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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS1992

Biomass Burning Airborne and Spaceborne Experiment in the Amazonas (BASE-A)

Results are presented on measurements of the trace gas and particulate matter emissions due to biomass burning during deforestation and grassland fires in South America, conducted as part of the Biomass Burning Airborne and Spaceborne Experiment in the Amazonas in September 1989. Field observations by an instrumented aircraft were used to estimate concentrations of O3, CO2, CO, CH4, and particulate matter. Fires were observed from satellite imagery, and the smoke optical thickness, particle size, and profiles of the extinction coefficient were measured from the aircraft and from the ground. Four smoke plumes were sampled, three vertical profiles were measured, and extensive ground measurements of smoke optical characteristics were carried out for different smoke types. The simultaneous measurements of the trace gases, smoke particles, and the distribution of fires were used to correlate biomass burning with the elevated levels of ozone.

Kaufman, Y. J.↗
NASA NTRS1991

Biomass burning and the production of greenhouse gases

The present discussion of related aspects of biomass burning describes a technique for estimating the instantaneous emission of trace gases generated by such fires on the basis of satellite imagery, and notes that burning results in significantly enhanced biogenic emissions of N2O, NO, and CH4. Biomass burning therefore has both immediate and long-term impacts on the trace-gas content of the atmosphere. The effects of Kuwait's oil fires, which encompass both combustion gases and particulates, are compared with those of the more general problem.

Levine, Joel S.↗
NASA NTRS1994

A trajectory modeling investigation of the biomass burning-tropical ozone relationship

The hypothesis that tropical total O3 maxima seen by the TOMS satellite derive from African biomass burning has been tested using isentropic trajectory analyses with global meteorological data fields. Two case studies from the 1989 biomass burning season demonstrate that a large fraction of the air arriving at the location of TOMS O3 maxima passed over regions of intense burning. Other trajectories initiated at a series of points over Africa and the Atlantic suggest flight strategies for field studies to be conducted in September 1992.

Pickering, Kenneth E.↗
NASA NTRS1994

Trace gas emissions to the atmosphere by biomass burning in the west African savannas

Savanna fires and atmospheric carbon dioxide (CO2) detection and estimating burned area using Advanced Very High Resolution Radiometer_(AVHRR) reflectance data are investigated in this two part research project. The first part involves carbon dioxide flux estimates and a three-dimensional transport model to quantify the effect of north African savanna fires on atmospheric CO2 concentration, including CO2 spatial and temporal variability patterns and their significance to global emissions. The second article describes two methods used to determine burned area from AVHRR data. The article discusses the relationship between the percentage of burned area and AVHRR channel 2 reflectance (the linear method) and Normalized Difference Vegetation Index (NDVI) (the nonlinear method). A comparative performance analysis of each method is described.

Frouin, Robert J.↗
NASA NTRS1994

Effects of biomass burning on summertime nonmethane hydrocarbon concentrations in the Canadian wetlands

Approximately 900 whole air samples were collected and assayed for selected C2-C10 hydrocarbons and seven halocarbons during the 5-week Arctic Boundary Layer Expedition (ABLE) 3B conducted in eastern Canadian wetland areas. In more than half of the 46 vertical profiles flown, enhanced nonmethane hydrocarbon (NMHC) concentrations attributable to plumes from Canadian forest fires were observed. Urban plumes, also enhanced in many NMHCs, were separately identified by their high correlation with elevated levels of perchloroethene. Emission factors relative to ethane were determined for 21 hydrocarbons released from Canadian biomass burning. Using these data for ethane, ethyne, propane, n-butane, and carbon monoxide enhancements from the literature, global emissions of these four NMHCs were estimated. Because of its very short atmospheric lifetime and its below detection limit background mixing ratio, 1,3-butadiene is an excellent indicator of recent combustion. No statistically significant emissions of nitrous oxide, isoprene, or CFC 12 were observed in the biomass-burning plumes encountered during ABLE 3B. The presence of the short-lived biogenically emitted isoprene at altitudes as high as 3000 m implies that mixing within the planetary boundary layer (PBL) was rapid. Although background levels of the longer-lived NMHCs in this Canadian region increase during the fire season, isoprene still dominated local hydroxyl radical photochemistry within the PBL except in the immediate vicinity of active fires. The average biomass-burning emission ratios for hydrocarbons from an active fire sampled within minutes of combustion were, relative to ethane, ethene, 2.45; ethyne 0.57; propane, 0.25; propene, 0.73; propyne, 0.06; n-butane, 0.09; i-butane, 0.01; 1-butene, 0.14; cis-2-butene, 0.02; trans-2-butene, 0.03; i-butylene, 0.07; 1,3-butadiene, 0.12; n-pentane, 0.05; i-pentane, 0.03; 1-pentene, 0.06; n-hexane, 0.05; 1-hexene, 0.07; benzene, 0.37; toluene, 0.16.

Blake, D. R.↗
NASA NTRS1994

Enhancement of acidic gases in biomass burning impacted air masses over Canada

Biomass-burning impacted air masses sampled over central and eastern Canada during the summer of 1990 as part of ABLE 3B contained enhanced mixing ratios of gaseous HNO3, HCOOH, CH3COOH, and what appears to be (COOH)2. These aircraft-based samples were collected from a variety of fresh burning plumes and more aged haze layers from different source regions. Values of the enhancement factor, delta X/delta CO, where X represents an acidic gas, for combustion-impacted air masses sampled both near and farther away from the fires, were relatively uniform. However, comparison of carboxylic acid emission ratios measured in laboratory fires to field plume enhancement factors indicates significant in-plume production of HCOOH. Biomass-burning appears to be an important source of HNO3, HCOOH, and CH3COOH to the troposphere over subarctic Canada.

Lefer, B. L.↗
NASA NTRS1990

Burning trees and bridges

Most burning of biomass is the result of human activity, and on a global scale it is increasing. Tropospheric concentrations of CO2, CO, CH4, non-methane hydrocarbons, and ozone are all increasing with time; global biomass burning may make an important contribution to this increase and thus to potential global climate change. The nitrogen cycle also can have important climatic effects. Nitrous oxide put into the atmosphere by biomass burning is a greenhouse gas 250 times more powerful (molecule for molecule) than carbon dioxide. Nitric oxide, as well as being a photochemical precursor of ozone, a major pollutant in the troposphere, produces nitric acid, the fastest-growing component of acid rain. Hence, the new bridge in the nitrogen cycle is of more than mere technical interest.

Levine, Joel S.↗
NASA NTRS1997

Experimental Observations of PMMA Spheres Burning at Reduced Gravity

Polymer combustion is a very complicated process which involves the coupling of gas-phase combustion, melting, pyrolysis, and possible charring of the condensed phase. Although only a few studies on the combustion of a spherically shaped polymer have been conducted, there is renewed interest in the subject. At the Third International Microgravity Combustion Workshop, we presented a preliminary experimental plan and proposed an apparatus to study the combustion of a PolyMethylMethAcrylate (PMMA) sphere at reduced gravity. In this paper, we describe the experimental hardware in detail, summarize our observations since the last workshop, and describe future studies. The main objective is to determine the burning rate of PMMA spheres at reduced gravity under different ambient oxygen concentrations and total pressures. The dependence of the burning rate on the initial sphere diameter will be examined. It is anticipated that the simple spherical geometry in conjunction with reduced gravity will facilitate an assessment of the effect of condensed phase behavior on polymer burning processes and can be used as a means to test polymer combustion models.

Yang, Ji-Ann C.↗
NASA NTRS1997

The Impact of Aerosols Generated from Biomass Burning, Dust Storms, and Volcanoes Upon the Earth's Radiative Energy Budget

A new technique for detecting aerosols from biomass burning and dust is developed. The radiative forcing of aerosols is estimated over four major ecosystems in South America. A new smoke and fire detection scheme is developed for biomass burning aerosols over South America. Surface shortware irradiance calculations are developed in the presence of biomass burning aerosols during the SCAR-B experiment. This new approach utilizes ground based, aircraft, and satellite measurements.

Christopher, Sundar A.↗
NASA NTRS1999

Biomass Burning Influences on the Composition of the Remote South Pacific Troposphere: Analysis Based on Observations from PEM Tropics-A

Airborne, in-situ measurements from PEM-Tropics-A (September/October 1996) are analyzed to show the presence of distinct pollution plumes in the middle-tropical troposphere of the remote South Pacific (10-30degS). These elevated plumes cause a relative maximum at about 5-7km attitude in the vertical distribution of primary and secondary species characteristic of fuel combustion and biomass burning (CO, C2H2, C2H6, CH3Cl, PAN, O3). Similar plumes were also observed at mid-latitudes in the middle troposphere during three flights east of New Zealand (40-45degS). In all, pollution plumes with CO larger than 100 ppb were observed 24 times on 7 separate flight days south of the equator. The observed plumes were generally embedded in very dry air. Ten-day back trajectory analysis supports the view that these originated from the biomass burning regions of South Africa (and South America) and were transported to the South Pacific along long-distance subsiding trajectories. The chemical composition of the southern Pacific troposphere analyzed from the PEM-Tropics-A data is compared with data from the tropical regions of the northern Pacific (PEM-West-A) and southern Atlantic (TRACE-A) during the same Sept/Oct time period. Sizable perturbations in the abundance of ozone and its key precursors, resulting from the transport of pollution originating from biomass burning sources, are observed in much of the Southern Hemispheric troposphere.

Singh, H. B.↗
NASA NTRS2000

A Model For The Burning of Teflon

Teflon has been identified as suitable material for use in oxygen-enriched atmospheres because of its low specific enthalpy of combustion that is, less than 1500 cal/gram. However, once ignited, Teflon burns in a heterogeneous reaction until total consumption or depletion of oxygen occurs. A model is developed for the burning of Teflon in pure, high-pressure oxygen, 3.4 to 68.9 MPa. The Teflon polymer chain dissociates via monomer units due to pyrolysis. These monomer units diffuse to the surface due to free convection. The model consists of coupled mass and energy balances for the polymer and an energy balance for the free convection of product gases. The model is used to obtain appropriate kinetic parameters for the dissociation and surface reactions. The model is validated against experimental measurements of Teflon discs supported on aluminum rods (2216) at oxygen pressures of 3.4, 6.8, 34.4, and 68.9 MPa. The model simulates the temperature distribution in the product gases above burning Teflon.

Waller, Jess M.↗
NASA NTRS2001

Tropospheric Ozone and Biomass Burning

This paper studies the significance of pyrogenic (e.g., biomass burning) emissions in the production of tropospheric ozone in the tropics associated with the forest and savanna fires in the African, South American, and Indonesian regions. Using aerosol index (Al) and tropospheric column ozone (TCO) time series from 1979 to 2000 derived from the Nimbus-7 and Earth Probe TOMS measurements, our study shows significant differences in the seasonal and spatial characteristics of pyrogenic emissions north and south of the equator in the African region and Brazil in South America. In general, they are not related to the seasonal and spatial characteristics of tropospheric ozone in these regions. In the Indonesian region, the most significant increase in TCO occurred during September and October 1997, following large-scale forest and savanna fires associated with the El Nino-induced dry season. However, the increase in TCO extended over most of the western Pacific well outside the burning region and was accompanied by a decrease in the eastern Pacific resembling a west-to-east dipole about the date-line. The net increase in TCO integrated over the tropical region between 15 deg N and 15 deg S was about 6-8 Tg (1 Tg = 10(exp 12) gm) over the mean climatological value of about 72 Tg. This increase is well within the range of interannual variability of TCO in the tropical region and does not necessarily suggest a photochemical source related to biomass burning. The interannual variability in TCO appears to be out of phase with the interannual variability of stratospheric column ozone (SCO). These variabilities seem to be manifestations of solar cycle and quasibiennial oscillations.

Chandra, Sushil↗
NASA NTRS1994

Simulating Local and Intercontinental Pollutant Effects of Biomass Burning: Integration of Several Remotely Sensed Datasets

Burning to clear land for crops and to destroy pests is an integral and largely unavoidable part of tropical agriculture. It is easy to note but difficult to quantify using remote sensing. This report describes our efforts to integrate remotely sensed data into our computer model of tropical chemical trace-gas emissions, weather, and reaction chemistry (using the MM5 mesoscale model and our own Global-Regional Atmospheric Chemistry Simulator). The effects of burning over the continents of Africa and South America have been noticed in observations from several satellites. Smoke plumes hundreds of kilometers long may be seen individually, or may merge into a large smoke pall over thousands of kilometers of these continents. These features are related to intense pollution in the much more confined regions with heavy burning. These emissions also translocate nitrogen thousands of kilometers in the tropical ecosystems, with large fixed-nitrogen losses balanced partially by locally intense fertilization downwind, where nitric acid is rained out. At a much larger scale, various satellite measurements have indicated the escape of carbon monoxide and ozone into large filaments which extend across the Tropical and Southern Atlantic Ocean. Our work relates the source emissions, estimated in part from remote sensing, in part from conventional surface reports, to the concentrations of these gases over these intercontinental regions. We will mention work in progress to use meteorological satellite data (AVHRR, GOES, and Meteosat) to estimate the surface temperature and extent and height of clouds, and explain why these uses are so important in our computer simulations of global biogeochemistry. We will compare our simulations and interpretation of remote observations to the international cooperation involving Brazil, South Africa, and the USA in the TRACE-A (Transport and Atmospheric Chemistry near the Equator - Atlantic) and SAFARI (Southern Africa Fire Atmosphere Research Initiative) and remote-sensing /aircraft/ecosystem observational campaigns.

Chatfield, Robert B.↗
NASA NTRS2002

Ram Burn Observations (RAMBO)

Ram Burn Observations (RAMBO) is a Department of Defense experiment that observes shuttle Orbital Maneuvering System engine burns for the purpose of improving plume models. On STS-107 the appropriate sensors will observe selected rendezvous and orbit adjust burns.

Source record↗
NASA NTRS2003

Preliminary Assessment Of The Burning Dynamics Of Jp8 Droplets In Microgravity

In this report we present new data for fuel droplet combustion in microgravity to examine the influence of ambient gas and fuel composition on flame structure and sooting dynamics for droplets with initial diameters in the range of 0.4mm to 0.5mm. The fuels are JP8 (a kerosene derivative) and nonane. The ambient gas is air and a mixture of 30% oxygen and 70% helium, the latter having been examined for burning under conditions where soot formation is minimal. Some data at elevated pressures are also reported. The burning process shows a nonlinear D2 progression which is independent of soot formation as burning in a helium inert showed the same nonlinear trend. Flames were proportionally farther from the droplet surface in helium than they were in air. A nondimensional parameter is presented that consolidates the three standoff distances for the droplet, flame and soot shell diameters within the initial diameter ranges examined.

Bae, J. H.↗
NASA NTRS2003

Airborne Measurements of Carbonaceous Aerosols in Southern Africa during the Dry Biomass Burning Season

Particulate matter collected aboard the University of Washington's (UW) Convair-580 research aircrafi over southem Afiica during the dry biomass burning season was analyzed for total carbon (TC), organic carbon (OC), and black carbon (BC) contents using thermal and optical methods. Samples were collected in smoke plumes of burning savanna and in regional haze. A known artifact, produced by the adsorption of organic gases on the quartz filter substrates used to collect the particulate matter samples, comprised a significant portion of the TC collected. Consequently, conclusions derived from the data are greatly dependent on whether or not OC concentrations are corrected for this artifact. For example, the estimated aerosol coalbedo (1 - single scattering albedo (SSA)), which is a measure of aerosol absorption, of the biomass smoke samples is 60% larger using corrected OC concentrations. Thus, the corrected data imply that the biomass smoke is 60% more absorbing than do the uncorrected data. The BC to (corrected) OC mass ratio (BC/OC) of smoke plume samples (0.18 plus or minus 0.06) is lower than that of samples collected in the regional haze (0.25 plus or minus 0.08). The difference may be due to mixing of biomass smoke with background air characterized by a higher BC/OC ratio. A simple source apportionment indicates that biomass smoke contributes about three quarters of the aerosol burden in the regional haze, while other souxes (e.g., fossil fuel burning) contribute the remainder.

Kirchstetter, Thomas W.↗
NASA NTRS2000

Burning Plastics Investigated in Space for Unique US/Russian Cooperative Project

It is well known that fires in the low-gravity environment of Earth-orbiting spacecraft are different from fires on Earth. The flames lack the familiar upward plume, which is the result of gravitational buoyancy. These flames, however, are strongly influenced by minor airflow currents. A recent study conducted in low gravity (microgravity) on the Russian orbital station Mir used burning plastic rods mounted in a small chamber with a controllable fan to expose the flame to airflows of different velocities. In this unique project, a Russian scientific agency, the Keldysh Research Center, furnished the apparatus and directed the Mir tests, while the NASA Glenn Research Center at Lewis Field provided the test materials and the project management. Reference testing and calibrations in ground laboratories were conducted jointly by researchers at Keldysh and at the NASA Johnson Space Center's White Sands Test Facility. Multiple samples of three different plastics were burned in the tests: Delrin, a common material for valve bodies; PMMA, a plastic "glass"; and polyethylene, a familiar material for containers and films. Each burned with a unique spherical or egg-shaped flame that spread over the rod. The effect of varying the airflow was dramatic. At the highest airflow attainable in the combustion chamber, nearly 10 cm/sec (a typical ventilation breeze), the flames were bright and strong. As airflow velocity decreased, the flames became shorter but wider. In addition, the flames became less bright, and for PMMA and polyethylene, they showed two colors, a bright part decreasing in volume and a nearly invisible remainder (see the photographs). Finally, at a very low velocity, the flames extinguished. For the plastics tested, this minimum velocity was very low, around 0.3 to 0.5 cm/sec. This finding confirms that at least a slight airflow is required to maintain a flame in microgravity for these types of materials.

Friedman, Robert↗
NASA NTRS2008

Effects of the 2006 El Nino on Tropospheric Ozone and Carbon Monoxide: Implications for Dynamics and Biomass Burning

We have studied the effects of the 2006 El Nino on tropospheric O3 and CO at tropical and sub-tropical latitudes measured from the OMI and MLS instruments on the Aura satellite. The 2006 El Nino-induced drought allowed forest fires set to clear land to burn out of control during October and November in the Indonesian region. The effects of these fires are clearly seen in the enhancement of GO concentration measured from the MLS instrument. We have used a global model of atmospheric chemistry and transport (GMI CTM) to quantify the relative irrrportance of biomass burning and large scale transport: in producing observed changes in tropospheric O3 and CO . The model results show that during October and November both biomass burning and meteorological changes contributed almost equally to the observed increase in tropospheric O3 in the Indonesian region. The biomass component was 4-6 DU but it was limited to the Indonesian region where the fires were most intense, The dynamical component was 4-8 DU but it covered a much larger area in the Indian Ocean extending from South East Asia in the north to western Australia in the south. By December 2006, the effect of biomass taming was reduced to zero and the obsemed changes in tropospheric O3 were mostly due to dynamical effects. The model results show an increase of 2-3% in the global burden of tropospheric ozone. In comparison, the global burdean of CO increased by 8-12%.

Chandra, S.↗