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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 361 records · Page 20

Quantum teleportation coexisting with classical communications in optical fiber

The ability for quantum and conventional networks to operate in the same optical fibers would aid the deployment of quantum network technology on a large scale. Quantum teleportation is a fundamental operation in quantum networking, but has yet to be demonstrated in fibers populated with high-power conventional optical signals. Here we report, to the best of our knowledge, the first demonstration of quantum teleportation over fibers carrying conventional telecommunications traffic. Quantum state transfer is achieved over a 30.2-km fiber carrying 400-Gbps C-band classical traffic with a Bell state measurement performed at the fiber’s midpoint. To protect quantum fidelity from spontaneous Raman scattering noise, we use optimal O-band quantum channels, narrow spectro-temporal filtering, and multi-photon coincidence detection. Fidelity is shown to be well maintained with an elevated C-band launch power of 18.7 dBm for the single-channel 400-Gbps signal, which we project could support multiple classical channels totaling many terabits/s aggregate data rates. These results show the feasibility of advanced quantum and classical network applications operating within a unified fiber infrastructure.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Quantum entanglement distribution coexisting with high-rate, broadband classical optical communications over a real-world fiber connecting remote, synchronized nodes

Compatibility with existing classical network infrastructure offers a scalable path towards deploying large-scale quantum networks. Here, we demonstrate O-band polarization-encoded quantum entanglement distribution over an installed 24.4-km fiber while coexisting with a state-of-the-art fully loaded C-band classical communications line system and a picosecond-level precision L-band synchronization signal. The classical system carries two 800-Gbps channels while the remainder of the C-band is filled with amplified spontaneous emission, as is standard for such state-of-the-art communications systems. We examine the spontaneous Raman scattering spectrum generated from this broadband C-band light and offer insights into wavelength allocation for O-band quantum channels. Optimal wavelength selection and narrow filtering enable well-preserved Bell state fidelity when coexisting with 21.4-dBm aggregate launch power across the C-band suitable for 36-Tbps transmission. To the best of our knowledge, this is the first implementation of entanglement-based quantum communications between two remote nodes coexisting with independent classical communications traffic. We demonstrate coexistence of quantum entanglement with ultra-high power levels and record classical bandwidth, offering promise for real-world entanglement-based networking integrated within high-capacity communications infrastructure.

Talcott, Gina M. [Northwestern U.] (ORCID:00000002↗

Advanced Model Development for Large Eddy Simulation of Oxy-Combustion and Supercritical Carbon Dioxide Power Cycles

A joint experimental and numerical study is performed to observe the characteristics of a supercritical carbon dioxide turbulent mixing layer in the presence of strong nonlinearities in the thermodynamic and transport properties. A bespoke experimental setup is designed and employed for this purpose and provides insight into macroscopic mixing behavior. The mixing is experimentally observed using two techniques: shadowgraphy and spontaneous Raman scattering. Qualitative and quantitative intensity fields obtained via these techniques yield instantaneous and mean density data. Spanwise temperature data is also collected using analogue resistance temperature detectors. These measurements are used to quantify the level of mixed material within the field. The experimental data are supplemented by a companion high-fidelity numerical study. The numerical results are obtained through fully resolved, three-dimensional direct numerical simulation. The numerical dataset permits observation of the near-field mixing characteristics, which are difficult to measure experimentally due to the rapid dynamics and sharp thermophysical gradients in this area. Qualitative field visualizations are presented, followed by quantitative mixed material results and observations regarding thermodynamic property trends at select locations within the field. One-dimensional spectra of the turbulent kinetic energy and solenoidal dissipation are provided to observe the spectral characteristics of the flow. Reynolds stress anisotropy is analyzed graphically through anisotropy invariance maps (Lumley triangles). The mixing quantification, spectral data and anisotropy analysis of a flow at these thermodynamic conditions represent the main outcomes of the work.

20 FOSSIL-FUELED POWER PLANTS↗

Time-dependent phenomena in correlated materials

Understanding time-dependent processes and light-matter interaction in strongly correlated materials, and the interplay between electronic, orbital, vibrational, and spin degrees of freedom, is a cornerstone of condensed matter. These mechanisms can be proven by measuring the response of the systems to time-dependent perturbations. The corresponding time scales are dictated by the way light couples to the different excitations, and how these excitations exchange energy and momentum. Our research advances our understanding of these processes, and the interpretation of different equilibrium and time-resolved spectroscopies. Our project encompasses two main themes: (i) developing and refining computational techniques to study non-equilibrium spectroscopies including non-perturbative effects and (ii) applications to non-equilibrium phenomena. We have developed a new computational approach that works directly in the time domain: by including all the degrees of freedom involved in the scattering process (e.g. electrons, photons, neutrons), we solve the time dependent problem: a faithful numerical simulation of the experiment. By measuring the energy and momentum of the outgoing particles, we can extract information about the energy and momentum absorbed by the system. Prior to our work, people attempting to model and calculate non-equilibrium spectral functions relied on a description of the scattering cross section based on a formulation in the frequency domain, a treatment that is extremely cumbersome and complex. Our technique works in and out of equilibrium and can reproduce spectra by several spectroscopic techniques, such as time-resolved photoemission, neutron scattering, Raman, X-ray spectroscopies (RIXS, Auger, XAS, XMCD), and, by not relying on analytical approximations, yields results that reveal novel overlooked transient mechanisms. These tools provide sorely needed intuition for understanding the phenomenology of strongly correlated materials and will help experimentalists in identifying signatures of relevant excitations in pump-probe experiments, such as those conducted in DOE supported facilities.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Aerospace sensor systems.

Aerospace sensor systems, discussing adaptive multimode sensors and multispectral sensing, electronic recognition of image components, laser radar and Raman scattering technique

Mannella, G. G.↗

Research investigation directed toward extending the useful range of the electromagnetic spectrum

The lifetimes and fine structure of He(-) were studied using time-of-flight techniques and quenching by a static axial magnetic field. Using level-crossing spectroscopy the hyperfine constants A and B and the lifetime of the 3 2P3/2 state of Li-7 were measured. Polarization of the Ru 7S level was created as a first step in determining the hyperfine structure of the alkali excited S state. The parametric interaction between light and microwaves in optically pumped Rb-87 vapor were investigated. Measurements and analyses of transitions in formaldehyde and its isotopic species and in the lowest two excited vibrational states of H2CO were also made, as well as of transitions in furan, pyrrole, formic acid, and cyanoacetylene. The Hanle effect was studied in the NO molecule, and RF oscillators were developed with flat, wideband output to observe excited state hyperfine transitions at zero field. Data was generated on the time-dependent behavior of photon echoes in ruby. Stimulated Raman scattering was studied in atomic Tl vapor. A Q switched, temperature-tuned ruby laser was developed which operates between 6934 and 6938 A. The frequency shift due to resonant interaction between identical radiating atoms was calculated.

Hartmann, S. R.↗

Parametric instability of a relativistically strong electromagnetic wave.

The stability of a circularly polarized electromagnetic wave that is strong enough to make plasma electrons, but not ions, relativistic is studied. Small perturbations are considered which propagate parallel to the large-amplitude driver. A relativistically strong wave can be unstable on time scales as short as twice its own oscillation period, and decays into a forward-going plasma oscillation and either one or two electromagnetic waves. Ion motion introduces an additional instability which can be important at short perturbation wavelengths, where the driver would otherwise be stable. The unstable ion and electron modes both have potential for producing anomalously large acceleration of relativistic particles, as well as significant amounts of backscattered light. These effects may be important in two applications: (1) the use of intense lasers to heat or compress plasma, and (2) the plasma surrounding a pulsar, if the pulsar is losing energy by radiation of electromagnetic waves at its rotation frequency. Instability persists in the nonrelativistic regime, reducing to stimulated Raman scattering as a special case.

Max, C. E.↗

Air pollution measurements from satellites

A study is presented on the remote sensing of gaseous and particulate air pollutants which is an extension of a previous report. Pollutants can be observed by either active or passive remote sensing systems. Calculations discussed herein indicate that tropospheric CO, CO2, SO2, NO2, NH3, HCHO, and CH4 can be measured by means of nadir looking passive systems. Additional species such as NO, HNO3, O3, and H2O may be measured in the stratosphere through a horizon experiment. A brief theoretical overview of resonance Raman scattering and resonance fluorescence is given. It is found that radiance measurements are most promising for general global applications, and that stratospheric aerosols may be measured using a sun occultation technique. The instrumentation requirements for both active and passive systems are examined and various instruments now under development are described.

Ludwig, C. B.↗

The polarizability of diatomic helium

The calculation of the electric dipole polarizability tensor of the He 2 dimer is described, and the results are used in the computation of several dielectric and optical properties of helium gas, at both high (322 K) and low (4 K) temperatures. The properties considered are the second dielectric virial coefficient, the second Kerr virial coefficient, and the depolarization ratio of the integrated intensities for the Raman scattering experiments. The thesis consists of five parts: the polarizability and various properties are defined; the calculation of the polarizability in the long-range region in terms of a quantum mechanical multipole expansion is described; the calculation of the He2 polarizability in the overlap region via coupled Hartree-Fock perturbation theory is described; the calculation of the quantum pair distribution function for both the He-3 and He-4 isotopes at 4 K is discussed; and the calculated values of the properties of helium gas are given.

Fortune, P. J.↗

Ultraviolet photometry from the Orbiting Astronomical Observatory. XIII - The albedos of Jupiter, Uranus, and Neptune

Presentation of OAO-2 broad-band ultraviolet photometry data for Jupiter, Uranus, and Neptune. These data have been combined with observations of 23 late-type stars to derive planetary albedos over the region 2000-4300 A. The new broad-band albedo for Jupiter agrees well with a previous measurement based on OAO-2 spectrometer data. The albedos for Uranus and Neptune are in good agreement with ground measurements in the region of overlap. The results for Uranus and Neptune have been compared with theoretical calculations for semiinfinite and finite pure H2 Rayleigh-Raman scattering atmospheres. Except for the shortest wavelengths, the measurements lie below the semiinfinite theoretical calculations. The calculations for the finite atmospheres suggest that an additional absorbing constituent will be needed to explain the observed albedos.

Savage, B. D.↗

Ruby laser induced emission from NO2

Two different types of emission from excited NO2 were observed using pulsed ruby laser light at 6943 A. The first type of fluorescence was seen in the near IR and results from the single photon excitation of NO2 from the ground 2-A1 state. By observing the emission as a function of time an unexpected behavior was observed in the near IR and could be explained by a consecutive deactivation mechanism, wherein a secondary species is preferentially detected. A second type of emission recently observed in the blue spectral region is weaker and is due to a multiphoton process. The intensity of the blue emission is a function of the cube of the laser intensity at low pressures and approaches the square at high pressures. This variation is attributed to simultaneous deactivation of the excited NO2 intermediate by collision (square) and by anti-Stokes Raman scattering off of the excited NO2 (cube).

Hakala, D. F.↗

Laser application to measure vertical sea temperature and turbidity, design phase

An experiment to test a new method was designed, using backscattered radiation from a laser beam to measure oceanographic parameters in a fraction of a second. Tyndall, Rayleigh, Brillouin, and Raman scattering all are utilized to evaluate the parameters. A beam from a continuous argon ion laser is used together with an interferometer and interference filters to gather the information. The results are checked by direct measurements. Future shipboard and airborne experiments are described.

Hirschberg, J. G.↗

Vapor transport mechanisms

The Raman scattering furnace for investigating vapor transport mechanisms was completed and checked out. Preliminary experiments demonstate that a temperature resolution of plus and minus 5 C is possible with this system operating in a backscatter mode. In the experiments presented with the GeI 4 plus excess Ge system at temperatures up to 600 C, only the GeI4 band at 150 cm superscript minus 1 was observed. Further experiments are in progress to determine if GeI2 does become the major vapor species above 440 C.

Workman, G. L.↗

Diagrammatic evaluation of the density operator for nonlinear optical calculations

Time-ordered diagrammatic representations are shown to precisely define and to simplify calculations of radiative perturbations to the density matrix. Nonlinear optical susceptibilities, here exemplified by that of CARS, can be obtained by simple propagator rules. An interpretation of transient Raman scattering in terms of time-ordered contributions is also discussed.

Yee, S. Y.↗

Investigation of laser induced parametric interactions in optical waveguides and fibers

Experimental and theoretical aspects of the laser pump depletion characteristics in an optical fiber due to stimulated Raman scattering, and stimulated Brillouin scattering were studied. A review is presented of research in fiber transmission accompanied by stimulated scattering. Results of experimental work with tunable dye lasers and argon lasers are presented. The spectral profiles of the laser pump and its transmitted light through the fiber are given.

Yu, C.↗