Field emission mitigation studies in the SLAC Linac Coherent Light Source II superconducting rf cavities via in situ plasma processing
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aExperiments were performed at The Fermilab Accelerator Science and Technology (FAST) facility to elucidate the effects of short-range wakefields (SRWs) in TESLA-type rf cavities. FAST has a unique configuration of a photocathode rf gun beam injecting two TESLA-type single cavities (CC1 and CC2) in series prior to the cryomodule. To investigate short-range wakefield effects, we have steered the beam to minimize the signals in the higher-order mode (HOM) detectors of CC1 and CC2 for a baseline, and then selected a vertical corrector to steer the beam off axis at an angle into CC1 or CC2. A Hamamatsu synchro-scan streak camera viewing a downstream OTR screen provided an image of y-t effects within the micropulses with ~10-micron spatial resolution and 2-ps temporal resolution. At 500 pC/b, 50 b, and 2 mrad off-axis steering into CC2, we observed an ~ 100-micron head-tail centroid shift in the streak camera image y(t)-profiles. This centroid shift value is consistent wit h a calculated short-range wakefield effect using ASTRA simulations.
Experiments were performed at The Fermilab Accelerator Science and Technology (FAST) facility to elucidate the effects of short-range wakefields (SRWs) in TESLA-type rf cavities. FAST has a unique configuration of a photocathode rf gun beam injecting two TESLA-type single cavities (CC1 and CC2) in series prior to the cryomodule. To investigate short-range wakefield effects, we have steered the beam to minimize the signals in the higher-order mode (HOM) detectors of CC1 and CC2 for a baseline, and then used a vertical corrector between the two cavities to steer the beam off axis at an angle into CC2. A Hamamatsu synchroscan streak camera viewing a downstream OTR screen provided an image of y-t effects within the micropulses with ~10-micron spatial resolution and 2-ps temporal resolution. At 500 pC/b, 50 b, and 4 mrad off-axis steering into CC2, we observed an ~ 100-micron head-tail centroid shift in the streak camera image y(t)-profiles. This centroid shift value is 5 times l arger than the observed HOM-driven centroid oscillation within the macropulse, and it is consistent with a calculated short-range wakefield effect using ASTRA simulations.
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In this DOE-funded project DE-SC0010081-020 Old Dominion University (ODU) in collaboration with University of Wisconsin (UW) and Jefferson Laboratory have investigated both experimentally and theoretically electromagnetic response and losses in multilayered superconducting structures made of new SRF materials which can push the field and Q performance limits of accelerating cavities.
Superconducting radio-frequency (SRF) cavities, usually manufactured from Niobium (Nb), are vital components of modern particle accelerators because of their ability to achieve high acceleration gradients with little power dissipation. Naturally forming Nb surface oxides significantly alter cavity performance by changing surface resistance. A nondestructive characterization of oxide thickness is helpful for relating surface processing treatments to cavity performance. This work develops a protocol to measure Nb oxide thickness using Angle-Resolved X-ray Photoelectron Spectroscopy (ARXPS) while correcting instrumental errors. Using uniform bulk standard samples (Silver, Aluminum oxide, and Germanium), we determined a baseline correction factor to account for analyzer-related intensity evolution as the measurement angle increases. The correction factor was then applied to Nb 3d ARXPS data. Applying the Strohmeier equation to the corrected data yielded a Nb2O5 thickness of 6.04 nm, closely matching the 5.5 (±.05) nm value obtained from cross-sectional transmission electron microscopy. Our approach will bring a method to incorporate inherent errors in the thickness measurements using ARXPS and can be broadly applied to improve the accuracy of thickness measurements in a wide range of heterostructures.
Superconducting radio-frequency (SRF) cavities, usually manufactured from Niobium (Nb), are vital components of modern particle accelerators because of their ability to achieve high acceleration gradients with little power dissipation. Naturally forming Nb surface oxides significantly alter cavity performance by changing surface resistance. A nondestructive characterization of oxide thickness is helpful for relating surface processing treatments to cavity performance. This work develops a protocol to measure Nb oxide thickness using Angle-Resolved X-ray Photoelectron Spectroscopy (ARXPS) while correcting instrumental errors. Using uniform bulk standard samples (Silver, Aluminum oxide, and Germanium), we determined a baseline correction factor to account for analyzer-related intensity evolution as the measurement angle increases. The correction factor was then applied to Nb 3d ARXPS data. Applying the Strohmeier equation to the corrected data yielded a Nb2O5 thickness of 6.04 nm, closely matching the 5.5 (±.05) nm value obtained from cross-sectional transmission electron microscopy. Our approach will bring a method to incorporate inherent errors in the thickness measurements using ARXPS and can be broadly applied to improve the accuracy of thickness measurements in a wide range of heterostructures.
We report radio-frequency measurements of quality factors and temperature mapping of a nitrogen doped Nb superconducting RF cavity. Cavity cutouts of hot and cold spots were studied with low temperature scanning tunneling microscopy and spectroscopy, X-ray photoelectron spectroscopy and secondary electron microscopy. Temperature mapping revealed a substantial reduction of the residual resistance upon cooling the cavity with a greater temperature gradient and hysteretic losses at the quench location, pointing to trapped vortices as the dominant source of residual surface resistance. Analysis of the tunneling spectra in the framework of a proximity effect theory shows that hot spots have a reduced pair potential and a wider distribution of the contact resistance between the Nb and the top Nb oxide. Alone, these degraded superconducting properties account for a much weaker excess dissipation as compared with the vortex contribution. Based on the correlation between the quasiparticle density of states and temperature mapping, we suggest that degraded superconducting properties may facilitate vortex nucleation or settling of trapped flux during cooling the cavity through the critical temperature.
Heterodyne detection using microwave cavities is a promising method for detecting high-frequency gravitational waves (GWs) or ultralight axion dark matter. In this work, we report on studies conducted on a spherical 2-cell cavity developed by the MAGO collaboration for high-frequency GWs detection. Although fabricated around 20 years ago, the cavity had not been used since. Due to deviations from the nominal geometry, we conducted a mechanical survey and performed room-temperature plastic tuning. Measurements and simulations of the mechanical resonances and electromagnetic properties were carried out, as these are critical for estimating the cavity’s GW coupling potential. Based on these results, we plan further studies in a cryogenic environment. The cavity characterisation does not only provide valuable experience for a planned physics run but also informs the future development of improved cavity designs.
Abstract Workbench-size particle accelerators, enabled by Nb 3 Sn-based superconducting radio-frequency (SRF) cavities, hold the potential of driving scientific discovery by offering a widely accessible and affordable source of high-energy electrons and x-rays. Thin-film Nb 3 Sn RF superconductors with high quality factors, high operation temperatures, and high-field potentials are critical for these devices. However, surface roughness, non-stoichiometry, and impurities in Nb 3 Sn deposited by conventional Sn-vapor diffusion prevent them from reaching their theoretical capabilities. Here we demonstrate a seed-free electrochemical synthesis that pushes the limit of chemical and physical properties in Nb 3 Sn. Utilization of electrochemical Sn pre-deposits reduces the roughness of converted Nb 3 Sn by five times compared to typical vapor-diffused Nb 3 Sn. Quantitative mappings using chemical and atomic probes confirm improved stoichiometry and minimized impurity concentrations in electrochemically synthesized Nb 3 Sn. We have successfully applied this Nb 3 Sn to the large-scale 1.3 GHz SRF cavity and demonstrated ultra-low BCS surface resistances at multiple operation temperatures, notably lower than vapor-diffused cavities. Our smooth, homogeneous, high-purity Nb 3 Sn provides the route toward high efficiency and high fields for SRF applications under helium-free cryogenic operations.
Surface preparation of niobium superconducting RF cavities is a critical step for achieving good RF performance under the superconducting state. Surface defect, roughness, and contamination affect the accelerating gradient and quality factor of the cavities. We report surface inspection methods used to control the surface processing of 650 MHz cavities designated for the pre-production and prototype cryomodules for PIP-II linac. The cavity surface was routinely inspected visually, with an optical camera, and by microscopic scanning of surface replicas. This article covers details on the surface inspection methods and surface polishing process used to repair the surface.
Electropolishing (EP) is the premier surface preparation method for high-Q, high-gradient superconducting RF cavities made of Nb. This leaves behind an apparently smooth surface, yet the achievable peak magnetic fields fall well below the superheating field of Nb, in most cases. In this work, the ultimate surface finish of EP was investigated by studying its effect on highly polished Nb samples. EP introduces high slope angle sloped-steps at grain boundaries. The magnetic field enhancement and superheating field suppression factors associated with such a geometry are calculated in the London theory. Despite the by-eye smoothness of electropolished Nb, such defects compromise the stability of the low-loss Meissner state, likely limiting the achievable peak accelerating fields in superconducting RF cavities. Finally, the impact of surface roughness on impurity diffusion is investigated which can link surface roughness to the effectiveness of heat treatments like low-temperature baking or nitrogen infusion in the vortex nucleation or hydride hypotheses. Surface roughness tends to decrease the effective dose of impurities as a result of the expansion of impurities into regions with greater internal angle. The effective dose of impurities can be protected by minimizing slope angles and step heights, ensuring uniformity.
Electropolishing (EP) is the premier surface preparation method for high-Q, high-gradient superconducting RF cavities made of Nb. This leaves behind an apparently smooth surface, yet the achievable peak magnetic fields fall well below the superheating field of Nb, in most cases. Here, in this work, the ultimate surface finish of EP was investigated by studying its effect on highly polished Nb samples. EP introduces high slope angle sloped-steps at grain boundaries. The magnetic field enhancement and superheating field suppression factors associated with such a geometry are calculated in the London theory. Despite the by-eye smoothness of electropolished Nb, such defects compromise the stability of the low-loss Meissner state, likely limiting the achievable peak accelerating fields in superconducting RF cavities. Finally, the impact of surface roughness on impurity diffusion is investigated which can link surface roughness to the effectiveness of heat treatments like low-temperature baking or nitrogen infusion in the vortex nucleation or hydride hypotheses. Surface roughness tends to decrease the effective dose of impurities as a result of the expansion of impurities into regions with greater internal angle. The effective dose of impurities can be protected by minimizing slope angles and step heights, ensuring uniformity.
Electropolishing (EP) of 1.3 GHz niobium (Nb) superconducting RF cavities is conducted to achieve a desired smooth and contaminant-free surface that yields good RF performance. Achieving a smooth surface of a large-sized elliptical cavity with the standard EP conditions was found to be challenging. This work aimed to conduct a systematic parametric EP study to understand the effects of various EP parameters on the surface of 650 MHz cavities used in PIP-II linac. Parameters optimized in this study provided a smooth surface of the cavities. The electropolished cavities met the baseline requirement of field gradient and qualified for further surface treatment to improve the cavity quality factor.
Higher-order modes (HOMs) in superconducting rf cavities present problems for an electron bunch traversing the cavity in the form of long-range wakefields from previous bunches. These may dilute the emittance of the macropulse average, especially with low emittance beams at facilities such as the European X-ray Free-electron Laser (XFEL) and the upgraded Linac Coherent Light Source (LCLS-II). Here we present observations of HOMs driven by the beam at the Fermilab Accelerator Science and Technology (FAST) facility. The FAST facility features two independent TESLA-type cavities (CC1 and CC2) after a photocathode rf gun followed by an 8-cavity cryomodule. The HOM signals were acquired from cavities using bandpass filters of 1.75 ± 0.15 GHz, 2.5 ± 0.2 GHz, and 3.25 ± 0.2 GHz and recorded using an 8-GHz, 20 GSa/s oscilloscope. The frequency resolution obtained is sufficient to separate polarization components of many of the HOMs. These HOM signals were captured from CC1 and cavities 1 and 8 of the cryomodule for various initial trajectories through the cavities, and we observe correlations between trajectory, HOM signals, and which polarization component of a mode is affected.
High-efficiency, high-velocity, sub-GHz elliptical superconducting RF cavities are a critical enabling technology for multiple upcoming accelerator development projects such as for the Powerful Energy Recovery Linac for Experiments (PERLE), and for the Future Circular Collider s (FCC) Booster, and future realizations of its Collider ring. The ambitious quality factor and gradient requirements of these applications require strong SRF R&D programs aimed at developing and optimizing advanced surface processing techniques for 800 MHz cavities. We report the initiation of the 800 MHz R&D program at Fermilab, with the aim of developing high-performance cavities compatible with PERLE and FCC applications.