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DOE OSTI2018

NSUF 2016 Annual Report

The Nuclear Science User Facilities (NSUF) and its partner facilities represent a prototype laboratory that utilizes a distributed partnership, with each facility bringing exceptional capabilities to the relationship including reactors, beamlines, state-of-the-art instruments, hot cells, and equally important, expertise. These capabilities and people together create a nationwide infrastructure that allows the best ideas to be tested using the most advanced capabilities. Through the NSUF, researchers and their collaborators are building on current knowledge to better understand the complex behavior of materials and fuels in a nuclear reactor. The NSUF’s partnership program in 2016 included eight universities, one research and education consortium, three national laboratories, and one industry partner. The avenues opened through these partnerships facilitate cooperative research across the country, matching people with capabilities and students with mentors. The NSUF in 2016 included Idaho National Laboratory (INL) and the following institutions: • Argonne National Laboratory • Center for Advanced Energy Studies (a research and education consortium between Boise State University, INL, Idaho State University, University of Idaho, and University of Wyoming) • Illinois Institute of Technology • Massachusetts Institute of Technology • North Carolina State University • Oak Ridge National Laboratory • Pacific Northwest National Laboratory • Purdue University • University of California, Berkeley • University of Michigan • University of Nevada, Las Vegas • University of Wisconsin • Westinghouse Materials Center of Excellence. This report contains details on new capabilities brought into the NSUF in 2016, the evidence of the increasing research facilitated by the NSUF, and new tools and activities to propel nuclear research and development forward to meet energy reliability and security needs. Learn about the NSUF Nuclear Fuels and Materials Library and the Nuclear Energy Infrastructure Database, and how the robust NSUF website continues to evolve to support new tools. Read about how the NSUF supports Department of Energy (DOE) missions through efforts like the 2016 NSUF Ion Beam Options Workshop, which led to a prioritiza-tion of ion beam facilities according to their ability to support Department of Energy Office of Nuclear Energy (DOE-NE) missions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2025

Perspectives on Tailoring Neutron Energy Spectra in Material Test Reactors

Material test reactors (MTRs) are used to irradiate nuclear fuels and materials to develop data for how they endure neutron bombardment in or near reactor cores. Most historic MTRs, and all that remain operational in the US today, are water-cooled types and produce a thermalized neutron flux. New irradiation facilities are needed which can produce neutron energy spectra relevant to fast and fusion reactor environments. Construction of these facilities will take several years of steadfast funding to complete, which poses a formidable schedule challenge for current fast and fusion reactor developers. Irradiation designs which modify the neutron energy spectra delivered to test specimens in thermal spectrum MTRs, an approach referred to as “spectral tailoring”, can be used to approximate several relevant phenomena in the materials needed to enable fast and fusion reactor technologies. This approach is imperfect, but still valuable in the present situation. Here, the two highest flux MTRs operational in the United States, the Advanced Test Reactor (ATR) and High Flux Isotope Reactor (HFIR), have rich histories, ongoing developments, and new potentials for spectral tailoring that will be reviewed and discussed in this paper.

36 MATERIALS SCIENCE↗

NASA NTRS1973

Preliminary neutronic analysis of a cavity test reactor

A reference configuration was calculated for a cavity test reactor to be used for testing the gascore nuclear rocket concept. A thermal flux of 4.1 x 10 to the 14th power neutrons per square centimeter per second in the cavity was provided by a driver fuel loading of 6.4 kg of enriched uranium in MTR fuel elements. The reactor was moderated and cooled by heavy water and reflected with 25.4 cm of beryllium. Power generation of 41.3 MW in the driver fuel is rejected to a heat sink. Design effort was directed toward minimization of driver power while maintaining 2.7 MW in the cavity during a test run. Ancillary data on material reactivity worths, reactivity coefficients, flux spectra, and power distributions are reported.

Whitmarsh, C. L., Jr.↗

DOE OSTI2022

Results of Initial Alloy 617 High Temperature Crack Growth Testing

Crack propagation data can provide valuable insights when performing a safety evaluation for a component. Alloy 617 is qualified in Section III, Division 5 of the American Society of Mechanical Engineers (ASME) Boiler and Pressure Vessel Code (BPVC) for elevated-temperature nuclear service up to 950°C. Little is known, however, about subcritical crack-growth phenomena in Alloy 617. Previous crack-growth studies of Alloy 617 did not investigate temperatures across the range which is currently qualified in Section III, Division 5. High-temperature crack-growth testing in air and in reactor-grade helium can provide data for establishing the crack-growth correlations in support of an ASME BPVC Section XI high-temperature flaw evaluation Code Case. Idaho National Laboratory (INL) has previously performed crack-growth testing, but the equipment requires revitalization. This report provides the status of crack-growth testing in Alloy 617 at INL.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NASA NTRS2007

Application of Simulated Reactivity Feedback in Nonnuclear Testing of a Direct-Drive Gas-Cooled Reactor

Nonnuclear testing can be a valuable tool in the development of an in-space nuclear power or propulsion system. In a nonnuclear test facility, electric heaters are used to simulate heat from nuclear fuel. Standard testing allows one to fully assess thermal, heat transfer, and stress related attributes of a given system but fails to demonstrate the dynamic response that would be present in an integrated, fueled reactor system. The integration of thermal hydraulic hardware tests with simulated neutronic response provides a bridge between electrically heated testing and full nuclear testing. By implementing a neutronic response model to simulate the dynamic response that would be expected in a fueled reactor system, one can better understand system integration issues, characterize integrated system response times and response and response characteristics, and assess potential design improvements with a relatively small fiscal investment. Initial system dynamic response testing was demonstrated on the integrated SAFE 100a heat pipe cooled, electrically heated reactor and heat exchanger hardware. This Technical Memorandum discusses the status of the planned dynamic test methodology for implementation in the direct-drive gas-cooled reactor testing and assesses the additional instrumentation needed to implement high-fidelity dynamic testing.

Bragg-Sitton, S. M.↗

DOE OSTI2022

Assessing the Impact of Effective Thermal Conductivity on Gas-cooled Reactor Transients in RELAP5-3D

In block-type high-temperature gas-cooled reactors (HTGRs), coolant holes in blocks lead to a reduction in heat transfer through conduction. In systems codes like RELAP5-3D, we must account for this degradation by using an effective thermal conductivity (ETC). This presentation discusses a few ETC relationships and demonstrates the impact of ETC for the modular High-Temperature Gas-Cooled Reactor 350 MW -- a computational benchmark for HTGR modeling -- and for the High Temperature Test Facility (HTTF) -- an HTGR thermal hydraulics test facility. We demonstrate that the use of ETC leads to temperatures that are higher than the bulk thermal conductivity of the block material would yield, but these differences have no meaningful impact on the transient performance of the reactors. The ETC also reduces the cooldown rate, leading to more time at elevated temperatures. Overall, while accounting for ETC is important in capturing the physics of the reactor, it is not expected to have a meaningful impact on transient performance.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2022

Conceptual Design of a Pumped Water Capsule for TREAT

This study performed mechanical design, thermal hydraulic, and fuel performance investigations to determine whether an existing large water capsule design could be modified to create forced convection boundary conditions on nuclear fuel specimens in the Transient Reactor Test facility. This concept was found to be viable and offers several advantages compared to a static water environment for a variety of transient power shape categories. The pumped capsule is not foreseen to be superior to a past concept for a larger water loop, but the pumped capsule approach is recommended for further engineering and deployment based on its high cost-to-value ratio primarily as a stop gap capability until a larger water loop can be realized.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2017

Precipitation of Epsilon Particles in Metal Doped Ceria Irradiated with Energetic Ions

Metallic particles precipitated from fission products in oxide fuel matrix (e.g., UO{sub 2}) have a great impact on the thermal and mechanical properties of the fuel. A burn-up of 40 MWd/kg U results in the conversion of 4% of the uranium to approximately 3% fission products and 1% transuranium elements. Epsilon phase is the major metallic phase of the precipitates with a hexagonal-closed packed (HCP) crystal structure. It can exist in a variety of metallic forms in UO{sub 2}, but typically, it consists of five metals: Mo, Pd, Rh, Ru and Tc. Epsilon particles can form over a wide range of stoichiometries in the five metal system. Simulated compositions with Re as a surrogate for Tc have been investigated as a waste form for {sup 99}Tc, an isotope with a long half-life of 2.13 10{sup 5} years and a high solubility under oxidizing conditions in addition to Mo in the corrosion process. There is a pressing need to understand the factors influencing the formation and growth of the metallic phase in fuel. Efforts are currently underway to perform careful neutron irradiation of nuclear fuel under controlled conditions in a test reactor, recover metallic phases that may be present, and characterize the resulting structure and chemistry. Due to the long duration, high cost and radiological concerns associated with neutron irradiation and sample characterizations, ion irradiation studies of a surrogate material with a full control of the processing parameters can emulate different stages of the particle precipitation, which can add a tremendous value to reactor-based studies. This presentation reports our recent ion irradiation results on the metallic particle precipitation under various irradiation and thermal annealing conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NASA NTRS2012

Nuclear Thermal Rocket Element Environmental Simulator (NTREES) Upgrade Activities

To support the on-going nuclear thermal propulsion effort, a state-of-the-art non nuclear experimental test setup has been constructed to evaluate the performance characteristics of candidate fuel element materials and geometries in representative environments. The facility to perform this testing is referred to as the Nuclear Thermal Rocket Element Environment Simulator (NTREES). This device can simulate the environmental conditions (minus the radiation) to which nuclear rocket fuel components will be subjected during reactor operation. Test articles mounted in the simulator are inductively heated in such a manner so as to accurately reproduce the temperatures and heat fluxes which would normally occur as a result of nuclear fission and would be exposed to flowing hydrogen. Initial testing of a somewhat prototypical fuel element has been successfully performed in NTREES and the facility has now been shutdown to allow for an extensive reconfiguration of the facility which will result in a significant upgrade in its capabilities

Emrich, William J. Jr.↗

NASA NTRS2013

Nuclear Thermal Rocket Element Environmental Simulator (NTREES) Phase II Upgrade Activities

Emrich, William J.↗

DOE OSTI2021

Reactor Pressure Vessel Fracture Mechanics Development and Concrete Application Testing for Grizzly

The Grizzly code is being developed to address degradation issues in nuclear reactor structures and components. For light-water reactors, Grizzly currently has capabilities to simulate degradation processes and their effects on structural integrity in two key areas: reactor pressure vessels (RPVs) and reinforced concrete structures. This report documents improvements made to Grizzly’s ability to address both of these structural systems. For RPVs, the reduced-order models (ROMs) used in fracture mechanics calculations have been expanded to allow their application over a broader range of the parameter space than was permitted by the previous models. The ROMs currently used in Grizzly for the evaluation of flaws that are fully embedded within the RPV (as opposed to surface-breaking flaws) are based on a model that is known to be conservative, indicating higher stress intensity factors than would be obtained from direct simulations. A more accurate model that eliminates these excess conservatisms has been recently included in the American Society of Mechanical Engineers Boiler and Pressure Vessel Code but was not applicable for flaws near the RPV surface, which is where the most critical flaws are usually located. That model has recently been extended for increased applicability in this near-surface region. The ROMs for embedded flaws in the Grizzly code have been expanded to include these recent extensions, which permit their use in a much broader set of cases than previously possible. Direct 3D simulations have been used to check these ROMs and have shown good agreement in most cases, although there are still some cases that need further investigation. There are considerable benefits to using these these more accurate and less conservative ROMs for embedded flaws. On a benchmark probabilistic fracture mechanics problem tested here, the conditional probability of fracture initiation computed for a population of flaws in a single plate in an RPV decreased by over a factor of 3. To address aging in reinforced concrete structures, a capability to simulate multiple degradation mechanisms, including alkali-silica reaction and radiation-induced volumetric expansion has been developed in Grizzly over the past several years. This had previously been demonstrated on laboratory-scale specimens but not on full-scale nuclear concrete structures with reinforcement. To demonstrate the applicability of Grizzly to the analysis of large-scale structures of interest, a full 3D model of a representative reinforced concrete structure, including a complex arrangement of reinforcing bars, was developed and demonstrated in Grizzly.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2016

Life Extension of Nuclear Plant Facilities through Monitoring and Detailed Analysis - 16175

The UK has accumulated a substantial legacy of radioactive waste from various civil nuclear and defence programmes. Presently, however most of the UK radioactive waste is generated from nine power stations which generate approximately one sixth of the of the country's electricity. Irradiated fuel is removed from these reactors and safe management of the radioactive solid and liquid effluents is required. The safe management of these effluents is essential. Sellafield, in West Cumbria UK, contains two reprocessing plants, one designed to process nuclear fuel from Magnox reactors (CO{sub 2} cooled with Uranium bar fuel) and the other to process nuclear fuel from Advanced Gas cooled Reactors and Pressurized Water Reactors. The reprocessing stage enables extraction of fissile material for recycling. This leaves a volume of dilute but high-level waste. The high-level radioactive liquid waste is concentrated to reduce its volume and then incorporated into borosilicate glass, using a process called vitrification. The glass is then poured into stainless steel containers and placed in long term storage. This required concentration of HLW liquor is achieved using a suite of aging evaporators. All evaporators are of similar design constructed from corrosion resistant stainless steel having dimensions height ∼11 m, internal diameter 3.05 m and capable of holding 13.7 m{sup 3} of liquor. The basic principle of operation is to heat the dilute liquor under partial vacuum, at constant volume, until the target concentration is achieved. Heating of the liquor is achieved using steam heated coils within the evaporator, and steam in the jacket which surrounds the lower half of the evaporator vessel. The evaporator is then brought to atmospheric pressure and the concentrated liquor is ejected whilst hot. The evaporator is then cooled with water cooled coils and a water filled jacket. New dilute liquor is then added for a new batch. The process is then repeated. As the evaporators reach the end of their original design life accurate prediction of the current condition of nuclear plant facilities is essential to safely justify continued plant operation by ensuring structural integrity. This poses a significant challenge as many aging UK nuclear facilities were not inherently built with inspection in mind. The potential life limiting components of the HA evaporators at Sellafield are the surfaces that contact the product liquor at elevated temperatures i.e. the steam heated surfaces of the coils within the evaporator vessel and the vessel base and wall surrounded by the steam jacket. Each heating component is critical to the operational life of the evaporator - the removal from service of a coil heating component significantly reduces the operational flexibility and remnant life of this plant. Over the last decade a variety of cutting-edge expertise and methodologies have been utilised to accurately measure and then predict the current condition of the plant and also to predict its remnant life. This paper provides an overview of the development of several techniques deployed, namely non-destructive testing/inspection, in-house software development and finite element modelling. These methods have been validated by lab-scale or full-scale experiments along with historical plant data. These techniques have been evolved and refined for over a decade, providing vital insights into the physical behaviour of this complex reprocessing system. This enables not only accurate assessment of the current condition of the plant equipment but also allows scientifically underpinned predictions to be made of how it will behave into the future. This is critical for Sellafield as this knowledge feeds into their safety case to the Office of Nuclear Regulation to justify continued operation. It is concluded that this integrated approach provides a robust analysis tool which has driven change and optimisation of plant procedures ensuring continued safe operation whilst extending the life of the facility. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2023

Post-irradiation examination of the Sirius-1 nuclear thermal propulsion fuel test

Nuclear Thermal Propulsion (NTP) systems hold promise in reducing transit times for exploration of the solar system by both crewed and uncrewed missions. NTP systems currently under investigation include a once-through high-temperature gas-cooled fission reactor to provide thermal energy to heat the coolant, which also serves as the propellant. The fuel system consists of angular UN fuel particles dispersed in a matrix of W/Re, creating a ceramic and metallic composite or cermet, which has been irradiated in Idaho National Laboratory's (INL) Transient Reactor Test Facility (TREAT). This enabled evaluation of these materials under representative nuclear heating rates (~95 K/s) and peak surface temperatures (~2527 K). Further, these surface conditions were indicative of achievement of the target peak internal temperature of approximately 2850 K. These tests named Sirius-1 (UN–W/Re), have been irradiated and this paper will present post-irradiation examination results. The Sirius-1 test produced minor, stable cracks in the fuel specimen and spalling of surface material. Volatilized uranium ‘soot’ was found deposited on the inner wall of the irradiation capsule indicating loss of some fissile material from the fuel specimen. Spalling from the surfaces was also noted upon visual inspection. Uranium diffusion from the fuel particles resulted in the formation of U/Re phases and the production of a laminar microstructure on the edge of the fuel system. Overall, the specimen was stable and remained within a coolable geometry upon conclusion of multiple thermal cycles to prototypical operating temperatures.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2024

Upsampling Monte Carlo Reactor Simulation Tallies in Depleted Sodium-Cooled Fast Reactor Assemblies Using a Convolutional Neural Network

The computational demand of neutron Monte Carlo transport simulations can increase rapidly with the spatial and energy resolution of tallied physical quantities. Convolutional neural networks have been used to increase the resolution of Monte Carlo simulations of light water reactor assemblies while preserving accuracy with negligible additional computational cost. Here, we show that a convolutional neural network can also be used to upsample tally results from Monte Carlo simulations of sodium-cooled fast reactor assemblies, thereby extending the applicability beyond thermal systems. The convolutional neural network model is trained using neutron flux tallies from 300 procedurally generated nuclear reactor assemblies simulated using OpenMC. Validation and test datasets included 16 simulations of procedurally generated assemblies, and a realistic simulation of a European sodium-cooled fast reactor assembly was included in the test dataset. We show the residuals between the high-resolution flux tallies predicted by the neural network and high-resolution Monte Carlo tallies on relative and absolute bases. The network can upsample tallies from simulations of fast reactor assemblies with diverse and heterogeneous materials and geometries by a factor of two in each spatial and energy dimension. The network’s predictions are within the statistical uncertainty of the Monte Carlo tallies in almost all cases. This includes test assemblies for which burnup values and geometric parameters were well outside the ranges of those in assemblies used to train the network.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2024

MARVEL Utilization Plan

This report provides a high-level overview of the utilization plan for the MARVEL microreactor. The main focus is on discussing testing and application-demonstration opportunities that leverage the reactor. With the reactor rapidly progressing towards demonstration, along with the short (2- year) operational window, it was deemed critical to establish a basis for how stakeholders can engage with the program and leverage the reactor as a testbed. This report discusses potential opportunities to use MARVEL, leveraging from data and design access to testing novel controls, and novel nuclear-electric and nuclear-heat applications. It provides guidance for interested stakeholders on potential funding opportunities that can be pursued to support tests during the operational lifetime of the reactor. The report discusses the recommended strategy for outreach and the organizational structure to review and select projects for participation. Interested stakeholders are encouraged to fill out a questionnaire on how they could leverage MAVEL at this link: https://qfreeaccountssjc1.az1.qualtrics.com/jfe/form/SV_72InKjSEz54Q2j4 It is important to emphasize that this is intended to be a living document (updated annually or as needed) with revisions issued as the MARVEL demonstration timeline evolves. Similarly, the framework for engagement is subject to change as the project progresses.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2019

Development of Waste Disposal Strategy for RH LLW Stored in the ATR Canal - 19453

The Advanced Test Reactor (ATR), located at Idaho National Laboratory (INL), is 250 megawatt research reactor designed and operated for the United States Department of Energy for irradiation testing of advanced nuclear fuels and material samples. The pressurized light-water moderated and cooled reactor achieved criticality in 1967. It is designed to allow high neutron flux irradiation of structural materials and nuclear fuels to replicate long-term exposure of materials in traditional lower-flux reactor cores. The ATR also produces rare isotopes for the use in the medical and other industries. The ATR is one of only four reactors in the world with this high-flux irradiation capability. Adjacent to the ATR is a water-filled canal which is used to handle casks, prepare experiments, perform irradiation experiments, and store irradiated components generated from reactor operations. The canal is used to store irradiated (activated) metals that are subsequently determined to be waste. In many instances, these items are too radioactive to remove from the canal and remain in temporary storage until a sufficient decay period has elapsed to where they can be safely removed. The more highly-radioactive remote-handled (RH) waste items requiring hundreds of years to decay have been in storage in the canal since the first ATR core internal changeout (CIC) which was conducted in the 1970's. The INL has recently completed construction and startup of a new Remote-Handled Low-Level Waste (RH LLW) Disposal Facility, which will serve as the final disposal capability for legacy RH (greater than 200 mR/hr on contact) metal waste currently stored in the canal. The ATR will need to develop a method for packaging, characterizing, removing, and shipping this material to the new disposal facility. Based on the configuration of the new disposal cells at the RH LLW Disposal Facility, the ATR must produce an entire new process for handing and packaging the legacy RH waste and preparing it for transport and final disposal. The ATR Canal RH LLW Cleanup Project scope is to develop the processes, tools, and equipment for safely sizing, packaging, and removing RH LLW from the canal. This paper presents highlights and challenges the project faces to develop and implement this capability: - Designing new tools, fabricating new equipment, and implementing new processes at an active Hazard Category-I nuclear facility. - Ensuring new equipment and tools are compatible with the existing equipment and processes at both the generator and the disposal facilities. - Sizing legacy waste under water using remote tools and equipment to minimize void space in waste disposal canisters while ensuring as low as reasonably achievable (ALARA) goals are met. - Loading waste containers underwater and preparing them to meet the liquid-free criteria of the disposal facility waste acceptance criteria (WAC). - Providing a new shielded transport container to transfer waste from ATR to the new on-site RH LLW Disposal Facility. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2022

Advanced Test Reactor Overview

Power Point presentation regarding ATR, intended to be presented to university students and/or new INL employees.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2016

Uncertainty Analysis in Critical Experiments of SORA Mockup

A series of static critical experiments were completed from September 1965 to August 1966 at the Oak Ridge National Laboratory Critical Experiments Facility (ORCEF) in support of the design of the Sorgente Rapida Reactor (SORA) under a cooperative agreement between EURATOM and the U.S. Atomic Energy Commission. The SORA which had been proposed by EURATOM and was described by Raievski and Larrimore was designed to be composed of rods of highly enriched uranium alloy latticed, as a fast, reflected, repetitively pulsed reactor to serve as a high-intensity source of neutrons for time-of-flight measurements. More information about the SORA design can be obtained in some references. The critical experiments, not including pulse testing, were performed with a mockup of the SORA reactor differing from the reactor principally in the use of iron in place of the coolant, of iron as reflector, and of uranium metal fuel in place of the alloy. A summary of the experiments for the mockup was compiled in report ORNL- 4263, in June, 1968, then published as a paper in 1969. Based on the available data from papers, reports mentioned above and the logbook, the typical 15 critical experiments were evaluated for experimental uncertainties for further benchmark analysis and inclusion in the ICSBEP Handbook. Through a series of rigorous procedures in analysis of the original experimental measurement data, the dimensions and displacement of individual components, and the isotopic contents, mass, and impurities of the individual components, the experimental uncertainties for the 15 configurations have been evaluated to be 0.00219 ∼0.00229 Δk{sub eff} for 11 configurations in type of the Reference Assembly, 0.00179 ∼0.00189 Δk{sub eff} for 4 configurations in type of the All-Iron Assembly. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗