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NASA NTRS1985

Development of algorithms for using satellite meteorological data sets to study global transport of stratospheric aerosols and ozone

The utilization of stratospheric aerosol and ozone measurements obtained from the NASA developed SAM II and SAGE satellite instruments were investigated for their global scale transports. The stratospheric aerosols showed that during the stratospheric warming of the winter 1978 to 1979, the distribution of the zonal mean aerosol extinction ratio in the northern high latitude exhibited distinct changes. Dynamic processes might have played an important role in maintenance role in maintenance of this zonal mean distribution. As to the stratospheric ozone, large poleward ozone transports are shown to occur in the altitude region from 24 km to 38 km near 55N during this warming. This altitude region is shown to be a transition region of the phase relationship between ozone and temperature waves from an in-phase one above 38 km. It is shown that the ozone solar heating in the upper stratosphere might lead to enhancement of the damping rate of the planetary waves due to infrared radiation alone in agreement with theoretical analyses and an earlier observational study.

Want, P. H.↗
NASA NTRS1986

Wavelength dependence of aerosol extinction coefficient for stratospheric aerosols

A simple empirical formula for the wavelength dependence of the aerosol extinction coefficient is proposed. The relationship between the constants in the formula and the variable parameter in the aerosol size distribution is explicitly expressed. Good agreement is found between the extinction coefficients calculated from the proposed formula and that calculated from Mie theory. The proposed expression is shown to be better than the Angstroem formula commonly used by atmospheric scientists.

Yue, Glenn K.↗
NASA NTRS2024

CREST: a Climate Data Record of Stratospheric Aerosols

Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived using data from six limb and occultation satellite instruments: SAGE (Stratospheric Aerosol and Gas Experiment) II on ERBS (Earth Radiation Budget Satellite), GOMOS (Global Ozone Monitoring by Occultation of Stars) and SCIAMACHY (Scanning Imaging Spectrometer for Atmospheric Chartography) on Envisat, OSIRIS (Optical Spectrograph and InfraRed Imaging System) on Odin, OMPS (Ozone Monitor Profiling Suite Limb Profiler) on Suomi NPP, and SAGE III on the ISS (International Space Station). The merging of aerosol profiles is performed via the transformation of the aerosol datasets from individual satellite instruments to the same wavelength (750 nm) and their de-biasing and homogenization by adjusting the seasonal cycles. After such homogenization, the data from individual satellite instruments are in good agreement. The merged aerosol extinction coefficient is computed as the median of the adjusted data from the individual instruments. The merged time series of vertically resolved monthly mean aerosol extinction coefficients at 750 nm is provided in 10° latitudinal bins from 90° S to 90° N, in the altitude range from 8.5 to 39.5 km. The time series of the stratospheric aerosol optical depth (SAOD) is created via the integration of aerosol extinction profiles from the tropopause to 39.5 km; it is also provided as monthly mean data in 10° latitudinal bins. The created aerosol climate record covers the period from October 1984 until December 2023, and it is intended to be extended in the future. The merged CREST aerosol dataset (v2) is available at https://doi.org/10.57707/fmib2share.dfe14351fd8548bcaca3c2956b17f665 (Sofieva et al., 2024a). It can be used in various climate-related studies.

Viktoria F Sofieva↗
NASA NTRS1991

SAM 2 measurements of the polar stratospheric aerosol. Volume 9: October 1982 - April 1983

The Stratospheric Aerosol Measurement (SAM) II sensor aboard Nimbus 7 is providing 1.0 micron extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM II measurement are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction and stratospheric optical depth in the Arctic are unusually large due to the presence of material from the El Chichon volcano eruption in the Spring of 1982. For example, the optical depth peaked at 0.068, more than 50 times background values. Typical values of aerosol extinction and stratospheric optical depth in the Antarctic varied considerably during this period due to the transport and arrival of the material from the El Chichon eruption. For example, the stratospheric optical depth varied from 0.002 in October 1982, to 0.021 in January 1983. Polar stratospheric clouds were observed during the Arctic winter, as expected. A representative sample is provided of the ninth 6-month period of data to be used in atmospheric and climatic studies.

Mcmaster, L. R.↗
NASA NTRS1984

Analysis of upper stratospheric Umkehr ozone profile data for trends and the effects of stratospheric aerosols

The effect of stratospheric aerosols on Umkehr estimates of long-term ozone depletion associated with chlorofluoromethanes (CFMs) is considered in a statistical time series trend analysis. Time series models are estimated using monthly averages of Umkehr measurements made over the last 15 to 20 years. The time series regression models incorporate seasonal, trend and noise factors and an additional factor to account for the effects of atmospheric aerosols on the Umkehr measurements. The analysis indicates a statistically significant relation with atmospheric aerosol transmission in the Umkehr layers and implies that the relation is an important factor in any time series trend analysis of Umkehr data. Taking this relation into account, statistically significant negative trends were found in the Upper Umkehr layers. It is pointed out that upper stratospheric ozone could be sensitive to long-term solar variability as well as other possible influences in addition to CFM-induced effects, and therefore the cause or causes of the estimated trend cannot be unambiguously estimated using current Umkehr data.

Reinsel, G. C.↗
NASA NTRS2019

CALIPSO Level 3 Stratospheric Aerosol Product: Version 1.00 Algorithm Description and Initial Assessment

In August 2018,the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) project released a new level 3 stratospheric aerosol profile data product derived from nearly 12 years of measurements acquired by the space-borne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP).This monthly averaged, gridded level 3 product is based on version 4.2 of the CALIOP level 1 and level 2 data products, which feature significantly improved calibration that now makes it possible to reliably retrieve profiles of stratospheric aerosol extinction and backscatter coefficients. This paper describes the science algorithm and data handling techniques that were developed to generate the CALIPSO version 1.00 level 3 stratospheric aerosol profile product. Further, we show that the retrieved extinction profiles capture the major stratospheric perturbations over the last decade resulting from volcanic eruptions, extreme smoke events, and signatures of stratospheric dynamics. Initial assessment of the product by inter-comparison with the stratospheric aerosol retrievals from the Stratospheric Aerosol and Gas Experiment III (SAGE III) on the International Space Station (ISS) indicates good agreement in the tropical stratospheric aerosol layer (30oN-30oS),where the average difference between zonal mean extinction profiles is typically less than 25% between 20km and 30km. However, differences can exceed 100% in the very low aerosol loading regimes found above 25 km at higher latitudes.

Jayanta Kar↗
NASA NTRS1983

SAM 2 measurements of the polar stratospheric aerosol. Volume 3: October 1979 to April 1980

The Stratospheric Aerosol Measurement (SAM) II sensor is aboard the Earth-orbiting Nimbus 7 spacecraft providing extinction measurements of the Antarctic and Arctic stratospheric aerosol with a vertical resolution of 1 km. Representative examples and weekly averages of aerosol data and corresponding temperature profiles for the time and place of each SAM II measurement (Oct. 1979 through Apr. 1980) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted and weekly aerosol optical depths are calculated. Seasonal variations and variations in space (altitude and longitude) for both polar regions are easily seen. Typical values of aerosol extinction at the SAM II wavelength of 1.0 microns for this time period are 2 to 4 times .0001/km in the main stratospheric aerosol layer. Optical depths for the stratosphere are about 0.002 to 0.003, up slightly over normal background levels (due to the eruption of Sierra Negra, Nov. 1979). Polar stratospheric clouds at altitudes of about 22 km were observed during the Arctic winter. A ready-to-use format containing a representative sample of the third 6 months of data to be used in atmospheric and climatic studies is presented.

Mccormick, M. P.↗
NASA NTRS1982

SAM 2 Measurements of the Polar Stratospheric Aerosol, volume 2. April 1979 to October 1979

The Stratospheric Aerosol Measurement (SAM) II sensor is abroad the Earth orbiting Nimbus 7 spacecraft proving extinction measurements of the Antarctic and Arctic stratospheric aerosol with a vertical resolution of 1 km. Representative examples and weekly averages of aerosol data and corresponding temperature profiles for the time and place of each SAM II measurement (April 29, 1979, to October 27, 1979) is presented. Contours of aerosol extinction as a function of altitude and longitude or time were plotted and weekly aerosol optical depths were calculated. Seasonal variations and variations in space (altitude and longitude) for both polar regions are easily seen. Typical values of aerosol extinction at the SAM II wavelength of 1.0 micron for the time priod were 1 to 3 x 10 to the -4th power km -1 in the main stratospheric aerosol layer. Optical depths for the stratosphere were about 0.002. Polar stratospheric clouds at altitudes between the tropopause and 20 km were observed during the Antarctic winter at various times and locations. A ready-to-use format containing a representative sample of the second 6 months of data to be used in atmospheric and climatic studies is presented.

Mccormick, M. P.↗
NASA NTRS1989

Background stratospheric aerosol reference model

In this analysis, a reference background stratospheric aerosol optical model is developed based on the nearly global SAGE 1 satellite observations in the non-volcanic period from March 1979 to February 1980. Zonally averaged profiles of the 1.0 micron aerosol extinction for the tropics and the mid- and high-altitudes for both hemispheres are obtained and presented in graphical and tabulated form for the different seasons. In addition, analytic expressions for these seasonal global zonal means, as well as the yearly global mean, are determined according to a third order polynomial fit to the vertical profile data set. This proposed background stratospheric aerosol model can be useful in modeling studies of stratospheric aerosols and for simulations of atmospheric radiative transfer and radiance calculations in atmospheric remote sensing.

Mccormick, M. P.↗
NASA NTRS1985

Variations in stratospheric aerosol optical depth during northern warmings

In this paper, the properties of the stratospheric aerosol optical depth (above 50 mbar) have been studied by using aerosol extinction profiles (at 1 micron) derived from the Stratospheric Aerosol Measurement and Stratospheric Aerosol and Gas Experiment (SAGE) during warming periods in the Northern Hemisphere. It is shown that, during the disturbed periods in winter, low values of aerosol optical depth (less than 0.0002) are found within the low-pressure system(s) (at the 30-mbar pressure surface), while high values are found outside. Similar characteristics are found to exist for the simultaneously observed SAGE O3 and NO2 columnar density distributions. Strong longitudinal gradients are shown with the low values within and wherever the vortex exists. This characteristic is maintained during and after the circumpolar vortex is disturbed, even after breakdown, indicating an isolation of the material within the vortex.

Wang, P.-H.↗
NASA NTRS2015

Stratospheric Aerosol and Gas Experiment III on the International Space Station (SAGE III/ISS)

The Stratospheric Aerosol and Gas Experiment III on the International Space Station (SAGE III/ISS) mission will extend the SAGE data record from the ideal vantage point of the International Space Station (ISS). The ISS orbital inclination is ideal for SAGE measurements providing coverage between 70 deg north and 70 deg south latitude. The SAGE data record includes an extensively validated data set including aerosol optical depth data dating to the Stratospheric Aerosol Measurement (SAM) experiments in 1975 and 1978 and stratospheric ozone profile data dating to the Stratospheric Aerosol and Gas Experiment (SAGE) in 1979. These and subsequent data records, notably from the SAGE II experiment launched on the Earth Radiation Budget Satellite in 1984 and the SAGE III experiment launched on the Russian Meteor-3M satellite in 2001, have supported a robust, long-term assessment of key atmospheric constituents. These scientific measurements provide the basis for the analysis of five of the nine critical constituents (aerosols, ozone (O3), nitrogen dioxide (NO2), water vapor (H2O), and air density using O2) identified in the U.S. National Plan for Stratospheric Monitoring. SAGE III on ISS was originally scheduled to fly on the ISS in the same timeframe as the Meteor-3M mission, but was postponed due to delays in ISS construction. The project was re-established in 2009.

Gasbarre, Joseph↗
NASA NTRS2023

The Calipso Version 4.5 Stratospheric Aerosol Subtyping Algorithm

The accurate classification of aerosol types injected into the stratosphere is important to properly characterize their chemical and radiative impacts within the Earth climate system. The updated stratospheric aerosol subtyping algorithm used in the version 4.5 (V4.5) release of the Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) level 2 data products now delivers more comprehensive and accurate classifications than its predecessor. The original algorithm identified four aerosol subtypes for layers detected above the tropopause: volcanic ash, smoke, sulfate/other, and polar stratospheric aerosol (PSA). In the revised algorithm, sulfates are separately identified as a distinct, homogeneous subtype, and the diffuse, weakly scattering layers previously assigned to the sulfate/other class are recategorized as a fifth “unclassified” subtype. By making two structural changes to the algorithm and revising two thresholds, the V4.5 algorithm improves the ability to discriminate between volcanic ash and smoke from pyrocumulonimbus injections, improves the fidelity of the sulfate subtype, and more accurately reflects the uncertainties inherent in the classification process. The 532 nm lidar ratio for volcanic ash was also revised to a value more consistent with the current state of knowledge. This paper briefly reviews the previous version of the algorithm (V4.1 and V4.2) then fully details the rationale and impact of the V4.5 changes on subtype classification frequency for specific events where the dominant aerosol type is known based on the literature. Classification accuracy is best for volcanic ash due to its characteristically high depolarization ratio. Smoke layers in the stratosphere are also classified with reasonable accuracy, though during the daytime a substantial fraction are misclassified as ash. It is also possible for mixtures of ash and sulfate to be misclassified as smoke. The V4.5 sulfate subtype accuracy is less than that for ash or smoke, with sulfates being misclassified as smoke about one-third of the time. However, because exceptionally tenuous layers are now assigned to the unclassified subtype and the revised algorithm levies more stringent criteria for identifying an aerosol as sulfate, it is more likely that layers labeled as this subtype are in fact sulfate compared to those assigned the sulfate/other classification in the previous data release.

Jason L Tackett↗
NASA NTRS2012

Toward a Combined SAGE II-HALOE Aerosol Climatology: An Evaluation of HALOE Version 19 Stratospheric Aerosol Extinction Coefficient Observations

Herein, the Halogen Occultation Experiment (HALOE) aerosol extinction coefficient data is evaluated in the low aerosol loading period after 1996 as the first necessary step in a process that will eventually allow the production of a combined HALOE/SAGE II (Stratospheric Aerosol and Gas Experiment) aerosol climatology of derived aerosol products including surface area density. Based on these analyses, it is demonstrated that HALOE's 3.46 microns is of good quality above 19 km and suitable for scientific applications above that altitude. However, it is increasingly suspect at lower altitudes and should not be used below 17 km under any circumstances after 1996. The 3.40 microns is biased by about 10% throughout the lower stratosphere due to the failure to clear NO2 but otherwise appears to be a high quality product down to 15 km. The 2.45 and 5.26 micron aerosol extinction coefficient measurements are clearly biased and should not be used for scientific applications after the most intense parts of the Pinatubo period. Many of the issues in the aerosol data appear to be related to either the failure to clear some interfering gas species or doing so poorly. For instance, it is clear that the 3.40micronaerosol extinction coefficient measurements can be improved through the inclusion of an NO2 correction and could, in fact, end up as the highest quality overall HALOE aerosol extinction coefficient measurement. It also appears that the 2.45 and 5.26 micron channels may be improved by updating the Upper Atmosphere Pilot Database which is used as a resource for the removal of gas species otherwise not available from direct HALOE measurements. Finally, a simple model to demonstrate the promise of mixed visible/infrared aerosol extinction coefficient ensembles for the retrieval of bulk aerosol properties demonstrates that a combined HALOE/SAGE II aerosol climatology is feasible and may represent a substantial improvement over independently derived data sets.

Thomason, L. W.↗
NASA NTRS1985

SAM II measurements of the polar stratospheric aerosol. Volume 6: April to October 1981

The Stratospheric Aerosol Measurement (SAM) II sensor is aboard the Earth-orbiting Nimbus 7 spacecraft providing extinction measurements of the Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages of these aerosol data and corresponding temperature profiles (Apr. 1981 to Oct. 1981) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted and weekly aerosol optical depths are calculated. Stratospheric optical depths are 0.002 to 0.003 for the Antarctic region and 0.006 to 0.007 at the beginning to 0.003 to 0.004 at the end of the time period for the Arctic region. Polar stratospheric clouds at altitudes between the tropopause and 20 km were observed during the Antarctic winter. A ready-to-use format containing a representative sample of the sixth 6 months of data to be used in atmospheric and climatic studies is reported.

Mccormick, M. P.↗
NASA NTRS1993

Stratospheric Aerosol and Gas Experiment (SAGE 3)

The proposed SAGE III instrument would be the principal source of data for global changes of stratospheric aerosols, stratospheric water vapor, and ozone profiles, and a contributing source of data for upper tropospheric water vapor, aerosols, and clouds. The ability to obtain such data has been demonstrated by the predecessor instrument, SAGE II, but SAGE III will be substantially more capable, as discussed below. The capabilities for monitoring the profiles of atmospheric constituents have been verified in detail, including ground-based validations, for aerosol, ozone, and water vapor. Indeed, because of its self-calibrating characteristics, SAGE II was an essential component of the international ozone trend assessments, and SAGE II is now proving to be invaluable in tracking the aerosols from Mt. Pinatubo. Although SAGE profiles generally terminate at the height of the first tropospheric cloud layer, it has been found that the measurements extend down to 3 km altitude more than 40 percent of the time at most latitudes. Thus, useful information can also be obtained on upper tropospheric aerosols, water vapor, and ozone.

Mccormick, M. P.↗
NASA NTRS2007

CALIPSO Observations of Stratospheric Aerosols: A Preliminary Assessment

We have examined the 532-nm aerosol backscatter coefficient measurements by the Cloud- Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) for their use in the observation of stratospheric aerosol. CALIPSO makes observations that span from 82 S to 82 N each day and, for each profile, backscatter coefficient values reported up to approx. 40 km. The possibility of using CALIPSO for stratospheric aerosol observations is demonstrated by the clear observation of the 20 May 2006 eruption of Montserrat in the earliest CALIPSO data in early June as well as by observations showing the 7 October 2006 eruption of Tavurvur (Rabaul). However, the very low aerosol loading within the stratosphere makes routine observations of the stratospheric aerosol far more difficult than relatively dense volcanic plumes. Nonetheless, we found that averaging a complete days worth of nighttime only data into 5-deg latitude by 1-km vertical bins reveals a stratospheric aerosol data centered near an altitude of 20 km, the clean wintertime polar vortices, and a small maximum in the lower tropical stratosphere. However, the derived values are clearly too small and often negative in much of the stratosphere. The data can be significantly improved by increasing the measured backscatter (molecular and aerosol) by approximately 5% suggesting that the current method of calibrating to a pure molecular atmosphere at 30 km is most likely the source of the low values.

Thomason, Larry W.↗
NASA NTRS1988

The relationship of satellite-inferred stratospheric aerosol extinction to the position of the 50-mb north polar jet stream

The relationship between stratospheric aerosols and the location of the north polar night stratospheric jet stream was investigated for selected periods of four successive winters (1979-1982), using measurements from SAM II (Stratospheric Aerosol Measurement II) and SAGE I (Stratospheric Aerosol and Gas Experiment I) satellite-borne sun photometers and corresponding meteorological observations. Each period investigated included a polar stratospheric warming during which major dynamic meteorological changes are known to have perturbed the structure of the polar vortex. The analysis of variations in aerosol extinction mixing ratio patterns among winters and during major stratospheric warming events within separate winters showed a well-defined positive gradient in extinction mixing ratio and temperature across the jet stream from the cyclonic side to the anticyclonic side at altitudes between 20 and 30 km during each winter period. Estimates of extinction mixing ratio profiles measured near the center of the polar vortex suggest that a gradual subsidence took place within the polar vortex during at least three of the four winter periods.

Livingston, John M.↗