DOE OSTI2010
Localized, transient heating of materials using micro-scale, highly absorbing laser light has been used in many industries to anneal, melt and ablate material with high precision. Accurate modeling of the relative contributions of conductive, convective and radiative losses as a function of laser parameters is essential to optimizing micro-scale laser processing of materials. In bulk semi-transparent materials such as silicate glass melts, radiation transport is known to play a significantly larger role as the temperature increases. Conventionally, radiation is treated in the frequency-averaged diffusive limit (Rosseland approximation). However, the role and proper treatment of radiative processes under rapidly heated, high thermal gradient conditions, often created through laser-matter interactions, is at present not clear. Starting from the radiation transport equation for homogeneous, refractive lossy media, they derive the corresponding time-dependent multi-frequency diffusion equations. Zeroth and first moments of the transport equation couple the energy density, flux and pressure tensor. The system is closed by neglecting the temporal derivative of the flux and replacing the pressure tensor by its diagonal analogue. The radiation equations are coupled to a diffusion equation for the matter temperature. They are interested in modeling infrared laser heating of silica over sub-millimeter length scales, and at possibly rapid rates. Hence, in contrast to related work, they retain the temporal derivative of the radiation field. They derive boundary conditions at a planar air-silica interface taking account of reflectivities obtained from the Fresnel relations that include absorption. The effect of a temperature-dependent absorption index is explored through construction of a multi-phonon dielectric function that includes mode dispersion. The spectral dimension is discretized into a finite number of intervals yielding a system of multigroup diffusion equations. Simulations are presented. To demonstrate the bulk heat loss due to radiation and the effect of the radiation's temporal derivative, they model cooling of a silica slab, initially at 2500 K, for 10 s. Retaining the derivative enables correctly modeling the loss of photons initially present in the slab. Other simulations model irradiating silica discs (of approximately 5 mm radii and thickness) with a CO2 laser: {lambda} = 10.59 and 4.6 um, Gaussian profile, r{sub 0} = 0.5 mm for 1/e decay. By surrounding the disks in room-temperature air, they make use of the boundary conditions described above.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗