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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 361 records · Page 20
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DOE OSTI2023

Uncertainty quantification of transition operators in the empirical shell model

While empirical shell model calculations have successfully described low-lying nuclear data for decades, only recently has significant effort been made to quantify the uncertainty in such calculations. Here, in this study, we quantify the statistical error in effective parameters for transition operators in empirical calculations in the sd (1s 1/2 -0d 3/2 -0d 5/2 ) valence space, specifically the quenching of Gamow-Teller transitions, effective charges for electric quadrupole (E2) transitions, and the effective orbital and spin couplings for magnetic dipole (M1) transitions and moments. We find the quenching factor for Gamow-Teller transitions relative to free-space values is tightly constrained. For effective M1 couplings, we found isoscalar components more constrained than isovector. This detailed quantification of uncertainties, while highly empirical, nonetheless is an important step towards interpretation of experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

First simultaneous measurement of the γ-ray and neutron emission probabilities in inverse kinematics at a heavy-ion storage ring

The probabilities for γ-ray and particle emission as a function of the excitation energy of a decaying nucleus are valuable observables for constraining the ingredients of the models that describe the deexcitation of nuclei near the particle emission threshold. These models are essential in nuclear astrophysics and applications. In this paper, we have for the first time simultaneously measured the γ-ray and neutron emission probabilities of 208 Pb. The measurement was performed in inverse kinematics at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, where a 208 Pb beam interacted through the 208 Pb (p,p') reaction with a hydrogen gas jet target. Instead of detecting the γ rays and neutrons emitted by 208 Pb, we detected the heavy beamlike residues produced after γ and neutron emission. These heavy residues were fully separated by a dipole magnet of the ESR and were detected with outstanding efficiencies. The comparison of the measured probabilities with model calculations has allowed us to test and select different descriptions of the γ-ray strength function and the nuclear level density available in the literature.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

First determination of ground state electromagnetic moments of Fe 53

Here, the hyperfine coupling constants of neutron deficient 53 Fe were deduced from the atomic hyperfine spectrum measured using the bunched-beam collinear laser spectroscopy technique. The low-energy 53 Fe beam was produced by projectile-fragmentation reactions followed by gas stopping, and used for the first time for laser spectroscopy. Ground state magnetic-dipole and electric-quadrupole moments were determined as μ= –0.65(1)μ N and Q=+35(15)e 2 fm 2 , respectively. The multiconfiguration Dirac-Fock method was used to calculate the electric field gradient to deduce Q from the quadrupole hyperfine coupling constant, since the quadrupole coupling constant has not been determined for any Fe isotopes. Both experimental values agree well with nuclear shell model calculations using the GXPF1A effective interaction performed in a full fp shell model space, which support the soft nature of the 56 Ni nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Prompt and delayed spectroscopy of At 203 : Observation of a shears band and a 29 / 2 + isomeric state

Using fusion-evaporation reactions, a gas-filled recoil separator, recoil-gating technique and recoil-isomer decay tagging technique we have extended the level scheme of 203 At(N=118) significantly. We have observed an isomeric [τ=14.1(3)μs] state with a spin and parity of 29/2 + . The isomeric state is suggested to originate from the π(h 9/2 )Ⓧ|| 202 Po;11 – > coupling, and it is depopulated through 286 keV E 2 and 366 keV E 3 transitions. Additionally, we have observed a cascade of magnetic-dipole transitions which is suggested to be generated by the shears mechanism.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Effective operators in two-nucleon systems

Effective Hamiltonians and effective electroweak operators are calculated with the Okubo-Lee-Suzuki formalism for two-nucleon systems. Working within a harmonic oscillator basis, first without and then with a confining harmonic oscillator trap, we demonstrate the effects of renormalization on observables calculated for truncated basis spaces. We illustrate the renormalization effects for the root-mean-square point-proton radius, electric quadrupole moment, magnetic dipole moment, Gamow-Teller transition and neutrinoless double-beta decay operator using nucleon-nucleon interactions from chiral Effective Field Theory. Renormalization effects tend to be larger in the weaker traps and smaller basis spaces suggesting applications to heavier nuclei with transitions dominated by weakly-bound nucleons would be subject to more significant renormalization effects within achievable basis spaces.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2019

Transition form factors: γ * + p → Δ ( 1232 ) , Δ ( 1600 )

We report that electroproduction form factors describing the γ * p → Δ + ( 1232 ) , Δ + ( 1600 ) transitions are computed using a fully dynamical diquark-quark approximation to the Poincaré-covariant three-body bound-state problem in relativistic quantum field theory. In this approach, the Δ ( 1600 ) is an analogue of the Roper resonance in the nucleon sector, appearing as the simplest radial excitation of the Δ ( 1232 ) . Precise measurements of the γ * p → Δ + ( 1232 ) transition already exist on 0 ≤ Q 2 ≲ 8 GeV 2 , and the calculated results compare favorably with the data outside the meson-cloud domain. The predictions for the γ * p → Δ + ( 1600 ) magnetic dipole and electric quadrupole transition form factors are consistent with the empirical values at the real photon point, and extend to Q 2 ≈ 6 m p 2 , enabling a meaningful direct comparison with experiment once analysis of existing data is completed. In both cases, the electric quadrupole form factor is particularly sensitive to deformation of the Δ -baryons. Interestingly, while the γ * p → Δ + ( 1232 ) transition form factors are larger in magnitude than those for γ * p → Δ + ( 1600 ) in some neighborhood of the real photon point, this ordering is reversed on Q 2 ≳ 2 m p 2 , suggesting that the γ * p → Δ + ( 1600 ) transition is more localized in configuration space.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Role of Chiral Two-Body Currents in 6 Li Magnetic Properties in Light of a New Precision Measurement with the Relative Self-Absorption Technique

A direct measurement of the decay width of the excited $0^+_1$ state of 6 Li using the relative self-absorption technique is reported. Our value of $Γ_{γ,0^{+}_{1}} → 1^{+}_{1}$ = 8.17 (14) stat. (11) syst. eV provides sufficiently low experimental uncertainties to test modern theories of nuclear forces. The corresponding transition rate is compared to the results of ab initio calculations based on chiral effective field theory that take into account contributions to the magnetic dipole operator beyond leading order. This allows for a precision test of the impact of two-body currents that enter at next-to-leading order.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Ab Initio Prediction of the 4 $\mathrm{H}$e($d, γ$) 6 $\mathrm{L}$i Big Bang Radiative Capture

We report the rate at which helium ( 4 He ) and deuterium (d) fuse together to produce lithium-6 ( 6 Li) and a γ ray, 4 $\mathrm{H}$e($d, γ$) 6 $\mathrm{L}$i, is a critical puzzle piece in resolving the discrepancy between big bang predictions and astronomical observations for the primordial abundance of 6 Li . The accurate determination of this radiative capture rate requires the quantitative and predictive description of the fusion probability across the big bang energy window (30 keV ≲ E ≲ 400 keV), where measurements are hindered by low counting rates. We present first-principle (or, ab initio) predictions of the 4 $\mathrm{H}$e($d, γ$) 6 $\mathrm{L}$i astrophysical S factor using validated nucleon-nucleon and three-nucleon interactions derived within the framework of chiral effective field theory. By employing the ab initio no-core shell model with continuum to describe 4 He-d scattering dynamics and bound 6 Li product on an equal footing, we accurately and consistently determine the contributions of the main electromagnetic transitions driving the radiative capture process. Our results reveal an enhancement of the capture probability below 100 keV owing to previously neglected magnetic dipole (M1) transitions and reduce by an average factor of 7 the uncertainty of the thermonuclear capture rate between 0.002 and 2 GK.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Effects of Rolling Reduction on Critical Current Density and Microstructure of Bi-2212 Wires

Bi-2212 Rutherford cables have been fabricated into flat racetrack coils and canted-cosine-theta dipole magnets. The performance gap between the magnets made with Rutherford cables and the “short-sample-limit” is about 30%. To better understand the influence of Rutherford cable processing on the strand performance, we studied three Bi-2212 wires with filament architectures of 37 × 18 and 55 × 18 and diameters of 0.8 and 1.0 mm. To simulate the deformation caused by cabling process, the three wires were rolled with thickness reductions ranging from 10% to 30%. The aspect ratios of rolled strands are between 1.29 and 2.05. The low aspect-ratio wire is also an interesting form for fabricating solenoid coils with higher packing density. The round and rolled strands were heat-treated under 50 bar and with maximum heat treatment temperatures of 885.5 °C and 890.5 °C. The rolling deformation reduced filament size uniformity, resulting in filament merging in fully heat-treated wires. It was found that rolling reduction reduced wire critical current density (JE) by 16 to 18%, but the JE decrease saturated at 15 to 20% of the thickness reduction. It is believed that the reduced JE results from the filament merging caused by rolling and non-uniform shrinking during overpressure heat treatment.

Bi-2212 wire↗
DOE OSTI2020

Special Issue: To Commemorate the Legacy of Malcolm J. Andrews—Scientist, Educator, and Leader

This special issue celebrates the scientific legacy of Dr. Malcolm J. Andrews, former Editor of the ASME Journal of Fluids Engineering (2010–2018). Malcolm devoted his career to the development and applications of computational, experimental, and analytical tools to investigate and solve diverse, complex fluid dynamics, and heat transfer problems. Malcolm’s most notable research accomplishments include: (i) contributions to innovative experiments, simulations, and theory to understand buoyancydriven turbulent mixing due to Rayleigh–Taylor instability; (ii) development of the multiphase particle-in-cell method for understanding fragmentation in spray jets, coal-water slurry, and other dense particulate flows; (iii) mixing in nano- and biomaterials in applications ranging from protein glues to carbon nanotube composites; (iv) determining dispersion in proteins to improve therapeutic drug delivery via micro-encapsulation; (v) innovative methods for storing information using nanopinned dipole magnetic vortices in superconducting materials; and (vi) modeling and design modifications for shell-and-tube heat exchangers, as well as heat transfer in rotating systems such as turbine blades. The results of his research have been published in a long series of trend-setting journal and conference papers, book chapters, and patents.

42 ENGINEERING↗
DOE OSTI2020

When the Moon had a magnetosphere

Apollo lunar samples reveal that the Moon generated its own global magnetosphere, lasting from ~4.25 to ~2.5 billion years (Ga) ago. At peak lunar magnetic intensity (4 Ga ago), the Moon was volcanically active, likely generating a very tenuous atmosphere, and, it is believed, was at a geocentric distance of ~18 Earth radii (R E ). Solar storms strip a planet’s atmosphere over time, and only a strong magnetosphere would be able to provide maximum protection. We present simplified magnetic dipole field modeling confined within a paraboloidal-shaped magnetopause to show how the expected Earth-Moon coupled magnetospheres provide a substantial buffer from the expected intense solar wind, reducing Earth’s atmospheric loss to space.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

CEPC booster design study

In September 2012, Chinese scientists proposed a Circular Electron Positron Collider (CEPC) in China at 240 GeV center-of-mass energy for Higgs studies. The booster provides 120 GeV electron and positron beams to the CEPC collider for top-up injection at 0.1 Hz. The design of the full energy booster ring of the CEPC is a challenge. The ejected beam energy is 120 GeV and the injected beam energy is 6 GeV. Here in this paper we describe two alternative schemes, the wiggler bend scheme and the normal bend scheme. For the wiggler bend scheme, we propose to operate the booster ring as a large wiggler at low energy and as a normal ring at high energy to avoid the problem of very low dipole magnet fields. Finally, for the normal bend scheme, we implement the orbit correction to correct the earth field.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2019

Hysteresis in the spontaneous emission induced by VO 2 phase change

We investigate the spontaneous emission of a two-level quantum emitter in the vicinity of a vanadium dioxide (VO 2 ) thin film. By taking advantage of effective medium techniques to describe the dielectric constant of the VO 2 , we demonstrate that, in the near-field regime, the spontaneous emission rate of both electric and magnetic dipole emitters can be maximized at the insulator-to-metal phase transition temperature of the film. We find that VO 2 ’s thermal hysteresis curve produces clear fingerprints in the emitter’s decay process, offering a new degree of freedom to dynamically control light emission at the nanoscale. We also find that the spontaneous emission rate is a non-monotonic function of the emitter transition wavelength, presenting a pronounced peak at infrared frequencies. Altogether, our results reveal that VO 2 phase transition is a promising mechanism to achieve on-demand tuning of an emitter’s lifetime.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Experimental realization of a terahertz all-dielectric metasurface absorber

Metamaterial absorbers consisting of metal, metal-dielectric, or dielectric materials have been realized across much of the electromagnetic spectrum and have demonstrated novel properties and applications. However, most absorbers utilize metals and thus are limited in applicability due to their low melting point, high Ohmic loss and high thermal conductivity. Other approaches rely on large dielectric structures and / or a supporting dielectric substrate as a loss mechanism, thereby realizing large absorption volumes. Here we present a terahertz (THz) all dielectric metasurface absorber based on hybrid dielectric waveguide resonances. We tune the metasurface geometry in order to overlap electric and magnetic dipole resonances at the same frequency, thus achieving an experimental absorption of 97.5%. A simulated dielectric metasurface achieves a total absorption coefficient enhancement factor of F T =140, with a small absorption volume. Our experimental results are well described by theory and simulations and not limited to the THz range, but may be extended to microwave, infrared and optical frequencies. In conclusion, the concept of an all-dielectric metasurface absorber offers a new route for control of the emission and absorption of electromagnetic radiation from surfaces with potential applications in energy harvesting, imaging, and sensing.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Plasmonic nanoarcs: a versatile platform with tunable localized surface plasmon resonances in octave intervals

The tunability of the longitudinal localized surface plasmon resonances (LSPRs) of metallic nanoarcs is demonstrated with key relationships identified between geometric parameters of the arcs and their resonances in the infrared. The wavelength of the LSPRs is tuned by the mid-arc length of the nanoarc. The ratio between the attenuation of the fundamental and second order LSPRs is governed by the nanoarc central angle. Beneficial for plasmonic enhancement of harmonic generation, these two resonances can be tuned independently to obtain octave intervals through the design of a non-uniform arc-width profile. Because the character of the fundamental LSPR mode in nanoarcs combines an electric and a magnetic dipole, plasmonic nanoarcs with tunable resonances can serve as versatile building blocks for chiroptical and nonlinear optical devices.

42 ENGINEERING↗
DOE OSTI2023

Highly luminescent ultra-thin films with rare earth for plasmonic applications

Amphiphilic complexes with luminescent rare earth metal ions suitable for Lanmuir-Blodgett (LB) deposition have been synthesized. LB monolayers with closely packed Eu complexes deposited directly on silver demonstrate significant far-field emission in contrast to the theoretical predictions of full quenching. Angular radiation and polarization patterns of the electric and magnetic dipole emission of Eu 3+ point to a high excitation efficiency of surface plasmon polaritons. Different luminescent behavior of closely packed emitters in comparison to diluted systems is tentatively attributed to the collective state of emitters in LB layers formed via near-field coupling with surface plasmons.

Munga, J.↗
DOE OSTI2025

New amphiphilic complexes with luminescent rare-earth ions

Organic compounds containing luminous rare-earth ions are of interest for numerous nanophotonic and plasmonic applications, including nanoscale lasers, biosensors, and optical magnetism studies. Optical studies of Eu 3+ complexes revealed that ultra-thin LB monolayers are highly luminescent even when deposited directly on plasmonic metal, which makes these materials very promising for plasmonic applications and studies, including control and enhancement of magnetic dipole emission with a plasmonic environment. In this work, we synthesize amphiphilic complexes with various rare-earth ions Nd 3+ , Yb 3+ , and DPT ligands and show that they all are suitable for monolayer or multilayer deposition with the Langmuir–Blodgett (LB) technique. Graphical abstract

36 MATERIALS SCIENCE↗