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At least 361 records · Page 20

Electron impact excitation of atomic oxygen - Revised cross sections

Revised cross-section values for the excitation of three O I resonance transitions at 1304, 1027, and 989 A, by electron impact on atomic oxygen are presented from threshold to 300 eV. These results are smaller than the excitation cross sections used in some airglow models by a factor of about 2.8. The revised values are in good agreement with recent quantum-scattering calculations. The downward revision is required by new laboratory studies in which the direct and dissociative cross sections for 1304 A excitation were normalized with small probable error to the O and O2 ionization cross sections. The results also reflect new advances in VUV optical calibration techniques. A number of outstanding airglow problems are simplified by these revisions.

Zipf, E. C.↗

Evaluation of an Ultra-Low Power Reed Solomon Encoder for NASA's Space Technology 5 Mission

Radiation test results and analyses are presented for ultra-low power Reed Solomon encoder circuits that are being considered for use on the Space Technology 5 (ST5) mission. The total ionizing dose tolerance is in excess of 100 krad(Si) and is due to the low supply voltage and the use of back-bias, which suppresses radiation-induced leakage currents in the n-channel devices. The circuits do not latch-up for ion LET values of at least 90 MeV-sq cm/mg. A hardened-by-design approach to SEU has achieved an upset threshold of about 20 MeV-sq cm/mg. The SEU rate expected for these circuits in the geosynchronous transfer orbit of ST5 is low.

Lei, K. E.↗

Test GammaPix™ Radiation Detection Software with Smartphones

GammaPix™ is a smartphone application that uses smartphone cameras to detect ionizing radiation. Brookhaven National Laboratory (BNL) evaluated the performance of the software in detecting radioactive materials. For this purpose, a series of tests were conducted at the Radiation Calibration Facility Annex at BNL. The experiments included dose measurements with three types of NIST-traceable calibration sources, 60Co, 241Am, and 137Cs. The recorded results by GammaPix™ were compared with the values measured by calibrated dosimeters to determine the detection thresholds. Several selected models of iPhones and Android cell phones with different pixel sizes and resolution were tested. In this paper, we present the test procedures and discuss the test results.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A sub-5 ps jitter time-to-digital converter ASIC with back-gate delay tuning in 22 nm CMOS

We present the design of a Time-to-Digital Converter (TDC) ASIC together with performance characterization results at cryogenic temperature (6-8 K), and at room temperature using emulated Low-Gain Avalanche Detector (LGAD) signals. The TDC design uses a two-step architecture with a ring-oscillator based counter and a Vernier delay line fine TDC. The TDC is implemented in an FD-SOI process, and back-gate tuning is used not only to correct threshold variation due to cryogenic operation, but also as a novel way to tune TDC delay elements with very little overhead. Using this technique, we demonstrate a design with very low power (0.5 mW) and area (0.003 mm 2 ). We present test results using the Fermilab Constant Fraction Discriminator (FCFD) ASIC to produce discriminated signals from an internal charge injection mechanism that mimics the waveform and signal amplitude of minimum ionizing particles impinging on LGAD sensors. We characterize the time precision of the full system and verify that the TDC ASIC contributes a negligible amount to the total system time precision, fully consistent with the expected jitter contribution of less than 5 ps. In conclusion, the results presented here demonstrate the utility of our TDC for applications in physics and quantum communications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Tonopah Test Range Air Monitoring: CY2017 Meteorological, Radiological, and Wind Transported Particulate Observations

In 1963, the U.S. Department of Energy (DOE) (formerly the Atomic Energy Commission [AEC]), implemented Operation Roller Coaster on the Tonopah Test Range (TTR) and an adjacent area of the Nevada Test and Training Range (NTTR) (formerly the Nellis Air Force Range). This operation resulted in radionuclide-contaminated soils at the Double Tracks site and Clean Slate I, II, and III sites. This report documents observations made during ongoing monitoring of radiological, meteorological, and dust conditions at stations installed adjacent to the Clean Slate sites and at the TTR Sandia National Laboratories (SNL) Range Operations Center (ROC). The primary objective of the monitoring effort is to support the DOE Environmental Management Nevada Program (EM NV) in the safe cleanup of the environmental legacy of nuclear device development and testing by determining if wind blowing across the Clean Slate sites is transporting particles of radionuclide-contaminated soil beyond the physical and administrative boundaries of the sites. The monitoring program underwent a significant change during 2017 with the decommissioning of one monitoring station and the establishment of three new stations. Station 400, located within TTR Area 3 and near the ROC, monitors conditions near the local workforce center and was in operation the full calendar year. Stations 401 and 403 are located on the northwest and southeast perimeter fence lines, respectively, of the Clean Slate III site. Station 401 operated throughout 2017, whereas Station 403 began operation at the end of April 2017. Stations 404 and 405 are along the northern and eastern boundary fence, respectively, at Clean Slate II and both began data collection at the end of April 2017. Also at the end of April, the Clean Slate I monitoring site, Station 402, was decommissioned. The stations are located to be generally downwind of the contaminated areas during either north-northwesterly or south-southeasterly winds, which are the predominant wind directions. The stations—which are similar in design to the Community Environmental Monitoring Program (CEMP) stations operating at locations surrounding the Nevada National Security Site and TTR—include meteorological instruments and continuous-flow, low-volume air samplers. Three pressurized ionization chambers for measuring gamma energy are in use at Stations 400, 401, and 403 (formerly at 402). Saltation sensors and saltation traps are deployed at the stations adjacent to the Clean Slate sites. Detailed meteorological data are recorded on data loggers, with periodic uploads via a satellite system to the Western Regional Climate Center (WRCC) at Desert Research Institute (DRI), to monitor instrument and site conditions. Air filter samples are collected every two weeks and the deposits in the saltation traps are collected when a sufficient sample mass for analysis has accumulated (generally a six- to eight-month interval). Dust transport by suspension and saltation is strongly dependent on wind speed. Concentrations of PM10 (particulate matter of aerodynamic diameter ≤10 micrometers [μm], a size fraction of small particles that are suspended in the air and can be easily inhaled) remain low until winds exceed approximately 32 km/hr (20 mph). Saltation particle counts also increase above the same general threshold wind speed. Wind speeds in excess of 32 km/hr (20 mph) occur less than three percent of the time. High winds are associated with two predominant directions: north-northwest and south. In 2017, the very highest winds were from the north, but all winds above 40 km/hr (25 mph) were approximately evenly split between south and northwest directions. The low-volume air samplers collect total suspended dust, and saltating particles are captured by the passive saltation traps, both for radiological analysis. Radionuclide monitoring at the ROC in TTR Area 3 (Station 400) found natural background levels of gross alpha and gross beta radiation. Similar background levels were found on filter samples analyzed using gamma and alpha spectroscopy. The gamma exposure rate data from pressurized ionization chambers (PIC) are comparable to those from the regional CEMP stations. Plutonium concentrations above background values were measured during 2017 from soil samples collected in passive saltation traps and on select air filters from the monitoring stations adjacent to the Clean Slate sites. The background for soils in the region is assumed to be 0.014 pCi/g plutonium-239+240 ( 239+240 Pu) as measured by Turner et al. (2003), whereas the background concentration of suspended 239+240Pu is assumed to be 9.5 x 10 -19 μCi/ml, which was determined by continuous air monitoring at the TTR airport in 1996 and 1997 (SNL, 1998). Background concentrations are exceeded by one to four orders of magnitude by the majority of samples from Clean Slate I, II, and III. The gross alpha and gross beta measurements of the air filters are also generally higher than those measured at the regional CEMP stations, although the gamma exposure rates determined by the PICs located at Clean Slate I and III are similar to CEMP measurements. The highest radionuclide concentrations of suspended dust are associated with individual filter samples from Clean Slate II Station 404 and Clean Slate III Station 401. Both of the stations are downwind of their respective sites during southerly winds, but they are also geographically closer to the highly contaminated detonation areas than the other monitoring stations. Considering all the analyzed samples, the 239+240Pu concentrations are generally higher for the Clean Slate II samples compared with those from Clean Slate III. The highest gross alpha and gross beta results are also observed for the Clean Slate II stations. The highest radionuclide concentrations are measured on the smaller (≤63 μm) saltation-sized particles and particulate matter collected downwind of each site. Nonetheless, traps oriented to collect dust moving toward the contamination areas also had plutonium concentrations significantly above background values, which is consistent with observations of low-level contamination dispersed beyond the fenced area. All the observed 239+240 Pu concentrations are below the risk-based action level (25 millirem per year, equivalent to a 239+240 Pu concentration of 4,120 pCi/g for an industrial worker scenario; U.S. DOE, 2014). The meteorological and particulate matter monitoring indicate that conditions for wind-borne contaminant movement exist at the Clean Slate sites, and that transport of radionuclide-contaminated soil by both suspension and saltation is occurring. The Corrective Action Unit (CAU) closure strategy uses a risk-based approach, whereby acceptable contaminant concentrations are determined as a function of anticipated human exposure. This strategy is consistent with the fence lines at the Clean Slate sites encircling areas of higher concentration and the observed presence of lower concentrations of contamination outside the fences.

54 ENVIRONMENTAL SCIENCES↗

Decreasing Proton Single Event Effects in CubeSats with Shielding

Shields-1, NORAD ID 43850,has been operating in polar low earth orbit since December 2018. The shielding has resulted in a lower total ionizing dose over time than typical aluminum thin-walled CubeSat structures. The reduced ionizing dosage caused by Shields-1 increases the reliability of commercial parts and reduces internal charging. Furthermore, the Shields-1 shielding reduces the ionizing particle fluence inside the spacecraft that contributes to the ionizing dose. NOVICE Sigma shielding software, using the (Aerospace Proton) AP8 –(Aerospace Electron) AE8 solar minimum trapped belt environment for a 1-year mission, estimates a 21.3 g/cm2 aluminum effective shielding for the Shields-1 electronics enclosure. This high areal density reduces not only the total number of energetic protons, but also reduces the number of ionizing particles over all modeled energies from the estimated shielded fluence for a 1-year mission. NOVICE Adjoint CAD modeling of the Shields-1 structure, with the detector located within the electronics enclosure, estimates that the total number of particles is reduced from 2.20x 10exp9 protons/cm2 to 1.52x 10exp8 protons/cm2, which represents 6.90% of the remaining particles(figure 1). By slowing down approximations of the integral proton fluence, a minimum proton threshold is estimated at 151 MeV. In comparison, a 0.204-cm aluminum thin-walled 3-unit (U) structure, with a 0.907 g/cm2 effective shielding, has 25.0% remaining particles and a minimum proton threshold of 36.2 MeV(figure 1). Proton energies that contribute to single event effects in radiation tolerant or higher semiconductor hardness are typically 100 MeV and higher. The Shields-1 electronics enclosure is estimated to attenuate energies: 100 MeV by 76.5%, 200 MeV by 61.7%, and 500 MeV by 63.0%(figure 2), when comparing the space environment proton differential fluence with the shielded differential fluence. The aluminum thin-walled structure is estimated to attenuate proton energies: 100 MeV by 13.7%, 200 MeV by 12.4%, and 500 MeV by 12.6%(figure 2), which are lower than for the Shields-1 electronics enclosure. The significant differences in attenuation between the Shields-1 electronics enclosure and aluminum thin-walled 3U structure show the additional utility of increasing shielding effectiveness for reducing the numbers of energetic protons that contribute to single event effects.

Larry Thomsen↗

Modeling and Numerical Simulation of Microwave Pulse Propagation in Air Breakdown Environment

Numerical simulation is used to investigate the extent of the electron density at a distant altitude location which can be generated by a high-power ground-transmitted microwave pulse. This is done by varying the power, width, shape, and carrier frequency of the pulse. The results show that once the breakdown threshold field is exceeded in the region below the desired altitude location, electron density starts to build up in that region through cascading breakdown. The generated plasma attenuates the pulse energy (tail erosion) and thus deteriorates the energy transmission to the destined altitude. The electron density saturates at a level limited by the pulse width and the tail erosion process. As the pulse continues to travel upward, though the breakdown threshold field of the background air decreases, the pulse energy (width) is reduced more severely by the tail erosion process. Thus, the electron density grows more quickly at the higher altitude, but saturates at a lower level. Consequently, the maximum electron density produced by a single pulse at 50 km altitude, for instance, is limited to a value below 10(exp 6) cm(exp -3). Three different approaches are examined to determine if the ionization at the destined location can be improved: a repetitive pulse approach, a focused pulse approach, and two intersecting beams. Only the intersecting beam approach is found to be practical for generating the desired density level.

Kuo, S. P.↗

Photoionization of the Fe lons: Structure of the K-Edge

X-ray absorption and emission features arising from the inner-shell transitions in iron are of practical importance in astrophysics due to the Fe cosmic abundance and to the absence of traits from other elements in the nearby spectrum. As a result, the strengths and energies of such features can constrain the ionization stage, elemental abundance, and column density of the gas in the vicinity of the exotic cosmic objects, e.g. active galactic nuclei (AGN) and galactic black hole candidates. Although the observational technology in X-ray astronomy is still evolving and currently lacks high spectroscopic resolution, the astrophysical models have been based on atomic calculations that predict a sudden and high step-like increase of the cross section at the K-shell threshold (see for instance. New Breit-Pauli R-matrix calculations of the photoionization cross section of the ground states of Fe XVII in the region near the K threshold are presented. They strongly support the view that the previously assumed sharp edge behaviour is not correct. The latter has been caused by the neglect of spectator Auger channels in the decay of the resonances converging to the K threshold. These decay channels include the dominant KLL channels and give rise to constant widths (independent of n). As a consequence, these series display damped Lorentzian components that rapidly blend to impose continuity at threshold, thus reformatting the previously held picture of the edge. Apparent broadened iron edges detected in the spectra of AGN and galactic black hole candidates seem to indicate that these quantum effects may be at least partially responsible for the observed broadening.

Palmeri, P.↗

Dissociative Ionization and Product Distributions of Benzene and Pyridine by Electron Impact

We report a theoretical study of the dissociative ionization (DI) and product distributions of benzene (C6H6) and pyridine (C5H5N) from their low-lying ionization channels. Our approach makes use of the fact that electronic motion is much faster than nuclear motion allowing DI to be treated as a two-step process. The first step is the electron-impact ionization resulting in an ion with the same nuclear geometry as the neutral molecule. In the second step, the nuclei relax from the initial geometry and undergo unimolecular dissociation. For the ionization process we use the improved binary-encounter dipole (iBED) model [W.M. Huo, Phys. Rev. A64,042719-I (2001)]. For the unimolecular dissociation, we use multiconfigurational self-consistent field (MCSCF) methods to determine the steepest descent pathways to the possible product channels. More accurate methods are then used to obtain better energetics of the paths which are used to determine unimolecular dissociation probabilities and product distributions. Our analysis of the dissociation products and the thresholds of their productions for benzene are compared with the recent dissociative photoionization meausurements of benzene by Feng et al. [R. Feng, G. Cooper, C.E. Brion, J. Electron Spectrosc. Relat. Phenom. 123,211 (2002)] and the dissociative photoionization measurements of pyridine by Tixier et al. [S. Tixier, G. Cooper, R. Feng, C.E. Brion, J. Electron Spectrosc. Relat. Phenom. 123,185 (2002)] using dipole (e,e+ion) coincidence spectroscopy.

Dateo, Christopher E.↗

s-wave threshold in electron attachment - Results in 2-C4F6 and CFCl3 at ultra-low electron energies

Electron attachment lineshapes and cross sections are reported for the processes 2-C4F6(-)/2-C4F6 and Cl(-)/CFCl3 at electron energies of 0-120 and 0-140 meV, and at resolutions of 6 and 7 meV (FWHM), respectively. As in previous measurements in CCl4 and SF6, the results show resolution-limited narrow structure in the cross section at electron energies below 15 meV. This structure arises from the divergence of the s-wave cross section in the limit of zero electron energy. Comparisons are given with swarm-measured results, and with collisional ionization (high-Rydberg attachment) data in this energy range.

Chutjian, A.↗

Molecular photoionization processes of astrophysical and aeronomical interest

An account is given of aspects of photoionization processes in molecules, with particular reference to recent theoretical and experimental studies of partial cross sections for production of specific final electronic states and of parent and fragment ions. Such cross sections help provide a basis for specifying the state of excitation of the ionized medium, are useful for estimating the kinetic energy distributions of photoejected electrons and fragment ions, provide parent-and fragment-ion yields, and clarify the possible origins of neutral fragments in highly excited rovibronic states. A descriptive account is given of photoionization phenomena, including tabulation of valence- and inner-shell potentials for some molecules of astrophysical and aeronomical interest. Cross sectional expressions are given. Various approximations currently employed in computational studies are described briefly, threshold laws and high-energy limits are indicated, and distinction is drawn between resonant and direct photoionization phenomena. Recent experimental and theoretical studies of partial photoionization cross sections in selected compounds of astrophysical and aeronomical relevance are described and discussed.

Langhoff, P. W.↗

Scintillation light detection performance for the DUNE ND-LAr 2 × 2 modules

The Deep Underground Neutrino Experiment (DUNE) will be using a liquid argon time projection chamber (LAr TPC) with optically separated modules in the Near Detector (ND) complex. A prototype experiment, DUNE ND-LAr 2 × 2, is composed of four test modules. They detect ionization charge through a pixel-based readout and scintillation light through fibers in light collection modules and light traps called ArCLights. The light detection performance for two modules of DUNE ND-LAr 2 × 2 that took cosmic ray data at the University of Bern is shown. We present further the role of the 2 × 2 prototype in DUNE and how it is used to demonstrate the reconstruction capabilities of its light detectors in terms of energy thresholds and timing resolution.

47 OTHER INSTRUMENTATION↗

Scintillation light detection performance for the DUNE ND-LAr 2 × 2 modules

The Deep Underground Neutrino Experiment (DUNE) will be using a liquid argon time projection chamber (LAr TPC) with optically separated modules in the Near Detector (ND) complex. A prototype experiment, DUNE ND-LAr 2 × 2, is composed of four test modules. They detect ionization charge through a pixel-based readout and scintillation light through fibers in light collection modules and light traps called ArCLights. The light detection performance for two modules of DUNE ND-LAr 2 × 2 that took cosmic ray data at the University of Bern is shown. We present further the role of the 2 × 2 prototype in DUNE and how it is used to demonstrate the reconstruction capabilities of its light detectors in terms of energy thresholds and timing resolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Classifying the full SDSS-IV MaNGA Survey using optical diagnostic diagrams: Presentation of AGN catalogs in flexible apertures

Accurate active galactic nucleus (AGN) identifications in large galaxy samples are crucial for the assessment of the role of AGN and AGN feedback in the co-evolution of galaxies and their central supermassive black holes. Emission-line flux-ratio diagnostics are commonly used to identify AGN in optical spectra. New large samples of integral field unit observations allow exploration of the role of aperture size in the classification process. In this paper, we present galaxy classifications for all 10010 galaxies observed within the Mapping Nearby Galaxies at Apache Point Observatory (MaNGA) survey. We use Baldwin-Philips-Terlevich line flux-ratio diagnostics combined with an Hα equivalent threshold in 60 apertures of varying size for the classification, and provide the corresponding catalogs. MaNGA-selected AGN primarily lie below the main sequence of star-forming galaxies, and reside in massive galaxies with stellar masses of ~10 11 M ⊙ and a median Hα-derived star formation rate of ~1.44M ⊙ yr -1 . We find that the number of “fake” AGN increases significantly beyond selection apertures of >1.0 R eff because of increased contamination from diffuse ionized gas (DIG). A comparison with previous works shows that the treatment of the underlying stellar continuum and flux measurements can significantly impact galaxy classification. Our work provides the community with AGN catalogs and galaxy classifications for the full MaNGA survey.

79 ASTRONOMY AND ASTROPHYSICS↗

Learned adaptive properties for mitigation of weight perturbations in embedded spiking networks

Recent years have seen an increased importance of neural network inference in edge-based scenarios, which impose size and power constraints requiring novel computing devices. These same edge scenarios may require operating over long periods of time, or exposure to extreme environments, resulting in a drift of neural network weights that cause degraded performance. In searching for ways to develop neural network approaches that perform robustly under these conditions, we propose a biologically-inspired mechanism for the dynamic adaptation of within-neuron parameters that is guided by a global context signal carrying information about perturbations and variability in incoming stimuli. Specifically, we demonstrate that adaptive voltage thresholds or neuronal time constants, when informed by a global context signal, can enable network-level mechanisms to recover from perturbed synaptic weights. Consistent with prior literature, the context-modulated approach is effective for recurrent, but not feedforward networks, by modulating network level dynamics. We demonstrate this approach successfully recovers performance in image classification tasks and spatiotemporal tracking tasks under idealized and Gaussian noise as well as for realistic perturbations from a memristive device when exposed to ionizing radiation. Finally, we discuss how this approach enables the design of robust and energy-efficient neuromorphic systems that perform well, even in resource-constrained scenarios with extreme environments such as edge processing.

context modulation↗

MCNP Simulation of the SFRC and Minimum Detection Threshold Determination (Rev. 1)

In this report the Minimum Detection Threshold (MDT) for the Spent Fuel Rod Counter (SFRC) was determined using Monte Carlo N-Particle transport computer code (MCNP). A model of the SFRC was simulated in addition to a fuel transport pipe and spent Magnox fuel at descending positions down the pipe. The neutron MDT for Magnox fuel free-falling along a discharge pipe was calculated to be equal to 4080 n/s. The gamma MDT for the same free falling fuel as measured by the SFRC’s ionization chamber was determined to be 455 γ/s. These values were determined to be a conservative value to use when the instrument is deployed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Linear polarization fractions of Fulcher- α fluorescence in electron collisions with H 2

We apply the molecular convergent close-coupling method to the calculation of linear polarization fractions for Fulcher-band fluorescence following electron-impact excitation of the H 2 d 3 Π u state. Furthermore, the results exhibit the opposite threshold behavior compared to the only previous calculations, but are in agreement with the most recent measurements for the Q(1), R(1), and Q(3) transitions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Accurate Cross Sections for Excitation of Resonance Transitions in Atomic Oxygen

Electron collision excitation cross sections for the resonance 2p(sup)4 (sup 3)P-2p(sup 3)3s (sup 3)S(sup 0), 2p(sup 4) (sup 3)P-2p(sup 3)3d (sup 3)D(sup 0), 2p4 (sup 3)P-2p(sup 3)3s (sup 3)D(sup 0), 2p(sup 4) (sup 3)P-2p(sup 3)3s (sup 3)P(sup 0) and 2p(sup 4) (sup 3)P-2s2p(sup 5) (sup 3)P(sup 0) transitions have been calculated by using the R matrix with a pseudostates approach for incident electron energies from near threshold to 100 eV. The excitation of these transition sgives rise to strong atomic oxygen emission features at 1304, 1027, 989, 878, and 792 Angstrom in the spectra of several planetary atmospheres. We included 22 spectroscopic bound and autoionizing states and 30 pseudostates in the close-coupling expansion. The target wave functions are chosen to properly account for the important correlation and relaxation effects. The effect of coupling to the continuum is included through the use of pseudostates. The contribution of the ionization continuum is significant for resonance transitions. Measured absolute direct excitation cross sections of 0 I are reported by experimental groups from the Jet Propulsion Laboratory and Johns Hopkins University. Good agreement is noted for the 2p(sup)4 (sup 3)P-2p(sup 3)3s (sup 3)S(sup 0) transition (lambda 1304 Ang) with measured cross sections from both groups that agree well with each other. There is disagreement between experiments for other transitions. Our results support the measured cross sections from the Johns Hopkins University for the 2p(sup 4) (sup 3)P-2p(sup 3)3d (sup 3)D(sup 0) and 2p4 (sup 3)P-2p(sup 3)3s (sup 3)D(sup 0) transitions, while for the 2p4 (sup 3)P-2p(sup 3)3s (sup 3)D(sup 0) transition the agreement is switched to the measured cross sections from the Jet Propulsion Laboratory.

Tayal, S. S.↗