), is no longer linearly dependent on laser intensity I, but increases at a slower rate, and in principle ultimately becomes independent of I. A conceptual picture of optical saturation using a two-level picture is described. This is, however, inadequate for the description of a real experiment involving a molecule, such as OH, for several reasons, which will be explained briefly; these are the multi-level nature of the electronic states and energy transfer among them and effects due to spatial, spectral, and temporal fluctuations in the laser pulse.
Source record↗
Validity of the Relation Between Spontaneous and Stimulated Emissions in Semiconductors
The Einstein relation between spontaneous emission and absorption was originally derived for a system consists of a two-state subsystem representing matter and harmonic fields representing radiation. The derivation is based on the detailed balance between these two subsystems under thermal equilibrium. The relationship was later investigated in connection with the interactions between radiation field and solids or semiconductors. The simple derivation dose not hold for semiconductors in general. In certain limiting cases, simple relation was obtained. The validity of this relation is important not only because of its fundamental role connecting two of the most fundamental optical processes in semiconductors, but mostly also because of its wide use as a practical method to measure the optical gain of a semiconductor. The validity of this relation for semiconductors has been an issue of controversial for some time. In this paper we numerically examine the validity of this relationship for several different lineshapes including Lorentzian, Gaussian, Sech, and a convoluted double Lorentzians (CDL). We find out that at relatively low density above transparency level, all first three lineshapes violate the Einstein relation. The relation is approximately valid at high density. At very high density, the validity of the Einstein relation holds well for all three lineshapes. The reason behind this observation is explained. The CDL lineshape has been shown analytically to obey the Einstein relationship previously. We show that for a 2D semiconductor with parabolic bands, the CDL lineshape can be integrated analytically. This analytic lineshape is compared with a simple Lorentzian lineshape.
Ning, Cun-Zheng↗
The saturation spectrum of parametric instabilities
Recent calculations on the nonlinear saturation spectrum of the parametric decay instability are described. The initial calculations did not use the correct expression for the spontaneous emission term and were aimed at obtaining the distribution of spectral energy in the unstable part of wave vector space. Results of those initial calculations are combined here with the correct expression for the spontaneous emission term to obtain the distribution of spectral energy in the stable part of wave vector space. These latter calculations are believed to be relevant to the interpretation of the so called plasma line spectra obtained in ionospheric heating experiments at Arecibo, Puerto Rico.
Fejer, J. A.↗
Radiative instabilities and 1000 second fluctuations in astrophysical masers
A stability analysis for small (linear) perturbations is presented for the radiation in astrophysical masers treated in the usual, linear maser approximation. Instabilities that oscillate with a period of about L/c, where L is the length of the maser are found. They occur (1) when the maser is partly but not heavily saturated, (2) when the decay rate Gamma for the molecular states is near c/L, and (3) when the product of the brightness temperature T sub 0 of the incident radiation and the angle for the beaming is less than a critical value that depends upon the particular masing transition. A fourth parameter, the fractional inversion in the pumping multiplied by (T sub 0/frequency), determines the importance of spontaneous emission which can eliminate the instabilities. These instabilities are a likely cause for the fluctuations in the radiation from the 18 cm OH masers that have been reported to occur on time scales as short as 1000 s. The calculations are applicable to other types of astrophysical masers as well, and suggest that spontaneous emission will prevent similar instabilities in the H2O and SiO masers.
Scappaticci, Gerardo A.↗
Resolving Wave-Particle Duality Could Accelerate the Mass Production of Quantum Computers
Quantum computers, hypothesized in 1980s, use concepts of superposition and entanglement phenomena. Although theoretical propositions and associated search algorithms for accurate measurements are being generated, the development of practical quantum computers themselves are advancing very slowly requiring enormous time and investments. The underlying concepts of a quantum computer are not new to the optical domain. However, the crucial enabling concepts of Entanglement and Superposition Principle are remaining clouded under the unresolved postulates, Wave-Particle Duality (WPD), and Wave Packet Reduction (WPR), implicating incompleteness in the interpretations of the mathematical formalism behind Quantum Mechanics. The WPD debate started during late1600 between Newton and Huygens. Young’s resolution of WPD through his double-slit experiment in 1802 was effectively overturned by Einstein’s interpretation of photoelectric effect as due to “indivisible light quanta”. However, Einstein disowned his “light quanta” postulate shortly before his death in1955, even though it had earned him the Nobel Prize. We resolve WPD by synthesizing Newton’s and Maxwell’s concepts and assume atoms do emit quanta but propagate as time-finite exponential pulses. This assumption also resolves WPR for light-matter interaction with the assumption that Schrodinger’s ψ represents atom’s internal dipolar amplitude stimulations. This over-turns Born’s interpretation that ψ only represents the abstract mathematical probability amplitude, rather than the physical “internal amplitude stimulation” of the quantum entity. However, our concept of atomic pulse emission forces us to re-derive the expression for the N-slit grating-spectrometer response since the classical derivation uses CW light, which does not exist. This pulsespectrometric response function strengthens our postulate since the grating response to the exponential pulse appears to be the convolution of a Lorentzian spectrum with the classical CW response function of the grating. The Fourier Transform of an exponential function is Lorentzian and QM predicts spontaneous emission line width to be Lorentzian. Then, conceptually one can extend the grating-expression (with N=2) to get the double-slit pattern. This approach preserves the classical causality that each of the two slits, like the N-signals out of a grating, are physically real and jointly stimulate the quantum detector array at the far field to generate the “Local” cosine fringes. The detector array executes the square modulus operation on its imposed dipolar amplitude stimulation and absorbs the necessary energy to fill up their quantum cups. Hence the double-slit pattern must also be “Local”, just as the N-slit grating spectrum is generated locally at the exit spectral-plane of the spectrometer. This removes the need to believe that “single photons” mysteriously generate the double slit pattern. Quantum computers, hypothesized in 1980s, use concepts of superposition and entanglement phenomena. Although theoretical propositions and associated search algorithms for accurate measurements are being generated, the development of practical quantum computers themselves are advancing very slowly requiring enormous time and investments. The underlying concepts of a quantum computer are not new to the optical domain. However, the crucial enabling concepts of Entanglement and Superposition Principle are remaining clouded under the unresolved postulates, Wave-Particle Duality (WPD), and Wave Packet Reduction (WPR), implicating incompleteness in the interpretations of the mathematical formalism behind Quantum Mechanics. The WPD debate started during late1600 between Newton and Huygens. Young’s resolution of WPD through his double-slit experiment in 1802 was effectively overturned by Einstein’s interpretation of photoelectric effect as due to “indivisible light quanta”. However, Einstein disowned his “light quanta” postulate shortly before his death in1955, even though it had earned him the Nobel Prize. We resolve WPD by synthesizing Newton’s and Maxwell’s concepts and assume atoms do emit quanta but propagate as time-finite exponential pulses. This assumption also resolves WPR for light-matter interaction with the assumption that Schrodinger’s ψ represents atom’s internal dipolar amplitude stimulations. This over-turns Born’s interpretation that ψ only represents the abstract mathematical probability amplitude, rather than the physical “internal amplitude stimulation” of the quantum entity. However, our concept of atomic pulse emission forces us to re-derive the expression for the N-slit grating-spectrometer response since the classical derivation uses CW light, which does not exist. This pulsespectrometric response function strengthens our postulate since the grating response to the exponential pulse appears to be the convolution of a Lorentzian spectrum with the classical CW response function of the grating. The Fourier Transform of an exponential function is Lorentzian and QM predicts spontaneous emission line width to be Lorentzian. Then, conceptually one can extend the grating-expression (with N=2) to get the double-slit pattern. This approach preserves the classical causality that each of the two slits, like the N-signals out of a grating, are physically real and jointly stimulate the quantum detector array at the far field to generate the “Local” cosine fringes. The detector array executes the square modulus operation on its imposed dipolar amplitude stimulation and absorbs the necessary energy to fill up their quantum cups. Hence the double-slit pattern must also be “Local”, just as the N-slit grating spectrum is generated locally at the exit spectral-plane of the spectrometer. This removes the need to believe that “single photons” mysteriously generate the double slit pattern.
Quantum Computer↗
On the efficiency of solar heating in the middle atmosphere
The efficiency at which solar ultraviolet radiation absorbed in the Hartley band of ozone is directly converted to heat in the terrestrial mesosphere and lower thermosphere (50-110 km) is calculated. The ozone molecule undergoes photolysis to yield the excited species O(1D) and O2(1Delta) with a quantum yield of about 0.9. Spontaneous emission from O2(1Delta) and from O2(1Sigma) (excited by energy transfer from O/1D/) significantly decreases the amount of energy available for heat. Similarly, the efficiency at which solar ultraviolet radiation absorbed by O2 in the Schumann-Runge continuum is directly converted to heat in the lower thermosphere (95-110 km) is calculated. The O2 undergoes photolysis and the excited product O(1D) is generated. Spontaneous emission from O2(1Sigma) (excited by energy transfer from O/1D/) reduces the amount of energy available for heat in the lower thermosphere. The consideration of these energy transfer and loss processes results in significantly reduced heating rates as compared to those conventionally calculated in models of the middle atmosphere.
Mlynczak, Martin G.↗
Spectral-line structures of saturated parametric instabilities.
The nonlinear saturation spectrum of parametric instabilities is shown to be restricted to discrete values of the propagation vector if spontaneous emission is neglected and a one-dimensional analysis is used. The purely growing instability is not excited for equal ion and electron temperatures if the power is less than 3.5 times the threshold power. The inadequacy of the present one-dimensional treatment is pointed out, and it is shown that waves with propagation vectors that are not parallel to the pump field must be present even if spontaneous emission is neglected.
Kuo, Y.-Y.↗
Structure in the nonlinear saturation spectrum of parametric instabilities.
The nonlinear saturation spectrum of the decay instability is obtained in the limit of small spontaneous emission, for comparable ion and electron temperatures, from numerical solutions of a kinetic equation based on an accurate expression for the nonlinearity. The spectral energy occupies several pairs of isolated saucer-shaped regions in wave-vector space. The regions increase in thickness, angular diameter, and number as the pump power is increased. The theory thus predicts the generation of waves propagating in directions which can differ substantially from the direction of the pump field. Ionospheric observations confirm this prediction; they were difficult to reconcile with the predictions of previous theories based on an approximated expression for the nonlinearity. The present work also corrects the results of previous one-dimensional theories that used an accurate expression for the nonlinearity and predicted 'spectral lines' in the limit of vanishing spontaneous emission.
Fejer, J. A.↗
Spontaneous Radio Frequency Emissions from Natural Aurora
At high latitudes, suitably sensitive radio experiments tuned below 5 MHz detect up to three types of spontaneous radio emissions from the Earth s ionosphere. In recent years, ground-based and rocket-borne experiments have provided strong evidence for theoretical explanations of the generation mechanism of some of these emissions, but others remain unexplained. Achieving a thorough understanding of these ionospheric emissions, accessible to ground-based experiments, will not only bring a deeper understanding of Earth s radio environment and the interactions between waves and particles in the ionosphere but also shed light on similar spontaneous emissions occurring elsewhere in Earth s environment as well as other planetary and stellar atmospheres.
LaBelle, J.↗
Development of Novel Composite and Random Materials for Nonlinear Optics and Lasers
A qualitative model explaining sharp spectral peaks in emission of solid-state random laser materials with broad-band gain is proposed. The suggested mechanism of coherent emission relies on synchronization of phases in an ensemble of emitting centers, via time delays provided by a network of random scatterers, and amplification of spontaneous emission that supports the spontaneously organized coherent state. Laser-like emission from powders of solid-state luminophosphors, characterized by dramatic narrowing of the emission spectrum and shortening of emission pulses above the threshold, was first observed by Markushev et al. and further studied by a number of research groups. In particular, it has been shown that when the pumping energy significantly exceeds the threshold, one or several narrow emission lines can be observed in broad-band gain media with scatterers, such as films of ZnO nanoparticles, films of pi-conjugated polymers or infiltrated opals. The experimental features, commonly observed in various solid-state random laser materials characterized by different particle sizes, different values of the photon mean free path l*, different indexes of refraction, etc.. can be described as follows. (Liquid dye random lasers are not discussed here.)
Noginov, Mikhail↗
Collisional excitation of carbon monoxide in interstellar clouds.
Investigation of different models for the collisional excitation of carbon monoxide (CO) by solving the rate equations for the ten lowest energy levels, including stimulated emission and absorption by 3 K isotropic radiation, spontaneous emission, and collisions. The results are qualitatively applicable to other linear molecules. They show that a wide range of rotational excitation temperatures, including population inversions, can be produced by the various kinetic temperatures and particle densities which are likely to occur in the interstellar regions containing molecules.
Goldsmith, P. F.↗
Iodine monofluoride emission spectrum and formation kinetics in electron-beam-produced plasmas
The observation of intense blue-green spontaneous emission attributed to IF from electron-beam-excited Ar/CF3I/NF3 gas mixtures is reported. Intense emission from a structured band centered at a wavelength of 484 nm was observed when mixtures of 2000-4000 Torr AR (or He or Ne), 3 Torr CF3I and 1 Torr NF3 (or F2) were irradiated with a 3-nsec FWHM electron beam. Analysis of ICl and IBr spectra, which the present spectrum closely resembles, indicates that the 484-nm emission originates from the E to A 3 pi 1 transition of IF. Examination of the time dependence of metastable IF and I2 emission reveals that the IF (E) level is formed primarily by excitation transfer from metastable I(4P) states. The fluorescence efficiency of the E-A transition and the radiative lifetime of the metastable IF (E) state are estimated to be approximately 6% and 15 nsec, respectively, and it is suggested that metastable IF is an attractive candidate for a blue-green laser.
Hutchison, S. B.↗
Organic materials able to detect analytes
The present invention generally relates to polymers with lasing characteristics that allow the polymers to be useful in detecting analytes. In one aspect, the polymer, upon an interaction with an analyte, may exhibit a change in a lasing characteristic that can be determined in some fashion. For example, interaction of an analyte with the polymer may affect the ability of the polymer to reach an excited state that allows stimulated emission of photons to occur, which may be determined, thereby determining the analyte. In another aspect, the polymer, upon interaction with an analyte, may exhibit a change in stimulated emission that is at least 10 times greater with respect to a change in the spontaneous emission of the polymer upon interaction with the analyte. The polymer may be a conjugated polymer in some cases. In one set of embodiments, the polymer includes one or more hydrocarbon side chains, which may be parallel to the polymer backbone in some instances. In another set of embodiments, the polymer may include one or more pendant aromatic rings. In yet another set of embodiments, the polymer may be substantially encapsulated in a hydrocarbon. In still another set of embodiments, the polymer may be substantially resistant to photobleaching. In certain aspects, the polymer may be useful in the detection of explosive agents, such as 2,4,6-trinitrotoluene (TNT) and 2,4-dinitrotoluene (DNT).
Rose, Aimee↗
Transition probability of the Si III 189.2-nm intersystem line
Measurement of the lifetime of the metastable 3s3p(3)P(0)1 level of Si(2+) (Si III), which decays by photon emission at 189.2 nm to the 3s2(1)S0 state, is reported. The data were taken from spontaneous emission from metastable Si III stored in an RF ion trap. The Si III ions were produced through electron bombardment of SiH4 and SiF4 at pressures of 1/100,000,000-1/10,000,000 Torr. A photomultiplier was employed to count the photon emissions from the transitions. A total of 11 decay curves were generated for analysis, with Poisson statistics used to set the uncertainties at within 8 pct. Significant systematic effects were controlled, and the lifetime was found to be within 3.6 microsec of 59.9 microsec. The method used is concluded valid for determining the lifetimes of metastable levels of low-Z ions with low charge, and thereby the transition probabilities.
Kwong, H. S.↗
Appendix: Limits on the use of heterodyning and amplification in optical interferometry
The development of optical fibers, lasers, and mixers at optical frequencies has offered the hope that active methods can contribute to optical interferometry. Heterodyning, in particular, looks attractive, even though bandwidths are narrower than one would like at present; one might expect this limitation to lessen as technology develops. That expectation, unfortunately, is not likely to benefit interferometry at optical wavelengths because of the intervention of quantum mechanics and the second law of thermodynamics, as Burke (1985a) pointed out. So much 'second quantization' noise is generated that only at infrared frequencies, somewhere in the 10-100 micron range, can one look forward to heterodyning in any realistic sense. The reason is easily understood. Every amplifier, in the quantum limit, works by stimulated emission, even though this basic truth is not obvious at radio frequencies. This means that there must be spontaneous emission occurring within every amplifier, and Strandberg (1957) showed that this implied a limiting noise temperature, T sub N = h nu/k, for any amplifier. Burke (1969) used this result to demonstrate that, if it were not for this quantum noise, the VLBI method would allow one to tell which slit a photon went through before forming an interference pattern, thus violating basic tenants of quantum mechanics. In essence, the second quantization condition Delta N Delta phi greater than or = 1 saves one from paradox. One can state the conclusion simply: any amplifier produces approximately one photon per Hertz of bandwidth. In optical interferometry, one will certainly want bandwidth in the 10(exp 12) to 10(exp 14) Hz range, and that implies an intolerable cacophony of noise photons. Only at infrared frequencies can one tolerate the quantum noise, where the natural noise background may be high and the mixers are not as efficient as one would hope for. The crossover at present is about 10 or 20 microns, but the boundary will shift to longer wavelengths as noise performance improves. One might guess that ultimately a wavelength of about 100 microns will mark the limit of useful amplification and heterodyning in astronomical aperture synthesis interferometry.
Burke, Bernard F.↗