An Algorithm for Hyperspectral Remote Sensing of Aerosols: 3. Application to the GEO-TASO Data in KORUS-AQ Field Campaign
This paper describes the third part of a series of investigations to develop algorithms for simultaneous retrieval of aerosol parameters and surface spectral reflectance from the data measured by GEOstationary Trace gas and Aerosol Sensor Optimization (GEO-TASO) instrument. Since the algorithm is designed for future hyperspectral and geostationary satellite sensors, such as Tropospheric Emissions: Monitoring of Pollution (TEMPO), it is applied to GEO-TASO data measured over the same area by different flights as part of the Korea-United Stated Air Quality Study (KORUS-AQ) field campaign in 2016. While GEO-TAOS has a spectral sampling interval of ~0.28 nm in the visible, its data is thinned through a band selection approach with consideration of atmospheric transmittance and different surface types, which yields 20 common spectral bands to be used by the algorithm. The algorithm starts with 4 common principal components (PCs) for surface spectral reflectance extracted from various spectral libraries, and the constraints of surface reflectance parameters and aerosol scattering models respectively from k- means clustering analysis of the Rayleigh-corrected GEO-TASO spectra and AERONET data. The algorithm then proceeds iteratively with an optimal estimation approach to update PCs and retrieve aerosol optical depth (AOD) until the best match between simulated and GEOS-TASO measured spectra is achieved. The spectral AODs are compared between those retrieved from GEO-TASO (x) and 7 AERONETS (y) in 440, 550, 550, 675 nm, respectively. The comparison reveals that iterative updates of surface spectral PCs (and so surface reflectance) yield significant enhancement in AOD retrievals, improving the mean linear fitting equations from y = 0.735x + 0.088 (without update of PCs) to y = 1.055x+ 0.01, and the Pearson correlation coefficient (𝑅𝑅2) from 0.54 to 0.76, respectively. Move case studies are need to further evaluate the algorithm for its application to TEMPO that carries a enhanced version of GEO-TASO instrument.