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DOE OSTI2022

A Hybrid Data-Driven and Model-Based Anomaly Detection Scheme for DER Operation: Preprint

This paper proposes a hybrid data and model-based anomaly detection for securing the operation of distributed energy resources (DERs) in distribution grids. Data-driven autoencoders (AE) are set up at the edge level by taking local DER data and detect anomalous operations by leveraging the reconstruction ability. In parallel, model-based state estimation (SE) is running at the system level by taking system models and measurements, the anomalies are identified by analyzing the measurements residual. The hybrid scheme preserves the benefits of both data-driven and model-based analysis and thus improves the robustness and accuracy of anomaly detection. It can be established by getting full use of the existing infrastructures in distribution grids. Numerical tests on a realistic distribution feeder in Southern California highlight the effectiveness as well as benefits of the proposed scheme.

anomaly detection↗

NASA NTRS2012

Subaru Imaging of Asymmetric Features in a Transitional Disk in Upper Scorpius

We report high-resolution (0.07 arcsec) near-infrared polarized intensity images of the circumstellar disk around the star 2MASS J16042165.2130284 obtained with HiCIAO mounted on the Subaru 8.2 m telescope. We present our H-band data, which clearly exhibit a resolved, face-on disk with a large inner hole for the first time at infrared wavelengths. We detect the centrosymmetric polarization pattern in the circumstellar material as has been observed in other disks. Elliptical fitting gives the semi-major axis, semi-minor axis, and position angle (P.A.) of the disk as 63 AU, 62 AU, and -14deg, respectively. The disk is asymmetric, with one dip located at P.A.s of approx. 85deg. Our observed disk size agrees well with a previous study of dust and CO emission at submillimeter wavelength with Submillimeter Array. Hence, the near-infrared light is interpreted as scattered light reflected from the inner edge of the disk. Our observations also detect an elongated arc (50 AU) extending over the disk inner hole. It emanates at the inner edge of the western side of the disk, extending inward first, then curving to the northeast. We discuss the possibility that the inner hole, the dip, and the arc that we have observed may be related to the existence of unseen bodies within the disk.

Mayama, S.↗

DOE OSTI2020

Josephson Junctions and Cosmic Microwave Background

The implementation of utilizing superconducting quantum interference device (SQUID) readout for constant voltage biased transition edge sensors (TES) has enabled the detection of the infinitesimal fluctuation in cosmic microwave background (CMB). The properties of the fluctuations will provide us the information of the universe at the time that this light was first emitted. In short, by measuring the CMB today, we learn about the distant, ancient universe—how the universe began, what it is made of, and how it evolved to its current state. Over the past 20 years, we have achieved many successful CMB measurements with Josephson junctions. Brian, I extend my congratulations on your eight decades of life—Happy 80th birthday!

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2025

Negative-Ion Formation upon Soft X-ray Photoexcitation of 2-Propanol

This study investigates the formation of negative ion fragments from gas-phase 2-propanol molecules after interaction with soft X-rays near the O K-edge. The experiment was performed by detecting negative and positive ions in coincidence with time-of-flight spectrometry. The analysis of two- and three-ion coincidence data revealed that nine different anions were produced: H – , C – , CH – , CH 2 – , O – , OH – , C 2 – , C 2 H – , and C 3 – . For all anions, the most common three-ion events were those involving two protons. The results highlight the sensitivity of negative-ion/positive-ion coincidence spectroscopy and provide new insight into the fragmentation processes of organic molecules under soft X-ray excitation.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2021

A Theory-Guided X-ray Absorption Spectroscopy Approach for Identifying Active Sites in Atomically Dispersed Transition-Metal Catalysts

Atomically dispersed supported metal catalysts offer new properties and the benefits of maximized metal accessibility and utilization. The characterization of these materials, however, remains challenging. Using atomically dispersed platinum supported on crystalline MgO (chosen for its well-defined bonding sites) as a prototypical example, we demonstrate in this work how systematic density functional theory calculations for assessing all the potentially stable platinum sites, combined with automated analysis of extended X-ray absorption fine structure (EXAFS) spectra, leads to unbiased identification of isolated, surface-enveloped platinum cations as the catalytic species for CO oxidation. The catalyst has been characterized by atomic-resolution imaging and EXAFS and high-energy resolution fluorescence detection X-ray absorption near edge spectroscopy. The proposed platinum sites are in agreement with experiment. This theory-guided workflow leads to rigorously determined structural models and provides a more detailed picture of the structure of the catalytically active site than what is currently possible with conventional EXAFS analyses. As this approach is efficient and agnostic to the metal, support, and catalytic reaction, we posit that it will be of broad interest to the materials characterization and catalysis communities.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Nanosecond anomaly detection with decision trees and real-time application to exotic Higgs decays

Abstract We present an interpretable implementation of the autoencoding algorithm, used as an anomaly detector, built with a forest of deep decision trees on FPGA, field programmable gate arrays. Scenarios at the Large Hadron Collider at CERN are considered, for which the autoencoder is trained using known physical processes of the Standard Model. The design is then deployed in real-time trigger systems for anomaly detection of unknown physical processes, such as the detection of rare exotic decays of the Higgs boson. The inference is made with a latency value of 30 ns at percent-level resource usage using the Xilinx Virtex UltraScale+ VU9P FPGA. Our method offers anomaly detection at low latency values for edge AI users with resource constraints.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

Electron energy loss spectroscopy database synthesis and automation of core-loss edge recognition by deep-learning neural networks

Abstract The ionization edges encoded in the electron energy loss spectroscopy (EELS) spectra enable advanced material analysis including composition analyses and elemental quantifications. The development of the parallel EELS instrument and fast, sensitive detectors have greatly improved the acquisition speed of EELS spectra. However, the traditional way of core-loss edge recognition is experience based and human labor dependent, which limits the processing speed. So far, the low signal–noise ratio and the low jump ratio of the core-loss edges on the raw EELS spectra have been challenging for the automation of edge recognition. In this work, a convolutional-bidirectional long short-term memory neural network (CNN-BiLSTM) is proposed to automate the detection and elemental identification of core-loss edges from raw spectra. An EELS spectral database is synthesized by using our forward model to assist in the training and validation of the neural network. To make the synthesized spectra resemble the real spectra, we collected a large library of experimentally acquired EELS core edges. In synthesize the training library, the edges are modeled by fitting the multi-Gaussian model to the real edges from experiments, and the noise and instrumental imperfectness are simulated and added. The well-trained CNN-BiLSTM network is tested against both the simulated spectra and real spectra collected from experiments. The high accuracy of the network, 94.9%, proves that, without complicated preprocessing of the raw spectra, the proposed CNN-BiLSTM network achieves the automation of core-loss edge recognition for EELS spectra with high accuracy.

36 MATERIALS SCIENCE↗

DOE OSTI2025

Multi-Analytical Investigation of Arsenical Transfer and Remediation on Nineteenth-Century Green Books

Books containing heavy metals, specifically nineteenth-century green arsenical books, have been identified at Northwestern University Libraries, raising health and safety concerns related to handling. Copper acetoarsenite pigments, such as emerald green, were detected on book covers, decorative page edges, labels, and other components using noninvasive analytical techniques including X-ray fluorescence (XRF), Raman spectroscopy, and Fourier-transform infrared (FTIR) spectroscopy. Further examination of selected volumes using synchrotron radiation (SR) techniques revealed pigment migration, degradation, and arsenic transfer to adjacent books. This paper expands on initial findings through two related experiments. The first explored the transfer of arsenic using mechanical friction; Staedtler Mars® white vinyl erasers rubbed on arsenical books generated crumbs which were analyzed via scanning electron microscopy–energy-dispersive X-ray spectroscopy (SEM-EDX). Results confirmed the transfer of arsenic, copper, and lead, with decorative page edges being particularly prone to shedding arsenic onto other materials. The second experiment tested remediation methods on a book contaminated by prolonged exposure to an arsenical neighbor. Surface cleaning using erasers and a vacuum removed flecks of pigment but did not eliminate non-chromophoric arsenic as confirmed by SR analyses, which highlights its presence either as a degradation product embedded within the paper or present in the paper as part of its production process. Findings demonstrate the acute toxicity risk posed by arsenical books and support the need for safe handling protocols. However, materials with only trace levels of arsenic embedded during production may pose a lower risk of transfer. Cross contamination beyond prolonged direct contact appears limited. These results highlight critical considerations for library preservation practices and future research on arsenic in historical materials.

arsenic↗

NASA NTRS1983

The dynamics of elliptical rings

The paper investigates the evolution of eccentric rings under the influence of (1) differential precession due to the planetary quadrupole moment; (2) self-gravity; (3) viscous forces due to interparticle collisions; and (4) eccentricity excitation by shepherd satellites. The principal conclusions are that: (1) uniform precession can be enforced by self-gravity; the resulting configuration is both dynamically and secularly stable. (2) due to viscous forces the line of apsides at the inner ring edge is not exactly aligned with the line of apsides at the outer edge; the apse shift may be detectable in the alpha and beta rings of Uranus; (3) the mean eccentricity is determined by a balance between viscous damping and excitation by shepherds; (4) and the dimensionless eccentricity gradient is expected to be positive and of order unity in most eccentric rings, as observed.

Borderies, N.↗

NASA NTRS1987

On autonomous terrain model acquistion by a mobile robot

The following problem is considered: A point robot is placed in a terrain populated by an unknown number of polyhedral obstacles of varied sizes and locations in two/three dimensions. The robot is equipped with a sensor capable of detecting all the obstacle vertices and edges that are visible from the present location of the robot. The robot is required to autonomously navigate and build the complete terrain model using the sensor information. It is established that the necessary number of scanning operations needed for complete terrain model acquisition by any algorithm that is based on scan from vertices strategy is given by the summation of i = 1 (sup n) N(O sub i)-n and summation of i = 1 (sup n) N(O sub i)-2n in two- and three-dimensional terrains respectively, where O = (O sub 1, O sub 2,....O sub n) set of the obstacles in the terrain, and N(O sub i) is the number of vertices of the obstacle O sub i.

Rao, N. S. V.↗

NASA NTRS1990

IUE observations of PG 1115 + 080 - The He I Gunn-Peterson test and a search for the lensing galaxy

Five observations of PG 1115 + 080 taken with the IUE SWP camera have been combined in order to carry out the He I Gunn-Peterson test and to search for a Lyman limit which could determine the redshift of the lens candidate reported by Christian et al. (1987). No Lyman-limit discontinuities are found, implying that the lensing galaxy does not intercept the line of sight or does not contain enough neutral hydrogen to be detected as a Lyman-limit edge. It is estimated that the lens column density for neutral hydrogen is 3 x 10 to the 16th/sq cm or less if it intercepts the line of sight.

Tripp, Todd M.↗

NASA NTRS1994

Development of an accurate transmission line fault locator using the global positioning system satellites

A highly accurate transmission line fault locator based on the traveling-wave principle was developed and successfully operated within B.C. Hydro. A transmission line fault produces a fast-risetime traveling wave at the fault point which propagates along the transmission line. This fault locator system consists of traveling wave detectors located at key substations which detect and time tag the leading edge of the fault-generated traveling wave as if passes through. A master station gathers the time-tagged information from the remote detectors and determines the location of the fault. Precise time is a key element to the success of this system. This fault locator system derives its timing from the Global Positioning System (GPS) satellites. System tests confirmed the accuracy of locating faults to within the design objective of +/-300 meters.

Lee, Harry↗

NASA NTRS2012

Fabrication and Performance of Large Format Transition Edge Sensor Microcalorimeter Arrays

We have produced a variety of superconducting transition edge sensor array designs for microcalorimetric detection of x-rays. Designs include kilopixel scale arrays of relatively small sensors (~75 micron pitch) atop a thick metal heatsinking layer as well as arrays of membrane-isolated devices on 250 micron pitch and smaller arrays of devices up to 600 micron pitch. We discuss the fabrication techniques used for each type of array focusing on unique aspects where processes vary to achieve the particular designs and required device parameters. For example, we evaluate various material combinations in the production of the thick metal heatsinking, including superconducting and normal metal adhesion layers. We also evaluate the impact of added heatsinking on the membrane isolated devices as it relates to basic device parameters. Arrays can be characterized with a time division SQUID multiplexer such that greater than 10 devices from an array can be measured in the same cooldown. Device parameters can be measured simultaneously so that environmental events such as thermal drifts or changes in magnetic fields can be controlled. For some designs, we will evaluate the uniformity of parameters impacting the intrinsic performance of the microcalorimeters under bias in these arrays and assess the level of thermal crosstalk.

Chervenak, James A.↗

NASA NTRS2012

Large Format Transition Edge Sensor Microcalorimeter Arrays

Chervenak, J. A.↗

NASA NTRS2012

Performance of Large Format Transition Edge Sensor Microcalorimeter Arrays

We have produced a variety of superconducting transition edge sensor array designs for microcalorimetric detection of x-rays. Arrays are characterized with a time division SQUID multiplexer such that greater than 10 devices from an array can be measured in the same cooldown. Designs include kilo pixel scale arrays of relatively small sensors (-75 micron pitch) atop a thick metal heatsinking layer as well as arrays of membrane-isolated devices on 250 micron and up to 600 micron pitch. We discuss fabrication and performance of microstripline wiring at the small scales achieved to date. We also address fabrication issues with reduction of absorber contact area in small devices.

Chervenak, J. A.↗

NASA NTRS2014

Revealing Asymmetries in the HD181327 Debris Disk: A Recent Massive Collision or Interstellar Medium Warping

New multi-roll coronagraphic images of the HD181327 debris disk obtained using the Space Telescope Imaging Spectrograph on board the Hubble Space Telescope reveal the debris ring in its entirety at high signal-to-noise ratio and unprecedented spatial resolution. We present and apply a new multi-roll image processing routine to identify and further remove quasi-static point-spread function-subtraction residuals and quantify systematic uncertainties. We also use a new iterative image deprojection technique to constrain the true disk geometry and aggressively remove any surface brightness asymmetries that can be explained without invoking dust density enhancements/ deficits. The measured empirical scattering phase function for the disk is more forward scattering than previously thought and is not well-fit by a Henyey-Greenstein function. The empirical scattering phase function varies with stellocentric distance, consistent with the expected radiation pressured-induced size segregation exterior to the belt. Within the belt, the empirical scattering phase function contradicts unperturbed debris ring models, suggesting the presence of an unseen planet. The radial profile of the flux density is degenerate with a radially varying scattering phase function; therefore estimates of the ring's true width and edge slope may be highly uncertain.We detect large scale asymmetries in the disk, consistent with either the recent catastrophic disruption of a body with mass greater than 1% the mass of Pluto, or disk warping due to strong interactions with the interstellar medium.

Henyey Greenstein function↗

NASA NTRS2020

Plasma-environment effects on K lines of astrophysical interest III. IPs, K thresholds, radiative rates, and Auger widths in Fe ix – Fe xvi

Aims. In the context of black-hole accretion disks, we aim to compute the plasma-environment e ects on the atomic parameters used to model the decay of K-vacancy states in moderately charged iron ions, namely Fe ix – Fe xvi. Methods. We used the fully relativistic multiconfiguration Dirac–Fock method approximating the plasma electron–nucleus and electron–electron screenings with a time-averaged Debye–Hückel potential. Results. We report modified ionization potentials, K-threshold energies, wavelengths, radiative emission rates, and Auger widths for plasmas characterized by electron temperatures and densities in the ranges 10^(5)-10^(7) K and 10^(18)-10^(22)/cu. cm. Conclusions. This study confirms that the high-resolution X-ray spectrometers onboard the future XRISM and Athena space missions will be capable of detecting the lowering of the K edges of these ions due to the extreme plasma conditions occurring in accretion disks around compact objects.

J. Deprince↗

NASA NTRS2020

Plasma environment effects on K lines of astrophysical interest IV. IPs, K thresholds, radiative rates, and Auger widths in Fe ii–Fe viii

Aims. Within the framework of compact-object accretion disks, we calculate plasma environment e ects on the atomic structure and decay parameters used in the modeling of K lines in lowly charged iron ions, namely Fe ii–Fe viii. Methods. For this study, we used the fully relativistic multiconfiguration Dirac–Fock method approximating the plasma electron–nucleus and electron-electron screenings with a time-averaged Debye-Hückel potential. Results. We report modified ionization potentials, K-threshold energies, wavelengths, radiative emission rates, and Auger widths for plasmas characterized by electron temperatures and densities in the ranges 10(exp 5)-10(exp 7) K and 10(exp 18)-10(exp 22) per cu.cm. In addition, we propose two universal fitting formulae to predict the IP and K-threshold lowerings in any elemental ion. Conclusions. We conclude that the high-resolution X-ray spectrometers onboard the future XRISM and ATHENA space missions will be able to detect the lowering of the K edges of these Fe ions due to the extreme plasma conditions occurring in the accretion disks around compact objects.

J. Deprince↗