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At least 361 records · Page 20

Stratospheric soot - Cloud forming properties and transport processes

Soot enters the stratosphere either from the troposphere in deep thunderstorm convection, predominantly in the tropics, from midlatitude forest fires, and directly from aircraft flying above the tropopause. Particles emitted from jet aircraft are relatively ineffective as cloud droplet condensation nuclei (less than 1 percent) compared with those from forest fires (above 50 percent). Chemical and other modification during aging of the particles may influence these results in some circumstances; cloud nucleating properties can be used as a soot tracer. Such aerosols, as they grow to haze drops and ilute in increasing humidity, may form ice particles in the cold polar stratosphere or in tropical cumuli anvils at 18 to 20 km altitude at temperatures as low as -90 C. Ice may also form as particles are removed by descent through troposphere folds and enter midlatitude cirrus at levels below -40 C. In the stratosphere, ice particles may provide surfaces that catalyze heterogeneous chemical reactions; in the upper troposphere, the optical depths of cirrus clouds may be significantly increased.

Hallett, John↗

Modifications Of Discrete Ordinate Method For Computations With High Scattering Anisotropy: Comparative Analysis

A numerical accuracy analysis of the radiative transfer equation (RTE) solution based on separation of the diffuse light field into anisotropic and smooth parts is presented. The analysis uses three different algorithms based on the discrete ordinate method (DOM). Two methods, DOMAS and DOM2+, that do not use the truncation of the phase function, are compared against the TMS-method. DOMAS and DOM2+ use the Small-Angle Modification of RTE and the single scattering term, respectively, as an anisotropic part. The TMS method uses Delta-M method for truncation of the phase function along with the single scattering correction. For reference, a standard discrete ordinate method, DOM, is also included in analysis. The obtained results for cases with high scattering anisotropy show that at low number of streams (16, 32) only DOMAS provides an accurate solution in the aureole area. Outside of the aureole, the convergence and accuracy of DOMAS, and TMS is found to be approximately similar: DOMAS was found more accurate in cases with coarse aerosol and liquid water cloud models, except low optical depth, while the TMS showed better results in case of ice cloud.

Korkin, Sergey V.↗

MODIS Aerosol and Low‐Cloud Retrievals: Orographic Effects in the Wake of Macquarie Island

Abstract Visible/infrared imagery from passive satellites is commonly relied upon to study low cloud microphysics over oceanic regions, including for the Southern Ocean (SO), but relatively little validation has been undertaken for the SO. In this article, we compare low‐cloud effective radius ( r e ), cloud droplet number concentration ( N d ) and cloud liquid water path (LWP) retrievals from the NASA Moderate Imaging Spectroradiometer (MODIS) with surface measurements collected during the Macquarie Island Cloud and Radiation Experiment (MICRE). MODIS 3.7‐μm band retrievals show little bias and moderately good correlation relative to MICRE retrievals for liquid‐phase low clouds when restricted to Solar Zenith Angles <65° on spatial scales of 50–100 km. However, the low overall bias in 3.7‐μm band effective radius ( r e 3.7 ) retrievals partly results from cancellation of errors: r e 3.7 is overestimated for non‐to‐lightly precipitating clouds, and underestimated for heavier drizzling clouds by ∼1–1.5 μm. 1.6‐μm and 2.1‐μm band r e retrievals are biased high. N d may likewise be slightly under‐ or overestimated depending on the concentration, but there is insufficient data to provide confidence in this result. Interestingly, a composite of MODIS retrievals from 2002 to 2020 show a distinct region of enhanced cloud cover and N d (and lower r e ) in the wake of Macquarie Island associated with orographic cloud formation. MODIS retrievals of aerosol optical depth (AOD) and Angstrom Exponent (AE) upwind and downwind of the island do not differ significantly. Comparison with MICRE measurements suggests that MODIS Collection 6 AOD retrievals are reasonable, while AE is problematically large.

54 ENVIRONMENTAL SCIENCES↗

Radio astronomy

A K-band reflected-wave ruby maser was used on the 64-meter (DSS-43) antenna at the Tidbinbilla Tracking Station, near Canberra, Australia. Spectral line observations were carried out near 22 GHz for water vapor sources and near 24 GHz for ammonia sources. The water vapor observations were made in the direction of known southern OH and H2O maser sources. All of the previously detected water line sources examined were detected. In addition, two new water vapor maser sources were discovered, G301.1+1.1and G308.9+0.1. The spectrum of G301.0+1.1 is presented six ammonia sources were found: G291.3-0.7, G305.4+0.2, G322.2+0.6, G327.3-0.5, G333.6-0.2, and G268.4-0.8. Spectra of two of these sources, G291.3-0.7 (RCW 57) and G305.4+0.2, are presented. Both show clearly the presence of the quadrupole splitting satellite lines that will allow the determination of NH3 optical depths in these clouds.

Shaffer, R. D.↗

Ammonia in the hot galactic centre cloud G 1.6-0.025

As part of an extensive southern survey of interstellar NH3 with the Parkes 64-m radio telescope (with a beamwidth of 81 arcsec), the (1,1), (2,2), and (3,3) transitions have been observed towards the galactic centre molecular cloud Gl.6-0.025. The cloud has an overall size of 10 arcmin, and contains several concentrations with differing velocities. It has several features also observed in other galactic centre clouds, e.g. high optical depths and kinetic temperatures above 50 K.

Gardner, F. F.↗

The origin and vertical distribution of carbon monoxide in Jupiter

Six clearly-resolved lines of the CO 1-0 vibration-rotation band near 4.7 microns have been observed in Jupiter at a resolution of 0.07/cm. CO is not found to be concentrated in the stratosphere, but is shown to be present in the troposphere at a mole fraction of 1.6 + or - 0.3 x 10 to the -9th, suggesting that rapid vertical mixing is the source of CO. Results indicate that the global oxygen abundance in Jupiter's gaseous envelope below the cloud-forming regions must be near the solar value, and that intervening clouds with an optical depth of 0.5-4 are present above the line-forming region.

Noll, Keith S.↗

Ultraviolet and optical spectra of high-ionization Seyfert galaxies with narrow lines

Ultraviolet and optical spectra are presented for three unusual Seyfert galaxies (Mrk 1239, Mrk 42, and Mrk 493) that resemble Seyfert 1 galaxies in that they have strong high-ionization lines and strong nonstellar continua, but resemble Seyfert 2 galaxies in that the widths of their permitted lines are as narrow as the widths of their forbidden lines. The He II lambda 1640 and He II lambda 4686 lines are used to determine an upper limit to the reddening experienced by the emission lines. Published optical data show that these particular high-ionization narrow-line (HINL) Seyferts have low lambda 5007 H beta ratios and strong Fe II emission, which suggest the presence of high-density regions. The low Lalpha/H-beta ratios in these objects indicate that high-density clouds are indeed present, and, like the broad-line region clouds in Seyfert 1 galaxies, these clouds have large optical depths with partially ionized zones. Overall, the line ratios and continuum fluxes of these particular HINL Seyferts are indistinguishable from those of broad-lined Seyfert 1 galaxies.

Crenshaw, D. Michael↗

Visible/Infrared Optical Depths of Cirrus as Seen by Satellite and Scanning Lidar

The High Spectral Resolution Lidar (HSRL) and the Volume Imaging Lidar (VIL) were combined to produce a quantitative image of the visible optical depth of cirrus clouds. The HSRL was used to calibrate the VIL signal into backscatter cross sections of particulates. The backscatter cross sections were related to extinction by a constant backscatter phase function determined from the HSRL data. This produced a three dimensional image of visual extinction in the cirrus clouds over a one hour period. Two lidar images were constructed from one hour VIL cross section records.

Wylie, Donald↗

Evaluation of the OMI Cloud Pressures Derived from Rotational Raman Scattering by Comparisons with other Satellite Data and Radiative Transfer Simulations

In this paper we examine differences between cloud pressures retrieved from the Ozone Monitoring Instrument (OMI) using the ultraviolet rotational Raman scattering (RRS) algorithm and those from the thermal infrared (IR) Aqua/MODIS. Several cloud data sets are currently being used in OMI trace gas retrieval algorithms including climatologies based on IR measurements and simultaneous cloud parameters derived from OMI. From a validation perspective, it is important to understand the OMI retrieved cloud parameters and how they differ with those derived from the IR. To this end, we perform radiative transfer calculations to simulate the effects of different geophysical conditions on the OMI RRS cloud pressure retrievals. We also quantify errors related to the use of the Mixed Lambert-Equivalent Reflectivity (MLER) concept as currently implemented of the OMI algorithms. Using properties from the Cloudsat radar and MODIS, we show that radiative transfer calculations support the following: (1) The MLER model is adequate for single-layer optically thick, geometrically thin clouds, but can produce significant errors in estimated cloud pressure for optically thin clouds. (2) In a two-layer cloud, the RRS algorithm may retrieve a cloud pressure that is either between the two cloud decks or even beneath the top of the lower cloud deck because of scattering between the cloud layers; the retrieved pressure depends upon the viewing geometry and the optical depth of the upper cloud deck. (3) Absorbing aerosol in and above a cloud can produce significant errors in the retrieved cloud pressure. (4) The retrieved RRS effective pressure for a deep convective cloud will be significantly higher than the physical cloud top pressure derived with thermal IR.

Vasilkov, Alexander↗

Tropical High Cloud Feedback Relationships to Climate Sensitivity

Clouds constitute a large portion of uncertainty in predictions of equilibrium climate sensitivity (ECS). While low cloud feedbacks have been the focus of intermodel studies due to their high variability among global climate models, tropical high cloud feedbacks also exhibit considerable uncertainty. Here, we apply the cloud radiative kernel technique of Zelinka et al. to 22 models across the CMIP5 and CMIP6 ensembles to survey tropical high cloud feedbacks and analyze their relationship to ECS. We find that the net high cloud feedback and its altitude and optical depth feedback components are significantly positively correlated with ECS in the tropical mean. On the other hand, the tropical mean high cloud amount feedback is not correlated with ECS. These relationships are most pronounced outside of areas of strong climatological ascent, suggesting the importance of thin cirrus feedbacks. Finally, we explore connections between high cloud feedbacks, climate sensitivity, and mean state high cloud properties. In general, high ECS models are cloudier in the upper troposphere but have a thinner high cloud population. Furthermore, we find that having more thin cirrus in the mean state relates to more positive high cloud altitude and optical depth feedbacks, and it either amplifies or dampens the high cloud amount feedback depending on the large-scale dynamical regime (amplifying in descent and dampening in ascent). In summary, our analysis highlights the importance of tropical high cloud feedbacks for driving intermodel spread in ECS and suggests that mean state high cloud characteristics might provide a unique opportunity for observationally constraining high cloud feedbacks.

atmosphere↗

Improvements in AVHRR Daytime Cloud Detection Over the ARM NSA Site

Clouds play an important role in the radiation budget over Arctic and Antarctic. Because of limited surface observing capabilities, it is necessary to detect clouds over large areas using satellite imagery. At low and mid-latitudes, satellite-observed visible (VIS; 0.65 micrometers) and infrared (IR; 11 micrometers) radiance data are used to derive cloud fraction, temperature, and optical depth. However, the extreme variability in the VIS surface albedo makes the detection of clouds from satellite a difficult process in polar regions. The IR data often show that the surface is nearly the same temperature or even colder than clouds, further complicating cloud detection. Also, the boundary layer can have large areas of haze, thin fog, or diamond dust that are not seen in standard satellite imagery. Other spectral radiances measured by satellite imagers provide additional information that can be used to more accurately discriminate clouds from snow and ice. Most techniques currently use a fixed reflectance or temperature threshold to decide between clouds and clear snow. Using a subjective approach, Minnis et al. (2001) found that the clear snow radiance signatures vary as a function of viewing and illumination conditions as well as snow condition. To routinely process satellite imagery over polar regions with an automated algorithm, it is necessary to account for this angular variability and the change in the background reflectance as snow melts, vegetation grows over land, and melt ponds form on pack ice. This paper documents the initial satellite-based cloud product over the Atmospheric Radiation Measurement (ARM) North Slope of Alaska (NSA) site at Barrow for use by the modeling community. Cloud amount and height are determined subjectively using an adaptation of the methodology of Minnis et al. (2001) and the radiation fields arc determined following the methods of Doelling et al. (2001) as applied to data taken during the Surface Heat and Energy Budget of the Arctic (SHEBA). The procedures and data produced in this empirically based analysis will also facilitate the development of the automated algorithm for future processing of satellite data over the ARM NSA domain. Results are presented for May, June, and July 1998. ARM surface data are use to partially validate the results taken directly over the ARM site.

Chakrapani, V.↗

Constraining the Global, Cloud-Free Reflected Solar Radiation Flux (RSRF) with Earth Observing System (EOS) Instruments

Variations in the top-of-atmosphere reflected solar radiation flux, and in the factors that determine its value, are among the most important diagnostic indicators of changes in Earth's energy balance. Data from the MISR (Multi-angle Imaging SpectroRadiometer), MODIS (Moderate-resolution Imaging Spectroradiometer), SAGE-3 (Stratospheric Aerosol and Gas Experiment), and CERES (Clouds and Earth's Radiant Energy System), all of which are spacecraft instruments scheduled for launch in 1999, will each constrain pieces of the RSRF budget. Prior to launch, we are performing studies to determine the sensitivity of these instruments to key factors that influence the cloud-free RSRF: aerosol optical depth, aerosol scattering properties, and surface visible bidirectional reflectance distribution function (BRDF). We are also assessing the ability of the aggregate of instruments to constrain the overall RSRF budget under natural conditions over the globe. Consider the MISR retrieval of aerosols: according to simulations over cloud-free, calm ocean, for pure particles with natural ranges of optical depth, particle size, and indices of refraction, MISR can retrieve column aerosol optical depth for all but the darkest particles, to an uncertainty of at most 0.05 or 20%, whichever is larger, even if the particle properties are poorly known. For one common particle type, soot, constraints on the optical depth over dark ocean are very poor. The simulated measurements also allow us to distinguish spherical from non-spherical particles, to separate two to four compositional groups based on indices of refraction, and to identify three to four distinct size groups between 0. 1 and 2.0 microns characteristic radius at most latitudes. Based on these results, we expect to distinguish air masses containing different aerosol types, routinely and globally, with multiangle remote sensing data. Such results far exceed current satellite aerosol retrieval capabilities, which provide only total optical depth for assumed particle properties; the new information will complement in situ data, which give details about aerosol size and composition locally. In addition, our team is using climatologies that reflect the constraints each instrument is expected to provide, along with ERBE (Earth Radiation Budget Experiment) data and a radiative transfer code, to study overall sensitivity to RSRF, helping us prepare for similar studies with new data from the EOS-era instruments.

Kahn, Ralph↗

Aerosol, Cloud and Trace Gas Observations Derived from Airborne Hyperspectral Radiance and Direct Beam Measurements in Recent Field Campaigns

The AERONET (AErosol RObotic NETwork) ground-based suite of sunphotometers provides measurements of spectral aerosol optical depth (AOD), precipitable water and spectral sky radiance, which can be inverted to retrieve aerosol microphysical properties that are critical to assessments of aerosol-climate interactions. Because of data quality criteria and sampling constraints, there are significant limitations to the temporal and spatial coverage of AERONET data and their representativeness for global aerosol conditions. The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument, jointly developed by NASA Ames and PNNL with NASA Goddard collaboration, combines airborne sun tracking and AERONET-like sky scanning with spectroscopic detection. Being an airborne instrument, 4STAR has the potential to fill gaps in the AERONET data set. Dunagan et al. [2013] present results establishing the performance of the instrument, along with calibration, engineering flight test, and preliminary scientific field data. The 4STAR instrument operated successfully in the SEAC4RS [Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys] experiment in Aug./Sep. 2013 aboard the NASA DC-8 and in the DoE [Department of Energy]-sponsored TCAP [Two Column Aerosol Project, July 2012 & Feb. 2013] experiment aboard the DoE G-1 aircraft (Shinozuka et al., 2013), and acquired a wealth of data in support of mission objectives on all SEAC4RS and TCAP research flights. 4STAR provided direct beam measurements of hyperspectral AOD, columnar trace gas retrievals (H2O, O3, NO2; Segal-Rosenheimer et al., 2014), and the first ever airborne hyperspectral sky radiance scans, which can be inverted to yield the same products as AERONET ground-based observations. In addition, 4STAR measured zenith radiances underneath cloud decks for retrievals of cloud optical depth and effective diameter. In this presentation, we provide an overview of the new 4STAR capabilities for airborne field campaigns, with an emphasis on comparisons between 4STAR and AERONET sky radiances, and retrievals of aerosol microphysical properties based on sky radiance measurements, column trace gas amounts from spectral direct beam measurements and cloud property retrievals from zenith mode observations for a few select case studies in the SEAC4RS and TCAP experiments. We summarize the aerosol, trace gas, cloud and airmass characterization studies made possible by the combined 4STAR direct beam, and sky/zenith radiance observations.

Aerosol-Climate↗

An observational search for CO2 ice clouds on Mars

CO2 ice clouds were first directly identified on Mars by the Mariner 6 and 7 infrared spectrometer limb scans. These observations provided support for early theoretical modeling efforts of CO2 condensation. Mariner 9 IRIS temperature profiles of north polar hood clouds were interpreted as indicating that these clouds were composed of H2O ice at lower latitudes and CO2 ice at higher latitudes. The role of CO2 condensation on Mars has recently received increased attention because (1) Kasting's model results indicated that CO2 cloud condensation limits the magnitude of the proposed early Mars CO2/H2O greenhouse, and (2) Pollack el al.'s GCM results indicated that the formation of CO2 ice clouds is favorable at all polar latitudes during the fall and winter seasons. These latter authors have shown that CO2 clouds play an important role in the polar energy balance, as the amount of CO2 contained in the polar caps is constrained by a balance between latent heat release, heat advected from lower latitudes, and thermal emission to space. The polar hood clouds reduce the amount of CO2 condensation on the polar caps because they reduce the net emission to space. There have been many extensive laboratory spectroscopic studies of H2O and CO2 ices and frosts. In this study, we use results from these and other sources to search for the occurrence of diagnostic CO2 (and H2O) ice and/or frost absorption features in ground based near-infrared imaging spectroscopic data of Mars. Our primary goals are (1) to try to confirm the previous direct observations of CO2 clouds on Mars; (2) to determine the spatial extent, temporal variability, and composition (H2O/CO2 ratio) of any clouds detected; and (3) through radiative transfer modeling, to try to determine the mean particle size and optical depth of polar hood clouds, thus, assessing their role in the polar heat budget.

Bell, James F., III↗

Broadband and filter radiometers at Ross Island, Antarctica: detection of cloud ice phase versus liquid water influences on shortwave and longwave radiation

Abstract. Surface radiometer data from Ross Island, Antarctica, collected during the austral summer 2015–2016 by the US Department of Energy Atmospheric Radiation Measurement (ARM) program West Antarctic Radiation Experiment (AWARE), are used to evaluate how shortwave and longwave irradiance respond to changing cloud properties as governed by contrasting meteorological regimes. Shortwave atmospheric transmittance is derived from pyranometer measurements, and cloud conservative-scattering optical depth is derived from filter radiometer measurements at 870 nm. With onshore flow associated with marine air masses, clouds contain mostly liquid water. With southerly flow over the Transantarctic Mountains, orographic forcing induces substantial cloud ice water content. These ice and mixed-phase clouds attenuate more surface shortwave irradiance than the maritime-influenced clouds and also emit less longwave irradiance due to colder cloud base temperature. These detected irradiance changes are in a range that can mean onset or inhibition of surface melt over ice shelves. This study demonstrates how basic and relatively low-cost broadband and filter radiometers can be used to detect subtle climatological influences of contrasting cloud microphysical properties at very remote locations.

54 ENVIRONMENTAL SCIENCES↗

A study of acoustic heating and forced convection in the solar corona

The S055 EUV spectra was used to perform emission measure and line intensity ratio analyses of loop plasma conditions in a study on the thermodynamics of magnetic loops in the solar corona. The evidence that loops contain plasma hotter than the background corona, and thus, require enhanced local dissipation of magnetic or mechanical energy is discussed. The S055 EUV raster pictures were used to study physical conditions in cool ultraviolet absorbing clouds in the solar corona, and optical data were used to derive constraints on the dimension, time scales and optical depths in dark opaque clouds not seen in H alpha and CaK as filaments or prominences. Theoretical modelling of propagation of magnetically guided acoustic shocks in the solar chromosphere finds it still unlikely that high frequency acoustic shocks could reach the solar corona. Dynamic modelling of spicules shows that such guided slow mode shocks can explain the acceleration of cool spicular material seen high in the corona.

Foukal, P. V.↗

Assessing Spectral Shortwave Cloud Observations at the Southern Great Plains Facility

The Atmospheric Radiation Measurement (ARM) program (now Atmospheric System Research) was established, in part, to improve radiation models so that they could be used reliably to compute radiation fluxes through the atmosphere, given knowledge of the surface albedo, atmospheric gases, and the aerosol and cloud properties. Despite years of observations, discrepancies still exist between radiative transfer models and observations, particularly in the presence of clouds. Progress has been made at closing discrepancies in the spectral region beyond 3 micron, but the progress lags at shorter wavelengths. Ratios of observed visible and near infrared cloud albedo from aircraft and satellite have shown both localized and global discrepancies between model and observations that are, thus far, unexplained. The capabilities of shortwave surface spectrometry have been improved in recent years at the Southern Great Plains facility (SGP) of the ARM Climate Research Facility through the addition of new instrumentation, the Shortwave Array Spectroradiometer, and upgrades to existing instrumentation, the Shortwave Spectroradiometer and the Rotating Shadowband Spectroradiometer. An airborne-based instrument, the HydroRad Spectroradiometer, was also deployed at the ARM site during the Routine ARM Aerial Facility Clouds with Low Optical Water Depths (CLOWD) Optical Radiative Observations (RACORO) field campaign. Using the new and upgraded spectral observations along with radiative transfer models, cloud scenes at the SGP are presented with the goal of characterizing the instrumentation and the cloud fields themselves.

McBride, P. J.↗

Constraints on the inner accretion flow of 4U/MXB 1636-53 (V 801 Arae) from a comparison of X-ray burst and persistent emission

A detailed analysis is presented of the importance of Comptonization in burst and persistent spectra of the low-mass X-ray binary 4U/MXB 1636-53, and from this analysis it is inferred that the inner accretion flow is geometrically thin. It is found that burst spectra of 1636-53 are very nearly Planckian in shape; from an upper limit to a high-energy excess in these spectra it is inferred that the Thomson scattering optical depth of a possible intervening hot cloud must be less than 1 during bursts, and that the Compton y parameter of that cloud must be less than 0.5. During persistent emission, Thomson optical depth of 4-8, an electron temperature of 2-5 keV, and a value of 0.8-1.1 for y are inferred.

Damen, E.↗