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The significance of gas phase reactions in determining the nuclear structure of comets is discussed. The sublimation of parent molecules such as H2O, CH4, CO2, and NH3 from the surface of the nucleus and their subsequent photodissociation and ionization in forming observed cometary molecular species are elaborated.
The spectra of energetic nuclei within astrophysical sources may be determined by studying gamma-ray line emissions above 8 MeV. Excited states which can be produced by inelastic scattering, charge exchange, and spallation reactions in the abundant nuclear species were considered in order to identify nuclear lines which may contribute to the gamma spectrum. The cross sections for production of most high-energy states are sparsely measured. Those which were determined are comparable to the cross section for production of the 15.11 MeV level in C-12 with few exceptions. The branching ratios for gamma-ray and particle emission are, however, better known. Of those states considered, 44 measured branching ratios greater than 40% for emission of a gamma-ray with energy above 8 MeV. For twelve more states the branching ratios, although not yet determined, are expected to be small. The gamma-ray emission from other individual nuclear states is not likely to be as great as that that for the 15.11 MeV state in C-12.
Processes which lead to the production of gamma rays with energy greater than 8 MeV in solar flares are reviewed and evaluated. Excited states produced by inelastic scattering, charge exchange, and spallation reactions in the abundant nuclear species are considered in order to identify nuclear lines which may contribute to the Gamma ray spectrum of solar flares. The flux of 15.11 MeV Gamma rays relative to the flux of 4.44 MeV Gamma rays from the de-excitation of the corresponding states in C12 is calculated for a number of assumed distributions of exciting particles. This flux ratio is a sensitive diagnostic of accelerated particle spectra. Other high energy nuclear levels are not so isolated as the 15.11 MeV state and are not expected to be so strong. The spectrum of Gamma rays from the decay of Pi dey is sensitive to the energy distribution of particles accelerated to energies greater than 100 MeV.
Processes that lead to the production of gamma rays with energy greater than 8 MeV in solar flares are reviewed and evaluated. Excited states that can be produced by inelastic scattering, charge exchange, and spallation reactions in the abundant nuclear species are considered in order to identify nuclear lines that may contribute to the gamma-ray spectrum of solar flares. The flux of 15.11-MeV gamma rays relative to the flux of 4.44-MeV gamma rays from the deexcitation of the corresponding states in C-12 is calculated for a number of assumed distributions of exciting particles. This flux ratio is shown to be a sensitive diagnostic of accelerated particle spectra. Other high-energy nuclear levels are not so isolated as the 15.11-MeV state and are not expected to be so strong. The spectrum of gamma rays from the decay of neutral pions is shown to be sensitive to the energy distribution of particles accelerated to energies greater than 100 MeV.
Reasons for mounting the Space Exploration Initiative, the variables facing U.S. planners, and the developmental technologies that will be needed to support this initiative are discussed. The three more advanced technological approaches in the field of power generation described include a lunar-based solar power system, a geosynchronous-based earth orbit solar power satellite system, and the utilization of helium-3/deuterium fusion reaction to create a nuclear fuel cycle. It is noted that the major elements of the SEI will include a heavy-lift launch vehicle, a transfer vehicle and a descent/ascent vehicle for use on lunar missions and adaptable to Mars exploration.
A method developed for the proton NIEL calculation previously is extended to incident alpha particles in this study: ZBL screened potential for Coulomb interactions and MCNPX 'thin target approximation' for nuclear interactions.
The He-3 (n,p)T reaction was examined as an energy source for a CO2 laser. For this purpose He-3 was added to a functioning CO2 electrically excited laser. Initially the laser was run electrically with 12 torr total pressure. The gas mixture was 1:1:8, CO2:N2:He. At zero reactor power, the laser was tested in place next to the core of the Georgia Tech. Research Reactor. After verification of laser action He-3 was added to the system. The He-3 partial pressures of 10 torr, 50 torr, and 300 torr were added in three separate reactor runs. Reactor power ranged from zero to 5 million watts, which corresponds to a peak flux of 10 to the 14th power/sq cm. At reactor powers greater than 10 kW, gain of up to 30 percent was shown. However, indications are this may be due to gamma excitation rather than caused by the He-3 (n,p)T reaction. These results do agree with the data of past CO2 nuclear pumped laser experiments.
The reliability and development of aerospace materials in extreme environments relies on a comprehensive understanding of their thermochemical properties. Such properties are commonly used for equilibrium phase stability calculations of interactions with corrosive environments at very high temperatures. These calculations can lead to in-depth understanding of degradation mechanisms in both coatings and components for applications such as nuclear thermal propulsion and gas turbine engines, both of which are part of NASA’s current R&D focus for improving propulsion systems for aerospace missions. The first part of this talk summarizes and discuss our current thermochemical calculations of the behavior of ceramic-ceramic (cercer) UN-based fuels and their coating systems during nuclear thermal rocket operation. The second part of the talk summarizes and discuss the energetics of reactions of ceramic coating materials and their binary oxide components with silicate melts measured by high temperature reaction calorimetry.
Sedimentary barites from South Africa and Western Australia (about 3 billion years old) contain spallogenic Xe isotopes produced by reactions of Ba with nuclear-active particles in cosmic rays. 'Surface residence time' of these samples was calculated from the observed concentrations of spallogenic Xe-126. Comparison of spallogenic ratios of Xe-131/Xe-126 in the two samples provides evidence for the reaction Ba-130(n, gamma) yields Xe-131, which is characterized by a large number of resonances for neutron absorption in the epithermal region. This observation lends additional support to the conclusions already reached regarding the origin of anomalous Xe-131 in lunar samples.
Added to the pure Coulomb potential, the contribution from vacuum polarization increases the barrier, reducing the wave function (u) for reacting nuclei within the range of nuclear forces. The cross section and reaction rate are then reduced accordingly by a factor proportional to u squared. The effect is treated by evaluating the vacuum polarization potential as a small correction to the Coulomb term, then computing u in a WKB formulation. The calculation is done analytically employing the small r power-series expansion for the Uehling potential to express the final result in terms of convenient parameters. At a temperature of 1.4 x 10 to the 7th K the (negative) correction is 1.3 percent for the fundamental fusion process p + p yields d + e(+) + nu.
High-temperature, crosslinked polyimides are typically insoluble, intractible materials. Consequently, in these systems it has been difficult to follow high-temperature curing or long-term degradation reactions on a molecular level. Selective labeling of the polymers with carbon-13, coupled with solid nuclear magnetic resonance spectrometry (NMR), enables these reactions to be followed. We successfully employed this technique to provide insight into both curing and degradation reactions of PMR-15, a polymer matrix resin used extensively in aircraft engine applications.
Thermonuclear reaction rates in medium and heavy nuclei determined from statistical properties
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The heavy isotopic anomalies observed recently in the fractionation and unknown nuclear inclusions from the Allende meteorite are explained by neutron reactions during the explosive carbon burning (ECB). This model produces heavy anomalies in the same zone where Al-26 and O-16 are produced, thus reducing the number of source zones required for the isotopic anomalies. Unlike the classical r-process, the ECB n-process avoids the problem with the Sr anomaly and may resolve the problem of conflicting time scales between Al-26 and the r-process isotopes I-129 and Pu-244. Experimental studies of Zr and Ce isotopic composition are proposed to test this model.
In order to effect large-scale return of extraterrestrial resources to Earth orbit, it is desirable to optimize the propulsion system to maximize the mass of payload returned per unit energy expended. This optimization problem is different from the conventional rocket propulsion optimization. A rocket propulsion system consists of an energy source plus reaction mass. In a conventional chemical rocket, the energy source and the reaction mass are the same. For the transportation system required, however, the best system performance is achieved if the reaction mass used is from a locally available source. In general, the energy source and the reaction mass will be separate. One such rocket system is the nuclear thermal rocket, in which the energy source is a reactor and the reaction mass a fluid which is heated by the reactor and exhausted. Another energy-limited rocket system is the hydrogen/oxygen rocket where H2/O2 fuel is produced by electrolysis of water using a solar array or a nuclear reactor. The problem is to choose the optimum specific impulse (or equivalently exhaust velocity) to minimize the amount of energy required to produce a given mission delta-v in the payload. The somewhat surprising result is that the optimum specific impulse is not the maximum possible value, but is proportional to the mission delta-v. In general terms, at the beginning of the mission it is optimum to use a very low specific impulse and expend a lot of reaction mass, since this is the most energy efficient way to transfer momentum. However, as the mission progresses, it becomes important to minimize the amount of reaction mass expelled, since energy is wasted moving the reaction mass. Thus, the optimum specific impulse will increase with the mission delta-v. Optimum I(sub sp) is derived for maximum payload return per energy expended for both the case of fixed and variable I(sub sp) engines. Sample missions analyzed include return of water payloads from the moons of Mars and of Saturn.
NASA has been primarily interested in nuclear-pumped lasers using the He-3 or U-235F6 reaction for lasant excitation. With He-3 excitation, a large volume, multiple-path He-3-Ar nuclear laser has produced an output of 1 kilowatt. Power deposition was shown to be homogeneous over this volume. The CO laser has been pumped for the first time using the He-3 reaction, producing approximately 200 Watts. Using a boron-10 coating to excite N2, nuclear lasing has been achieved in CO2 in a transfer laser configuration. Nuclear lasing of Ar-Xe has been demonstrated using fission fragment excitation from U-235F6. Research on the gas core reactor has resulted in a steady state operational power of 30 kilowatts with flowing U-235F6 in an argon vortex.
Plasma current sheet dynamics - thermonuclear fusion - space propulsion