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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 379 records · Page 21

Lidar observations of Arctic polar stratospheric clouds, 1988 - Signature of small, solid particles above the frost point

The paper presents recent (January 1988) Arctic airborne lidar data which suggest that Type I polar stratospheric clouds (PSCs) are composed of small solid particles with radii on the order of 0.5 micron. PSCs were observed remotely in the 21-24 km altitude range north of Greenland during a round-trip flight from Andenes, Norway on January 29, 1988, aboard the NASA Wallops Flight Facility P-3 Orion aircraft. Synoptic analyses at the 30-mb level show local temperatures of 191-193 K, which are well above the estimated frost point temperature of 185 K; this suggests that the PSCs were probably of the binary HNO3-H2O (Type I) class.

Poole, L. R.↗

Ka-Band Scanning ARM Cloud Radar (KASACR), 2nd Generation CF-Radial Spectral Data, Vertically-Pointing Scan, Cross Mode (a1-level)

The Ka-Band Scanning ARM Cloud Radar (KASACR) records cloud properties. ARM's scanning cloud radars are dual-frequency, dual-polarization Doppler radars mounted on a common scanning pedestal. Each pedestal includes a Ka-band radar (2kW peak power) and the deployment location determines whether the second radar is a W-band (1.7 kW peak power) or an X-band (20 kW peak power). Beamwidths for Ka-bands paired with W-bands are roughly matched at 0.3 degrees. The X-band beamwidth is approximately 1 degree. Due to the narrow antenna beamwidth, ARM’s scanning cloud radars use scanning strategies unlike typical weather radars. Rather than focusing on plan position indicator, or PPI, scans, the KASACR uses range height indicator, or RHI, scans at numerous azimuths to obtain cloud volume data. Measurements collected with the KASACR are copolar and cross-polar radar reflectivity, Doppler velocity, spectra width and spectra when not scanning, and linear depolarization ratio. KASACR data from the 2018–2019 Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign in Argentina are now available as b1-level products. Building on the original CACTI operational data, the b1-level products feature improved data quality resulting from extensive analyses and corrections. The data are cross-calibrated to a common point, datastreams are corrected for operational issues that occurred during the campaign, and several data quality masks and basic derived products are incorporated. For more information, read the CACTI radar b1-level processing report.

54 ENVIRONMENTAL SCIENCES↗

Peridynamic elastic waves in two-dimensional unbounded domains: Construction of nonlocal Dirichlet-type absorbing boundary conditions

The focus of this paper is on application of peridynamics (PD) to propagation of elastic waves in unbounded domains. We construct absorbing boundary conditions (ABCs) derived from a semi-analytical solution of the PD governing equation at the exterior region. This solution is made up of a finite series of plane waves, as fundamental solutions (modes), which satisfy the PD dispersion relations. The modes are adjusted to transmit the energy from the interior region (near field) to the exterior region (far field). The corresponding unknown coefficients of the series are found in terms of the displacement field at a layer of points adjacent to the absorbing boundary. This is accomplished through a collocation procedure at subregions (clouds) around each absorbing point. The proposed ABCs offer appealing advantages, which facilitate their application to PD. They are of Dirichlet-type, hence their implementation is relatively simple as no derivatives of the field variables are required. They are constructed in the time and space domains and thus application of Fourier and Laplace transforms, cumbersome for nonlocal models, is not required. At the discrete level, the modes satisfy the same numerical dispersion relations of the near field, which makes the far-field solution compatible with that of the near field. We scrutinize the performance of the proposed ABCs through several examples. So our investigation shows that the proposed ABCs perform stably in time with an appropriate level of accuracy even in problems characterized by highly-dispersive propagating waves, including crack propagation in semi-unbounded brittle solids.

42 ENGINEERING↗

Boundary Layer Controls on the Shallow-to-Deep Cumulus Transition (Final Technical Report)

This project advanced our understanding of the processes governing cumulus cloud formation and provides an improved observational basis for validating earth system models. To be specific, the project used laser- and radar-remote sensors to examine the physical properties of updrafts that rise from earth’s surface and initiate clouds deeper in the atmosphere. These updrafts comprise “thermals” and “plumes” and occur at small spatial and temporal scales (e.g., 10s of minutes, 100s of meters). These small scales preclude explicit representation in most earth system and climate models, and thus necessitate “sub-grid-scale” parameterization of updraft processes. The innovation of this project was to directly measure the size, shape, strength and water vapor content of these updrafts with Doppler and Raman lidars, respectively, and to link these updraft properties to cloud processes using vertically pointed weather radars. The resulting data sets comprise 100s of thousands of updrafts and thousands of clouds, which far exceeds previous efforts, and thereby provides a robust statistical and physical representation of these processes. From these large datasets the project produced a sequence of scientific analyses that: (1) Elucidate how variations in the turbulent structure of the convective boundary layer control shallow cumulus convection, (2) Quantify the upward transport of water vapor to cloud base via thermals and plumes, (3) Validate large-eddy simulations of updrafts and shallow convective clouds, (4) Demonstrate a size-to-strength relationship between updraft width and updraft speed, and (5) Demonstrate how updrafts interact with the stability at the top of the convective boundary layer to modulate the depth and vigor of convective clouds. These results have been disseminated via several published journal articles, academic theses, and conference presentations. Collectively these results contribute to the Atmospheric System Research (ASR) program’s goal to “improve understanding of the key cloud, aerosol, precipitation, and radiation processes that affect the Earth’s radiative balance and hydrological cycle, particularly processes that limit the predictive ability of regional and global earth system models”.

54 ENVIRONMENTAL SCIENCES↗

Reconstructing Subgrid Cloud Variability Guided by CloudSat/CALIPSO Observations

Predicting realistic cloud subgrid variability remains a challenge for Global Climate Models (GCMs) even though it can play an important role for proper representation of processes pertaining to cloud microphysics, precipitation, and radiation, but also for comparisons with satellite observations which are of much higher resolution than model grids. The diagnostic approach of subgrid cloud variability is commonly handled by subcolumn cloud generators. For a specific GCM, one ideally wants the subgrid variability used for comparisons with satellite observations to be created by the same generator and with the same rules as the one used for model integration. With this in mind, we have embarked in an effort to test and improve cloud subcolumn generators appropriate for GCMs. For this purpose, we use cloud (hydrometeor) products from active observations by the CloudSat radar (CPR) and the CALIPSO lidar (CALIOP). Cloud products from active sensors while suffering significant sampling and coverage drawbacks have the advantage of resolving both horizontal and vertical variability. The main question is: given a profile of cloud condensate mean and variance, can we create a subgrid cloud field that is statistically similar to the observed subgrid cloud field? By “statistically”, we suggest that we do not aspire to reproduce “well” each individual subgrid cloud field of a GCM-scale region, but that our generator performs well for a large ensemble of cases. We simulate radar, passive imager, and radiation flux fields from the observed 2D cloud fields and create one-point statistics; we use the profiles of cloud condensate mean and variance as input to the generator to create subgrid cloud fields; we compare the statistics; we adjust the rules of the generator to create the best possible agreement between the radar, imager and radiation field statistics. In this process, the active observations have actually a dual role: they provide the actual subgrid cloud field which can be reduced to a profile of mean and variance used by the subcolumn generator, but they also provide the rules needed by the generator, such as measures (e.g, decorrelation length) of the vertical overlap of cloud fraction and of the condensate horizontal variability. This presentation will show our progress using Cloudsat and CALIPSO products in this dual fashion.

cloud↗

Reconstructing Subgrid Cloud Variability Guided by CloudSat/CALIPSO Observations

Predicting realistic cloud subgrid variability remains a challenge for Global Climate Models (GCMs) even though it can play an important role for proper representation of processes pertaining to cloud microphysics, precipitation, and radiation, but also for comparisons with satellite observations which are of much higher resolution than model grids. The diagnostic approach of subgrid cloud variability is commonly handled by subcolumn cloud generators. For a specific GCM, one ideally wants the subgrid variability used for comparisons with satellite observations to be created by the same generator and with the same rules as the one used for model integration. With this in mind, we have embarked in an effort to test and improve cloud subcolumn generators appropriate for GCMs. For this purpose, we use cloud (hydrometeor) products from active observations by the CloudSat radar (CPR) and the CALIPSO lidar (CALIOP). Cloud products from active sensors while suffering signi􀂦cant sampling and coverage drawbacks have the advantage of resolving both horizontal and vertical variability. The main question is: given a profile of cloud condensate mean and variance, can we create a subgrid cloud field that is statistically similar to the observed subgrid cloud field? By “statistically”, we suggest that we do not aspire to reproduce “well” each individual subgrid cloud field of a GCM-scale region, but that our generator performs well for a large ensemble of cases. We simulate radar, passive imager, and radiation flux fields from the observed 2D cloud fields and create one-point statistics; we use the profiles of cloud condensate mean and variance as input to the generator to create subgrid cloud fields; we compare the statistics; we adjust the rules of the generator to create the best possible agreement between the radar, imager and radiation field statistics. In this process, the active observations have actually a dual role: they provide the actual subgrid cloud field which can be reduced to a profile of mean and variance used by the subcolumn generator, but they also provide the rules needed by the generator, such as measures (e.g, decorrelation length) of the vertical overlap of cloud fraction and of the condensate horizontal variability. This presentation will show our progress using Cloudsat and CALIPSO products in this dual fashion.

clouds↗

Ka-Band Scanning ARM Cloud Radar (KASACR), 2nd Generation CF-Radial Spectral Data, Vertically-Pointing Scan, Cross-Polarization Mode (a1-level)

The Ka-Band Scanning ARM Cloud Radar (KASACR) records cloud properties. ARM's scanning cloud radars are dual-frequency, dual-polarization Doppler radars mounted on a common scanning pedestal. Each pedestal includes a Ka-band radar (2kW peak power) and the deployment location determines whether the second radar is a W-band (1.7 kW peak power) or an X-band (20 kW peak power). Beamwidths for Ka-bands paired with W-bands are roughly matched at 0.3 degrees. The X-band beamwidth is approximately 1 degree. Due to the narrow antenna beamwidth, ARM’s scanning cloud radars use scanning strategies unlike typical weather radars. Rather than focusing on plan position indicator, or PPI, scans, the KASACR uses range height indicator, or RHI, scans at numerous azimuths to obtain cloud volume data. Measurements collected with the KASACR are copolar and cross-polar radar reflectivity, Doppler velocity, spectra width and spectra when not scanning, and linear depolarization ratio. KASACR data from the 2018–2019 Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign in Argentina are now available as b1-level products. Building on the original CACTI operational data, the b1-level products feature improved data quality resulting from extensive analyses and corrections. The data are cross-calibrated to a common point, datastreams are corrected for operational issues that occurred during the campaign, and several data quality masks and basic derived products are incorporated. For more information, read the CACTI radar b1-level processing report.

54 ENVIRONMENTAL SCIENCES↗

158 micron forbidden C II mapping of the Orion molecular cloud

A fully sampled, 1000-point, 1-arcmin-resolution map of the inner 6.5 x 10 arcmin (alpha x delta) regions of the Orion Nebula in the 157.7409-micron forbidden fine-structure line is constructed. Large-scale strip maps in forbidden C II across the face of the Orion molecular cloud, and CO(17-16), (14-13), and (7-6) spectra are obtained at selected positions in the Orion H II region/molecular cloud interface. Strong forbidden C II line emission is observed across the face of the Orion molecular. The total forbidden C II luminosity from the Orion molecular cloud is about 1500 solar luminosities, or 0.3 percent of the FIR luminosity. The extended forbidden C II emission probably arises in either the UV-exposed surface of the molecular cloud or from the surfaces of UV-exposed clumps within the molecular cloud.

Stacey, G. J.↗

Convective and Turbulent Motions in Nonprecipitating Cu. Part III: Characteristics of Turbulence Motions

Velocity field in a nonprecipitating Cu under BOMEX conditions, simulated by SAM with 10-m resolution and spectral bin microphysics is separated into the convective part and the turbulent part, using a wavelet filtering. In Part II of the study properties of convective motions of this Cu were investigated. Here in Part III of the study, the parameters of cloud turbulence are calculated in the cloud updraft zone at different stages of cloud development. The main points of this study are (i) application of a fine-scale LES model of a single convective cloud allowed a direct estimation of turbulence parameters using the resolved flow in the cloud and (ii) the separation of the resolved flow into the turbulence flow and the nonturbulence flow allowed us to estimate different turbulent parameters with sufficient statistical accuracy. We calculated height and time dependences of the main turbulent parameters such as turbulence kinetic energy (TKE), spectra of TKE, dissipation rate, and the turbulent coefficient. It was found that the main source of turbulence in the cloud is buoyancy whose contribution is described by the buoyancy production term (BPT). The shear production term (SPT) increases with height and reaches its maximum near cloud top, and so does BPT. In agreement with the behavior of BPT and SPT, turbulence in the lower cloud part (below the inversion level) is weak and hardly affects the processes of mixing and entrainment. The fact that BPT is larger than SPT determines many properties of cloud turbulence. For instance, the turbulence is nonisotropic, so the vertical component of TKE is substantially larger than the horizontal components. Another consequence of the fact that BPT is larger than STP manifests itself in the finding that the turbulence spectrum largely obeys the -11/5 Bolgiano–Obukhov scaling. The classical Kolmogorov -5/3 scaling dominates for the low part of a cloud largely at the dissolving stage of cloud evolution. Using the spectra obtained we evaluated an “effective” dissipation rate which increases with height from nearly zero at cloud base up to 20 cm 2 s -3 near cloud top. The coefficient of turbulent diffusion was found to increase with height and ranged from 5 m 2 s -1 near cloud base to 25 m 2 s -1 near cloud top. In conclusion, the possible role of turbulence in the process of lateral entrainment and mixing is discussed.

54 ENVIRONMENTAL SCIENCES↗

The ionization equilibrium inside the RHO Ophiuchi cloud

Observational technology is now reaching the point where optical absorption-line studies of dark interstellar clouds are becoming feasible. Such studies are of great interest. In particular, it will be important to discover the degree of depletion which has occurred in dark clouds. In order to assess depletions on the basis of observations of a limited range of ionization stages, it is necessary to analyze the ionization balance. The present investigation is concerned with such an analysis. The two key parameters necessary for deducing the ionization balance are the electron density and the radiation field intensity. A summary is provided regarding the existing data on the cloud density using data from the literature, and the radiation field intensity is derived from the observed H2 rotational excitation. The implications of both the density and radiation field data for the ionization balance of several species are discussed. It is found that for all species treated the first ion is dominant in the line of sight toward HD 147889.

Snow, T. P., Jr.↗

KAZR Hydrometeor and Insect Masks

The Ka-band ARM zenith pointing radar (aka, KAZR) is so sensitive that it detects cloud particles and individual insects. While detecting insects with Ka-band radar is beneficial and desirable to advance radar entomology, this sensitivity can be detrimental to radar meteorology because insects could be interpreted as clouds or precipitation. For example, misclassifying insects as clouds has been a problem for the ARM Active Remote Sensing of Clouds (ARSCL) Value Added Product since its inception (Clothiaux et al. 2000). Based on cloud particle and insect radar scattering properties, an algorithm was developed that identifies clouds, raindrops, ice particles, and insects in KAZR co- and cross-polarimeteric Doppler velocity spectra. The algorithm produces affirmative masks in the KAZR native time and height resolution indicating time-height locations of hydrometeors and insects. The hydrometeor mask contains binary information (e.g., yes/no hydrometeor presence), and the insect mask includes a proxy for insect activity that increases when more insects are detected in the Doppler velocity spectra. The algorithm was developed using KAZR medium sensitivity mode (MD) observations and was applied to two summer seasons of KAZR observations at the Southern Great Plains (SGP) Central Facility: May-October 2018 and 2019. In the future, this data set will be expanded to include other KAZR operating modes and observations from other ARM field sites. Details of the algorithm and data set can be found in: Williams, C.R., K.L. Johnson, S.E. Giangrande, J. C. Hardin, R. Oktem, and D. M. Romps, 2021: Identifying Insects, Clouds, and Precipitation using Vertically Pointing Polarimetric Radar Doppler Velocity Spectra. Atmospheric Measurement Techniques, submitted 6-Feb-2021. https://amt.copernicus.org/preprints/amt-2021-27/#discussion.For more information on the ARSCL VAP, see Clothiaux, E. E., T. P. Ackerman, G. G. Mace, K. P. Moran, R. T. Marchand, M. A. Miller, and B. E. Martner, 2000; J. Appl. Meteor., 39, 645-665.

54 ENVIRONMENTAL SCIENCES↗

Cloud Impacts on Photochemistry: Building a Climatology of Photolysis Rates from the Atmospheric Tomography Mission

Measurements from actinic flux spectroradiometers on board the NASA DC-8 during the Atmospheric Tomography (ATom) mission provide an extensive set of statistics on how clouds alter photolysis rates (J values) throughout the remote Pacific and Atlantic Ocean basins. J values control tropospheric ozone and methane abundances, and thus clouds have been included for more than three decades in tropospheric chemistry modeling. ATom made four profiling circumnavigations of the troposphere capturing each of the seasons during 2016–2018. This work examines J values from the Pacific Ocean flights of the first deployment, but publishes the complete Atom-1 data set (29 July to 23 August 2016). We compare the observed J values (every 3 s along flight track) with those calculated by nine global chemistry– climate/transport models (globally gridded, hourly, for a mid-August day). To compare these disparate data sets, we build a commensurate statistical picture of the impact of clouds on J values using the ratio of J -cloudy (standard, sometimes cloudy conditions) to J -clear (artificially cleared of clouds). The range of modeled cloud effects is inconsistently large but they fall into two distinct classes: (1) models with large cloud effects showing mostly enhanced J values aloft and or diminished at the surface and (2) models with small effects having nearly clear-sky J values much of the time. The ATom-1 measurements generally favor large cloud effects but are not precise or robust enough to point out the best cloud-modeling approach. The models here have resolutions of 50–200 km and thus reduce the occurrence of clear sky when averaging over grid cells. In situ measurements also average scattered sunlight over a mixed cloud field, but only out to scales of tens of kilometers. A primary uncertainty remains in the role of clouds in chemistry, in particular, how models average over cloud fields, and how such averages can simulate measurements.

actinic flux spectroradiometers↗

An Unbiased CO Survey Toward the Northern Region of the Small Magellanic Cloud with the Atacama Compact Array. II. CO Cloud Catalog

The nature of molecular clouds and their statistical behavior in subsolar metallicity environments are not fully explored yet. We analyzed data from an unbiased CO (J = 2–1) survey at the spatial resolution of ∼2 pc in the northern region of the Small Magellanic Cloud with the Atacama Compact Array to characterize the CO cloud properties. A cloud-decomposition analysis identified 426 spatially/velocity-independent CO clouds and their substructures. Based on the cross-matching with known infrared catalogs by Spitzer and Herschel, more than 90% CO clouds show spatial correlations with point sources. We investigated the basic properties of the CO clouds and found that the radius–velocity linewidth (R–σ v ) relation follows the Milky Way-like power-law exponent, but the intercept is ∼1.5 times lower than that in the Milky Way. The mass functions (dN/dM) of the CO luminosity and virial mass are characterized by an exponent of ∼1.7, which is consistent with previously reported values in the Large Magellanic Cloud and in the Milky Way.

Local Group↗

Do interstellar gas clouds exist between spiral arms.

This paper discusses what can happen to clouds as they move from arm regions to interarm regions, through a density-wave shock, and back to arm regions again. Shu et al. (1972) have taken the viewpoint that interstellar clouds will survive the trip between arms. Biermann et al. (1972) have taken the viewpoint that they will not. We shall point out that cloud-cloud collisions and other processes may lead to the destruction of interstellar clouds in less time than the 100 m.y. it takes clouds to travel across arms. A possible observational test is suggested to distinguish between the two possibilities.

Quirk, W. J.↗

New Concepts for Refinement of Cumulus Parameterization in GCM's the Arakawa-Schubert Framework

Several state-of-the-art models including the one employed in this study use the Arakawa-Schubert framework for moist convection, and Sundqvist formulation of stratiform. clouds, for moist physics, in-cloud condensation, and precipitation. Despite a variety of cloud parameterization methodologies developed by several modelers including the authors, most of the parameterized cloud-models have similar deficiencies. These consist of: (a) not enough shallow clouds, (b) too many deep clouds; (c) several layers of clouds in a vertically demoralized model as opposed to only a few levels of observed clouds, and (d) higher than normal incidence of double ITCZ (Inter-tropical Convergence Zone). Even after several upgrades consisting of a sophisticated cloud-microphysics and sub-grid scale orographic precipitation into the Data Assimilation Office (DAO)'s atmospheric model (called GEOS-2 GCM) at two different resolutions, we found that the above deficiencies remained persistent. The two empirical solutions often used to counter the aforestated deficiencies consist of a) diffusion of moisture and heat within the lower troposphere to artificially force the shallow clouds; and b) arbitrarily invoke evaporation of in-cloud water for low-level clouds. Even though helpful, these implementations lack a strong physical rationale. Our research shows that two missing physical conditions can ameliorate the aforestated cloud-parameterization deficiencies. First, requiring an ascending cloud airmass to be saturated at its starting point will not only make the cloud instantly buoyant all through its ascent, but also provide the essential work function (buoyancy energy) that would promote more shallow clouds. Second, we argue that training clouds that are unstable to a finite vertical displacement, even if neutrally buoyant in their ambient environment, must continue to rise and entrain causing evaporation of in-cloud water. These concepts have not been invoked in any of the cloud parameterization schemes so far. We introduced them into the DAO-GEOS-2 GCM with McRAS (Microphysics of Clouds with Relaxed Arakawa-Schubert Scheme).

Sud, Y. C.↗

Peak Rain Rate Sensitivity to Observed Cloud Condensation Nuclei and Turbulence in Continental Warm Shallow Clouds During CACTI

Abstract Warm clouds strongly affect Earth's energy budget but remain imperfectly represented in climate models, partly due to the complexity and covariability of relevant processes influencing warm rain. This work presents a detailed analysis of different factors affecting rain rate peak intensity (RR) in continental warm clouds. Clouds were identified with vertically pointing radar and lidar observations and categorized via a temperature‐based cloud type classification algorithm from which warm clouds were isolated. Observations and retrievals of liquid water path (LWP), cloud condensation nuclei concentration (N CCN ), cloud depth, and cloud duration of more than 3,000 separate warm clouds sampled during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign are analyzed in this work. Multiple linear regression (MLR) and random forest (RF) models are applied to assess the relative impact of these variables on RR. Overall, RR tends to increase as cloud depth, LWP, and cloud duration increase, or N CCN decreases. Cloud depth affects RR the most while N CCN impacts it the least. When considering over 170 warm clouds observed at least 1 hr in which in‐cloud turbulence is retrieved, the effect of N CCN on RR remains most likely suppressive, but it is not significant at a 75% level for MLR and is highly uncertain for RF. The impact of in‐cloud turbulence depends on the moment and location it is sampled. Cloud base turbulence around the time of RR suppresses RR, while cloud top turbulence effects are inconclusive. Possible difficulties in isolating robust CCN and turbulence effects on RR are discussed.

54 ENVIRONMENTAL SCIENCES↗

Dataset for "FLEXPART-WRF simulations to assess dust transport in the convective boundary layer at the Southern Great Plains site"

Soil dusts are an important source of aerosol in agricultural regions and can affect the Earth’s radiation budget through the modification of cloud properties, and in particular, through their ability to act as ice nucleating particles. In order to impact cloud properties, agricultural soil dusts need to be transported from the point of emission to cloud-relevant altitudes. Vertical transport within the planetary boundary layer is strongly controlled by turbulence and is challenging to represent accurately in regional and global models. Large-eddy simulations (LES) are run at resolutions capable of resolving most of the turbulent energy directly and can thus better simulate vertical transport. In this study, we leverage the LES ARM Symbiotic Simulation and Observation (LASSO) large-eddy simulations to simulate vertical transport of agricultural dust within the turbulent boundary layer using a modified version of the stochastic dispersion model FLEXPART-WRF. We find that the modified model is better capable of simulating particle transport due to turbulence, and that particle size was the greatest factor in determining particle lifetime. Individual meteorology and particle density had intermediate effects upon particle transport, while release height had little effect upon simulation results. Finally, we utilize a quasi-single column model (QSCM) approach to determine how our results compare to a parameterized treatment of turbulence. The QSCM simulations led to greater tracer transport out of the boundary layer, with ramifications for any studies utilizing a Lagrangian stochastic model to understand tracer dispersion. These results highlight the importance of accurately simulating turbulence for understanding particle transport.

54 ENVIRONMENTAL SCIENCES↗