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DOE OSTI2021

Strain-modulated helimagnetism and emergent magnetic phase diagrams in highly crystalline MnP nanorod films

Here, we explore strain-modulated helimagnetism in highly crystalline MnP nanorod films grown on Si(100) substrates using molecular beam epitaxy. The strained MnP film exhibits a paramagnetic to ferromagnetic (FM) phase transition at $T_C$ ~ 279 K, and the FM to helical phase transition at $T_N$ ~ 110 K. The value of $T_N$ is greater than $T_N$ ~ 47K for the MnP single crystal, indicating strong strain-modulated helimagnetic states in the MnP nanorod film. The presence of significant thermal hysteresis in the helical phase indicates the coexistence of competing magnetic interactions, leading to the first-order metamagnetic transition. Similar to its single-crystal counterpart, an anisotropic magnetic effect is observed in the MnP film, which is independently confirmed by magnetic hysteresis loop and radio-frequency transverse susceptibility (TS) measurements. The evolution of the screw to the cone and fan phases is precisely tracked from magnetization vs magnetic field/temperature measurements. The temperature dependence of the anisotropy fields, extracted from the TS spectra, yields further insight into the competing nature of the magnetic phases. Unfolding of the different helical phases at $\textit{T}$ < 120 K (~$T_N$) is analyzed by the temperature- and field-dependent magnetic entropy change. Based on these findings, the comprehensive magnetic phase diagrams of the MnP nanorod film are constructed for both the in-plane and out of plane magnetic field directions, revealing emergent strain/dimensionality-driven helical magnetic features that are absent in the magnetic phase diagram of the MnP single crystal.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

Antiferromagnetic real-space configuration probed by dichroism in scattered x-ray beams with orbital angular momentum

X-ray beams with orbital angular momentum (OAM) are a promising tool for x-ray characterization techniques. Beams with OAM have a helicity - an azimuthally varying phase - which leads to a gradient of the light field. New material properties can be probed by utilizing the helicity of an OAM beam. Here, we demonstrate a dichroic effect in resonant diffraction from an artificial antiferromagnet with a topological defect. We found that the scattered OAM beam has circular dichroism at the antiferromagnetic Bragg peak whose sign is coupled to its helicity, which reveals the real-space configuration of the antiferromagnetic ground state. Thermal cycling of the artificial antiferromagnet can change the ground state, as indicated by reversal of the sign of circular dichroism. This result is one of the first demonstrations of a soft x-ray spectroscopy characterization technique utilizing the OAM of x rays. In conclusion, this helicity-dependent circular dichroism exemplifies the potential to utilize OAM beams to probe matter in a way that is inaccessible using currently available x-ray techniques.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Polarized dipole scattering amplitudes meet the valence quark model

The recently revised small- x helicity evolution [], resumming the double-logarithmic factor, α s ln 2 ( 1 / x ) , allows for the study of helicity distributions of quarks and gluons at small Bjorken x , corresponding to high center-of-mass energy. In this work, we calculate the moderate- x initial conditions in the regime, α s ln 2 ( 1 / x ) ∼ 1 , for the small- x helicity evolution using a light-front valence quark model of the proton, which provides additional physical information about the target. The perturbative emission and absorption of a gluon by the valence quarks are also included. The results, given in Eqs. (35), provide a new set of initial conditions with a significantly reduced number of free parameters than conventional models []. Consequently, the predictive power of small- x helicity evolution is expected to improve once the initial conditions from this work are incorporated. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Stabilization of Liner Implosions via a Dynamic Screw Pinch

Magnetically driven implosions are susceptible to magnetohydrodynamic instabilities, including the magneto-Rayleigh-Taylor instability (MRTI). To reduce MRTI growth in solid-metal liner implo-sions, the use of a dynamic screw pinch (DSP) has been proposed [P. F. Schmit et al., Phys. Rev. Lett. 117, 205001 (2016)]. In a DSP con guration, a helical return-current structure surrounds the liner, resulting in a helical magnetic eld that drives the implosion. Here, we present the rst experimental tests of a solid-metal liner implosion driven by a DSP. Using the 1-MA, 100{200-ns COBRA pulsed-power driver, we tested three DSP cases (with peak axial magnetic elds of 2 T, 14 T, and 20 T) and a standard z-pinch (SZP) case (with a straight return-current structure and thus zero axial eld). The liners had an initial radius of 3.2 mm and were made from 650-nm-thick aluminum foil. Images collected during the experiments reveal that helical MRTI modes developed in the DSP cases, while non-helical (azimuthally symmetric) MRTI modes developed in the SZP case. Additionally, the MRTI amplitudes for the 14-T and 20-T DSP cases were smaller than in the SZP case. Speci cally, when the liner had imploded to half of its initial radius, the MRTI amplitudes for the SZP case and for the 14-T and 20-T DSP cases were, respectively, 1.1-0.3 mm, 0.7-0.2 mm, and 0.3-0.1 mm. Relative to the SZP, the stabilization obtained using the DSP agrees reasonably well with theoretical estimates.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2025

EMT-TS Hybrid Simulation for Large Power Grids Considering IBR-Driven Dynamics

The escalating integration of inverter-based resources (IBRs) poses new challenges to power systems by introducing fast dynamics with higher frequencies, which may need to be simulated by an electromagnetic transient (EMT) program. As an alternative to conducting EMT simulations for the entire system, which is typically time consuming, hybrid simulation between EMT and phasor-domain transient stability (TS) can greatly reduce the computational burden while preserving the detailed fast dynamics in the EMT zone. This paper establishes an EMT-TS hybrid simulation platform using open-source tools, specifically ParaEMT, GridPACK, and HELICS, which are the EMT simulator, TS simulator, and interface framework, respectively. Case studies on the 240-bus Western Electricity Coordinating Council (WECC) system demonstrate that the developed ParaEMT-HELICS-GridPACK hybrid simulator can accurately capture both slow electromechanical and fast IBR-driven dynamics with a 2.4x speedup.

electromagnetic transient↗

DOE OSTI2022

Crystal structure of an RNA/DNA strand exchange junction

Short segments of RNA displace one strand of a DNA duplex during diverse processes including transcription and CRISPR-mediated immunity and genome editing. These strand exchange events involve the intersection of two geometrically distinct helix types—an RNA:DNA hybrid (A-form) and a DNA:DNA homoduplex (B-form). Although previous evidence suggests that these two helices can stack on each other, it is unknown what local geometric adjustments could enable A-on-B stacking. Here we report the X-ray crystal structure of an RNA-5′/DNA-3′ strand exchange junction at an anisotropic resolution of 1.6 to 2.2 Å. The structure reveals that the A-to-B helical transition involves a combination of helical axis misalignment, helical axis tilting and compression of the DNA strand within the RNA:DNA helix, where nucleotides exhibit a mixture of A- and B-form geometry. These structural principles explain previous observations of conformational stability in RNA/DNA exchange junctions, enabling a nucleic acid architecture that is repeatedly populated during biological strand exchange events.

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2020

Integrated Data Analysis to Improve Te and Zeff Measurement on NSTX-U

The multi-energy soft x-ray (ME-SXR) camera is a new concept for a fusion plasma diagnostic based on a pixelated detector with adjustable photon cutoff thresholds. It is a single, compact, solid-state detector which combines spatial and spectral sensitivity and can be configured remotely at run time, making it ideal for a fusion environment. The detector can be configured for application to a wide range of physics problems including impurity transport, electron temperature profiles, and non-thermal effects. The detector has been installed on the Madison Symmetric Torus (MST) as part of a collaboration between Princeton Plasma Physics Laboratory and the University of Wisconsin–Madison to develop the technology and analysis techniques. A full diagnostic forward model of the ME-SXR diagnostic has been developed to enable analysis of the raw photon count data. This model incorporates the atomic physics underlying the plasma emission, diagnostic geometry, and detector response characteristics. Employing this model, a Bayesian analysis approach is used to extract electron temperature from the raw data. This analysis approach uses all available information, clearly quantifies prior information, and handles uncertainties transparently. The ME-SXR camera is being used to study the 3D (helical, stellarator-like) state that forms in the MST device. This helical core structure has improved energy confinement. The transition to the helical state is accompanied by a rise in electron temperature in the central part of the helical structure, but then this enhancement fluctuates. The characteristics of this fluctuation are being compared to a magneto-hydrodynamics model.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2021

Dependence of Solar Wind Proton Temperature on the Polarization Properties of Alfvénic Fluctuations at Ion-kinetic Scales

In this work, we use fluctuating magnetic helicity to investigate the polarization properties of Alfvénic fluctuations at ion-kinetic scales in the solar wind as a function of β p , the ratio of proton thermal pressure to magnetic pressure, and θ vB , the angle between the proton flow and local mean magnetic field, B 0 . Using almost 15 yr of Wind observations, we separate the contributions to helicity from fluctuations with wavevectors, k, quasi-parallel and oblique to B 0 , finding that the helicity of Alfvénic fluctuations is consistent with predictions from linear Vlasov theory. This result suggests that the nonlinear turbulent fluctuations at these scales share at least some polarization properties with Alfvén waves. Furthermore, we also investigate the dependence of proton temperature in the β p –θ vB plane to probe for possible signatures of turbulent dissipation, finding that it correlates with θ vB . The proton temperature parallel to B 0 is higher in the parameter space where we measure the helicity of right-handed Alfvénic fluctuations, and the temperature perpendicular to B 0 is higher where we measure left-handed fluctuations. This finding is inconsistent with the general assumption that by sampling different θ vB in the solar wind we can analyze the dependence of the turbulence distribution on θ kB , the angle between k and B 0 . After ruling out both instrumental and expansion effects, we conclude that our results provide new evidence for the importance of local kinetic processes that depend on θ vB in determining proton temperature in the solar wind.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Turbulent Heating in Collisionless Low-beta Plasmas: Imbalance, Landau Damping, and Electron–Ion Energy Partition

An understanding of how turbulent energy is partitioned between ions and electrons in weakly collisional plasmas is crucial for modeling many astrophysical systems. Using theory and simulations of a four-dimensional reduced model of low-beta gyrokinetics (the “Kinetic Reduced Electron Heating Model”), we investigate the dependence of collisionless heating processes on plasma beta and imbalance (normalized cross-helicity). These parameters are important because they control the helicity barrier, the formation of which divides the parameter space into two distinct regimes with remarkably different properties. In the first, at lower beta and/or imbalance, the absence of a helicity barrier allows the cascade of injected power to proceed to small (perpendicular) scales, but its slow cascade rate makes it susceptible to significant electron Landau damping, in some cases leading to a marked steepening of the magnetic spectra on scales above the ion Larmor radius. In the second, at higher beta and/or imbalance, the helicity barrier halts the cascade, confining electron Landau damping to scales above the steep “transition-range” spectral break, resulting in dominant ion heating. We formulate quantitative models of these processes that compare well to simulations in each regime, and combine them with results of previous studies to construct a simple formula for the electron–ion heating ratio as a function of beta and imbalance. This model predicts a “winner takes all” picture of low-beta plasma heating, where a small change in the fluctuations' properties at large scales (the imbalance) can cause a sudden switch between electron and ion heating.

Interplanetary turbulence↗

DOE OSTI2021

Photoproduction of the b 1 (1235) Meson off the proton at E gamma = 6-12 GeV

The GlueX Experiment at Jefferson Lab directs a linearly polarized photon beam on a liquid hydrogen target surrounded by an almost hermetic detector. The experiment aims to study the meson spectrum in the light-quark sector and search for exotic spin-parity states predicted by lattice QCD calculations. The lightest exotic candidate is the π 1 meson, which is predicted to decay dominantly to b 1 π. In this thesis, we present efforts to characterize the ωπ 0 decay channel of the b 1 meson as precursor to an analysis of the sought-after π 1 exotic state. We present an introduction to the physics involved and an overview of the detector subsystems with a focus on the Barrel Calorimeter gain monitoring system, as part of the service work expected by the GlueX Collaboration. We discuss the data analysis method used and present two frameworks, for angular moments and partial waves analyses. Details of the simulation used to calculate the detector acceptance. A proof of concept partial wave analysis is presented along with experimental angular moments as first step to a full analysis of the angular distribution Our partial wave analysis indicates that both S- and D-waves are needed, in qualitative agreement with theoretical expectations. The cross-section of the omega π 0 channel is extracted to be of the scale of 1 μb in agreement with previous measurements. The differential cross-section indicates the presence of two production processes with p 1 = -5:24 ± 0:04 for 0:25 < -t < 0:95 GeV 2 ~c 2 and p 2 = -1:24 ± 0:05 for 0:95 < -t < 2:0 GeV 2 ~c 2 , which does not agree with results from previous experiments. The s-channel helicity conservation and helicity amplitudes of the b 1 meson are presented as additional experimental observables. Our results confirm that the b1 photoproduction process does not conserve s-channel helicity though they do not align with previous measurements. The helicity amplitude of the omega are extracted to be |F 1 | 2 = 0:3037 ± 0:0003 which does not agree with the expected value of a b 1 decay or results from a previous experiment. Future steps in all these analyses will be continued by a new graduate student in the group, culminating in a publication.

Foda, Ahmed↗

DOE OSTI2023

Tooling assembly and method for explosively forming features in a thin-walled cylinder

The present invention provides a method of explosively forming a helical tube from at least one thin-walled cylinder using a tooling assembly. The method includes inserting the at least one thin-walled cylinder into a die of the tooling assembly. The die surrounds the at least one thin-walled cylinder and includes an interior surface that defines a helical thread pattern. The method further includes surrounding the at least one thin-walled cylinder and the die with a casing of the tooling assembly. A cavity is defined by the casing and the thin-walled cylinder. The method further includes positioning an explosive charge within the cavity. The method additionally includes at least partially submerging the tooling assembly. The method further includes detonating the explosive charge. As a result, the at least one thin-walled cylinder is formed into a helical tube that corresponds with helical thread pattern of the interior surface of the die.

Eberl, Kurt R.↗

DOE OSTI2024

Supports with integrated sensors for nuclear reactor steam generators, and associated systems and methods

Supports with integrated sensors for nuclear reactor steam generators, and associated systems and methods, are disclosed. A representative method for forming a nuclear-powered steam generator includes forming an instrumented support, the instrumented support including a carrier portion and a retainer portion, with at least one of the carrier portion or the retainer portion being integrally formed with a sensor via an additive manufacturing process. The method can further include coupling the sensor to a communication link, supporting a helical steam conduit on the instrumented support, and installing the helical steam conduit and the instrumented support in a nuclear reactor. The helical steam conduit is positioned along a primary flow path, which is in turn positioned to circulate a heated primary flow in thermal communication with the helical steam conduit.

Welter, Kent↗

DOE OSTI2023

Patterns in interactions of variably acetylated xylans with hydrophobic cellulose surfaces

The recalcitrance of plant cell wall lignocellulosic biomass to deconstruction is a major hurdle to sustainable biofuel/bioproduct economy. A multitude of interactions stabilize lignocellulosic biomass structure. Among these, tight packing of hemicellulose-cellulose is partly responsible for biomass recalcitrance. Here, unrestrained molecular dynamics simulations are employed to understand the influence of the nature and pattern of naturally-occuring acetyl decorations of the xylan backbone on interactions with the (100) hydrophobic cellulose surface. Periodically O2-acetylated xylan (2AcX) assume twofold helical screw conformations that are stabilized by a combination of multiple hydrophobic contacts and hydrogen bonds with the hydrophobic cellulose surface. In contrast, acetylation at the O3 position in xylan obstructs interactions, thereby adopting threefold helical screw conformations that potentially preferably interact with lignin rather than cellulose. Fully acetylated xylan desorbs from the surface implying a minimum number of unsubstituted residues on the xylan backbone is required for interaction with the surface. Here, the substituted residues must form ~ 20% fewer contacts than the unsubstituted residues to sustain stable twofold helical screw xylan conformations on the cellulose surface. Thus, specific roles of macromolecular conformations of cellulose and hemicellulose in influencing the supramolecular interactions and function of plant cell walls have been determined.

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2025

Origin of Large Effective Phonon Magnetic Moments in Monolayer MoS 2

Recent helicity-resolved magneto-Raman spectroscopy measurement demonstrates large effective phonon magnetic moments of ~2.5 μ B in monolayer MoS 2 , highlighting resonant excitation of bright excitons as a feasible route to activate Γ-point circularly polarized phonons in transition metal dichalcogenides. However, a microscopic picture of this intriguing phenomenon remains lacking. In this work, we show that an orbital transition between the split conduction bands (Δ 0 = 4 meV) of MoS 2 couples to the doubly degenerate E" phonon mode (Ω 0 = 33 meV), forming two hybridized states. Our phononic and electronic Raman scattering measurements capture these two states: (i) one with predominantly phonon contribution in the helicity-switched channels and (ii) one with primarily orbital contribution in the helicity-conserved channels. An orbital-phonon coupling model successfully reproduces the large effective magnetic moments of the circularly polarized phonons and explains their thermodynamic properties. Strikingly, the Raman mode from the orbital transition is superimposed on a strong quasi-elastic scattering background, indicating the presence of spin fluctuations. As a result, the electrons excited to the conduction bands through the exciton exhibit paramagnetic behavior although MoS 2 is generally considered as a nonmagnetic material. By depositing nanometer-thickness nickel thin films on monolayer MoS 2 , we tune the electronic structure so that the A exciton perfectly overlaps with the 633 nm laser. The optimization of resonance excitation leads to pronounced tunability of the orbital-phonon hybridized states. Our results generalize the orbital-phonon coupling model of effective phonon magnetic moments to material systems beyond the paramagnets and magnets.

2D transition metal dichalcogenide↗

DOE OSTI2021

Physics‐based iterative reconstruction for dual‐source and flying focal spot computed tomography

Purpose For single‐source helical Computed Tomography (CT), both Filtered‐Back Projection (FBP) and statistical iterative reconstruction have been investigated. However, for dual‐source CT with flying focal spot (DS‐FFS CT), a statistical iterative reconstruction that accurately models the scanner geometry and acquisition physics remains unknown to researchers. Therefore, our purpose is to present a novel physics‐based iterative reconstruction method for DS‐FFS CT and assess its image quality. Methods Our algorithm uses precise physics models to reconstruct from the native cone‐beam geometry and interleaved dual‐source helical trajectory of a DS‐FFS CT. To do so, we construct a noise physics model to represent data acquisition noise and a prior image model to represent image noise and texture. In addition, we design forward system models to compute the locations of deflected focal spots, the dimension, and sensitivity of voxels and detector units, as well as the length of intersection between x‐rays and voxels. The forward system models further represent the coordinated movement between the dual sources by computing their x‐ray coverage gaps and overlaps at an arbitrary helical pitch. With the above models, we reconstruct images by an advanced Consensus Equilibrium (CE) numerical method to compute the maximum a posteriori estimate to a joint optimization problem that simultaneously fits all models. Results We compared our reconstruction with Siemens ADMIRE, which is the clinical standard hybrid iterative reconstruction (IR) method for DS‐FFS CT, in terms of spatial resolution, noise profile, and image artifacts through both phantoms and clinical scan datasets. Experiments show that our reconstruction has a higher spatial resolution, with a Task‐Based Modulation Transfer Function (MTF task ) consistently higher than the clinical standard hybrid IR. In addition, our reconstruction shows a reduced magnitude of image undersampling artifacts than the clinical standard. Conclusions By modeling a precise geometry and avoiding data rebinning or interpolation, our physics‐based reconstruction achieves a higher spatial resolution and fewer image artifacts with smaller magnitude than the clinical standard hybrid IR.

Wang, Xiao↗

DOE OSTI2022

Highly Symmetric, Self-Assembling 3D DNA Crystals with Cubic and Trigonal Lattices

The rational design of nanoscopic DNA tiles has yielded highly ordered crystalline matter in 2D and 3D. The most well-studied 3D tile is the DNA tensegrity triangle, which is known to self-assemble into macroscopic crystals. However, contemporary rational design parameters for 3D DNA crystals nearly universally invoke integer numbers of DNA helical turns and Watson–Crick (WC) base pairs. Here, in this study, 24-bp edges are substituted into a previously 21-bp (two helical turns of DNA) tensegrity triangle motif to explore whether such unconventional motif can self-assemble into 3D crystals. The use of noncanonical base pairs in the sticky ends results in a cubic arrangement of tensegrity triangles with exceedingly high symmetry, assembling a lattice from winding helical axes and diamond-like tessellation patterns. Reverting this motif to sticky ends with Watson–Crick pairs results in a trigonal hexagonal arrangement, replicating this diamond arrangement in a hexagonal context. These results showcase that the authors can generate unexpected, highly complex, pathways for materials design by testing modifications to 3D tiles without prior knowledge of the ensuing symmetry. This study expands the rational design toolbox for DNA nanotechnology; and it further illustrates the existence of yet-unexplored arrangements of crystalline soft matter.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Loops and trees in generic EFTs

We consider aspects of tree and one-loop behavior in a generic 4d EFT of massless scalars, fermions, and vectors, with a particular eye to the high-energy limit of the Standard Model EFT at operator dimensions 6 and 8. First, we classify the possible Lorentz structures of operators and the subset of these that can arise at tree-level in a weakly coupled UV completion, extending the tree/loop classification through dimension 8 using functional methods. Second, we investigate how operators contribute to tree and one-loop helicity amplitudes, exploring the impact of non-renormalization theorems through dimension 8. We further observe that many dimension 6 contributions to helicity amplitudes, including rational parts, vanish exactly at one-loop level. This suggests the impact of helicity selection rules extends beyond one loop in non-supersymmetric EFTs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

First measurement of prompt and non-prompt D* + vector meson spin alignment in pp collisions at $\sqrt{s}$ = 13 TeV

This letter reports the first measurement of spin alignment, with respect to the helicity axis, for D* + vector mesons and their charge conjugates from charm-quark hadronisation (prompt) and from beauty meson decays (non-prompt) in hadron collisions. The measurements were performed at midrapidity (|y| < 0.8) as a function of transverse momentum (p T ) in proton–proton (pp) collisions collected by ALICE at the centre-of-mass energy $\sqrt{s}$ = 13 TeV. The diagonal spin density matrix element $ρ$00 of D* + mesons was measured from the angular distribution of the D* + → D 0 (→ K - π + )π + decay products, in the D* + rest frame, with respect to the D* + momentum direction in the pp centre of mass frame. The $ρ$00 value for prompt D* + mesons is consistent with 1/3, which implies no spin alignment. However, for non prompt D* + mesons an evidence of $ρ$00 larger than 1/3 is found. The measured value of the spin density element is $ρ$00 = 0.455±0.022(stat.)±0.035(syst.) in the 5 < p T < 20 GeV/c interval, which is consistent with a Pythia 8 Monte Carlo simulation coupled with the EvtGen package, which implements the helicity conservation in the decay of D* + meson from beauty mesons. In non-central heavy-ion collisions, the spin of the D* + mesons may be globally aligned with the direction of the initial angular momentum and magnetic field. Based on the results for pp collisions reported in this letter it is shown that alignment of non-prompt D* + mesons due to the helicity conservation coupled to the collective anisotropic expansion may mimic the signal of global spin alignment in heavy-ion collisions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗