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At least 379 records · Page 21

Conjugate Observations of Optical Aurora with POLAR Satellite and Ground Based Imagers in Antarctica

Operation of the ultraviolet imager on the POLAR satellite permits the observation of Aurora Borealis in daylight during northern summer. With optical imagers in the Automatic Geophysical Observatories (AGO-s) large regions of the oval of Aurora Australis can be observed simultaneously during the southern winter polar night. This opportunity permits conducting a systematic study of the properties of auroras on opposite ends of the same field line. It is expected that simultaneously observed conjugate auroras occurring on closed field lines should be similar to each other in appearance because of the close connection between the two hemispheres through particle scattering and mirroring processes. On open or greatly distorted field lines there is no a priori expectation of similarity between conjugate auroras. To investigate the influence of different IMF conditions on auroral behavior we have examined conjugate data for periods of southward IMF. Sudden brightening and subsequent poleward expansions are observed to occur simultaneously in both hemispheres. The POLAR data show that sudden brightening are initiated at various local time regions. When the local time of this region is in the field of view of the AGO station network then corresponding brightening is also found to occur in the southern hemisphere. Large features such as substorm induced westward propagation and resulting auroral brightening seem to occur simultaneously on conjugate hemispheres. The widely different view scales make it difficult to make unique identification of individual auroral forms in the POLAR and in the ground based data but in a general sense the data is consistent with conjugate behavior.

Mende, S. H.↗

Radio properties of the highly polarized, quiescent quasar OI 287

The highly polarized, quiescent quasar OI 287 has been observed with high resolution at 2 cm and 6 cm in an effort to determine the origin of some of the object's peculiar properties. The results seem to rule out the classification of OI 287 as a blazar. Extrapolation of the radio core spectrum to midinfrared wavelengths fails to predict the infrared flux by at least an order of magnitude. This supports the conclusion that the infrared emission and the radio emission do not originate in the same synchrotron-emitting component. The high optical polarization could be related to possible broad absorption lines in the unobserved UV regime, or it could be caused by reflection into the line of sight by scattering agents distributed in a thin disk.

Ulvestad, James S.↗

Variations of light emission and carrier dynamics around V-defects in InGaN quantum wells

Time- and spectrally-resolved scanning near-field optical microscopy was applied to study spatial variations of photoluminescence (PL) spectra and carrier dynamics in polar InGaN/GaN single quantum wells (QWs) emitting from 410 nm to 570 nm. The main attention was devoted to variations of PL properties and carrier dynamics around V-defects. The PL intensity, peak wavelength, and linewidth, as well as the radiative and nonradiative recombination times, were found to be different in V-defect-rich and defect-free regions. The radiative lifetime close to the defects was longer up to several times, which is attributed to an increased electron and hole wave function separation in the QW plane. PL decay times, measured using excitation and collection through the near-field probe, were one to two orders of magnitude shorter than PL decay times measured in the far field. This shows that the near-field PL decay and the integrated PL intensity are primarily determined by the carrier out-diffusion from under the probe. Only in the immediate vicinity of the V-defects, the near-field PL decays due to the nonradiative recombination at dislocations. The area of such enhanced nonradiative recombination is limited to just a few percent of the total QW area. This shows that recombination via dislocations and V-defects does not play a decisive role in the overall nonradiative recombination and internal quantum efficiency of polar InGaN/GaN QWs.

36 MATERIALS SCIENCE↗

Continuum emission in active galactic nuclei; Proceedings of the Workshop, Tucson, AZ, January 11-14, 1986

Papers are presented on IRAS observations of active galactic nuclei, 0.3-100 micron continua of Seyfert 1 galaxies, the diverse soft X-ray slopes of QSOs, and the continuum variability of the optically-active radio-quiet quasar GQ Comae. Also considered are the polarization signatures of accretion disks in active galactic nuclei, X-ray spectra of BL Lacertae objects, diffusive shock acceleration and quasar variability, and radio-optical broadband spectra and variability of quasars. Other topics include the radio properties of optically selected Seyfert galaxies, and the structure of the emission region in blazars.

Sitko, Michael L.↗

Scattering and Absorption by Nonspherical Particles in Planetary Atmospheres

The atmospheres of Mars, the giant planets, and Titan all support populations of nonspherical particles. Analyses of observations of these atmospheres therefore rely on an understanding of the optical properties of nonspherical particles. We can glean information on particle size and composition from the wavelength dependence of the optical depth and from the shape of the forward peak of the scattering phase function. Additional information comes from polarization measurements which have been especially fruitful for Titan's haze. The Mars atmosphere contains mineral dust particles with effective radii near 1.6 micro meters, and water ice particles with radii between about 1 and 4 micro meters. The uppermost tropospheric hazes in Jupiter and Saturn are composed of ice crystals of ammonia, water and possibly traces of ammonium hydrosulfide, Methane ice and hydrogen sulfide ice are present in the atmospheres of Uranus and Neptune. Size estimation for these hazes in the giant planets is difficult, and even the expected spectral signatures are elusive, Titan's haze is both forward scattering and strongly polarized - a combination which points toward a fractal aggregate struc1.ure of 10 - 100 or more organic monomers whose radius is about 0.06 micro meters. Polar stratospheric hazes on Jupiter and Saturn also display this characteristic.

nonsperical particles↗

Optical Thin Film Modeling: Using FTG's FilmStar Software

Every material has basic optical properties that define its interaction with light: The index of refraction (n) and extinction coefficient (k) vary for the material as a function of the wavelength of the incident light. Also significant are the phase velocity and polarization of the incident light These inherent properties allow for the accurate modeling of light s behavior upon contact with a surface: Reflectance, Transmittance, Absorptance.

Freese, Scott↗

Nearly a Decade of CALIPSO Observations of Asian and Saharan Dust Properties Near Source and Transport Regions

The lidar on the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission, makes robust measurements of dust and has generated a length of record that is significant both seasonally and inter-annually. We exploit this record to determine a multi-year climatology of the properties of Asian and Saharan dust, in particular seasonal optical depths, layer frequencies, and layer heights of dust gridded in accordance with the Level 3 data products protocol, between 2006-2015. The data are screened using standard CALIPSO quality assurance flags, cloud aerosol discrimination (CAD) scores, overlying features and layer properties. To evaluate the effects of transport on the morphology, vertical extent and size of the dust layers, we compare probability distribution functions of the layer integrated volume depolarization ratios, geometric depths and integrated attenuated color ratios near the source to the same distributions in the far field or transport region. CALIPSO is collaboration between NASA and Centre National D'études Spatiales (CNES), was launched in April 2006 to provide vertically resolved measurements of cloud and aerosol distributions. The primary instrument on the CALIPSO satellite is the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), a near-nadir viewing two-wavelength polarization-sensitive instrument. The unique nature of CALIOP measurements make it quite challenging to validate backscatter profiles, aerosol type, and cloud phase, all of which are used to retrieve extinction and optical depth. To evaluate the uncertainty in the lidar ratios, we compare the values computed from dust layers overlying opaque water clouds, considered nominal, with the constant lidar ratio value used in the CALIOP algorithms for dust. We also explore the effects of noise on the CALIOP retrievals at daytime by comparing the distributions of the properties at daytime to the nighttime distributions.

Omar, Ali H.↗

Large Enhancements in Optical and Piezoelectric Properties in Ferroelectric Zn 1- x Mg x O Thin Films through Engineering Electronic and Ionic Anharmonicities

Multifunctionality as a paradigm requires materials exhibiting multiple superior properties. Integrating second-order optical nonlinearity and large bandgap with piezoelectricity can, for example, enable broadband, strain-tunable photonics. Though very different phenomena at distinct frequencies, both second-order optical nonlinearity and piezoelectricity are third-rank polar tensors present only in acentric crystal structures. However, simultaneously enhancing both phenomena is highly challenging since it involves competing effects with tradeoffs. Recently, a large switchable ferroelectric polarization of ≈80 μC cm –2 was reported in Zn 1-x Mg x O films. Here, ferroelectric Zn 1-x Mg x O is demonstrated to be a platform that hosts simultaneously a 30% increase in the electronic bandgap, a 50% enhancement in the second harmonic generation (SHG) coefficients, and a near 200% improvement in the piezoelectric coefficients over pure ZnO. These enhancements are shown to be due to a 400% increase in the electronic anharmonicity and a ≈200% decrease in the ionic anharmonicity with Mg substitution. Precisely controllable periodic ferroelectric domain gratings are demonstrated down to 800 nm domain width, enabling ultraviolet quasi-phase-matched optical harmonic generation as well as domain-engineered piezoelectric devices.

36 MATERIALS SCIENCE↗

Exciton–Polaritons in CsPbBr 3 Crystals Revealed by Optical Reflectivity in High Magnetic Fields and Two-Photon Spectroscopy

Cesium lead bromide (CsPbBr3) is a representative material of the emerging class of lead halide perovskite semiconductors that possess remarkable optoelectronic properties. Its optical properties in the vicinity of the bandgap energy are greatly contributed by excitons, which form exciton polaritons due to strong light–matter interactions. Exciton–polaritons in solution-grown CsPbBr 3 crystals are examined by means of circularly polarized reflection spectroscopy measured in high magnetic fields up to 60 T. The excited 2P exciton state is measured by two-photon absorption. Comprehensive modeling and analysis provides detailed quantitative information about the exciton–polariton parameters: exciton binding energy of 32.5 meV, oscillator strength characterized by longitudinal–transverse splitting of 5.3 meV, damping of 6.7 meV, reduced exciton mass of 0.18$m$ 0 , exciton diamagnetic shift of 1.6 μeV T -2 , and exciton Landé factor $g$ x = + 2.35. It is shown that the exciton states can be described within a hydrogen-like model with an effective dielectric constant of 8.7. From the measured exciton longitudinal–transverse splitting, Kane energy of E p = 15 eV is evaluated, which is in reasonable agreement with values of 11.8–12.5 eV derived from the carrier effective masses.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Generation of entangled-photons by a quantum dot cascade source in polarized cavities: Using cavity resonances to boost signals and preserve the entanglements

Motivated by recent advances in the development of single photon emitters for quantum information sciences, here we design and formulate a quantum cascade model that describes cascade emission by a quantum dot (QD) in a cavity structure while preserving entanglement that stores information needed for single photon emission. The theoretical approach is based on a photonic structure that consists of two orthogonal cavities in which resonance with either the first or second of the two emitted photons is possible, leading to amplification and rerouting of the entangled light. The cavity–QD scheme uses a four-level cascade emitter that involves three levels for each polarization, leading to two spatially entangled photons for each polarization. By solving the Schrodinger equation, we identify the characteristic properties of the system, which can be used in conjunction with optimization techniques to achieve the “best” design relative to a set of prioritized criteria or constraints in our optical system. The theoretical investigations include an analysis of emission spectra in addition to the joint spectral density profile, and the results demonstrate the ability of the cavities to act as frequency filters for the photons that make up the entanglements and to modify entanglement properties. The results provide new opportunities for the experimental design and engineering of on-demand single photon sources.

Chemistry↗

Quantum confining excitons with an electrostatic moiré superlattice

Quantum confining excitons has been a persistent challenge in the pursuit of strong exciton interactions and quantum light generation. Unlike electrons, which can be readily controlled via electric fields, imposing strong nanoscale potentials on excitons to enable quantum confinement has proven challenging. In this study, we utilize piezoelectric force microscopy to image the domain structures of twisted hexagonal boron nitride (h – BN), revealing evidence of strong in-plane electric fields at the domain boundaries. By placing a monolayer MoSe 2 only one to two nanometers away from the twisted h – BN interface, we observe energy splitting of neutral excitons and Fermi polarons by several millielectronvolts at the moiré domain boundaries. By directly correlating local structural and optical properties, we attribute such observations to excitons confined in a nanoscale one-dimensional electrostatic potential created by the strong in-plane electric fields at the moiré domain boundaries. Intriguingly, this 1D quantum confinement results in pronounced polarization anisotropy in the excitons’ reflection and emission, persistent to temperatures as high as ~80 Kelvins. Furthermore, these findings open new avenues for exploring and controlling strongly interacting excitons for classical and quantum optoelectronics.

2-dimensional systems↗

Ultraviolet observations of interstellar molecules and grains from Spacelab

The paper presents observational results obtained on interstellar grains and molecules and suggests promising areas for Spacelab research. Regarding grains, useful data can be expected on the shape of the ultraviolet extinction curve for new interstellar regions, on the nature of UV extinction at short wavelengths, the presence of structure in the UV extinction curve comparable to the visible-wavelength diffuse bands, and the polarization properties of grains in UV wavelengths. The advances in observations of molecules will include the ability to prove more heavily-obscured regions, coverage of wavelength regions inadequately studied with previous instruments, and the capability of observing in optical absorption species detected in the same line of sight in radio emission.

Snow, T. P., Jr.↗

Retrieval of cloud cover parameters from multispectral satellite images

A technique is described for extracting cloud cover parameters from multispectral satellite radiometric measurements. Utilizing three channels from the AVHRR (Advanced Very High Resolution Radiometer) on NOAA polar orbiting satellites, it is shown that one can retrieve four parameters for each pixel: cloud fraction within the FOV, optical thickness, cloud-top temperature and a microphysical model parameter. The last parameter is an index representing the properties of the cloud particle and is determined primarily by the radiance at 3.7 microns. The other three parameters are extracted from the visible and 11 micron infrared radiances, utilizing the information contained in the two-dimensional scatter plot of the measured radiances. The solution is essentially one in which the distributions of optical thickness and cloud-top temperature are maximally clustered for each region, with cloud fraction for each pixel adjusted to achieve maximal clustering.

Arking, A.↗

Poincaré beams from a free electron laser

Poincaré beams are light beams that have spatially inhomogeneous polarization structure that spans a finite portion of the Poincaré sphere. This feature bestows the beams with intriguing topological properties and has led to a surge in research on their fundamental characteristics, their controlled generation and on emerging applications. Here we present an experimental demonstration of a Poincaré beam generated in the extreme ultraviolet (16.7 nm) at the FERMI free electron laser (FEL). The ‘star’ type Poincaré beam is generated by exploiting the phase and intensity structure intrinsic to FEL radiation without relying on optical elements. Here, we controlled the spatial polarization distribution through a precise overlap and power balance between two FEL pulses, each with different transverse phase distributions and orthogonal circular polarizations. The spatial polarization structure was mapped in detail and shows extensive coverage of the Poincaré sphere, in agreement with analytic predictions. This method of in situ Poincaré beam production in FELs enables straightforward flexibility in the orientation and balance of polarization states, and can readily be extended to other vector beams and to shorter wavelengths enabling novel science applications in modern light sources.

Morgan, Jenny [SLAC National Accelerator Laborator↗

SPEX Airborne Spectropolarimeter Calibration and Performance

To improve our understanding of the complex role of aerosols in the climate system and on air quality, measurements are needed of optical and microphysical aerosol. From many studies, it has become evident that a satellite-based multiangle, multiwavelength polarimeter will be essential to provide such measurements. Here, high accuracy (∼0.003) on the degree of linear polarization (DoLP) measurements is important to retrieve aerosol properties with an accuracy needed to advance our understanding of the aerosol effect on climate. SPEX airborne, a multiangle hyperspectral polarimeter, has been developed for observing and characterizing aerosols from NASA’s high-altitude research aircraft ER-2. It delivers measurements of radiance and DoLP at visual wavelengths with a spectral resolution of 3 and 7–30 nm, respectively, for radiance and polarization, at nine fixed equidistant viewing angles from −56° to +56° oriented along the ground track, and a swath of 7° oriented across-track. SPEX airborne uses spectral polarization modulation to determine the state of linear polarization of scattered sunlight. This technique has been developed in the Netherlands and has been demonstrated with ground-based instruments. SPEX airborne serves as a demonstrator for a family of space-based SPEX instruments that have the ability to measure and characterize atmospheric aerosol by multiangle hyperspectral polarimetric imaging remotely from a satellite platform. SPEX airborne was calibrated radiometrically and polarimetrically using Jet Propulsion Laboratory (JPL) facilities including the Polarization Stage Generator-2 (PSG-2), which is designed for polarimetric calibration and validation of the Airborne Multiangle SpectroPolarimetric Imager (AirMSPI). Using the PSG-2, the accuracy of the SPEX airborne DoLP measurements in the laboratory setup is found to be 0.002–0.004. Radiometric calibration is realized with an estimated accuracy of 4%. In 2017, SPEX airborne took part in the “Aerosol Characterization from Polarimeters and Lidar” campaign on the ER-2 that included four polarimeters and two lidars. Polarization measurements of SPEX airborne and the coflying Research Scanning Polarimeter (RSP), recorded during the campaign, were compared and display root-mean-square (RMS) differences ranging from 0.004 (at 555 nm) up to 0.02 (at 410 nm). For radiance measurements, excellent agreement between SPEX airborne and RSP is obtained with an RMS difference of ∼4%. The lab- and flight-performance values for polarization are similar to those recently published for AirMSPI, where also an intercomparison with RSP was made using data from field campaigns in 2013. The intercomparison of radiometric and polarimetric data both display negligible bias. The in-flight comparison results provide verification of SPEX airborne’s capability to deliver high-quality data.

Aerosols↗

Cs X Si 15 P 21 ( X = Sn or Pb): Polar Noncentrosymmetric Si–P Frameworks Stabilized by Covalent X –P Bonding

Metal silicon phosphides composed of earth-abundant Si and P tend to exhibit semiconducting properties and adopt diverse crystal structures with relatively small additions of structure-directing elements. The potential of silicon phosphide materials in nonlinear optical applications has been hindered by the inability to systematically produce noncentrosymmetric structures with such a flexible framework. Here, in this work, two isostructural compounds with a novel noncentrosymmetric structure were made possible by the inclusion of elements with stereochemically active lone pairs (Sn 2+ and Pb 2+ ). The structures were determined through single-crystal and synchrotron powder X-ray diffraction. Analysis of chemical bonding in real space through the electron localization function revealed stereochemically active Pb 2+ and Sn 2+ species in a trigonal pyramidal coordination with {Pb/Sn}–P bonds. Such covalent bonding between Pb and P is quite uncommon in extended solids and has been reported in a few rare instances. Band structure calculations and linear optical measurements confirm the semiconducting nature of Cs X Si 15 P 21 ( X = Sn or Pb). The synthesis was optimized to yield high-purity polycrystalline samples. The nonlinear optical properties show promising second-harmonic generation (SHG) coefficients from the Kurtz–Perry method. First-principles calculations of the nonlinear optical properties support the experimentally determined SHG values and provide moderate values of birefringence, suggesting Cs X Si 15 P 21 could be phase-matchable and practical nonlinear optical materials in the mid-IR region.

crystal structure↗

The optical polarization of Scorpius X-1.

The X-ray source Sco X-1 is known to have a slight linear polarization in visible light. An investigation was conducted to determine whether the origin of the polarization is intrinsic to the source or interstellar. No evidence could be found for unusual polarization properties in Sco X-1 that would point to an intrinsically polarized source, although this cannot be excluded. It is pointed out that the case for interstellar polarization would become very strong if stars in the immediate vicinity are found to be polarized with the same position angle.

Landstreet, J. D.↗

High-fidelity imaging of a band insulator in a three-dimensional optical lattice clock

Here, we report on the observation of a high-density, band insulating state in a three-dimensional optical lattice clock. Filled with a nuclear-spin-polarized degenerate Fermi gas of 87 Sr, the three-dimensional (3D) lattice has one atom per site in the ground motional state, thus guarding against frequency shifts due to contact interactions. At this high density where the average distance between atoms is comparable to the probe wavelength, conventional imaging techniques at saturation intensity suffer from large systematic errors. To spatially probe frequency shifts in the clock and measure thermodynamic properties of this system, accurate imaging techniques at high optical depths are required. Using a combination of highly saturated fluorescence and absorption imaging, we confirm the density distribution in our 3D optical lattice in agreement with a single spin band insulating state. Combining our clock platform with this high filling fraction opens the door to studying new classes of long-lived, many-body states arising from dipolar interactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗