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DOE OSTI2021

Optical and Electronic Losses Arising from Physically Mixed Interfacial Layers in Perovskite Solar Cells

Perovskite solar cell device performance is affected by optical and electronic losses. To minimize these losses in solar cells, it is important to identify their sources. Here, we report the optical and electronic losses arising from physically mixed interfacial layers between the adjacent component materials in highly efficient two terminal (2T) all-perovskite tandem, single junction wide-bandgap, and single junction narrow-bandgap perovskite-based solar cells. Physically mixed interfacial layers as the sources of optical and electronic losses are identified from spectroscopic ellipsometry measurements and data analysis followed by comparisons of simulated and measured external quantum efficiency spectra. Parasitic absorbance in the physically mixed regions between silver metal electrical contacts and electron transport layers (ETLs) near the back contact and a physical mixture of commercial indium tin oxide and hole transport layers (HTL) near the front electrical contact lead to substantial optical loss. Here, a lower-density void + perovskite nucleation layer formed during perovskite deposition at the interface between the perovskite absorber layer and the HTL causes electronic losses due to incomplete collection of photogenerated carriers likely originating from poor coverage and passivation of the initially nucleating grains.

14 SOLAR ENERGY↗

NASA NTRS1983

Testing a dynamical model for mid-latitude sea surface temperature anomalies

The present investigation is concerned with the development and testing of a dynamical model for sea surface temperature (SST) anomalies in the midlatitudes. The model is an extension of the stochastic forcing model, suggested by Frankignoul and Hasselmann (1977), in which SST anomalies arise naturally as a response of the slowly varying upper ocean to the rapidly varying air-sea fluxes. The conducted analysis confirms strongly the validity of this model. The results suggest that advection by mean ocean currents plays an important role in some regions. Attention is given to the governing equations, a statistical model, SST anomaly advection, heat flux anomalies, wind-driven mass transport in the mixed layer, mixed-layer depth, aspects of model testing, and the atmospheric forcing.

Frankignoul, C.↗

DOE OSTI2024

Self-similar Reynolds-averaged mechanical–scalar turbulence models for reshocked Richtmyer–Meshkov instability-induced mixing in the small Atwood number limit

Analytical self-similar solutions to two-, three-, and four-equation Reynolds-averaged mechanical–scalar turbulence models describing incompressible turbulent Richtmyer–Meshkov instability-induced mixing in planar geometry derived in the small Atwood number limit are extended to construct models for reshocked Richtmyer–Meshkov mixing. In this study, the models are based on the turbulent kinetic energy K and its dissipation rate ε, together with the scalar variance S and its dissipation rate χ modeled either differentially or algebraically. The three- and four-equation models allow for a simultaneous description of mechanical and scalar mixing, i.e., mixing layer growth and molecular mixing. Mixing layer growth parameters and other physical observables were obtained explicitly as functions of the model coefficients and were used to calibrate the model coefficients. Here, the solutions for the singly shocked Richtmyer–Meshkov case for the mixing layer width and the turbulent fields are used to construct piecewise-continuous generalizations of these quantities for times after reshock. For generality, the post-reshock mixing layer width is not assumed to grow with the same power-law as the pre-reshock width, and an impulsive approximation applied to Rayleigh–Taylor instability growth is used to establish the expression for the post-reshock width. A four-equation model is then used to illustrate the spatiotemporal behavior of the mean and turbulent fields and late-time turbulent equation budgets across the mixing layer. The reference solutions derived here can provide systematic calibrations and better understanding of mechanical–scalar turbulence models and their predictions for reshocked Richtmyer–Meshkov instability-induced turbulent mixing in the very large Reynolds number limit.

42 ENGINEERING↗

NASA NTRS1984

Airborne lidar observations of long-range transport in the free troposphere

Airborne lidar measurements of ozone and aerosols in the lower troposphere show the presence of pollutant layers above the mixed layer. Two case studies are analyzed to identify probable source regions and mechanisms for material injection into the free troposphere above local mixed layers. An elevated haze/oxidant layer observed over South Carolina on Aug. 2, 1980, was found to originate in cumulus convection over Georgia on Aug. 1, 1980. An extensive haze/oxidant layer observed over southeastern Virginia on July 31, 1981, is shown to have been in contact with the New England mixed layer on July 30, 1981. This transported air mass is estimated to contribute approximately 30 percent of the ozone maximum measured at the surface in the Norfolk, VA, area on July 31, 1981. Such elevated 'reservoir' layers are transported over long ranges and are not detected by sensors which are confined to the surface.

Shipley, S. T.↗

NASA NTRS1996

Mixing and Transition Control Studied

Considerable progress in understanding nonlinear phenomena in both unbounded and wallbounded shear flow transition has been made through the use of a combination of high- Reynolds-number asymptotic and numerical methods. The objective of this continuing work is to fully understand the nonlinear dynamics so that ultimately (1) an effective means of mixing and transition control can be developed and (2) the source terms in the aeroacoustic noise problem can be modeled more accurately. Two important aspects of the work are that (1) the disturbances evolve from strictly linear instability waves on weakly nonparallel mean flows so that the proper upstream conditions are applied in the nonlinear or wave-interaction streamwise region and (2) the asymptotic formulations lead to parabolic problems so that the question of proper out-flow boundary conditions--still a research issue for direct numerical simulations of convectively unstable shear flows--does not arise. Composite expansion techniques are used to obtain solutions that account for both mean-flow-evolution and nonlinear effects. A previously derived theory for the amplitude evolution of a two-dimensional instability wave in an incompressible mixing layer (which is in quantitative agreement with available experimental data for the first nonlinear saturation stage for a plane-jet shear layer, a circular-jet shear layer, and a mixing layer behind a splitter plate) have been extended to include a wave-interaction stage with a three-dimensional subharmonic. The ultimate wave interaction effects can either give rise to explosive growth or an equilibrium solution, both of which are intimately associated with the nonlinear self-interaction of the three dimensional component. The extended theory is being evaluated numerically. In contrast to the mixing-layer situation, earlier comparisons of theoretical predictions based on asymptotic methods and experiments in wall-bounded shear-flow transition have been somewhat lacking in one aspect or another. The current work strongly suggests that the main weakness is the underlying asymptotic representation of the linear "part" of the problem and not the explicit modeling of the nonlinear/wave-interaction effects. Consequently, the long-wave-length/high-Reynolds-number asymptotic limit for the Blasius boundary-layer stability problem was reexamined, and a new dispersion relationship for the instability waves that is uniformly valid for both the upper- and lower branch regions to the required order of approximation was obtained. A comparison with numerical results, obtained by solving the Orr-Sommerfeld stability problem, shows that the asymptotic formula provides surprisingly good results, even for values of the frequency parameter usually encountered in experimental investigations. This is particularly evident in the dynamically important upper-branch region, where much of the nonlinear interactions in transition experiments are believed to take place. The result is important in that it can be used to greatly improve the accuracy of weakly nonlinear critical-layer-based theories, and a consistent nonlinear theory is currently under evaluation.

Source record↗

DOE OSTI2026

Upper ocean mixing, surface heat fluxes, and heat content variability in the upper 150 m during Hurricane Laura (2020)

Observations (from thermistor sensors and a hurricane glider) and model-based temperature were used to answer questions including the following: 1) What physical and environmental conditions explain the rapid intensification of Hurricane Laura? 2) How did the pre-existing warm mixed layer at Stone mooring (StM) influence the degree of cooling in the mixed layer? 3) How did vertical mixing, surface heat fluxes, and advective processes collectively shape the mixed layer heat evolution at StM? Observations measured by thermistor sensors showed that Hurricane Laura induced a cooling of -1.2oC in the mixed layer when Hurricane Laura’s wind speed increased to 47 m/s on 26 August. This contrasts with the -1.04oC mixed layer temperature change estimated from model-based temperature. At StM, the presence of a 31oC warm mixed layer and elevated heat content (60-80kJ/cm2) effectively preconditioned the upper ocean ahead of Hurricane Laura’s passage. After Hurricane Laura passed, turbulent mixing associated with the storm transported the heat anomalies downward into subsurface layers. In addition, this study shows that a surface heat flux of 5.04 kJ/cm2 supported the intensity of Hurricane Laura as it traversed over the StM. Using a mixed layer heat balance model, this study shows that entrainment flux and surface flux mostly contributed to the observed change in the mixed layer temperature.

Tsai, Senam↗

NASA NTRS2020

Characterizing 15 Years of Saharan-like, Dry, Well-Mixed Air Layers in North Africa

The Saharan Air Layer (SAL) is a dry, well-mixed layer (WML) of warm and sometimes dusty air of nearly constant water vapor mixing ratio generated by the intense surface heating and strong, dry convection in the Sahara Desert, which has notable downstream impacts on the surface energy balance, organized convective system development, seasonal precipitation, and air quality. Characterizing both WMLs and SALs from the existing rawinsonde network has proven challenging because of its sparseness and inconsistent data reporting. Spurred on by this challenge, we previously created a detection methodology and supporting software to automate the identification and characterization of WMLs from multiple data sources including rawinsondes, remote sensing platforms, and model products. We applied our algorithm to each dataset at both its native and at a common (most coarse data product) vertical resolution to detect WMLs and their characteristics (temperature, mixing ratio, AOD, etc.) at each of the 53 rawinsonde launch sites in north Africa.

Nicholls, Stephen D.↗

NASA NTRS1994

The Roles of Large- and Small-Scale Structures in Turbulent Free Shear Layers

The occurrence of large-scale coherent structures in turbulent free shear flows (especially the planar mixing layer) has been recognized for some time. Indeed, the observation of such structures in mixing layers did much to promote interest in the study of coherent structures in turbulence. It has been widely assumed that the large-scale structures in these flows are responsible for the entrainment of free-stream fluid and the overall growth of the layer, while the small-scale structures provide mixing and dissipation. A model of scalar mixing based on these ideas was proposed for these flows. However, recent experimental and computational evidence suggests that the dominance of the large-scale structures in turbulent mixing layers is not universal. In addition, there is a substantial variation among experiments in several statistical measures of self-similar mixing layers, for example growth rate and velocity variances. To investigate the importance of large-scale structures, several free shear flows (mixing layers and wakes) have been simulated via direct numerical simulation. The simulations are designed to mimic experimental mixing layers in which the splitter plate boundary layers are turbulent. Different levels of two-dimensional forcing are included resulting in large-scale structures of differing strength and importance. These simulations are used to investigate the role of large-scale coherent structures in free shear layers and the effect of these structures on relevant turbulence statistics and scalar mixing. It is found that the statistics and structures in several experiments involving turbulent mixing layers are in better agreement with simulations that do not exhibit dominant large-scale structures than those in which the common mixing layer structures do dominate. It is also found that the level of forcing can have a profound effect on the qualitative and quantitative features of these shear layer, even when they are nominally self-similar.

Moser, Robert D.↗

NASA NTRS1994

Air pollutant transport in a coastal environment. Part 1: Two-dimensional simulations of sea-breeze and mountain effects

Over the southern California coastal region, observations of the vertical distributions of pollutants show that maximum concentrations can occur within temperature inversion layers well above the surface. A mesoscale model is used to study the dynamical phenomena that cause such layers, including sea breezes and mountain flows, and to study the characteristics of air pollutant transport in a coastal environment capped by a temperature inversion. The mathematical and physical structure of the model is described. Two-dimensional simulations corresponding to four configurations of coastal plains and mountains are discussed. The simulations reveal that pollutant transport over a coastal plain is strongly influenced by the topographic configuration, including the height of coastal mountains and their distance from the coastline. Sea breezes induced by land-sea thermal contrasts, as well as upslope winds induced along mountain flanks, both create vertical transport that can lead to the formation of elevated pollution layers. The sea-breeze circulation generates pollution layers by undercutting the mixed layer and lofting pollutants into the stable layer. Heating of mountain slopes acts to vent pollutants above the mountain ridge during the day; during the evening, pollutants can be injected directly into the inversion layer from the decaying upslope flows. In a land-sea configuration with mountains close to the coastline, the sea breeze and heated-mountain flow are strongly coupled. In the afternoon, this interaction can produce upslope flow from which polluted air is detrained into the inversion layer as a return circulation. When the mountains lie farther inland, however, pollutants may be trapped aloft when the mixed layer stabilizes in the late afternoon. As the nocturnal boundary layer forms over the coast in the evening, polluted mixed-layer air is effectively left behind in the inversion layer. In the Los Angeles Basin, the formation mechanism for elevated polluted layers is most similar to our cases with inland mountains.

Lu, Rong↗

DOE OSTI2021

Self-similar Reynolds-averaged mechanical–scalar turbulence models for Rayleigh–Taylor, Richtmyer–Meshkov, and Kelvin–Helmholtz instability-induced mixing in the small Atwood number limit

Analytical self-similar solutions to two-, three-, and four-equation Reynolds-averaged mechanical–scalar turbulence models describing incompressible turbulent Rayleigh–Taylor, Richtmyer–Meshkov, and Kelvin–Helmholtz instability-induced mixing in planar geometry are derived in the small Atwood number (Boussinesq) limit. The models are based on the turbulent kinetic energy K and its dissipation rate ε, together with the scalar (heavy-fluid mass fraction) variance S and its dissipation rate Χ modeled either differentially or algebraically. The models allow for a simultaneous description of mechanical and scalar mixing, i.e., mixing layer growth and molecular mixing, respectively. Mixing layer growth parameters and other physical observables relevant to each instability are obtained explicitly as functions of the model coefficients. The turbulent fields are also expressed in terms of the model coefficients, with their temporal power-law scalings obtained by requiring that the self-similar equations are explicitly time-independent. The model calibration methodology is described and discussed. Expressions for a subset of the various physical observables are used to calibrate each of the two-, three-, and four-equation models, such that the self-similar solutions are consistent with experimental and numerical simulation data corresponding to these values of the observables and to specific canonical Rayleigh–Taylor, Richtmyer–Meshkov, and Kelvin–Helmholtz turbulent flows. A calibrated four-equation model is then used to reconstruct the mean and turbulent fields, and late-time turbulent equation budgets for each instability-induced flow across the mixing layer. The reference solutions derived here can provide systematic calibrations and better understanding of mechanical–scalar turbulence models and their predictions for instability-induced turbulent mixing in the very large Reynolds number limit.

42 ENGINEERING↗

NASA NTRS1992

Compressibility effects on large structures in free shear flows

Space-time correlations were used to study compressibility effects on large structures in mixing layers. Two high-Reynolds number mixing layers with M(c) = 0.51 (case 1) and 0.86 (case 2) were studied. The results indicate that the structures in case 1 are similar to those in the incompressible case, but less organized. The structures in case 2 are highly three-dimensional, with a good spatial but a poor temporal orgnization. The streamwise correlations showed a decay rate four to five times greater for case 2 relative to case 1. While the spanwise correlations for case 1 showed trends similar to incompressible mixing layers, the behavior of case 2 was very different. The pressure fluctuations in the fully developed region of case 2 displayed significant rms variation in the spanwise direction with a well-defined pattern. Based on these measurements, the structures in case 2 seem to be of a horseshoe type, transversely spanning the mixing layer with the head in the low-speed side and the legs inclined in both the x-y and the x-z planes.

Samimy, M.↗

NASA NTRS1994

Effects of Heat Release on a Two-Dimensional Reacting Shear Layer

The diffusion controlled binary reaction between initially segregated reactants in a two-dimensional low Mach number mixing layers is studied via numerical simulation. The stoichiometric ratio of the reactants is chosen to be much larger than one, as is typical of hydrocarbon flames in air. This results is a flame that is offset from the main vortical region of the mixing layer. In agreement with experimental observations, the flame remains surprisingly uncontorted during the flow evolution and is not entrained into the mixing layer. The effect of the heat release of the flame on the evolution of the mixing layer is thus similar to the effect of a difference in free-stream density between the two sides of the layer. The resulting baroclinic torque inhibits the familiar rolup and pairing of mixing layer vortices common in constant density flows. This also contributes to the layers inability to entrain the flame. The increase in viscosity caused by the heating of the flame reduces the effective Reynolds number of the flow. But, contrary to what has commonly been suggested, this is not the major reason for the inhibition of the usual large-scale mixing layer structures.

Moser, Robert↗

NASA NTRS1984

The coupling between scales in shear flows

The relationship between large and small-scale motions in turbulent shear flows is studied using short-time correlation measurements. Boundary layers, plane and axisymmetric mixing layers, plane wakes, and the far fields of plane and circular jets are examined. The coupling is found to be significant in all flows. Phase reversal across the shear region is found to occur in the boundary layers and the mixing layers only. This is interpreted to mean that in these layers the streamwise extent of the large structure over which the small-scale activity reaches a peak moves from one transverse end of the large structure over which its ensemble-averaged u-fluctuation is positive to another where it is negative. In the far field of jets and wakes, the small-scale peak activity remains confined to that half of the streamwise extent of the large structure where its ensemble-averaged u-fluctuation is positive.

Bandyopadhyay, P. R.↗

NASA NTRS1974

Interaction of a cumulus cloud ensemble with the large-scale environment. I

A theory of the interaction of a cumulus cloud ensemble with the large-scale environment is developed. In this theory, the large-scale environment is divided into the subcloud mixed layer and the region above. The time changes of the environment are governed by the heat and moisture budget equations for the subcloud mixed layer and for the region above, and by a prognostic equation for the depth of the mixed layer. In the environment above the mixed layer, the cumulus convection affects the temperature and moisture fields through cumulus-induced subsidence and detrainment of saturated air containing liquid water which evaporates in the environment. In the subcloud mixed layer, the cumulus convection does not act directly on the temperature and moisture fields, but it affects the depth of the mixed layer through cumulus-induced subsidence.

Arakawa, A.↗

DOE OSTI2020

A passive model for the evolution of subgrid-scale instabilities in turbulent flow regimes

In this work, a zero-dimensional model for the development of turbulent mixing layers driven by Rayleigh–Taylor (RT) or Richtmyer–Meshkov (RM) instabilities is presented, for application in Reynolds-Averaged Navier–Stokes (RANS) simulations. The model approximates the behavior of the turbulent mixing layer at a passively advected tracer particle that sits on the material interface of interest in the simulation, and is used to provide initial conditions for the RANS model once the mixing layer width has developed to a size that may be resolved on the computational mesh. The model relies on approximations to the Besnard–Harlow–Rauenzahn (BHR) RANS closure equations and is thus consistent the turbulent development of the mixing layer, unlike previous models of this type which have focused on the early-time laminar development of RT or RM instabilities. These instabilities will often grow through an initially laminar state before developing into turbulence, and criteria for switching from an existing laminar model to the proposed turbulent model are considered. The proposed model reproduces the mixing layer development of RT and RM instabilities seen in mixed width resolving BHR RANS simulations to a reasonable degree of accuracy, and relaxes the need for the RANS simulation to resolve the mixed width as soon as the mixing layer becomes turbulent, which may be impractical in cases where the mixing layer grows through a wide range of scales.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS1995

Grid resolution and turbulent inflow boundary condition recommendations for NPARC calculations

The effects of grid resolution and specification of turbulent inflow boundary conditions were examined using the NPARC code with the Baldwin-Lomax and Chien k-e turbulence models. Three benchmark turbulent test cases were calculated: two were wall bounded flows and the third was a compressible mixing layer. The wall bounded flows were essentially insensitive to axial grid density; however, the location of the first point off the wall had a substantial effect on flow solutions. It was determined that the first point off the wall must be in the laminar sublayer (y+ less than or equal to 5) for the entire boundary layer. For the compressible mixing layer cases, the axial grid density affected the capturing of oblique shock waves in the mixing region, but the overall mixing rate was not strongly dependent on grid resolution. In specifying the inflow turbulent boundary conditions, it was very important to match the boundary layer and momentum thicknesses of the two flows entering the mixing region; calculations obtained with smaller or no boundary layers resulted in substantially reduced mixing. The solutions were relatively insensitive to freestream turbulence level.

Georgiadis, Nicholas J.↗

NASA NTRS1994

Control of an Axisymmetric Jet Using Vortex Generators

The results of an experimental investigation on the effect of vortex generators, in the form of small tabs at the nozzle exit on the evolution of a jet, are reported in this paper. Primarily tabs of triangular shape are considered, and the effect is studied up to a jet Mach number of 1.8. Each tab is found to produce a dominant pair of counter-rotating streamwise vortices having a sense of rotation opposite to that expected from the wrapping of the boundary layer. This results in an inward indentation of the mixing layer into the core of the jet. A triangular-shaped tab with its apex leaning downstream, referred to as a delta tab, is found to be the most effective in producing such vortices, with a consequential large influence on the overall jet evolution. Two delta tabs, spaced 180 deg apart, completely bifurcate the jet. Four delta tabs stretch the mixing layer into four 'fingers,' resulting in a significant increase in the jet mixing downstream. For six delta tabs the mixing layer distortion settles back to a three finger configuration through an interaction of the streamwise vortices. The tabs are found to be equally effective in jets with turbulent or laminar initial boundary layers. Two sources of streamwise vorticity are postulated for the flow under consideration. One is the upstream 'pressure hill,' generated by the tab, which constitutes the main contributor of vorticity to the dominant pair. Another is due to vortex filaments shed from the sides of the tab and reoriented downstream by the mean shear of the mixing layer. Depending on the orientation of the tab, the latter source can produce a vortex pair having a sense of rotation opposite to that of the dominant pair. In the case of the delta tab, vorticity from the two sources add, explaining the strong effect in that configuration.

Zaman, K. B. M. Q.↗

NASA NTRS1988

Modeling of supersonic reacting flow fields

A detailed understanding of the scramjet combustor flow field is critical to the achievement of a successful design. Even though the combustor flow field is quite complex, it can be realistically viewed as a collection of spatially developing and reacting supersonic mixing layers that are initially discrete, but that ultimately merge into larger more complex zones. These mixing layers begin downstream of a set of fuel injectors that introduce gaseous hydrogen in both a parallel and transverse direction into a supersonic air stream entering from the engine inlet. The behavior of the initial portion of the combustor flow, in the mixing layers near the fuel injectors, appears to be most critical, since this is where the mechanism for efficient high speed mixing must be established to achieve the required degree of combustion downstream. Because of the structure of the flow field in this initial portion of the combustor, a single supersonic, spatially developing and reacting mixing layer serves as an excellent physical model for the overall flow field. Even though this reacting mixing layer flow is geometrically simple, it can still be made to retain all of the fluid mechanical and chemical complexities present in the actual combustor flow field.

Drummond, J. P.↗