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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 379 records · Page 21

Analysis of MINERvA tunings of GENIE based on Hadron Multiplicity using Machine Learning

Scientists with the MINERvA neutrino interaction experiment have long studied distributions of hadrons (protons and pions) to improve the models for these reactions. Until now, most work has relied on easy to find, energetic, and well tracked hadrons. But in order to take full advantage of MINERνA data it is necessary to develop an efficient enough tool to recognize hadron tracks with lower energy, more transverse angle and more challenging patterns of activity. In this analysis, a Machine Learning tool based on Convolutional Neural Network and Transfer Learning has been developed to tackle that issue. It is found to be extremely capable of recognizing hadron activities especially when there are few and not very energetic hadrons, the accuracy is 76%. But it is also found that this network is very reluctant to classify too many hadrons. The classification is also affected by the presence of other particles in the event such photons, hadrons below a threshold or neutrons. This network is used to compare hadron multiplicity of data to the MC models and distinguish between different MC tunes. Some MINERνA tunes are explored in this analysis, but none of them described the data very well, especially not for all different hadrons multiplicities at once. Four combinations of those tunes were more successful, but none of them could be recognized as the best one. Nevertheless, this analysis develops an ML network that sets the basis of further exploration of hadron multiplicity as a tool to analyze MC tunes at MINERνA and beyond.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Imaging Based Detector with Efficient Scintillators for Neutron Diffraction Measurements

The Anger Camera developed by the detector group at the Oak Ridge National Laboratory was utilized for the present work for its unique advantage of employing multiple modules to obtain large active measurement area for detecting diffracted/scattered thermal neutrons. Considering the relatively small flux associated with diffracted/scattered neutrons, suitable efficiency with high spatial resolution is a requirement for utilizing two-dimensional imaging detectors. The potential to implement pulse shape (in addition to pulse height) discrimination-based scintillators further enhances the ability to detect diffracted neutrons with improved signal to noise ratio. In this paper, initial results associated with 6Li glass-based scintillator will be presented. The authors explored the feasibility of using this system to detect and quantify diffraction peaks and peak shifts at the Neutron Residual Stress Facility (NRSF2), High Flux Isotope Reactor (HFIR) in the Oak Ridge National Laboratory (ORNL). Suitable camera mounting and shielding had to be developed. Reference measurements using polycrystalline powders with known atomic planar spacing will be discussed along with measurement settings associated with expected resolution for peak shift measurements. Initial results are promising and demonstrate that a suitable scintillation-based neutron detecting system is viable for residual stress-based diffraction measurements. Small area detectors are also feasible with suitable consideration to scattering volume and distance to detector.

Seals, Matthew↗

Gantryless Associated-Particle Neutron Radiography

The present work reports on the development of techniques for in-field fast-neutron radiography measurements using the associated-particle imaging (API) method. The API method employs alpha-neutron coincidences from the d+t→α+n reaction to enable fast neutron transmission imaging with excellent contrast using a wide cone beam. However, for field radiography applications, the API method is burdened by the need for the relative positions of the source and detector to be known. Fortunately, these relative positions can be inferred from transmission data. The inferred positions also enable accurate stitching of multiple images into a composite image even when using a low-resolution detector panel and acquiring images having few overlapping pixels. The developed techniques address analysis of measurements where (1) the source and detector panel are separately hand positioned rather than held in registration by a gantry, (2) multiple detector panel positions within the “coincident cone” of tagged neutrons are required to piece together an image of an item of interest, and (3) normalization measurements that have identical source-detector positioning but without the inspected object are not possible. The present work will describe the system calibrations (including timing calibrations and neutron direction calibrations) necessary for subsequent analyses, the method of locating the detector in the coincident cone of neutrons with millimeter precision using the timing and directions of coincident neutrons, the method of calculating a normalization image for a given detector panel position, and the method used to project multiple images into a common image.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Multiple fermion scattering in the weakly coupled spin-chain compound YbAlO 3

The Heisenberg antiferromagnetic spin-1/2 chain, originally introduced almost a century ago, is one of the best studied models in quantum mechanics due to its exact solution, but nevertheless it continues to present new discoveries. Its low-energy physics is described by the Tomonaga-Luttinger liquid of spinless fermions, similar to the conduction electrons in one-dimensional metals. In this work we investigate the Heisenberg spin-chain compound YbAlO3 and show that the weak interchain coupling causes Umklapp scattering between the left- and right-moving fermions and stabilizes an incommensurate spin-density wave order at q = 2k F under finite magnetic fields. These Umklapp processes open a route to multiple coherent scattering of fermions, which results in the formation of satellites at integer multiples of the incommensurate fundamental wavevector Q = nq. Our work provides surprising and profound insight into bandstructure control for emergent fermions in quantum materials, and shows how neutron diffraction can be applied to investigate the phenomenon of coherent multiple scattering in metals through the proxy of quantum magnetic systems.

36 MATERIALS SCIENCE↗

Fused x-ray and fast neutron CT reconstruction for imaging large and dense objects

Megavolt x-ray computed tomography (CT) is a powerful tool for three-dimensional characterization. However, its utility is limited for large objects composed of high-atomic number (Z) materials, where x rays fail to penetrate. Information from fast neutron CT (FNCT) can complement x-ray CT reconstructions since fast neutrons can more readily penetrate high-Z objects. In this work, we demonstrate a method for combining FNCT and x-ray CT data to create a single reconstruction, more accurate than could be achieved with either x rays or fast neutrons alone. The algorithm was tested on an exemplar comprising multiple concentric, nested cylinders of different materials. Simulated and empirical x-ray CT data were acquired for the exemplar using a 9 MV bremsstrahlung spectrum. Additional simulated and empirical FNCT data were acquired using an accelerator based fast neutron source. The FNCT data were used to synthesize x-ray CT data and augment the x-ray CT data missing due to lack of penetration. This approach mitigates artifacts that would otherwise negatively affect the accuracy and resolution of a single-modality reconstructed volume.

47 OTHER INSTRUMENTATION↗

Elucidating Structural Disorder in Ultra‐Thin Bi‐Rich Bismuth Oxyhalide Photocatalysts

Abstract Advancing the field of photocatalysis requires the elucidation of structural properties that underpin the photocatalytic properties of promising materials. The focus of the present study is layered, Bi‐rich bismuth oxyhalides, which are widely studied for photocatalytic applications yet poorly structurally understood, due to high levels of disorder, nano‐sized domains, and the large number of structurally similar compounds. By connecting insights from multiple scattering techniques, utilizing electron‐, X‐ray‐ and neutron probes, the crystal phase of the synthesized materials is allocated as layered Bi 24 O 31 X 10 (X = Cl, Br), albeit with significant deviation from the reported 3D crystalline model. The materials comprise anisotropic platelet‐shaped crystalline domains, exhibiting significant in‐plane ordering in two dimensions but disorder and an ultra‐thin morphology in the layer stacking direction. Increased synthesis pH tailored larger, more ordered crystalline domains, leading to longer excited state lifetimes determined via femtosecond transient absorption spectroscopy (fs‐TAS). Although this likely contributes to improved photocatalytic properties, assessed via the photooxidation of benzylamine, increasing the overall surface area facilitated the most significant improvement in photocatalytic performance. This study, therefore, enabled both phase allocation and a nuanced discussion of the structure‐property relationship for complicated, ultra‐thin photocatalysts.

Chemistry↗

Monte Carlo calculation of the average neutron depolarization for the NPDGamma experiment

The NPDGamma experiment measures the asymmetry in γ-ray emission in the capture of polarized neutrons on liquid parahydrogen. The beam polarization is measured using 3 He spin analysis, but this measurement does not account for the contribution of depolarization from spin–flip scattering primarily due to orthohydrogen in the bulk liquid. This is a systematic effect that dilutes the experimental asymmetry and is modeled using Monte Carlo. Finally, methods for tracking neutron spin in MCNPX were developed in order to calculate the average neutron polarization upon capture for use as a multiplicative correction to the measured beam polarization for the NPDGamma experiment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Thermonuclear performance variability near ignition at the National Ignition Facility

We describe our current understanding of the variability and degradation mechanisms observed through a series of five indirectly driven inertial fusion implosions fielded at the National Ignition Facility in the fall of 2021, four of which attempted to reproduce the first experiment to achieve Lawson's criterion for ignition with a thermonuclear yield of 1.35 MJ on August 8, 2021. A large number of absolutely calibrated (imaging, time-resolved, and spectrally resolved) x-ray and neutron diagnostics are fielded on the NIF along multiple lines of sight for each experiment. This allows for a reconstruction of the DT fuel and ablator mix injected into the hotspot around peak burn. We show that nuclear yield variations are well reproduced by numerical modeling when the measured low mode asymmetries and mix mass are included. Furthermore, these observed perturbations during burn are linked to small variations in laser delivery and capsule defects. Stringent specifications are then set to achieve robust ignition with the implosion design studied in this paper.

Divol, L. (ORCID:0000000269699898)↗

Spallation Neutron Source Hydrogen Relief Analysis for the Cryogenic Moderator System

The Spallation Neutron Source at Oak Ridge National Laboratory operates the Cryogenic Moderator System (CMS) which provides hydrogen cooling at 20K to three neutron moderators. Each hydrogen loop is protected by multiple burst discs and reclosing relief valves. As a result of the Proton Power Upgrade project, the CMS moderator loops will hold more hydrogen and thus require piping modifications. Operational experience has demonstrated that transient pressure increases in these hydrogen loops occasionally result in the rupture of the burst discs. The causes for pressure transients in the system that might lead to hydrogen venting are varied and complex, for example loss of vacuum or cooling. Dynamic simulation and analysis of the parameters considered as the worst-case relief venting scenario were performed and will be presented.

47 OTHER INSTRUMENTATION↗

Spin excitations in the kagome-lattice metallic antiferromagnet Fe 0.89 Co 0.11 Sn

Kagome-lattice materials have attracted tremendous interest due to the broad prospect for seeking superconductivity, quantum spin liquid states, and topological electronic structures. Among them, the transition-metal kagome lattices are high-profile objects for the combination of topological properties, rich magnetism, and multiple-orbital physics. Here we report an inelastic neutron scattering study on the spin dynamics of a kagome-lattice antiferromagnetic metal Fe 0.89 Co 0.11 Sn. Although the magnetic excitations can be observed up to ~250 meV, well-defined spin waves are only identified below ~90 meV and can be modeled using Heisenberg exchange with ferromagnetic in-plane nearest-neighbor coupling J 1 , in-plane next-nearest-neighbor coupling J 2 , and antiferromagnetic (AFM) interlayer coupling J c under linear spin-wave theory. Above ~90 meV, the spin waves enter the itinerant Stoner continuum and become highly damped particle-hole excitations. At the K point of the Brillouin zone, we reveal a possible band crossing of the spin wave, which indicates a potential Dirac magnon. Finally, our results uncover the evolution of the spin excitations from the planar AFM state to the axial AFM state in Fe 0.89 Co 0.11 Sn, solve the magnetic Hamiltonian for both states, and confirm the significant influence of the itinerant magnetism on the spin excitations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Benchmark evaluation of one dimensional array of HEU moderated and reflected by Lucite

The evaluation of two HEU-Lucite experiments is presented. The critical experiments were performed using the Planet Universal Critical Assembly Machine at Los Alamos National Laboratory in 2019. In these experiments, HEU foils were interleaved with Lucite in a column stack and were moderated and reflected from the square Lucite plates. The neutron data produced were used to approximate the multiplication of each measured configuration. The evaluation of the experiments using calculational techniques is presented in the paper. A Monte-Carlo computational model to be used with MCNP6 was developed for the determination of uncertainties and the effects of various uncertainties on the multiplication factor were studied. The evaluation of the benchmark was performed for comparison of calculation results with the experimental data and validation of calculation techniques in particular the newly available thermal scattering data for the Lucite material. The sensitivity studies include parametric variations of material composition and geometry. Experimental uncertainties were low, with the overall height of the HEU/Lucite stack being the largest contributor to the overall uncertainty in k{sub eff}. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Uncertainties Associated with the Nucleosynthesis in Ejecta of a Black Hole Accretion Disk

Abstract The simulation of heavy element nucleosynthesis requires input from yet-to-be-measured nuclear properties. The uncertainty in the values of these off-stability nuclear properties propagates to uncertainties in the predictions of elemental and isotopic abundances. However, for any given astrophysical explosion, there are many different trajectories, i.e., temperature and density histories, experienced by outflowing material, and thus different nuclear properties can come into play. We consider combined nucleosynthesis results from 460,000 trajectories from a black hole accretion disk and find the spread in elemental predictions due solely to unknown nuclear properties to be a factor of a few. We analyze this relative spread in model predictions due to nuclear variations and conclude that the uncertainties can be attributed to a combination of properties in a given region of the abundance pattern. We calculate a cross-correlation between mass changes and abundance changes to show how variations among the properties of participating nuclei may be explored. Our results provide further impetus for measurements of multiple quantities on individual short-lived neutron-rich isotopes at modern experimental facilities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Additive manufacturing of composite neutron absorbing components

Collimators and other components for use in neutron scattering experiments or to provide neutron shielding in nuclear reactors or accelerator based neutron sources are produced by additive manufacturing from multiple different types of material, such as boron carbide (B4C), steel, isotopically enriched boron carbide (10B4C), and blends thereof.

Anderson, David C.↗

Combined Environments: Driving multiple loads on Z

Pulsed power drivers such as the Z generator of Sandia National Laboratories typically deliver high current (>20MA) to single experiments. This project is intended to develop and assess ways to simultaneously drive multiple targets on a single pulsed power driver (specifically a neutron and an x-ray producing target driven in a single experiment). The combined x-ray/neutron environment produced will then be used to investigate potential synergistic effects in integrated circuits. A pre-requisite for being able to design and study multiple targets on Z is first adapting simulation tools to be able to model them effectively. This will enable us to assess the tradeoffs between the different ways multiple targets can be combined, and to better understand how existing and future pulsed power machines can be used to generate combined testing environments. This report is limited to documenting the initial development of a parallel load modeling capability that is presently being applied to design experiments to produce combined neutron/x-ray environments on Z.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The Role of a Neutron Component in the Photospheric Emission of Long Duration Gamma-Ray Burst Jets

Long-duration gamma-ray bursts (LGRBs), thought to be produced during core-collapse supernovæ, may have a prominent neutron component in the outflow material. If present, neutrons can change how photons scatter in the outflow by reducing its opacity, thereby allowing the photons to decouple sooner than if there were no neutrons present. Understanding the details of this process could therefore allow us to probe the central engine of LGRBs, which is otherwise hidden. Here, we present results of the photospheric emission from an LGRB jet, using a combination of relativistic hydrodynamic simulations and radiative transfer post-processing using the Monte Carlo Radiation Transfer (MCRaT) code. We control the size of the neutron component in the jet material by varying the equilibrium electron fraction Y e , and we find that the presence of neutrons in the GRB fireball affects the Band parameters α and E 0 , while the picture with the β parameter is less clear. In particular, the break energy E 0 is shifted to higher energies. Additionally, we find that increasing the size of the neutron component also increases the total radiated energy of the outflow across multiple viewing angles. Our results not only shed light on LGRBs, but are also relevant to short-duration gamma-ray bursts associated with binary neutron star mergers, due to the likelihood of a prominent neutron component in such systems.

Gamma-ray bursts↗

Inferring Water Content from Neutron Die-away Curves for Planetary Science Applications

Signatures of liquid water on planetary bodies may provide evidence for past, present, or future life elsewhere in the solar system. Multiple current and upcoming planetary science missions are prioritizing the search for water, using innovative technologies and creative algorithms. For this project, we explore the capabilities of an instrument similar to the Dragonfly spacecraft to map water content on the surface of Titan, the largest moon of Saturn. We simulate Dragonfly’s neutron observations for a variety of soil compositions and develop multiple techniques to extract water content from the resultant neutron data. Additionally, we supplement neutron observations with gamma spectroscopy in an attempt to further refine water content estimates. This work is part of a larger study to employ Gaussian process regression to estimate a map of water content along the surface of Titan. Using the estimated map, an algorithm based on prediction difference mapping is employed to optimally move multiple Dragonfly detectors around the surface of Titan, fully autonomously.

79 ASTRONOMY AND ASTROPHYSICS↗

Overview of the Neutron Radiography Reactor (NRAD) for Neutron Imaging and In-Core Experiment Capabilities at Idaho National Laboratory

NRAD is a 250-kilowatt TRIGA research reactor that first went online at INL in 1977. (TRIGA stands for Training, Research, Isotopes, General Atomics.) Historically, NRAD was utilized as a neutron radiography reactor that provides comprehensive, non-destructive information about the internal condition of irradiated nuclear fuel. Idaho National Laboratory (INL) has multiple nuclear fuels research and development programs that routinely evaluate irradiated fuels using neutron radiography at NRAD. In recent years, NRAD has gone through a transformation from the single purpose radiography reactor for which it was designed into a multipurpose research reactor, and expanding its in-core irradiation capabilities to support a broader mission for the US Department of Energy (DOE) Nuclear Energy (NE) programs, Basic Energy Science (BES) Programs, as well as Fusion Energy programs. NRAD is a designated user facility under the DOE Nuclear Science User Facility (NSUF) program, and is available for access for general public via a competitive proposal process. More information about NSUF and NRAD are available from the website: https://nsuf.inl.gov/Home/Facility/654.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗