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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 361 records · Page 20

Neutron activation diagnostics at the National Ignition Facility (invited)

Neutron yields are measured at the National Ignition Facility (NIF) by an extensive suite of neutron activation diagnostics. Neutrons interact with materials whose reaction cross sections threshold just below the fusion neutron production energy, providing an accurate measure of primary unscattered neutrons without contribution from lower-energy scattered neutrons. Indium samples are mounted on diagnostic instrument manipulators in the NIF target chamber, 25-50 cm from the source, to measure 2.45 MeV deuterium-deuterium fusion neutrons through the {sup 115}In(n,n'){sup 115m} In reaction. Outside the chamber, zirconium and copper are used to measure 14 MeV deuterium-tritium fusion neutrons via {sup 90}Zr(n,2n), {sup 63}Cu(n,2n), and {sup 65}Cu(n,2n) reactions. An array of 16 zirconium samples are located on port covers around the chamber to measure relative yield anisotropies, providing a global map of fuel areal density variation. Neutron yields are routinely measured with activation to an accuracy of 7% and are in excellent agreement both with each other and with neutron time-of-flight and magnetic recoil spectrometer measurements. Relative areal density anisotropies can be measured to a precision of less than 3%. These measurements reveal apparent bulk fuel velocities as high as 200 km/s in addition to large areal density variations between the pole and equator of the compressed fuel.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

BARYON LOADING OF ACTIVE GALACTIC NUCLEUS JETS MEDIATED BY NEUTRONS

Plasmas of geometrically thick, black hole (BH) accretion flows in active galactic nuclei (AGNs) are generally collisionless for protons, and involve magnetic field turbulence. Under such conditions a fraction of protons can be accelerated stochastically and create relativistic neutrons via nuclear collisions. These neutrons can freely escape from the accretion flow and decay into protons in the dilute polar region above the rotating BH to form relativistic jets. We calculate geometric efficiencies of the neutron energy and mass injections into the polar region, and show that this process can deposit luminosity as high as L{sub j}{approx}2 Multiplication-Sign 10{sup -3} M-dot c{sup 2} and mass loading M-dot{sub j}{approx}6 Multiplication-Sign 10{sup -4} M-dot for the case of the BH mass M {approx} 10{sup 8} M{sub Sun }, where M-dot is the mass accretion rate. The terminal Lorentz factors of the jets are {Gamma} {approx} 3, and they may explain the AGN jets having low luminosities. For higher luminosity jets, which can be produced by additional energy inputs such as Poynting flux, the neutron decay still can be a dominant mass loading process, leading to, e.g., {Gamma} {approx} 50 for L{sub j,tot}{approx}3 Multiplication-Sign 10{sup -2} M-dot c{sup 2}.

79 ASTRONOMY AND ASTROPHYSICS↗

Impact of common clandestine structural modifications on synthetic cathinone “bath salt” pharmacokinetics

Since 2009, the synthetic cathinones (“bath salts”) have risen in popularity as drugs of abuse. However, there are a paucity of studies that have determined the impact of functional group modifications in the synthetic cathinone chemical structures on plasma and central nervous system (CNS) pharmacokinetics. In the present study, we investigated the in vivo plasma and CNS pharmacokinetics of three synthetic cathinones whose structures differ by lengthening of the α-alkyl chain: methylone (-CH{sub 3}), butylone (-CH{sub 2}CH{sub 3}), and pentylone (-CH{sub 2}CH{sub 2}CH{sub 3}). Male Sprague-Dawley rats were treated with a 20 mg/kg subcutaneous dose of the individual synthetic cathinone. Blood samples were obtained at specific times from a jugular vein cannula over an 8 hour period. Over a separate three-hour period, CNS samples were obtained using a microdialysis cannula surgically implanted into the lateral ventricle. In the plasma, pentylone, with the longest α-alkyl chain, displayed the highest C{sub max} and AUC{sub 0–∞}, and the longest t{sub 1/2.} Decreasing the α-alkyl chain length as in butylone and methylone significantly decreased the C{sub max}, AUC{sub 0–∞}, and t{sub 1/2}. The plasma pharmacokinetic values are consistent with the greater lipophilicity associated with α-alkyl side chain lengthening. Conversely, in the CNS, methylone and butylone displayed higher C{sub max} and AUC{sub 0–∞} values than pentylone. These contrary findings in the CNS and plasma demonstrate that lengthening of the α-alkyl chain of methylone, butylone, and pentylone yields differential pharmacokinetic properties in the CNS as compared to the plasma. - Highlights: • Adding α-methyl groups increase synthetic cathinone plasma C{sub max}, AUC{sub 0–∞,} t{sub 1/2.} • Adding α-methyl groups decrease synthetic cathinone CNS C{sub max}, AUC{sub 0–∞,} t{sub 1/2.} • The CNS has greater exposure to the synthetic cathinones as compared to the plasma.

60 APPLIED LIFE SCIENCES↗

Xenon excimer emission from multicapillary discharges in direct current mode

Microdischarges in xenon have been generated in a pressure range of 400-1013 mbar with a fixed flow rate of 100 sccm. These microdischarges are obtained from three metallic capillary tubes in series for excimer emission. Total discharge voltage is thrice as large as that of a single capillary discharge tube at current levels of up to 12 mA. Total spectral irradiance of vacuum ultraviolet (VUV) emission also increases significantly compared to that of the single capillary discharge. Further, the irradiance of the VUV emission is strongly dependent on pressure as well as the discharge current.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

On the Rydberg transitions and elemental compositions in the laser produced Al (6063) plasma

We present new studies on the optical emission spectra of the laser produced Al 6063 alloy plasma generated by the 1064 nm Nd: YAG laser. The spectrum reveals Rydberg transitions; nd {sup 2}D{sub 3/2,5/2}{yields} 3p {sup 2}P{sub 1/2,3/2} (n = 3 - 8), ns {sup 2}S{sub 1/2}{yields} 3p {sup 2}P{sub 1/2,3/2} (n 4-6), and the dominant spectral lines of the other constituent elements. We have extracted the relative abundance of the impurities using the relative intensity ratio method. Besides, we have calculated the electron temperature ({approx}7580 K) from the Boltzmann plot method and the electron number densities ({approx}1.4 x 10{sup 17}/cm{sup 3}) from the Stark widths of the aluminum spectral lines. The plasma parameters determined in the present work are in agreement with that reported in the literature. The molecular vibrational transitions of the AlO free radical associated with the B {sup 2}{Sigma}{yields}X {sup 2}{Sigma} band system have also been identified.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Beyond Zeeman spectroscopy: Magnetic-field diagnostics with Stark-dominated line shapes

A recently suggested spectroscopic approach for magnetic-field determination in plasma is employed to measure magnetic fields in an expanding laser-produced plasma plume in an externally applied magnetic field. The approach enables the field determination in a diagnostically difficult regime for which the Zeeman-split patterns are not resolvable, as is often encountered under the conditions characteristic of high-energy-density plasmas. Here, such conditions occur in the high-density plasma near the laser target, due to the dominance of Stark broadening. A pulsed-power system is used to generate magnetic fields with a peak magnitude of 25 T at the inner-electrode surface in a coaxial configuration. An aluminum target attached to the inner electrode surface is then irradiated by a laser beam to produce the expanding plasma that interacts with the applied azimuthal magnetic field. A line-shape analysis of the Al III 4s-4p doublet (5696 and 5722 A) enables the simultaneous determination of the magnetic field and the electron density. The measured magnetic fields are generally found to agree with those expected in a vacuum based on the pulsed-power system current. Examples of other transitions that can be used to diagnose a wide range of plasma and magnetic field parameters are presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Statistical spatial properties of speckle patterns generated by multiple laser beams

This paper investigates hot spot characteristics generated by the superposition of multiple laser beams. First, properties of speckle statistics are studied in the context of only one laser beam by computing the autocorrelation function. The case of multiple laser beams is then considered. In certain conditions, it is shown that speckles have an ellipsoidal shape. Analytical expressions of hot spot radii generated by multiple laser beams are derived and compared to numerical estimates made from the autocorrelation function. They are also compared to numerical simulations performed within the paraxial approximation. Excellent agreement is found for the speckle width as well as for the speckle length. Application to the speckle patterns generated in the Laser MegaJoule configuration in the zone where all the beams overlap is presented. Influence of polarization on the size of the speckles as well as on their abundance is studied.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser induced electron acceleration in an ion-channel guiding

Direct electron acceleration by a propagating laser pulse of circular polarization in an ion-channel guiding is studied by developing a relativistic three-dimensional single particle code. The electron chaotic dynamic is also studied using time series, power spectrum, and Liapunov exponent. It is found that the electron motion is regular (non-chaotic) for laser pulse with short time duration, while for long enough time duration, the electron motion may be chaotic. In the case of non-chaotic motion, the electron can gain and retain very high energy in the presence of ion-channel before reaching the steady-state, whereas in the case of chaotic motion, the electron gains energy and then loses it very rapidly in an unpredictable manner.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Generation of laser-induced plasma in supercritical water and vibrational spectroscopic study of accompanying stimulated Raman scattering

We have formed a laser-induced plasma (LIP) in supercritical water (SCW) and studied associated molecular vibrations using spectroscopic methods. The accompanying forward and backward stimulated Raman scattering (SRS) of water molecules showed anisotropic behavior at supercritical conditions (>647 K and >22.1 MPa). The Raman shift of the backward SRS indicated that attractive interactions between water molecules and excess electrons generated by the LIP were dominant in the SCW. The backward SRS spectrum provided a microscopic view of the hydration environment around an excess electron, which is useful for controlling electron-driven chemical reactions and materials processing in SCW.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Late-time particle emission from laser-produced graphite plasma

We report a late-time ''fireworks-like'' particle emission from laser-produced graphite plasma during its evolution. Plasmas were produced using graphite targets excited with 1064 nm Nd: yttrium aluminum garnet (YAG) laser in vacuum. The time evolution of graphite plasma was investigated using fast gated imaging and visible emission spectroscopy. The emission dynamics of plasma is rapidly changing with time and the delayed firework-like emission from the graphite target followed a black-body curve. Our studies indicated that such firework-like emission is strongly depended on target material properties and explained due to material spallation caused by overheating the trapped gases through thermal diffusion along the layer structures of graphite.

36 MATERIALS SCIENCE↗

Charge resolved electrostatic diagnostic of colliding copper laser plasma plumes

The collision of two laser generated plasma plumes can result, under appropriate conditions, in the formation of a ''stagnation layer.'' The processes underlying this phenomenon are complex and time dependent. The majority of experiments over the last few decades have focused upon spectroscopic diagnostic of colliding plasmas. We have performed electrostatic diagnosis of multiply charged copper ions (Cu{sup +} to Cu{sup 5+}) generated via Q-switched pulsed laser ({lambda} = 1.06 {mu}m, {tau} = 6 ns, and E{sub L} = 52-525 mJ) generation of copper plasma plumes from a planar target. Time dependent current traces, charge yields, and kinetic energy (K{sub e}) distributions are obtained for single plasma plumes (S{sub p}) and colliding plasma plumes (C{sub p}). The charge yield from a C{sub p} relative to twice that from a S{sub p} is characterized by a charge yield ratio (CYR) parameter. Superior ion yields for all charge states occur for a discrete range of fluences (F) from colliding plasma plumes leading to a CYR parameter exceeding unity. The kinetic energy distributions from colliding plasma plumes display well defined energy compression via narrowing of the distributions for all fluences and charge states. The extent of this energy compression is charge dependent. Space charge forces within the stagnation layer and the resulting charge dependent acceleration of ions are proposed to account for the transfer of ion kinetic energy in favour of collisional ionization mechanisms.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Operation Status of the J-PARC Negative Hydrogen Ion Source

A cesium-free negative hydrogen ion source driven with a lanthanum hexaboride (LaB{sub 6}) filament is being operated without any serious trouble for approximately four years in J-PARC. Although the ion source is capable of producing an H{sup -} ion current of more than 30 mA, the current is routinely restricted to approximately 16 mA at present for the stable operation of the RFQ linac which has serious discharge problem from September 2008. The beam run is performed during 1 month cycle, which consisted of a 4-5 weeks beam operation and a few days down-period interval. At the recent beam run, approximately 700 h continuous operation was achieved. At every runs, the beam interruption time due to the ion source failure is a few hours, which correspond to the ion source availability of more than 99%. The R and D work is being performed in parallel with the operation in order to enhance the further beam current. As a result, the H{sup -} ion current of 61 mA with normalized rms emittance of 0.26 {pi}mm.mrad was obtained by adding a cesium seeding system to a J-PARC test ion source which has the almost same structure with the present J-PARC ion source.

43 PARTICLE ACCELERATORS↗

Ion Source Development For The Proposed FNAL 750 keV Injector Upgrade

Currently there is a Proposed FNAL 750 keV Injector Upgrade for the replacement of the 40 year old Fermi National Laboratory (FNAL) Cockcroft-Walton accelerators with a new ion source and 200 MHz Radio Frequency Quadruple (RFQ). The slit type magnetron being used now will be replaced with a round aperture magnetron similar to the one used at Brookhaven National Lab (BNL). Operational experience from BNL has shown that this type of source is more reliable with a longer lifetime due to better power efficiency. The current source development effort is to produce a reliable source with >60 mA of H{sup -} beam current, 15 Hz rep-rate, 100 {mu}s pulse width, and a duty factor of 0.15%. The source will be based on the BNL design along with development done at FNAL for the High Intensity Neutrino Source (HINS).

43 PARTICLE ACCELERATORS↗

Impedance Measurement of an Antenna with Hydrogen Plasma Driven by 13.56 MHz-rf for J-PARC H{sup -} ion source

In order to satisfy the Japan Proton Accelerator Research Complex (J-PARC) second stage requirements of an H{sup -} ion beam current of 50 mA and a life-time of 2000 hours, the development of a 13.56 MHz-rf-driven H{sup -} ion source was started by using an antenna developed at the Spallation Neutron Source (SNS). As the first step, the impedance of an antenna with hydrogen plasma, which is one of the most important parameters, was measured. For an rf-power of 0 kW, 1.25 kW or 7.45 kW, it was measured as j84.19+5.107 {Omega}, j80.22+11.82 {Omega} or j58.24+21.16 {Omega}, respectively. Its real-part had a rather large value and rather large rf-power dependence unexpectedly. By using the measured impedance, the circuit to produce rf-plasma in the plasma chamber on a -50 kV potential with a 13.56 MHz-rf-source on the ground potential was designed by the circuit simulation code LTSpice IV.

43 PARTICLE ACCELERATORS↗

Quantification Of Cesium In Negative Hydrogen Ion Sources By Laser Absorption Spectroscopy

The use of cesium in negative hydrogen ion sources and the resulting cesium dynamics caused by the evaporation and redistribution in the vacuum and plasma phase makes a reliable and on-line monitoring of the cesium amount in the source highly desirable. For that purpose, a robust and compact laser absorption setup suitable for the ion source environment has been developed utilizing the Cs D{sub 2} resonance line at 852.1 nm. First measurements are taken in a small laboratory plasma chamber with cesium evaporation. A detection limit of {approx_equal}5x10{sup 13} m{sup -3} at a typical path length of 15 cm has been obtained with a dynamic range of more than three orders of magnitude, limited by line saturation at high densities. For on-line monitoring an automatic data analysis is established achieving a temporal resolution of 100 ms. The setup has then been applied to the ITER prototype ion sources developed at IPP. It is been shown that the method is well suited for routine measurements revealing a new insight into the cesium dynamics during source operation and cesium conditioning.

43 PARTICLE ACCELERATORS↗

Gas dynamic effects on formation of carbon dimers in laser-produced plasmas

We investigated the effect of helium and nitrogen pressures on the dynamics of molecular species formation during laser ablation of carbon. For producing plasmas, planar carbon targets were irradiated with 1064 nm, 6 ns pulses from an Nd:yttrium aluminum garnet laser. The emission from excited C{sub 2} and CN molecules was studied using space resolved optical time-of-flight emission spectroscopy and spectrally resolved fast imaging. The intensity oscillations in C{sub 2} and CN monochromatic fast imaging and their emission space-time contours suggest that recombination is the major mechanism of C{sub 2} formation within the laser ablation carbon plumes in the presence of ambient gas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Collisional current drive in two interpenetrating plasma jets

The magnetic field generation in two interpenetrating, weakly collisional plasma streams produced by intense lasers is considered. The generation mechanism is very similar to the neutral beam injection current drive in toroidal fusion devices, with the differences related to the absence of the initial magnetic field, short interaction time, and different geometry. Spatial and temporal characteristics of the magnetic field produced in two counterstreaming jets are evaluated; it is shown that the magnetic field of order of 1 T can be generated for modest jet parameters. Conditions under which this mechanism dominates that of the ''Biermann battery'' are discussed. Other settings where the mechanism of the collisional current drive can be important for the generation of seed magnetic fields include astrophysics and interiors of hohlraums.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Enhancements of extreme ultraviolet emission using prepulsed Sn laser-produced plasmas for advanced lithography applications

Laser-produced plasmas (LPP) from Sn targets are seriously considered to be the light source for extreme ultraviolet (EUV) next generation lithography, and optimization of such a source will lead to improved efficiency and reduced cost of ownership of the entire lithography system. We investigated the role of reheating a prepulsed plasma and its effect on EUV conversion efficiency (CE). A 6 ns, 1.06 {mu}m Nd:yttrium aluminum garnet laser was used to generate the initial plasma that was then reheated by a 40 ns, 10.6 {mu}m CO{sub 2} laser to generate enhanced EUV emission from a planar Sn target. The effects of prepulsed laser intensity and delay timings between the prepulsed and the pumping pulse were investigated to find the optimal pre-plasma conditions before the pumping pulse. The initial optimization of these parameters resulted in 25% increase in CE from the tin LPP. The cause of increased EUV emission was identified from EUV emission spectra and ion signal data.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗