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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 361 records · Page 20

Optimization of X-ray event screening using ground and in-orbit data for the Resolve instrument onboard the XRISM satellite

The X-Ray Imaging and Spectroscopy Mission (XRISM) satellite was successfully launched and put into a low-Earth orbit on September 6, 2023 (UT). The Resolve instrument onboard XRISM hosts an X-ray microcalorimeter detector, which was designed to achieve a high-resolution ( ≤ 7 eV FWHM at 6 keV), high-throughput, and non-dispersive spectroscopy over a wide energy range. It also excels in a low background with a requirement of < 2 × 10 -3 s -1 keV -1 (0.3 to 12.0 keV), which is equivalent to only one background event per spectral bin per 100-ks exposure. Event screening to discriminate X-ray events from background is a key to meeting the requirement. We present the result of the Resolve event screening using data sets recorded on the ground and in orbit based on the heritage of the preceding X-ray microcalorimeter missions, in particular, the Soft X-ray Spectrometer onboard ASTRO-H. We optimize and evaluate 19 screening items of three types based on (1) the event pulse shape, (2) relative arrival times among multiple events, and (3) good time intervals. We show that the initial screening, which is applied for science data products in the performance verification phase, reduces the background rate to 1.8 × 10 -3 s -1 keV -1 meeting the requirement. We further evaluate the additional screening utilizing the correlation among some pulse shape properties of X-ray events and show that it further reduces the background rate, particularly in the < 2 keV band. Over 0.3 to 12 keV, the background rate becomes 1.0 × 10 -3 s -1 keV -1 .

47 OTHER INSTRUMENTATION↗

A Fast Radio Burst Backend for the Tianlai Dish Pathfinder Array

The Tianlai Dish Pathfinder Array is a radio interferometer array consisting of 16 six-meter dish antennas. The original digital backend integration time is at the seconds level, designed for H I intensity mapping experiment. A new digital backend with millisecond response is added to enable it to search for fast radio burst during its observations. The design and calibration of this backend, and the real time search pipeline for it are described in this paper. It is capable of forming 16 digital beams for each linear polarization, covering an area of 19.6 square degrees. The search pipeline is capable of searching for, recording and classifying FRBs automatically in real time. Finally, in commissioning, we succeeded in capturing the signal pulses from the pulsars PSR B0329+54 and B2021+51.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Multispectral and thermal surface imagery and surface elevation mosaics (camspec-air)

This dataset contains high resolution image products (orthomosaics) acquired from midsized uncrewed aerial systems, which have been processed for value added quality. The instrument itself, a multispectral imager, the Altum by Micasense, captures 6 spectral bands (red, green blue, NIR, red edge, and LWIR/thermal1) as radiance, which is converted to reflectance. The code used to develop these images first uses tools from the Micasense python library2 to apply dark level corrections, row gradient corrections, and radiometric corrections. Next it uses the processing API from Agisoft Metashape software to align and mosaic the processed imagery, following the processes developed by the USGS' structure from motion workflow documentation3. Captures at different altitudes (recorded in MSL) produce an orthomosaic, a tif image containing information related to the 6 spectral bands, and a digital elevation model (DEM), a tif image containing information related to the elevation of the surveyed terraine. Metadata included in every image can be used to extract lat, lon, and reflectance values. 1https://www.arm.gov/publications/tech_reports/handbooks/doe-sc-arm-tr-281.pdf 2https://micasense.github.io/imageprocessing/MicaSense%20Image%20Processing%20Setup.html 3https://pubs.usgs.gov/of/2021/1039/ofr20211039.pdf

54 ENVIRONMENTAL SCIENCES↗

Efficiency analysis of helium-cooled MAS DNP: case studies of surface-modified nanoparticles and homogeneous small-molecule solutions

Despite the growing number of successful applications of dynamic nuclear polarization (DNP)-enhanced magic-angle spinning (MAS) NMR in structural biology and materials science, the nuclear polarizations achieved by current MAS DNP instrumentation are still considerably lower than the theoretical maximum. Here, the method could be significantly strengthened if experiments were performed at temperatures much lower than those currently widely used (~100 K). Recently, the prospects of helium (He)-cooled MAS DNP have been increased with the instrumental developments in MAS technology that uses cold helium gas for sample cooling. Despite the additional gains in sensitivity that have been observed with He-cooled MAS DNP, the performance of the technique has not been evaluated in the case of surfaces and interfaces that benefit the most from DNP. Herein, we studied the efficiency of DNP at temperatures between ~30 K and ~100 K for organically functionalized silica material and a homogeneous solution of small organic molecules at a magnetic field B 0 = 16.4 T. We recorded the changes in signal enhancement, paramagnet-induced quenching and depolarization effects, DNP build-up rate, and Boltzmann polarization. For these samples, the increases in MAS-induced depolarization and DNP build-up times at around 30 K were not as severe as anticipated. In the case of the surface species, we determined that MAS DNP at 30 K provided ~10 times higher sensitivity than MAS DNP at 90 K, which corresponds to the acceleration of experiments by multiplicative factors of up to 100.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Foil backlighter development at the OMEGA laser facility for extended x-ray absorption fine structure experiments

Extended x-ray absorption fine structure (EXAFS) measurements require a bright and continuous x-ray source and a detection system with high spectral resolution to capture the modulations of the absorption coefficient above the material absorption edge. When performing EXAFS measurements under laser-driven dynamic compression, it is hence critical to optimize the backlighter x-ray emission. In this study, a series of experiments has been conducted at the OMEGA laser facility to characterize titanium (Z = 22), iron (Z = 26), germanium (Z = 32), molybdenum (Z = 42), silver (Z = 47), and gold (Z = 79) foil backlighters irradiated with 3 kJ–12 kJ of laser energy. The spectra have been recorded using a dual crystal spectrometer (DCS), a two-channel transmission spectrometer covering 11 keV–45 keV and 19 keV–90 keV energy bands. The DCS has been calibrated so that the spectral intensities can be compared between different campaigns.

47 OTHER INSTRUMENTATION↗

Fusion product measurements by nuclear diagnostics in the Joint European Torus deuterium–tritium 2 campaign (invited)

We report a new deuterium–tritium experimental, DTE2, campaign has been conducted at the Joint European Torus (JET) between August 2021 and late December 2021. Motivated by significant enhancements in the past decade at JET, such as the ITER-like wall and enhanced auxiliary heating power, the campaign achieved a new fusion energy world record and performed a broad range of fundamental experiments to inform ITER physics scenarios and operations. New capabilities in the area of fusion product measurements by nuclear diagnostics were available as a result of a decade long enhancement program. These have been tested for the first time in DTE2 and a concise overview is provided here. Confined alpha particle measurements by gamma-ray spectroscopy were successfully demonstrated, albeit with limitations at neutron rates higher than some 10 17 n/s. High resolution neutron spectroscopy measurements with the magnetic proton recoil instrument were complemented by novel data from a set of synthetic diamond detectors, which enabled studies of the supra-thermal contributions to the neutron emission. In the area of escaping fast ion diagnostics, a lost fast ion detector and a set of Faraday cups made it possible to determine information on the velocity space and poloidal distribution of the lost alpha particles for the first time. This extensive set of data provides unique information for fundamental physics studies and validation of the numerical models, which are key to inform the physics and scenarios of ITER.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Multispectral and thermal surface imagery and surface elevation mosaics - SGP July 2022

This data set contains high-resolution image products (orthomosaics) acquired from midsized uncrewed aerial systems that have been processed for value-added quality. The instrument itself, a multispectral imager, the Altum by Micasense, captures six spectral bands (red, green blue, NIR, red edge, and LWIR/thermal1) as radiance, which is converted to reflectance via custom code. The code used to develop these images first uses tools from the Micasense Python library2 to apply dark level corrections, row gradient corrections, and radiometric corrections. Next, it uses the processing API from Agisoft Metashape software to align and mosaic the processed imagery, following the processes developed by the USGS' structure from motion workflow documentation.3 Captures at different altitudes (recorded in MSL) produce an orthomosaic, a tif image containing information related to the six spectral bands, and a digital elevation model (DEM), a tif image containing information related to the elevation of the surveyed terraine. Metadata included in every image can be used to extract lat, lon, and reflectance values. 1 https://www.arm.gov/publications/tech_reports/handbooks/doe-sc-arm-tr-281.pdf 2 https://micasense.github.io/imageprocessing/MicaSense%20Image%20Processing%20Setup.html 3 https://pubs.usgs.gov/of/2021/1039/ofr20211039.pdf

54 ENVIRONMENTAL SCIENCES↗

Chip-integrated metasurface full-Stokes polarimetric imaging sensor

Abstract Polarimetric imaging has a wide range of applications for uncovering features invisible to human eyes and conventional imaging sensors. Chip-integrated, fast, cost-effective, and accurate full-Stokes polarimetric imaging sensors are highly desirable in many applications, which, however, remain elusive due to fundamental material limitations. Here we present a chip-integrated Meta surface-based Full-Stokes Polar imetric Im aging sensor (MetaPolarIm) realized by integrating an ultrathin (~600 nm) metasurface polarization filter array (MPFA) onto a visible imaging sensor with CMOS compatible fabrication processes. The MPFA is featured with broadband dielectric-metal hybrid chiral metasurfaces and double-layer nanograting polarizers. This chip-integrated polarimetric imaging sensor enables single-shot full-Stokes imaging (speed limited by the CMOS imager) with the most compact form factor, records high measurement accuracy, dual-color operation (green and red) and a field of view up to 40 degrees. MetaPolarIm holds great promise to enable transformative applications in autonomous vision, industry inspection, space exploration, medical imaging and diagnosis.

47 OTHER INSTRUMENTATION↗

Diagnosing low-mode (ℓ < 6) and mid-mode (6 ≤ ℓ ≤ 60) asymmetries in the post-stagnation phase of laser-direct-drive deuterium–tritium cryogenic implosions on OMEGA

Low- and mid-mode perturbations are possible candidates for performance limitations in cryogenic direct-drive implosions on the OMEGA laser at the Laboratory of Laser Energetics. Simulations with a 3D hydrocode demonstrated that hotspot imagers do not show evidence of the shell breakup in the dense fuel. However, these same simulations revealed that the low- and mid-mode perturbations in the dense fuel could be diagnosed more easily in the post-stagnation phase of the implosion by analyzing the peak in the x-ray emission limb at the coronal–fuel interface than before or at the stagnation phase. In experiments, the asymmetries are inferred from gated images of the x-ray emission of the implosion by using a 16-pinhole array imager filtered to record x-ray energies >800 eV and an x-ray framing camera with 40-ps time integration and 20-μm spatial resolution. Furthermore, a modal analysis is applied to the spatial distribution of the x-ray emission from deuterium and tritium cryogenic implosions on OMEGA recorded after the bang time to diagnose the low- and mid-mode asymmetries, and to study the effect that the beam-to-target ratio (Rb/Rt) has on the shell integrity.

47 OTHER INSTRUMENTATION↗

Low-cost sensors and analytics for a digital factory

ORNL Manufacturing Demonstration Facility and Perisense worked on a low-cost solution for machining process monitoring to enable a digital factory. Enabling machine connectivity for digital factors is expensive for many small to medium manufacturers. The hypothesis for the research project is that a lowcost sensor suite, which can be retrofitted to a legacy machine tool or a new machine tool, can effectively provide real-time, in-situ sensing for manufacturing processes, which can enable improvements in process performance and efficiency. The Perisense sensor node was installed on the Haas TM1 machine with a current sensor and an accelerometer. Cutting tests were performed at different process parameters and sensor data was recorded. Results show a correlation of the current sensor to the spindle load. The accelerometer, mounted on the machine base, showed a correlation to the spindle speed as well as the spindle load. The sensor data can be used to monitor the machining process and provide insights on the machine spindle load utilization.

42 ENGINEERING↗

Photon-shot-noise-limited transient absorption soft X-ray spectroscopy at the European XFEL

Femtosecond transient soft X-ray absorption spectroscopy (XAS) is a very promising technique that can be employed at X-ray free-electron lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here, a dedicated setup for soft X-rays available at the Spectroscopy and Coherent Scattering (SCS) instrument at the European X-ray Free-Electron Laser (European XFEL) is presented. It consists of a beam-splitting off-axis zone plate (BOZ) used in transmission to create three copies of the incoming beam, which are used to measure the transmitted intensity through the excited and unexcited sample, as well as to monitor the incoming intensity. Since these three intensity signals are detected shot by shot and simultaneously, this setup allows normalized shot-by-shot analysis of the transmission. For photon detection, an imaging detector capable of recording up to 800 images at 4.5 MHz frame rate during the FEL burst is employed, and allows a photon-shot-noise-limited sensitivity to be approached. The setup and its capabilities are reviewed as well as the online and offline analysis tools provided to users.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Single-Particle Soot Photometer (SP2) Black Carbon Number and Mass Concentrations

The single-particle soot photometer (SP2) records particle-by-particle measurements of the intensity of both the scattering signature and incandescence signature of particles that enter its laser beam. These intensities are then used to calculate refractory black carbon (rBC) masses and particle diameters. In previous U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility field campaigns, the SP2 data was difficult to process because the manufacturer-supplied code was not scalable to distributed machines, making it unusable for the large amounts of data output by the SP2. This prohibited the SP2 from becoming an operational instrument for ARM. Therefore, PySP2 was developed to solve this issue and enable SP2 to be an operational instrument for ARM. This technical document summarizes the test data sets from the ARM North Slope of Alaska (NSA) site and the Multidisciplinary Drifting Observatory for the Study of Arctic Climate (MOSAiC) field campaign that were used to develop and test PySP2.

54 ENVIRONMENTAL SCIENCES↗

Leaf temperature raw data, 2015 - 2017, at Manaus, Brazil

This data package contains raw leaf surface temperature data from the NGEE Tropics K34 tower site on a plateau near Manaus, Brazil, including automated and manually collected time series data on leaf surface temperature (thermocouples, IR radiometer, thermocamera). Leaf surface temperature (LST) was determined throughout diurnal periods using individual type T thermocouples (Omega Engineering) on 8 individual leaves of a single tree. Mature leaves at the same height and general area near the tower were selected. LST measurements were taken every 15 s and recorded on a field portable self-powered data logger (OM-CP-OCTTEMP-A, Omega Engineering). Measurements were stopped in the case of a storm or rain which can remove the attached thermocouple wires from the leaf due to large wind-driven branch movements. Included in the attached zip file are six folders: three with LST data in Excel and CSV file formats from both the K34 and B34 towers, one folder with data logger configuration programs that were used for data collection, a fifth folder with PDF files of manuals for instruments used and a final folder with two Excel metadata files. See dataset references for associated metadata package. This dataset replaces the leaf surface temperature data of two retired packages, http://dx.doi.org/10.15486/ngt/1507764 and http://dx.doi.org/10.15486/ngt/1507767

54 ENVIRONMENTAL SCIENCES↗

List Mode Data from the Modular Vehicle Detector System

In 2022 measurements were made with the Modular Vehicle Detectors (MVD) at the National Criticality Experiments Research Center (NCERC), located in the Device Assembly Facility (DAF) on the Nevada National Security Site (NNSS), Nevada. These detectors were supplied by the Naval Information Warfare Center (NIWC) Pacific. The MVDs were connected to an Advanced List Mode Module (ALMM) which records when an MVD detected a neutron. This is a summary of the measurement configurations as well as a list of the list-mode data files from each configuration. In addition to the measurements taken at NCERC additional measurements with the MVDs were taken at Los Alamos National Laboratory (LANL).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Atmospheric H 2 observations from the NOAA Cooperative Global Air Sampling Network

Abstract. The NOAA Global Monitoring Laboratory (GML) measures atmospheric hydrogen (H2) in grab samples collected weekly as flask pairs at over 50 sites in the Cooperative Global Air Sampling Network. Measurements representative of background air sampling show higher H2 in recent years at all latitudes. The marine boundary layer (MBL) global mean H2 was 552.8 ppb in 2021, 20.2 ± 0.2 ppb higher compared to 2010. A 10 ppb or more increase over the 2010–2021 average annual cycle was detected in 2016 for MBL zonal means in the tropics and in the Southern Hemisphere. Carbon monoxide measurements in the same-air samples suggest large biomass burning events in different regions likely contributed to the observed interannual variability at different latitudes. The NOAA H2 measurements from 2009 to 2021 are now based on the World Meteorological Organization Global Atmospheric Watch (WMO GAW) H2 mole fraction calibration scale, developed and maintained by the Max Planck Institute for Biogeochemistry (MPI-BGC), Jena, Germany. GML maintains eight H2 primary calibration standards to propagate the WMO scale. These are gravimetric hydrogen-in-air mixtures in electropolished stainless steel cylinders (Essex Industries, St. Louis, MO), which are stable for H2. These mixtures were calibrated at the MPI-BGC, the WMO Central Calibration Laboratory (CCL) for H2, in late 2020 and span the range 250–700 ppb. We have used the CCL assignments to propagate the WMO H2 calibration scale to NOAA air measurements performed using gas chromatography and helium pulse discharge detector instruments since 2009. To propagate the scale, NOAA uses a hierarchy of secondary and tertiary standards, which consist of high-pressure whole-air mixtures in aluminum cylinders, calibrated against the primary and secondary standards, respectively. Hydrogen at the parts per billion level has a tendency to increase in aluminum cylinders over time. We fit the calibration histories of these standards with zero-, first-, or second-order polynomial functions of time and use the time-dependent mole fraction assignments on the WMO scale to reprocess all tank air and flask air H2 measurement records. The robustness of the scale propagation over multiple years is evaluated with the regular analysis of target air cylinders and with long-term same-air measurement comparison efforts with WMO GAW partner laboratories. Long-term calibrated, globally distributed, and freely accessible measurements of H2 and other gases and isotopes continue to be essential to track and interpret regional and global changes in the atmosphere composition. The adoption of the WMO H2 calibration scale and subsequent reprocessing of NOAA atmospheric data constitute a significant improvement in the NOAA H2 measurement records.

Pétron, Gabrielle↗

Evaluation of an x-ray multilayer mirror for radiography at sub-1-keV photon energies

An x-ray multilayer mirror on a spherical substrate designed for near-normal incidence with a photon energy of ~738 eV (F He α ) was procured and tested. This device is intended to be used for in-flight radiography of the shell in inertial confinement fusion experiments with cryogenic targets on the OMEGA laser at the Laboratory for Laser Energetics. Experiments in self-emission on a small (~10 J) laser system showed that the reflectivity of the mirror is high enough to record an image at laser energies as low as 0.1 J. Furthermore, a second set of tests in backlighting geometry on a larger (kJ)-scale, short-pulse laser yielded usable radiographs with laser energies as low as 40 J with a spatial resolution of ~10 μm.

47 OTHER INSTRUMENTATION↗

Ultraviolet digital holographic microscopy (DHM) of micron-scale particles from shocked Sn ejecta

A cloud of very fast, O (km/s), and very fine, O (µm), particles may be ejected when a strong shock impacts and possibly melts the free surface of a solid metal. To quantify these dynamics, this work develops an ultraviolet, long-working distance, two-pulse Digital Holographic Microscopy (DHM) configuration and is the first to replace film recording with digital sensors for this challenging application. A proposed multi-iteration DHM processing algorithm is demonstrated for automated measures of the sizes, velocities, and three-dimensional positions of non-spherical particles. Ejecta as small as 2 µm diameter are successfully tracked, while uncertainty simulations indicate that particle size distributions are accurately quantified for diameters ≥4 µm. These techniques are demonstrated on three explosively driven experiments. Measured ejecta size and velocity statistics are shown to be consistent with prior film-based recording, while also revealing spatial variations in velocities and 3D positions that have yet to be widely investigated. Having eliminated time-consuming analog film processing, the methodologies proposed here are expected to significantly accelerate future experimental investigation of ejecta physics.

47 OTHER INSTRUMENTATION↗

Integrated Risk-Informed Condition Based Maintenance Capability and Automated Platform: Technical Report 3

This project is a collaborative research effort between PKMJ Technical Services LLC, Idaho National Laboratory, and Public Service Enterprise Group (PSEG) Nuclear, LLC. The collaboration, led by PKMJ Technical Services LLC, is part of the industry Funding Opportunity Announcement (FOA) award under Advanced Nuclear Technology Development FOA #DE-FOA-0001817. The pilot demonstration focuses on the Circulating Water System (CWS), an important non-safety-related system that impacts the power generation capability of the plant site. Achieving riskinformed condition-based Predictive Maintenance (PdM) on the CWS will result in significant economic benefits, and the developed methodologies can also be applied to other plant systems. This approach supports an industry goal of ensuring that nuclear power generation remains a viable, economically competitive option in the energy market. Operation and Maintenance (O&M) costs include labor-intensive Preventive Maintenance (PM) programs that involve manually performed inspection, calibration, testing, and maintenance of plant assets at periodic frequencies as well as time-based replacement of assets, irrespective of condition. This project offers an alternative by focusing on riskinformed condition-based maintenance to reduce O&M costs while still maintaining plant health and safety. This report summarizes the progress made toward achieving a risk-informed condition-based maintenance approach. The research and development (R&D) activities presented in this report are associated with development of a nuclear digital platform application, integration of fault signature models, and automated work management processes. The fault signatures and Machine Learning (ML) models are key components in predictive analytics and are heavily leveraged to improve the insights received by existing plant process data sources. Availability of the analysis results within a centralized digital platform enhances efficiency by enabling automation of activities otherwise performed manually. Personnel are presented with enhanced information that can be used to evaluate plant status and risks. Utilizing the enhancements to data analytics supports automated responses, (i.e. issuance of work orders) to address developing equipment faults and thus preventing forced, unplanned shutdowns of components or systems. The R&D activities described within this report lay the foundation for developing and demonstrating a digital automated platform to centralize the implementation of condition monitoring and response to equipment faults. The digital automated platform is cloud-based and designed to enable improved efficiency of plant processes. The digital platform includes content related to maintenance optimization, fault signature analysis, and plant records, which can all be used to support efficiencies when located within a centralized digital platform. These efficiencies could be further enhanced when deployed through industry-wide deployment of the technology to improve insights and processes based upon economies of scale.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗