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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 379 records · Page 21

Microstructural evolutions, phase transformations and hard magnetic properties in polycrystalline Ce–Co–Fe–Cu alloys

This work focuses on systematic studies of Ce–Co based 1:5 permanent magnet alloys of CeCo 4.4-x Fe x Cu 0.6 and CeCo 3.9-x Fe x Cu 1.2 (x = 0, 0.3, 0.6, 0.9, 1.2, 1.8) by varying Co:Fe. The overarching aim of this manuscript is to elucidate the hard-magnetic properties through a better understanding of phase formation by the structural, microstructural, and magnetic properties in these materials. Improved mutual solubility of Fe in the 1:5 phase has been observed with an extended homogeneity range by Cu substitution. For both composition series, Fe contents of x ≤ 0.6 show a homogeneous microstructure with a single 1:5 phase and good magnetic properties. The composition region 0.6 < x ≤ 0.9 appears to be near the boundary of solubility and evolution of other phases. At x = 1.8, it is found that the homogeneous 1:5 phase and magnetic hardness deteriorated due to the evolution of secondary phases such as 2:17, 2:7, and Fe–Co. Furthermore, the addition of Fe improved both the magnetization and Curie temperature via increased effective exchange interactions, while an increase in Cu content enhanced coercivity.

33 ADVANCED PROPULSION SYSTEMS↗

The onset of alloying in Cu-Ni powders under high-shear consolidation

Friction consolidation (FC) is a solid phase processing methodology that densifies a material through high-shear deformation and pressure at elevated temperature. The method has garnered interest in the scientific community because of its ability to produce extremely refined and homogeneous microstructures, off-axis texture development, and improved material properties. This manuscript presents an investigation of Cu and Ni material mixing via evaluation of morphological evolution, grain boundary characterization, and compositional analysis to provide insights on the operational alloying mechanisms occurring under high shear and elevated temperature. Using correlative microscopy techniques, we show alloying progresses via a combination of grain boundary diffusion and interfacial roughening at heterophane boundaries. Evidence supporting Cu infiltration along Ni-Ni grain boundaries along with asymmetric diffusion of Cu into Ni grains is highlighted. The resultant, consolidated microstructure was produced directly from a powder compact in ~30 s and exhibited a submicron, equiaxed grain size.

36 MATERIALS SCIENCE↗

Influence of post deposition annealing on the microstructural evolution and tensile behavior of austenitic stainless-steel alloy 709 made by laser powder bed fusion

Structural materials used in the next generation nuclear reactors or other advanced energy systems are often required to withstand higher operating temperatures for a longer service life. Alloy 709 (A709), a Nb-containing and N-stabilized Fe-25Ni-20Cr austenitic stainless steel, has been recommended for high-temperature reactor constructions due to the better performance over the baseline Type 316H stainless steel. Here, in the current manuscript, for the first time, the microstructure evolution and tensile behavior of an A709 made by laser powder bed fusion (LPBF) is discussed. The as deposited and heat treated LPBF alloys are compared with a reference wrought alloy. Owing to the chemical segregation and a higher number of dislocations, the LPBF materials show a significantly higher density of precipitates formed during high temperature treatments when compared to the wrought samples. This is reflected when looking at the tensile properties, both at room and elevated temperatures, where LPBF samples show higher strengths compared to wrought materials.

36 MATERIALS SCIENCE↗

Porosity evolution during heating of copper made from powder by friction extrusion

Here, friction extrusion was used to compact and extrude solid copper rod from feedstock powders. Following extrusion, considerable porosity was observed throughout the extrudate cross section due to the entrained porosity in the feedstock material and the extrusion process. The thermal stability of the extrudate was investigated via a series of heat treatments. Porosity evolution exhibited three distinct stages—an unchanged plateau (0°C–300°C) followed by an abrupt increase (400°C–500°C) and ultimately a reduction, as the temperature increases (>500°C). The peak porosity measured was ~25%. The underlying driving force for pore evolution is described as the competition between the internal pore pressure, material strength, and sintering kinetics, as a function of temperature. The observed porosity evolution and driving force are not expected to be limited to copper. Thus, this manuscript reveals an important consideration regarding elevated-temperature thermal stability as advanced manufacturing methods involving direct powder extrusion are explored.

36 MATERIALS SCIENCE↗

The fast non-ferric kicker system for the Muon g–2 Experiment at Fermilab

Here we describe the installation, commissioning, and characterization of the new injection kicker system in the Muon g – 2 Experiment (E989) at Fermilab, which makes a precision measurement of the muon magnetic anomaly. Three Blumlein pulsers drive each of the 1.27-m-long non-ferric kicker magnets, which reside in a storage ring vacuum (SRV) that is subjected to a 1.45 T magnetic field. The new system has been redesigned relative to Muon g – 2 ’s predecessor experiment, and we present those details in this manuscript.

43 PARTICLE ACCELERATORS↗

The Timepix4 analog front-end design: Lessons learnt on fundamental limits to noise and time resolution in highly segmented hybrid pixel detectors

This manuscript describes the optimization of the front-end readout electronics for high granularity hybrid pixel detectors. The theoretical study aims at minimizing the noise and jitter. The model presented here is validated with both circuit post layout simulations and measurements on the Timepix4 Application Specific Integrated Circuit (ASIC). The analog front-end circuit and the procedure to optimize the dimensions of the main transistors are described with detail. The Timepix4 is the most recent ASIC designed in the framework of the Medipix4 Collaboration. It was manufactured in 65nm CMOS process, and consists of a four side buttable matrix of 448 × 512 pixels with 55µm pitch. The analog front-end has a gain of ~36mV/ke - when configured in High Gain Mode, and ~20mV/ke - when configured in Low Gain Mode. The Equivalent Noise Charge (ENC) is ~68e - rms and ~80e - rms in High Gain Mode and in Low Gain Mode respectively. In event driven mode the incoming hits can be time stamped within a ~ 200ps time bin and the chip can deal with a maximum flux of ~ 3.6MHzmm –2 s –1 . In photon counting mode, the chip can deal with up to ~ 5GHzmm –2 s –1 . The routine designed to optimize the Timepix4 front-end is then used to analyze the performance limits in terms of jitter and noise for Charge Sensitive Amplifiers in pixel detectors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Comparative assessment of different aluminum alloys for neutron beam window applications

The choice of an aluminum alloy window along a neutron beam requires careful consideration depending on the requirements of the instrument end station. The windows should generally be thin to minimize loss of neutrons from the beam due to scattering and absorption but still thick enough to be structurally sound for safety requirements. Further, the microstructure of the material is dependent on the alloy and the preparation method and may introduce scattering artifacts or smearing of the instrument resolution that are not desirable. In this manuscript, SANS and total cross section measurements of several different aluminum alloys will be presented and compared in order to provide some useful insight to engineers working on future neutron instrument design.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Design, construction, and performance of the GEM based radial time projection chamber for the BONuS12 experiment with CLAS12

Here, a new radial time projection chamber based on Gas Electron Multiplier amplification layers was developed for the BONuS12 experiment in Hall B at Jefferson Lab. This device represents a significant evolutionary development over similar devices constructed for previous experiments, including cylindrical amplification layers constructed from single continuous GEM foils with less than 1% dead area. Particular attention had been paid to producing excellent geometric uniformity of all electrodes, including the very thin metalized polyester film of the cylindrical cathode. This manuscript describes the design, construction, and performance of this new detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The ATLAS ITk Strip detector system for the Phase-II LHC upgrade

In the view of the luminosity increase foreseen by the High-Luminosity Large Hadron Collider program at CERN, the ATLAS experiment initiated an R&D program to replace its complete inner detector (ID) system. The new Inner Tracker (ITk) system, anticipated to be installed by 2028, will be a new all-silicon based tracker including Strip and Pixel detector technologies. The new detector is designed to meet the requirements of operating under a harsh environment namely, high radiation levels, increased pile-up and data rates while decrease the material budget and maintain or even improve the performance. The Strip project has advanced in several areas the last years while facing challenges moving from pre-production to production. Here, this manuscript gives an overview of the ITk Strip system and describes the advancements and challenges to date.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Artificial intelligence time series forecasting for feed-forward laser stabilization

Laser plasma accelerators, typically operating at 1–10 Hz repetition rates, have the ability to produce high-quality electron beams in compact, all-optical-driven configurations, with the electron beams uniquely suited for a wide variety of accelerator-based applications. However, fluctuations and drifts in the laser delivery to the meter-scaled and below plasma target (the electron beam source) will translate into electron beam source variations that can limit their utility for demanding applications like light sources or linear colliders. Commercially available active feedback laser stabilization systems are intrinsically bandwidth limited due to their integration with multi-inch corrective mirror mounts which minimizes their effectiveness. In this manuscript, we present a Neural Network time series forecaster that can predict laser position fluctuations of the laser delivery to the final target well ahead of a future laser shot. The Root-Mean-Square-Error (RMSE) of the prediction accuracy was < 2 μ m for a 1 / e 2 beam radius of 34 μ m . Our feed-forward approach serves as a first-step in circumventing the bandwidth limitations imposed by the currently available stabilization systems since it allows for mirrors to be moved into position ahead of time to offset the predicted future position drift. This will help advance laser plasma accelerator research by providing greater robustness and stability needed for its applications.

Berger, Curtis↗

Radiation hot spot formation on UF 6 30B cylinders

The accurate material accountancy of a country's enriched uranium hexafluoride (UF 6 ) stockpiles is imperative to the International Atomic Energy Agency (IAEA) for determining appropriate material safeguards. Uranium hexafluoride is typically stored in large cylinders with enrichment verification typically performed with a NaI gamma detector using the enrichment meter method. This approach for calculating enrichment assumes that the UF 6 is homogeneous inside the cylinder. Here, the measurements and tests presented in this manuscript show that the UF 6 in cylinders left outside in the elements can experience fractionation, leading to inhomogeneity, and subsequent development of radiation hot spots. These hot spot locations can produce errant enrichment measurements. In dark-colored cylinders that experience significant surface heating from the sun, UF 6 sublimates off the cylinder walls, leaving only the uranium daughter products in a horizontal patch (stripe) along the cylinder's midline. This daughter patch is hypothesized to be the source of the radiation hot spots. The patch forms during the summer and tends to decay away during the winter, when solar intensity and temperatures are reduced.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Characterization of the optical model of the T2K 3D segmented plastic scintillator detector unit cube

The magnetized near detector (ND280) of the T2K long-baseline neutrino oscillation experiment has been recently upgraded aiming to satisfy the requirement of reducing the systematic uncertainty from measuring the neutrino–nucleus interaction cross section, which is the largest systematic uncertainty in the search for leptonic charge-parity symmetry violation. A key component of the upgrade is SuperFGD, a 3D segmented plastic scintillator detector made of approximately 2,000,000 optically-isolated 1 cm 3 cubes. The SuperFGD cube unit shows promising optical performance, including a high light yield of about 40 photoelectrons (p.e.) per channel, a low cube-to-cube crosstalk rate below 3%, and a sub-nanosecond time resolution of 0.96 ns. By combining tracking and stopping power measurements of final state particles, this novel detector enables precise 3D-imaging of GeV neutrino interactions with reduced systematic uncertainties. A detailed Geant4 based optical simulation of the SuperFGD building block, i.e. a plastic scintillating cube read out by three wavelength shifting fibers, has been developed and validated with the different datasets collected in various beam tests. In this manuscript the description of the optical model as well as the comparison with data are reported.

Neutrino oscillations↗

Temperature-dependent calibration procedures for the silicon photomultiplier readout of the cosmic ray veto detector for the Mu2e experiment

The cosmic ray veto detector for the Mu2e experiment consists of scintillation bars embedded with wavelength-shifting fibers and read out by silicon photomultipliers (SiPMs). Here, in this manuscript, the calibration procedures of the SiPMs are described including corrections for the temperature dependence of their light yield. These corrections are needed as the SiPMs are not kept at a constant temperature due to the complexity and cost of implementing a cooling system on such a large detector. Rather, it was decided to monitor the temperature to allow the appropriate corrections to be made. The SiPM temperature dependence has been measured in a dedicated experiment and the calibration procedures were validated with data from production detectors awaiting installation at Fermilab.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Design and commissioning of the Correlated Gamma-Neutron Array for sCattering (CoGNAC)

The Correlated Gamma-Neutron Array for sCattering (CoGNAC) is a dual $n$-$γ$ detector array fielded at the Weapons Neutron Research facility at the Los Alamos Neutron Science Center. Here, the detector array utilizes elpasolite detectors and liquid scintillators to perform measurements of neutron elastic and inelastic scattering cross sections and emitted particle angular distributions. This manuscript details the design and experimental setup of CoGNAC as well as some of the preliminary studies performed to select the elpasolite detectors deployed in the array. Examples of the analysis methods available to CoGNAC are given in the context of past CoGNAC measurements of neutron scattering reactions on 28 Si and 56 Fe.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterization of dynamics and decay in the St. Benedict Paul trap

The St. Benedict experiment includes a linear Paul trap designed to measure the beta-neutrino angular correlation coefficient 𝑎 𝛽ν of mixed superallowed 𝛽-decay transitions between mirror nuclei via coincidence detection of 𝛽-particles and recoiling ions. The emitted 𝛽 particle and daughter ion are detected with plastic scintillators and micro-channel plate detectors, respectively, allowing for accurate measurements of their time-of-flights. From the shape of the coincidence time-of-flight distribution, a value of 𝑎 𝛽ν can be determined. This manuscript presents detailed simulations of the St. Benedict Paul trap, with a focus on ion cloud dynamics and recoiling daughter trajectories.

Linear Paul trap↗

Deep glassy state dynamic data challenge glass models: Elastic models

The idea of an “ideal” glass transition temperature has persisted at least since the work from Kauzmann when it was observed that the entropy of glass-forming liquids extrapolated to below that of the crystal, thus suggesting the need for a phase transition at a finite or non-zero absolute temperature. This thermodynamic paradox was also found to be related to the observations of a diverging of the extrapolated viscosity or relaxation times at a temperature near to this ideal glass transition. Recently, however, we have carried out experiments using both an ancient amber material and an ultra-stable amorphous fluoropolymer that challenge the ideas of the divergence of the viscosity or relaxation times at this ideal glass transition. In the present manuscript we have evaluated two theories of the glass transition that are based on ideas related to elasticity of the amorphous glass-forming material. We find that the models from both J. Dyre and his group and of K.S. Schweizer and his group not only show non-diverging behavior but are also in some agreement with the new data, though still showing somewhat slower dynamics than those observed in the experiments. The work shows that the data are good enough to distinguish between theories and it is suggested that other mechanisms may be needed to fully describe the non-diverging responses of the ultra-stable glasses.

36 MATERIALS SCIENCE↗

Limitations of traditional tools for beyond design basis external hazard PRA

Probabilistic risk assessment (PRA) is being used increasingly by the nuclear industry for safety during normal operations as well as for the protection against external hazards. Computation of total risk in an external hazard PRA is dependent on hazard assessment, fragility assessment, and systems analysis. A systems analysis for propagation of component fragilities is conducted using event and fault trees. The event and fault trees for an actual power plant can be fairly large in size, which imposes computational challenges. Hence, certain assumptions are employed for computational efficiency. These assumptions typically represent the conditions imposed during the design basis (DB) scenario. The traditional PRA tools based on these assumptions are also widely applied to perform risk assessment in the context of beyond design basis (BDB) scenarios. However, some of these assumptions may not be valid for certain BDB scenarios. In addition, the probability of dependent failures also increases in BDB scenarios due to common cause failures (CCF) which usually results from design modifications, human errors, etc. In this manuscript, a simple and a relatively more complex illustrative examples are used to show the limitation of these assumptions in the numerical quantification of risk for the case of BDB conditions. Case studies with CCF events across multiple fault trees are also presented to illustrate the effect of these assumptions when traditional approach is used in BDB risk assessment. It is shown that the assumptions are valid for the case of DB conditions but may lead to excessively conservative risk estimates in the case of BDB conditions. Finally, a Bayesian network based top-down algorithm is proposed as an alternative tool for accurate numerical quantification of total risk in systems analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Revisiting Bayesian constraints on the transport coefficients of QCD

Multistage models based on relativistic viscous hydrodynamics have proven successful in describing hadron measurements from relativistic nuclear collisions. These measurements are sensitive to the shear and the bulk viscosities of QCD and provide a unique opportunity to constrain these transport coefficients. Bayesian analyses can be used to obtain systematic constraints on the viscosities of QCD, through methodical model-to-data comparisons. In this manuscript, we discuss recent developments in Bayesian analyses of heavy ion collision data. Furthermore, we highlight the essential role of closure tests in validating a Bayesian analysis before comparison with measurements. We discuss the role of the emulator that is used as proxy for the multistage theoretical model. We use an ongoing Bayesian analysis of soft hadron measurements by the JETSCAPE Collaboration as context for the discussion.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗