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Diffuse spectral reflectance of optically thick cloud and powder layers composed of particles with strong IR resonance, noting effect of particle size
Diffuse spectral reflectance of optically thick cloud and powder layers composed of particles with strong IR resonance, noting effect of particle size
The contributions of diffuse and specular reflection to the total canopy reflection of sunlight are determined experimentally for wheat at two stages of development using spectroradiometer measurements obtained at 13 wavelengths in the 480-720-nm range with a polarizing film in maximum and minimum signal-amplitude positions. The data and computation techniques are presented in tables, diagrams, and graphs, and the need to take specular reflection into account in constructing models of light/canopy interaction is stressed.
X-ray diffuse scattering measurements of nickel- palladium, iron-aluminum, and nickel-tungsten alloy systems
Uncontrolled beam loss at the electrostatic septum is a performance limit for several existing or planned high power hadron accelerators delivering slow-extracted spills to fixed targets. A passive diffuser, or pre-scatterer, in a suitable configuration has been shown to reduce such beamloss significantly, with the actual gain factor depending on the parameters and details of the extraction process and hardware. In this paper, the optimization of diffuser configurations is investigated for a range of beam energies and extraction conditions, and the sensitivity to the available parameters explored via simulation results. The advantages and limitations of the diffuser are discussed and conclusions drawn concerning the specific case studies of the 8 GeV Fermilab debuncher ring and 400 GeV CERN SPS.
The nature of defect clusters in Ni and Ni$_{50}$Co$_{50}$ (NiCo) irradiated at room temperature with 2–16 MeV Ni ions is studied using asymptotic diffuse X-ray scattering and transmission electron microscopy (TEM). Analysis of the scattering data provides separate size distributions for vacancy and interstitial type defect clusters, showing that both types of defect clusters have a smaller size and higher density in NiCo than in Ni. Diffuse scattering results show good quantitative agreement with TEM results for cluster sizes greater than 4 nm diameter, but find that the majority of vacancy clusters are under 2 nm in NiCo, which, if not detected, would lead to the conclusion that defect density was actually lower in the alloy. Interstitial dislocation loops and stacking fault tetrahedra are identified by TEM. Lastly comparison of diffuse scattering lineshapes to those calculated for dislocation loops and SFTs indicates that most of the vacancy clusters are SFTs.
The propagation of elastic waves in the moon, where the first seismograms were characterized by the presence of a long coda attributed to strongly scattered waves, is modeled with the aid of the time-dependent equation of radiative transfer. The average energy density as a function of time and space is described by the diffusion equation with linear dissipation on the assumption that all the energy present has been scattered many times and the time and distance scales of the problem are long compared to the scales of the scattering process. Ultrasonic experiments in the laboratory confirm the applicability of the formalism.
Significance A major challenge of protein crystallography is to accurately describe protein structure variations. Whereas Bragg peaks only yield a picture in which the variations are superimposed, diffuse X-ray scattering (diffraction between the peaks) reports on the way different atoms move together and can be used to increase the accuracy of models. We have performed a molecular-dynamics (MD) simulation of crystalline staphylococcal nuclease, yielding a rich picture of functionally important motions. This simulation is 100-fold longer than previous studies and yields reproducible calculations of diffuse intensity, overcoming a major challenge in the field. Experimental data support the MD models and indicate that diffuse scattering can be used both to validate and to improve MD simulations.
The influence of Dupree diffusivity on the occurrence scattering time advance for the electron-ion collision is investigated in turbulent plasmas. The second-order eikonal method and the effective Dupree potential term associated with the plasma turbulence are employed to obtain the occurrence scattering time as a function of the diffusion coefficient, impact parameter, collision energy, thermal energy, and Debye length. The result shows that the occurrence scattering time advance decreases with an increase of the Dupree diffusivity. Hence, we have found that the influence of plasma turbulence diminishes the occurrence time advance in forward electron-ion collisions in thermal turbulent plasmas. The occurrence time advance shows that the propensity of the occurrence time advance increases with increasing scattering angle. It is also found that the effect of turbulence due to the Dupree diffusivity on the occurrence scattering time advance decreases with an increase of the thermal energy. In addition, the variation of the plasma turbulence on the occurrence scattering time advance due to the plasma parameters is also discussed.
Recent Monte Carlo computations, based on a speculative extrapolation of the electron spectrum, suggested that repeated scatterings contribute most of the extragalactic X-ray background around 3 MeV in a Compton model. We have redone this calculation analytically with a similar electron spectrum, but with very different results. The double-scatter contribution near 3 MeV does not exceed 1 percent and cannot improve the fit to data. The effect is largest near 1 keV but will probably not be observable.
Carrier diffusion is of paramount importance in many semiconductor devices, such as solar cells, photodetectors, and power electronics. Structural defects prevent such devices from reaching their full performance potential. Although a large carrier diffusion length indicates high material quality, it also implies increased carrier depletion by an individual extended defect (for instance, a dislocation) and obscures the spatial resolution of neighboring defects using optical techniques. For commonly utilized photoluminescence (PL) imaging, the spatial resolution is dictated by the diffusion length rather than by the laser spot size, no matter the spot is at or below the diffraction limit. We show how Raman imaging of the LO phonon-plasmon-coupled mode can be used to recover the intrinsic spatial resolution of the optical system, and we demonstrate the effectiveness of the technique by imaging defects in GaAs with diffraction-limited optics, achieving a 10-fold improvement in resolution. Furthermore, by combining Raman and PL imaging, we can independently and simultaneously determine the spatial dependence of the electron density, hole density, radiative recombination rate, and non-radiative recombination rate near a dislocation-like defect, which has not been possible using other techniques.
The results of studies of the surface of GaAs in the presence of indium and phosphorus surfactants are reported. It is shown that, as a result of their diffusion (annealing) at a temperature of 650–670°C, clusters enriched with indium are formed in the GaAs surface region. The clusters can be seen as bright spots in an image obtained by a scanning electron microscope with the use of an in-lens detector. At the same time, studies of the morphology of this surface with an atomic-force microscope show a decrease in the root-meansquare roughness of the surface after annealing (diffusion), which is indicative of the incorporation of In atoms into the GaAs crystal lattice. The clusters are responsible for changes in the Raman spectra. Specifically, an increase in the signal intensity due to surface-enhanced Raman scattering and a shift of the vibration frequency in the surface region are observed. It is found that cluster formation is defined by the crystallographic orientation of the surface and by the technological conditions of surface preparation.
Measurements of energetic solar flare electrons, Jovian electrons, and low-energy solar protons have led to the suggestion that the inner heliosphere is essentially scatter free. Consideration is given to a model in which scattering is only important within the corotating interaction regions (CIR's), while the cavity formed by the CIR's in the inner heliosphere is scatter free, as compared to an interplanetary diffusion model wherein scattering is determined by the solar wind and magnetic field microstructure everywhere in the heliosphere. The two models are compared in terms of the solar wind stream associated Forbush decreases at 1 AU and the longitudinal cosmic ray nucleonic intensity variations at larger heliocentric distances (Pioneer 11 measurements at about 3 AU). It is shown that the diffusion model is able to explain consistently all longitudinal galactic cosmic ray intensity modulation measurements.
The diffusion approximation to the Fokker-Planck equation is commonly used to model the transport of solar energetic particles in interplanetary space. In this study, we present exact analytical predictions of a higher order telegraph approximation for particle transport and compare them with the corresponding predictions of the diffusion approximation and numerical solutions of the full Fokker-Planck equation. We specifically investigate the role of the adiabatic focusing effect of a spatially varying magnetic field on an evolving particle distribution. Comparison of the analytical and numerical results shows that the telegraph approximation reproduces the particle intensity profiles much more accurately than does the diffusion approximation, especially when the focusing is strong. However, the telegraph approximation appears to offer no significant advantage over the diffusion approximation for calculating the particle anisotropy. The telegraph approximation can be a useful tool for describing both diffusive and wave-like aspects of the cosmic-ray transport.
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The Apollo 17 wide-field far-ultraviolet spectrometer was used to scan six large bands of the sky during trans-earth coast. After accounting for internal scattered light and the light expected from stars in the field of view, no significant residual flux remains. This imposes important constraints on the scattering properties of the interstellar dust grains: either the grains are extremely strongly forward scattering, or the albedo of the grains is low. The absence of a scattered light signal from dusty, moderate galactic latitude regions of the sky indicates that the high galactic latitude flux reported by Henry et al. (1977) and by Anderson et al. (1979) does not represent starlight backscattered by dust.
We report a comparative neutron single crystal diffraction study of the structural and magnetic properties of layered halides CrCl3 and 𝛼−RuCl3. They host a honeycomb arrangement of transition metal ions with distinct electronic configurations and undergo a first-order structural transition between high-temperature 𝐶2/𝑚 and low-temperature 𝑅‾‾‾3. Both compounds show a step-like change in the 𝑐-lattice parameter across the structure transition. In contrast, the in-plane lattice response is quite different: 𝛼−RuCl3 exhibits an abrupt hysteretic change across the transition accompanied by progressive crystalline degradation upon thermal cycling, whereas CrCl3 shows a smooth in-plane lattice evolution and remains structurally robust. Magnetically, CrCl3 orders into an A-type antiferromagnetic structure at 𝑇𝑁=14 K and exhibits pronounced diffuse magnetic scattering extending up to about 40 K. 𝛼−RuCl3 shows no observable magnetic diffuse scattering above its zigzag antiferromagnetic ordering temperature 𝑇𝑁=7.6 K. These results suggest that the contrasting structural responses arise from an interplay between interlayer sliding energetics, stacking-strain coupling, and elastic accommodation of the stacking transition. The distinct chemical bonding and electronic configurations of the two compounds provide a microscopic basis for their different lattice responses to the structure transition and magnetic correlations.
The paper deals with a model-free approach to the analysis of quasielastic neutron scattering intensities from anomalously diffusing quantum particles. All quantities are inferred from the asymptotic form of their time-dependent mean square displacements which grow ∝t{sup α}, with 0 ≤ α < 2. Confined diffusion (α = 0) is here explicitly included. We discuss in particular the intermediate scattering function for long times and the Fourier spectrum of the velocity autocorrelation function for small frequencies. Quantum effects enter in both cases through the general symmetry properties of quantum time correlation functions. It is shown that the fractional diffusion constant can be expressed by a Green-Kubo type relation involving the real part of the velocity autocorrelation function. The theory is exact in the diffusive regime and at moderate momentum transfers.