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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 379 records · Page 21
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Exactly solvable model of light-scattering errors in quantum simulations with metastable trapped-ion qubits

Here, we analytically solve a model for light scattering in Ising dynamics of metastable atomic qubits, generalizing the approach of Foss-Feig et al. to include leakage outside the qubit manifold. We analyze the influence of these fundamental errors in simulations of proposed experiments with metastable levels of 40 Ca + ions in a Penning trap. We find that “effective magnetic fields” generated by leaked qubits have significant impacts on spin-spin correlation functions for Greenberger-Horne-Zeilinger state preparation or for quantum simulations with strong coupling, while spin squeezing uses a much weaker coupling and is largely insensitive to the simulated leakage errors, even with a few hundred ions. Our theory and results are expected to be useful in modeling a variety of metastable qubit experiments in the future.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Observation of High-Frequency Transverse Phonons in Metallic Glasses

Here, using inelastic neutron scattering and molecular dynamics simulations on a model Zr-Cu-Al metallic glass, we show that transverse phonons persist well into the high-frequency regime, and can be detected at large momentum transfer. Furthermore, the apparent peak width of the transverse phonons was found to follow the static structure factor. The one-to-one correspondence, which was demonstrated for both Zr-Cu-Al metallic glass and a three-dimensional Lennard-Jones model glass, suggests a universal correlation between the phonon dynamics and the underlying disordered structure. This remarkable correlation, not found for longitudinal phonons, underscores the key role that transverse phonons hold for understanding the structure-dynamics relationship in disordered materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Pressure Evolution of Ultrafast Photocarrier Dynamics and Electron–Phonon Coupling in FeTe 0.5 Se 0.5

Understanding the coupling between electrons and phonons in iron chalcogenides FeTe x Se 1–x has remained a critical but arduous project in recent decades. The direct observation of the electron–phonon coupling effect through electron dynamics and vibrational properties has been lacking. Here, we report the first pressure-dependent ultrafast photocarrier dynamics and Raman scattering studies on an iron chalcogenide FeTe 0.5 Se 0.5 to explore the interaction between electrons and phonons in this unconventional superconductor. The lifetime of the excited electrons evidently decreases as the pressure increases from 0 to 2.2 GPa, and then increases with further compression. The vibrational properties of the A 1g phonon mode exhibit similar behavior, with a pronounced frequency reduction appearing at approximately 2.3 GPa. The dual evidence reveals the enhanced electron–phonon coupling strength with pressure in FeTe 0.5 Se 0.5 . Our results give an insight into the role of the electron–phonon coupling effect in iron-based superconductors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1966

Dust belt of the earth.

Dynamical and light scattering properties of small dust grains orbiting Earth

TERRESTRIAL DUST BELT↗
NASA NTRS1975

Remote monitoring of environmental particulate pollution - A problem in inversion of first-kind integral equations

The determination of the microstructure, chemical nature, and dynamical evolution of scattering particulates in the atmosphere is considered. A description is given of indirect sampling techniques which can circumvent most of the difficulties associated with direct sampling techniques, taking into account methods based on scattering, extinction, and diffraction of an incident light beam. Approaches for reconstructing the particulate size distribution from the direct and the scattered radiation are discussed. A new method is proposed for determining the chemical composition of the particulates and attention is given to the relevance of methods of solution involving first kind Fredholm integral equations.

Fymat, A. L.↗
NASA NTRS1984

Comprehensive Understanding for Vegetated Scene Radiance Relationships

The improvement of our fundamental understanding of the dynamics of directional scattering properties of vegetation canopies through analysis of field data and model simulation data is discussed. Directional reflectance distributions spanning the entire existance hemisphere were measured in two field studies; one using a Mark III 3-band radiometer and one using rapid scanning bidirectional field instrument called PARABOLA. Surfaces measured included corn, soybeans, bare soils, grass lawn, orchard grass, alfalfa, cotton row crops, plowed field, annual grassland, stipa grass, hard wheat, salt plain shrubland, and irrigated wheat. Some structural and optical measurements were taken. Field data show unique reflectance distributions ranging from bare soil to complete vegetation canopies. Physical mechanisms causing these trends are proposed based on scattering properties of soil and vegetation. Soil exhibited a strong backscattering peak toward the Sun. Complete vegetation exhibited a bowl distribution with the minimum reflectance near nadir. Incomplete vegetation canopies show shifting of the minimum reflectance off of nadir in the forward scattering direction because both the scattering properties or the vegetation and soil are observed.

Kimes, D. S.↗
NASA NTRS1985

The HEAO-2 Guest Investigator Program: Non-linear growth of instabilities in line-driven stellar winds

The linear instability of line-driven stellar winds to take proper account of the dynamical effect of scattered radiation were analyzed. It is found that: (1) the drag effect of the mean scattered radiation does greatly reduce the contribution of scattering lines to the instability at the very base of the wind, but the instability growth rate associated with such lines rapidly increases as the flow moves outward from the base, reaching more than 50% of the growth rate for pure absorption lines within a stellar radius of the surface, and eventually reaching 80% of that rate at large radii; (2) perturbations in the scattered radiation field may be important for the propagation of wind disturbances, but they have little effect on the wind instability; and (3) the contribution of strongly shadowed lines to the wind instability is often reduced compared to that of unshadowed lines, but their overall effect is not one of damping in the outer parts of the wind. It is concluded that, even when all scattering effects are taken into account, the bulk of the flow in a line-driven stellar wind is still highly unstable.

Rybicki, G. B.↗
NASA NTRS1998

Towards quantifying mesoscale flows in the troposphere using Raman lidar and Sondes

Water vapor plays an important role in the energetics of the boundary layer processes which in turn play a key role in regulating regional and global climate. It plays a primary role in Earth's hydrological cycle, in radiation balance as a direct absorber of infrared radiation, and in atmospheric circulation as a latent heat energy source, as well as in determining cloud development and atmospheric stability. Water vapor concentration, expressed as a mass mixing ratio (g kg(exp -l)), is conserved in all meteorological processes except condensation and evaporation. This property makes it an ideal choice for studying many of the atmosphere's dynamic features. Raman scattering measurements from lidar also allow retrieval of water vapor mixing ratio profiles at high temporal and vertical resolution. Raman lidars sense water vapor to altitudes not achievable with towers and surface systems, sample the atmosphere at much higher temporal resolution than radiosondes or satellites, and do not require strong vertical gradients or turbulent fluctuations in temperature that is required by acoustic sounders and radars. Analysis of highly-resolved water vapor profiles are used here to characterize two important mesoscale flows: thunderstorm outflows and a cold front passage. The data were obtained at the Atmospheric Radiation Measurement Site (CART) by the groundbased Department of Energy/Sandia National Laboratories lidar (CART Raman lidar or CARL) and Goddard Space Flight Center Scanning Raman Lidar (SRL). A detailed discussion of the SRL and CARL performance during the IOPs is given by others in this meeting.

Demoz, B.↗
NASA NTRS1999

The Dissolution of an Interfween Miscible Liquids

The disappearance of the surface tension of the interface of a binary mixture, measured using the dynamic surface light scattering technique, is slower for a binary mixture of higher density contrast. A comparison with a naive diffusion model, expected to provide a lower limit for the speed of dissolution in the absence of gravity shows that the interfacial surface tension disappears much slower than even by diffusion with the effect becoming much more pronounced when density contrast between the liquid phases is increased. Thus, the factor most likely to be responsible for this anomalously slow dissolution is gravity. A mechanism could be based on the competition between diffusive relaxation and sedimentation at the dissolving interface.

Vlad, D.H.↗
NASA NTRS2012

Keck/NIRC2 Imaging of the Warped, Asymmetric Debris Disk Around HD 32297

We present Keck/NIRC2 K(sub s) band high-contrast coronagraphic imaging of the luminous debris disk around the nearby, young A star HD 32297 resolved at a projected separation of r = 0.3 - 2.5" (approx equals 35 - 280 AU). The disk is highly warped to the north and exhibits a complex, "wavy" surface brightness profile interior to r approx equals 110 AU, where the peaks/plateaus in the profiles are shifted between the NE and SW disk lobes. The SW side of the disk is 50 - 100% brighter at r = 35 - 80 AU, and the location of its peak brightness roughly coincides with the disk's mm emission peak. Spectral energy distribution modeling suggests that HD 32297 has at least two dust populations that may originate from two separate belts likely at different locations, possibly at distances coinciding with the surface brightness peaks. A disk model fur a single dust belt including a phase function with two components and a 5 - 10 AU pericenter offset explains the disk's warped structure and reproduces some of the surface brightness profile's shape (e.g. the overall "wavy" profile, the SB peak/plateau shifts) but more poorly reproduces the disk's brightness asymmetry and the profile at wider separations (r > 110 AU). Although there may be a1ternate explanations, agreement between the SW disk brightness peak and disk's peak rom emission is consistent with an overdensity of very small, sub-blowout-sized dust and large, 0.1 - 1 mm-sized grains at approx equal 45 AU tracing the same parent population of planetesimals. New near-IR and submm observations may be able to clarify whether even more complex grain scattering properties or dynamical sculpting by an unseen planet are required to explain HD 32297's disk structure.

Currie, Thayne↗
NASA NTRS2012

Keck/NIRC2 Imaging of the Warped, Asymmetric Debris Disk Around HD 32297

We present Keck/NIRC2 Ks band high-contrast coronagraphic imaging of the luminous debris disk around the nearby, young A star HD 32297 resolved at a projected separation of r = 0.3-2.5 arcse (approx 35-280 AU). The disk is highly warped to the north and exhibits a complex, "wavy" surface brightness profile interior to r approx 110 AU, where the peaks/plateaus in the profiles are shifted between the NE and SW disk lobes. The SW side of the disk is 50 - 100% brighter at r = 35 - 80 AU, and the location of its peak brightness roughly coincides with the disk's mm emission peak. Spectral energy distribution modeling suggests that HD 32297 has at least two dust populations that may originate from two separate belts likely at different locations, possibly at distances coinciding with the surface brightness peaks. A disk model for a single dust belt including a phase function with two components and a 5-10 AU pericenter offset explains the disk's warped structure and reproduces some of the surface brightness profile's shape (e.g. the overall "wavy" profile, the SB peak/plateau shifts) but more poorly reproduces the disk's brightness asymmetry. Although there may be alternate explanations, agreement between the SW disk brightness peak and disk's peak mm emission is consistent with an overdensity of very small, sub-blowout-sized dust and large, 0.1-1 mm-sized grains at approx 45 AU tracing the same parent population of planetesimals. New near-IR and submm observations may be able to clarify whether even more complex grain scattering properties or dynamical sculpting by an unseen planet are required to explain HD 32297's disk structure.

Currie, Thayne↗
NASA NTRS2022

Alma Images the Eccentric HD 53143 Debris Disk

We present ALMA 1.3 mm observations of the HD 53143 debris disk—the first infrared or millimeter image produced of this ∼1 Gyr old solar analog. Previous HST STIS coronagraphic imaging did not detect flux along the minor axis of the disk, which could suggest a face-on geometry with two clumps of dust. These ALMA observations reveal a disk with a strikingly different structure. In order to fit models to the millimeter visibilities and constrain the uncertainties on the disk parameters, we adopt a Markov Chain Monte Carlo approach. This is the most eccentric debris disk observed to date with a forced eccentricity of 0.21 ± 0.02, nearly twice that of the Fomalhaut debris disk, and also displays an apocenter glow. Although this eccentric model fits the outer debris disk well, significant interior residuals remain, which may suggest a possible edge-on inner disk, which remains unresolved in these observations. Combined with the observed structure difference between HST and ALMA, these results suggest a potential previous scattering event or dynamical instability in this system. We also note that the stellar flux changes considerably over the course of our observations, suggesting flaring at millimeter wavelengths. Using simultaneous TESS observations, we determine the stellar rotation period to be 9.6 ± 0.1 days.

Radio astronomy↗
DOE OSTI2021

Effects of the dynamical magnetization state on spin transfer

We utilize simulations of electron scattering by a chain of dynamical quantum spins to analyze the interplay between the spin transfer effect and the magnetization dynamics.We show that the complex interactions between the spin-polarized electrons and the dynamical states of the local spins can be decomposed into separate processes involving electron reflection and transmission, as well as absorption and emission of magnons—the quanta of magnetization dynamics. Analysis shows that these processes are substantially constrained by the energy and momentum conservation laws, resulting in a significant dependence of spin transfer on the electron’s energy and the dynamical state of the local spins. Here, our results suggest that exquisite control of spin transfer efficiency and of the resulting dynamical magnetization states may be achievable by tailoring the spectral characteristics of the conduction electrons and of the magnetic systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Ultralow thermal conductivity from transverse acoustic phonon suppression in distorted crystalline α-MgAgSb

Low thermal conductivity is favorable for preserving the temperature gradient between the two ends of a thermoelectric material, in order to ensure continuous electron current generation. In high-performance thermoelectric materials, there are two main low thermal conductivity mechanisms: the phonon anharmonic in PbTe and SnSe, and phonon scattering resulting from the dynamic disorder in AgCrSe2 and CuCrSe2, which have been successfully revealed by inelastic neutron scattering. Using neutron scattering and ab initio calculations, we report here a mechanism of static local structure distortion combined with phononanharmonic-induced ultralow lattice thermal conductivity in α-MgAgSb. Since the transverse acoustic phonons are almost fully scattered by the compound’s intrinsic distorted rocksalt sublattice, the heat is mainly transported by the longitudinal acoustic phonons. The ultralow thermal conductivity in α-MgAgSb is attributed to its atomic dynamics being altered by the structure distortion, which presents a possible microscopic route to enhance the performance of similar thermoelectric materials.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Phonon excitations in Eu 2 Ir 2 O 7 probed by inelastic x-ray scattering

The study of phonon dynamics and its interplay with magnetic ordering is crucial for understanding the unique quantum phases in the pyrochlore iridates. Here, through inelastic x-ray scattering on a single crystal sample of the pyrochlore iridate Eu 2 Ir 2 O 7 , we map out the phonon excitation spectra in Eu 2 Ir 2 O 7 and compare them with the theoretical phonon spectra calculated using the density functional theory. Further, possible phonon renormalization across the magnetic long-range order transition is observed in our experiments, which is consistent with the results of the previous Raman scattering experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Direct Correlation of the Salt-Reduced Diffusivities of Organic Solvents with the Solvent’s Mole Fraction

We report that lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) in organic solvents (especially propylene carbonate) has demonstrated extraordinary pseudocapacitive performance as an electrolyte in the supercapacitor configuration. However, the influence of the solvated ions on the diffusivity of the solvent molecules is yet to be understood. We examine the impact of LiTFSI on the diffusivity in five organic solvents: acetonitrile (ACN), tetrahydrofuran (THF), methanol (MeOH), dimethyl sulfoxide (DMSO), and propylene carbonate (PC) using a combination of neutron scattering, conductivity measurements, and molecular dynamics simulations. The extent of the diffusivity reduction in the concentration regime of ≤1 M directly correlates with the solvent mole fraction at which the solvation shells around Li + ions are of similar size in all the solvents, resulting in a universal ~50% reduction in the solvent diffusivity. These results provide guidance for formulation of the new electrolytes to enhance the performance of energy storage devices.

conductivity↗