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At least 379 records · Page 21

CeNTREX: a new search for time-reversal symmetry violation in the 205 Tl nucleus

The Cold molecule Nuclear Time-Reversal EXperiment (CeNTREX) is a new effort aiming for a significant increase in sensitivity over the best present upper bounds on the strength of hadronic time reversal (T) violating fundamental interactions. The experimental signature will be shifts in nuclear magnetic resonance frequencies of 205 Tl in electrically-polarized thallium fluoride (TlF) molecules. Here we describe the motivation for studying these T-violating interactions and for using TlF to do so. To achieve higher sensitivity than earlier searches for T-violation in TlF, CeNTREX uses a cryogenic molecular beam source, optical state preparation and detection, and modern methods of coherent quantum state manipulation. Details of the measurement scheme and the current state of the apparatus are presented, with quantitative measurements of the TlF beam. Lastly, the estimated sensitivity and methods to control systematic errors are discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

The invisible black widow PSR J1720−0534: implications for the electron density towards the North Polar Spur

Radio emission from pulsars can be used to map out their distances through dispersion measure (DM), which quantifies the amount of radio pulse dispersion. However, this method relies on accurately modelling the free electron density in the line of sight. Here, we present a detailed study of the multiwavelength emission from PSR J1720−0534, a black widow compact binary millisecond pulsar discovered in 2021, which the latest electron density model of the Galaxy places at only 191 pc. We obtained and analysed deep multiwavelength observations in the γ-ray ( Fermi -Large Area Telescope, 2008–2022), optical (Las Cumbres Observatory, 2.7 h), near-infrared (Nordic Optical Telescope, 3.5 h), and X-ray ( Swift -X-Ray Telescope, 10 ks) bands. We found no significant detection of γ-ray, optical, near-infrared, or X-ray counterparts around the radio-timing position of PSR J1720−0534, which we thus nickname ‘the invisible black widow’. Employing the most constraining near-infrared limit ( J > 23.4 mag), we established a lower limit on the source distance, d > 1.1 kpc, assuming conservative properties for the black widow companion star. This distance lower limit differs drastically (by a factor of more than 5) from the Yao et al. DM distance estimate. We attribute this difference to the inclusion in the Yao et al. model of a large and dense component towards the North Polar Spur. Considering our results and recent parallax distances to other pulsars in this direction, we argue that such a local and large component in the electron density model of the Galaxy is unnecessary.

79 ASTRONOMY AND ASTROPHYSICS↗

A VLBA-uGMRT search for candidate binary black holes: study of six X-shaped radio galaxies with double-peaked emission lines

ABSTRACT Identifying methods to discover dual active galactic nucleus (AGN) has proven to be challenging. Several indirect tracers have been explored in the literature, including X/S-shaped radio morphologies and double-peaked (DP) emission lines in the optical spectra. However, the detection rates of confirmed dual AGN candidates from the individual methods remain extremely small. We search for binary black holes (BBH) in a sample of six sources that exhibit both X-shaped radio morphology and DP emission lines using the Very Long Baseline Array (VLBA). Three out of the six sources show dual VLBA compact components, making them strong candidates for BBH sources. In addition, we present deep uGMRT images revealing the exquisite details of the X-shaped wings in three sources. We present a detailed precession modeling analysis of these sources. The black hole separations estimated from the simplistic geodetic precession model are incompatible with those estimated from emission line offsets and the VLBA separations. However, precession induced by a non-coplanar secondary black hole is a feasible mechanism for explaining the observed X-shaped radio morphologies and the black hole separations estimated from other methods. The black hole separations estimated from the double-peaked emission lines agree well with the VLBA compact component separations. Future multifrequency VLBA observations will be critical in ruling out or confirming the BBH scenario in the three galaxies with dual component detections.

Sebastian, Biny (ORCID:0000000184286525)↗

Superradiance and Subradiance due to Quantum Interference of Entangled Free Electrons

When multiple quantum emitters radiate, their emission rate may be enhanced or suppressed due to collective interference in a process known as super- or subradiance. Such processes are well known to occur also in light emission from free electrons, known as coherent cathodoluminescence. Unlike atomic systems, free electrons have an unbounded energy spectrum, and, thus, all their emission mechanisms rely on electron recoil, in addition to the classical properties of the dielectric medium. To date, all experimental and theoretical studies of super- and subradiance from free electrons assumed only classical correlations between particles. However, dependence on quantum correlations, such as entanglement between free electrons, has not been studied. Recent advances in coherent shaping of free-electron wave functions motivate the investigation of such quantum regimes of super- and subradiance. In this Letter, we show how a pair of coincident path-entangled electrons can demonstrate either super- or subradiant light emission, depending on the two-particle wave function. By choosing different free-electron Bell states, the spectrum and emission pattern of the light can be reshaped, in a manner that cannot be accounted for by a classical mixed state. We show these results for light emission in any optical medium and discuss their generalization to many-body quantum states. Furthermore, our findings suggest that light emission can be sensitive to the explicit quantum state of the emitting matter wave and possibly serve as a nondestructive measurement scheme for measuring the quantum state of many-body systems.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Adapt: A Weather Radar Data Analysis and Nowcasting Platform for Informed Adaptive Scanning

SF-26-021 Adapt is a data processing platform for real-time data analysis, short term prediction of targets convective cells and tracking for archived data. It provides tools for downloading, processing, segmenting, projecting, analyzing, and visualizing storm cell data from weather radar. The pipeline includes cell detection, motion estimation using optical flow, cell property extraction, and persistence to NetCDF and SQLite/Parquet for guiding adaptive scanning.

Raut, Bhupendra Ashokrao [Argonne National Laborat↗

Significantly enhanced near-field coupling via tip engineering

The ability to significantly enhance near-field coupling between light and matter at the nanoscale is crucial for advancing the fields of nanophotonics and nanopolariotonics. However, conventional probes face challenges in achieving optimal light–matter interaction. In this study, we propose a novel, to the best of our knowledge, simulation-based strategy that leverages tip engineering to dramatically amplify the scattering field through tailored double-layer geometries. By employing a core-shell structure with a thin shell layer optimized for specific dielectric permittivity and effective polarizability, we demonstrate a near-field enhancement of up to 10 times compared to conventional probes. Our findings highlight exciting new possibilities for optimizing near-field interactions through probe designs with customized resonances, paving the way for substantially improved nano-optical sensing, imaging, and detection.

Shiravi, H.↗

Nephelometer Instrument Handbook

The Integrating Nephelometer (Figure 1) is an instrument that measures aerosol light scattering. It measures aerosol optical scattering properties by detecting (with a wide angular integration – from 7 to 170°) the light scattered by the aerosol and subtracting the light scattered by the carrier gas, the instrument walls and the background noise in the detector (zeroing). Zeroing is typically performed for 5 minutes every day at midnight UTC. The scattered light is split into red (700 nm), green (550 nm), and blue (450 nm) wavelengths and captured by three photomultiplier tubes. The instrument can measure total scatter as well as backscatter only (from 90 to 170°) (Heintzenberg and Charlson 1996; Anderson et al. 1996; Anderson and Ogren 1998; TSI 3563 2015) At ARM (Atmospheric Radiation Measurement), two identical Nephelometers are usually run in series with a sample relative humidity (RH) conditioner between them. This is possible because Nephelometer sampling is non-destructive and the sample can be passed on to another instrument. The sample RH conditioner scans through multiple RH values in cycles, treating the sample. This kind of setup allows to study how aerosol particles’ light scattering properties are affected by humidification (Anderson et al. 1996). For historical reasons, the two Nephelometers in this setup are labeled “wet” and “dry”, with the “dry” Nephelometer usually being the one before the conditioner and sampling ambient air (the names are switched for the MAOS measurement site due to the high RH of the ambient air).

47 OTHER INSTRUMENTATION↗

FORESTR: Finding, Organizing, Representing, Explaining, Summarizing, and Thinning Random forests

Random forests have become popular models used for data driven predictions. As a result, random forests are currently used or being considered for high-consequence mission applications in national security, such as the prediction of yield from optical signals and malware detection. While random forests may provide accurate predictions, the complexity of the algorithm causes a lack of interpretability. Random forests are an ensemble of regression or decision trees. Individual regression and decision trees are interpretable, but ensembles are inherently difficult to interpret due to the compilation of many models. We aim to increase the interpretability of random forests by finding patterns in the ensemble of trees that can be used to “thin” (or remove) trees. As a starting point, in this report, we develop a new distance metric for quantifying the similarity between trees based on their topologies (i.e., shapes). We base the metric on a novel distance metric for graphs that is a proper mathematical distance, is invariant to transformations, has registration between graphs, and computes topological evolutions between graphs. We use the tree distance metric to compute tree statistics such as a “mean tree” and to identify clusters of trees. We apply the developed methodology to a toy dataset and a mission relevant product inspection dataset to demonstrate how the metric can provide insight into random forests. Furthermore, we discuss the limitations of the approach and ideas for future research into how the metric could be used as a thinning tool to develop less complex models.

97 MATHEMATICS AND COMPUTING↗

Resolving femtosecond photoinduced energy flow: capture of nonadiabatic reaction pathway topography and wavepacket dynamics from photoexcitation through the conical intersection seam (Final Technical Report)

The dynamics that take place within just tens to hundreds of femtoseconds following the absorption of light by a molecule can play a critical role in how the absorbed energy is directed, allowing it to be used for a specific function or dissipated harmlessly. The form of chemical change that occurs rapidly in these molecules is called a “nonadiabatic electronic transition.” Such transitions are known to mediate energy flow in natural biological systems such as the ultraviolet photoprotection mechanism of DNA and the first step of the human vision response. Understanding how these mechanisms work precisely may help scientists achieve controlled manipulation of solar energy or optical control of a wide range of energy management functions in artificial systems. Experimental methods, however, have not yet allowed a precisely resolved and complete measurement of nonadiabatic electronic transitions. This constitutes a major obstacle to progress in the field. For progress to occur that would inform a wide body of research aiming to efficiently harness the energy of light for practical purposes, it is especially important to benchmark computational models of the molecules undergoing these rapid changes with experimental measurements, in order to learn which models are accurate. With Dept. of Energy funding, we have made strong progress towards establishing a new optical method for experimentally detecting the full nonadiabatic electronic transition. This requires having coordinated pulses of light covering the visible through the mid-infrared range of the electromagnetic spectrum that last only ten femtoseconds. We have developed a new, relatively simple approach for generating such pulses of laser light, and have incorporated them into a time-resolved spectrometer for measuring rapid changes in molecules. These tools can provide the greater precision and new types of data that are needed to benchmark computational models of molecular change and thus to make progress in the field. Our tools were tested on graphene, an excellent solid-state sample for verifying the capabilities and limitations of our instrumentation. The investment made in these tools by the Dept. of Energy Office of Science will allow new fundamental scientific understanding of energy dynamics in molecules in future studies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NREL Hydrogen Sensor Testing Laboratory and Smart Hydrogen Wide Area Monitoring

The NREL Hydrogen sensor laboratory aims to ensure that hydrogen sensor technology is available to meet end-user needs and to foster the proper use of sensors by advancing next generation sensing and analysis techniques, supporting codes and standards development, and improving component reliability systems.

08 HYDROGEN↗

Satellite-Based Assessment of Rocket Launch and Coastal Change Impacts on Cape Canaveral Barrier Island, Florida, USA

The Cape Canaveral Barrier Island, home to the National Aeronautics and Space Administration (NASA)’s Kennedy Space Center and the United States (U.S.) Space Force’s Cape Canaveral Space Force Station, is situated in a unique ecological transition zone that supports diverse wildlife. This study evaluates the recent changes in vegetation cover (2016–2023) and dune elevation (2007–2017) within the Cape Canaveral Barrier Island using high-resolution optical satellite and light detection and ranging (LiDAR) data. The study period was chosen to depict the time period of a recent increase in rocket launches. The study objectives include assessing changes in vegetation communities, identifying detectable impacts of liquid propellant launches on nearby vegetation, and evaluating dune elevation and tide level shifts near launchpads. The results indicate vegetation cover changes, including mangrove expansion in wetland areas and the conversion of coastal strands to denser scrubs and hardwood forests, which were likely influenced by mild winters and fire management. While detectable impacts of rocket launches on nearby vegetation were observed, they were less severe than those caused by solid rocket motors. Compounding challenges, such as rising tide levels, beach erosion, and wetland loss, potentially threaten the resilience of launch operations and the surrounding habitats. The volume and scale of launches continue to increase, and a balance between space exploration and ecological conservation is required in this biodiverse region. This study focuses on the assessment of barrier islands’ shorelines.

54 ENVIRONMENTAL SCIENCES↗

Fast image acquisition system and method using pulsed light illumination and sample scanning to capture optical micrographs with sub-micron features

An optical inspection system for detecting sub-micron features on a sample component. The system may have a controller, a camera responsive to the controller for capturing images, an objective lens able to capture submicron scale features on the sample component, and a pulsed light source. The pulsed light source may be used to generate light pulses. The camera may be controlled to acquire images, using the objective lens, only while the pulsed light source is providing light pulses illuminating a portion of the sample component. Relative movement between the sample component and the objective lens is provided to enable at least one of a desired subportion or an entirety of the sample component to be scanned with the camera.

Yoo, Jae Hyuck↗

Laser Based Ultrasound for Verification of Circuit Card Assemblies

This IR is a follow-up conference Paper to the IR approved abstract; PNNL-SA-194096. --- Verification that equipment is authentic and not changed; even at the circuit card assembly (CCA) level will likely be an important component of future arms control treaties. This effort was an initial evaluation of the potential for laser-based ultrasound (LBU) as an inspection tool for Unique Identification (UID) of Circuit Card Assembly (CCA) boards and CCA components. The LBU system used a laser pulse for ultrasound generation and an Optical Microphone for ultrasound detection to image subsurface structures without physical contact and in a dry state. This paper described the selected CCA surrogate, CCA components that were examined, the LBU system, LBU images of the CCA components, and the initial development of UID algorithms. Receiver operating characteristics (ROC) curves indicated good performance for two algorithms as a potential means for UID of CCA boards and CCA components.

Laser Ultrasound, Equipment Verification, Arms Con↗

Thermal Conductivity Degradation in High Burnup U-Pu-Zr Fuel

Recent advancements in the characterization of irradiated U-Pu-Zr fuels have revealed complexities that challenge existing understanding of constituent redistribution. Traditionally, models have proposed three concentric regions within the fuel, each characterized by distinctive phases and porosity. However, through detailed analysis of high burnup U-Pu-Zr, we discovered the presence of four distinct constituent redistribution regions. Particularly novel is the observation of significant Pu redistribution, a previously unreported phenomenon that necessitates a reevaluation of current models. This work aims to delve deeper into these findings, seeking to correlate mesoscale measurements of thermal diffusivity and respective thermal conductivity with the phases present in each redistribution region. To achieve this objective, we employed mesoscale thermoreflectance methods using the unique, Idaho National Laboratory (INL) developed, Thermal Conductivity Microscope (TCM) at INL’s Irradiated Materials Characterization Laboratory. The TCM employs two tightly focused lasers: one for heating to generate periodic thermal waves in the substrate, and another spatially separated probe laser to detect changes in the optical reflectivity of the gold-coated substrate resulting from thermal wave diffusion. We conducted several thermal diffusivity measurements within each region of constituent redistribution of a U-19Pu-10Zr fuel pin cross section irradiated to 11 at. % burnup. The TCM measurement positions strategically aligned with transmission electron microscopy (TEM) lift-out locations previously collected from the fuel sample. Complementary microstructural analysis techniques such as optical and scanning electron microscopy (OM/SEM), electron probe microanalysis for chemical compositions, and TEM-based selective area electron diffraction (SAED) analysis for crystallographic insights into each phase were also utilized. This comprehensive approach allowed us to correlate local thermal diffusivity data with microstructural characteristics, enabling the computation of local thermal conductivity at each position. The significance of this contribution lies in its pioneering use of the TCM for ternary fuel mesoscale examination, shedding light on the previously overlooked effects of Pu redistribution on local thermal conductivity. By informing current models capturing constituent redistribution and heat transfer, our findings pave the way for more accurate predictions of metallic fuel performance. Moreover, this work sets the stage for future comparisons with similar TCM examinations on U-19Pu-10Zr fuels at ultra-low burnup, facilitating a comprehensive understanding of thermal property changes across different burnup levels. Ultimately, our study not only enriches our understanding of the thermophysical properties of individual redistribution regions within U-Pu-Zr fuel but also offers valuable insights for the design and operational parameters of proposed next-generation fast reactors.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Chip-Scale Oscillation-Mode Optomechanical Inertial Sensor Near the Thermodynamical Limits

Modern navigation systems integrate the global positioning system (GPS) with an inertial navigation system (INS), which complement each other for correct attitude and velocity determination. Here, the core of the INS integrates accelerometers and gyroscopes used to measure forces and angular rate in the vehicular inertial reference frame. With the help of gyroscopes and by integrating the acceleration to compute velocity and distance, precision and compact accelerometers with sufficient accuracy can provide small–error location determination. Solid–state implementations, through coherent readout, can provide a platform for high performance acceleration detection. In contrast to prior accelerometers using piezoelectric or capacitive readout techniques, optical readout provides narrow–linewidth high–sensitivity laser detection along with low–noise resonant optomechanical transduction near the thermodynamical limits. Here an optomechanical inertial sensor with an 8.2 µg Hz –1/2 velocity random walk (VRW) at an acquisition rate of 100 Hz and 50.9 µg bias instability is demonstrated, suitable for applications, such as, inertial navigation, inclination sensing, platform stabilization, and/or wearable device motion detection. Driven into optomechanical sustained–oscillation, the slot photonic crystal cavity provides radio–frequency readout of the optically–driven transduction with an enhanced 625 µg Hz –1 sensitivity. Measuring the optomechanically–stiffened oscillation shift, instead of the optical transmission shift, provides a 220× VRW enhancement over pre–oscillation mode detection.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

When can we detect lianas from space? Toward a mechanistic understanding of liana‐infested forest optics

Abstract Lianas, woody vines acting as structural parasites of trees, have profound effects on the composition and structure of tropical forests, impacting tree growth, mortality, and forest succession. Remote sensing could offer a powerful tool for quantifying the scale of liana infestation, provided the availability of robust detection methods. We analyze the consistency and global geographic specificity of spectral signals—reflectance across wavelengths—from liana‐infested tree crowns and forest stands, examining the underlying mechanisms of these signals. We compiled a uniquely comprehensive database, including leaf reflectance spectra from 5424 leaves, fine‐scale airborne reflectance data from 999 liana‐infested canopies, and coarse‐scale satellite reflectance data covering 775 ha of liana‐infested forest stands. To unravel the mechanisms of the liana spectral signal, we applied mechanistic radiative transfer models across scales, establishing a synthesis of the relative importance of different mechanisms, which we corroborate with field data on liana leaf chemistry and canopy structure. We find a consistent liana spectral signal at canopy and stand scales across globally distributed sites. This signature mainly arises at the canopy level due to direct effects of more horizontal leaf angles, resulting in a larger projected leaf area, and indirect effects from increased light scattering in the near and short‐wave infrared regions, linked to lianas' less costly leaf construction compared with trees on average. The existence of a consistent global spectral signal for lianas suggests that large‐scale quantification of liana infestation is feasible. However, because the traits responsible for the liana canopy‐reflectance signal are not exclusive to lianas, accurate large‐scale detection requires rigorously validated remote sensing methods. Our models highlight challenges in automated detection, such as potential misidentification due to leaf phenology, tree life history, topography, and climate, especially where the scale of liana infestation is less than a single remote sensing pixel. The observed cross‐site patterns also prompt ecological questions about lianas' adaptive similarities in optical traits across environments, indicating possible convergent evolution due to shared constraints on leaf biochemical and structural traits.

Environmental Sciences & Ecology↗

X-ray emission from a rapidly accreting narrow-line Seyfert 1 galaxy at z = 6.56

The space density of X-ray-luminous, blindly selected active galactic nuclei (AGN) traces the population of rapidly accreting super-massive black holes through cosmic time. It is encoded in the X-ray luminosity function, whose bright end remains poorly constrained in the first billion years after the Big Bang as X-ray surveys have thus far lacked the required cosmological volume. With the eROSITA Final Equatorial-Depth Survey (eFEDS), the largest contiguous and homogeneous X-ray survey to date, X-ray AGN population studies can now be extended to new regions of the luminosity–redshift space (L 2 - 10 keV > 10 45 erg s -1 and z > 6). The current study aims at identifying luminous quasars at z > 5.7 among X-ray-selected sources in the eFEDS field in order to place a lower limit on black hole accretion well into the epoch of re-ionisation. A secondary goal is the characterisation of the physical properties of these extreme coronal emitters at high redshifts. Cross-matching eFEDS catalogue sources to optical counterparts from the DESI Legacy Imaging Surveys, we confirm the low significance detection with eROSITA of a previously known, optically faint z = 6.56 quasar from the Subaru High-z Exploration of Low-luminosity Quasars (SHELLQs) survey. We obtained a pointed follow-up observation of the source with the Chandra X-ray telescope in order to confirm the low-significance eROSITA detection. Using new near-infrared spectroscopy, we derived the physical properties of the super-massive black hole. Finally, we used this detection to infer a lower limit on the black hole accretion density rate at z > 6. The Chandra observation confirms the eFEDS source as the most distant blind X-ray detection to date. The derived X-ray luminosity is high with respect to the rest-frame optical emission of the quasar. With a narrow MgII line, low derived black hole mass, and high Eddington ratio, as well as its steep photon index, the source shows properties that are similar to local narrow-line Seyfert 1 galaxies, which are thought to be powered by young super-massive black holes. In combination with a previous high-redshift quasar detection in the field, we show that quasars with L 2 - 10 keV > 10 45 erg s -1 dominate accretion onto super-massive black holes at z ~ 6.

79 ASTRONOMY AND ASTROPHYSICS↗